Instrumentation and Detectors · Cross-listed from quant-ph
Cross-Sensor RGB Spectrograms: A Visual Method for Anomaly Detection in Classical and Quantum Magnetometer Triads
Manas Pandey
Stationary multi-magnetometer arrays are routinely deployed in geomagnetic observatories, laboratory shielded rooms, and ground-based monitoring stations. The standard analysis pipeline reduces each sensor to an independent power spectrum, discarding any inter-sensor structure that is itself diagnostic of measurement health and of localised
magnetic activity. This paper develops a purely theoretical framework for a deliberately simple visualisation that maps the short-time
Fourier (STFT) power spectra of three concurrent magnetometers into the red, green, and blue channels of a single image: the cross-sensor RGB spectrogram. Inter-sensor coherence appears as neutral grey or white, while spectral energy that is unique to one or two sensors stands out as saturated colour. We formalise the construction of the image, derive its time-frequency resolution properties, give an explicit account of the per-channel normalisation choice, and present a colour-anomaly taxonomy that distinguishes coherent broadband activity, single-sensor faults, asymmetric pairwise sources, and slow temporal drift. A companion long-window variant is described for resolving features in the ultra-low frequency (ULF) band. The construction is presented without reference to any particular
dataset or implementation; it is intended as a self-contained methodological building block that can be inserted into any monitoring pipeline whose front end is a synchronously sampled magnetometer triad. Because the construction operates on scalar magnitude time series alone, it applies equally to classical fluxgate sensors and to
quantum magnetometers – optically pumped magnetometers (OPMs), nitrogen-vacancy (NV) centre arrays, and superconducting
quantum interference devices (SQUIDs) – where distinguishing
quantum-limited noise from technical artefacts is a central diagnostic challenge.
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Optics
Iterative approach for high-quality binary intensity hologram generation in augmented reality applications
Anik Ghosh, Matteo Ziliani, Marco Astarita et al. (+8 more)
Binary amplitude spatial light modulators, such as digital micromirror devices (DMDs), are increasingly relevant for computer generated holography due to their high refresh rates, low cost, and due to the emergence of subwavelength pixel architectures. However, the binary constraint limits the reconstruction quality, as conventional approaches rely on a binarization applied as a final step after hologram computation which leads to reduced efficiency and contrast. We introduce an iterative estimation approach for the generation of off axis binary amplitude holograms, in which the binarization constraint is applied at each iteration. We validate the approach through numerical simulations and experimental reconstruction using a DMD based optical setup. Quantitative and qualitative comparisons with random superposition and Gerchberg Saxton methods demonstrate significant improvements in image contrast, light efficiency, and reconstruction fidelity, with comparable computational cost. The proposed method provides a practical route toward high quality CGH using binary modulators and supports emerging applications requiring high speed and high resolution
holographic projection.
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All authors Anik Ghosh, Matteo Ziliani, Marco Astarita, Samuele Trezzi, Alessandro Cerioni, Anna Cesaratto, Mara Galli, Gianluca Valentini, Andrea Bassi, Giulio Cerullo, Paolo Pozzi
Computational Physics · Cross-listed from math.NA
From Exact Space-Time Symmetry Conservation to Automatic Mesh Refinement in Discrete Initial Boundary Value Problems
Alexander Rothkopf, W.A. Horowitz and Jan Nordström
In this contribution we present recent developments in the formulation and solution of Initial Boundary Value Problems (IBVPs). Building upon a modern variational action formulation of classical dynamics, we treat Initial Boundary Value Problems directly on the action level, bypassing governing equations. We show that by including coordinate maps as dynamical degrees of freedom together with propagating fields two key results emerge. Space-time
symmetries remain protected even after discretization, leading to an exact conservation of Noether charges even for discrete IBVPs. The dynamical nature of the coordinate maps leads to an adjustment of space-time resolution, guided by Noether charge conservation, realizing a form of automatic adaptive mesh refinement. We stress that as long as SBP operators are used for the discretization, our results are independent of whether the dynamics are solved on the action or governing equation level and hold in particular also at high order. As proof-of-principle for our approach we present its application to scalar wave-propagation in 1+1 dimensions.
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Instrumentation and Detectors
Correcting the Energy-Dependent Asymmetry in Low-Energy $\mu$SR
G. Janka, Z. Salman, A. Suter et al. (+1 more)
Low-energy $\mu$SR (LE-$\mu$SR) enables depth-resolved studies of
magnetic and electronic properties from the surface into the near-surface region, but the measured transverse-field asymmetry is not an intrinsic constant and depends on implantation energy and beamline conditions. Following an upgrade of the single-
muon tagging system at the LEM beamline at PSI in 2023, updated asymmetry calibrations became necessary. Here, we present updated reference measurements that establish the energy-dependent maximum asymmetry using a silver reference and quantify spurious contributions from reflected
muons using a nickel reference. In addition, we address systematic reductions of the measured asymmetry arising from incomplete beam–sample overlap by introducing a sample-size-dependent correction factor. This factor is obtained from musrSim/Geant4 simulations incorporating an updated electrostatic field map of the sample environment and is benchmarked using implantation-energy scans on SrTiO$_3$ samples of different lateral dimensions. Together, these updated calibrations and the simulation-based overlap correction provide a practical and up-to-date framework for LE-$\mu$SR data correction under current beam conditions and enable quantitative depth-resolved analysis of volume fractions.
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All authors G. Janka, Z. Salman, A. Suter, T. Prokscha
Atomic Physics · Cross-listed from quant-ph
Autonomous Quantum Error Correction of Spin-Oscillator Hybrid Qubits
Sungjoo Cho, Ju-yeon Gyhm, Hyukjoon Kwon et al. (+1 more)
We propose a novel measurement-free scheme for stabilizing a
spin-oscillator hybrid
qubit via autonomous
quantum error correction. The engineered Lindbladian renders the code space into an attractive steady-state subspace, realized by coupling the storage mode to a rapidly cooled bath through a controlled beam-splitter and
spin-dependent displacement interactions. The continuous variable-discrete variable hybrid approach to autonomous
quantum error correction preserves the hardware efficiency of conventional dissipation engineering while simplifying the required system-bath coupling. The construction is compatible with simple logical gates and leverages primitives already demonstrated in experimental platforms, such as trapped-ion systems, suggesting a practical route to hardware-efficient, noise-biased logical
qubits without repeated syndrome measurements and feedforward.
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All authors Sungjoo Cho, Ju-yeon Gyhm, Hyukjoon Kwon, Hyunseok Jeong
Fluid Dynamics · Cross-listed from quant-ph
Schrödinger-Navier-Stokes Equation for the Quantum Simulation of Navier-Stokes Flows
Luca Cappelli, Sauro Succi, Monica Lacatus et al. (+2 more)
The search for
quantum-like wave formulations of the Navier-Stokes (Schrödinger-Navier-Stokes, SNS for short) equations describing classical dissipative fluids has met with increasing
attention in the recent years, due to the large portfolio of potential applications in science and engineering. A SNS formulation of classical fluids was first presented in a largely un-noticed paper by Dietrich and Vautherin back in 1985(Journal de Physique). In this paper, we revisit this specific SNS approach and assess its viability for
quantum implementations based on Carleman
embedding/linearization techniques. Specifically, we i) Clarify in full mathematical detail why the SNS dissipator presents a steep challenge for
quantum computers and propose a way out strategy based on the Hamilton-Jacobi (HJ) formulation of fluid dynamics; ii) Develop a corresponding
quantum algorithm using a new technique based on a tensor-network representation of Carleman
embedding of the HJ equations (CHJ) which permits substantial
memory savings; iii) Emulate the CHJ
quantum algorithm on a classical computer and analyse its convergence and accuracy for the specific case of Kolmogorov-like flows at moderate Reynolds numbers. To the best of our knowledge, this is the first
quantum algorithm based on a
quantum-like wave formulation of the genuine Navier-Stokes equations, including pressure, dissipation and vorticity.
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All authors Luca Cappelli, Sauro Succi, Monica Lacatus, Alessandro Zecchi, Alessandro Roggero
Chemical Physics · Cross-listed from cs.DS
Computational Generation of Substrate-Specific Molecular Cages
Noé Demange, Yann Strozecki and Sandrine Vial
In this paper, we propose a method to build molecular cages designed to capture a specific substrate. We model a cage as a graph of atoms with coordinates in space, and several constraints on their edges (degree, length and angle). We use a simple method to place binding patterns which are able to interact with certain parts of the substrate. We then propose an
algorithm which considers all possible ways of connecting these binding patterns and try to construct the smallest possible molecular paths realizing these connections. We investigate many variants of our method in order to obtain the most efficient
algorithm, able to build cages of more than a hundred atoms.
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Fluid Dynamics
Patchy Polymeric Scalar Turbulence
Rahul K. Singh and Marco E. Rosti
Turbulent polymeric flows show strong deviations from Kolomogorov-like behaviour resulting from more complex dynamics compared to Newtonian
turbulence. We now study the nature of mixing in polymeric
turbulence via Eulerian passive scalar fields of varying molecular diffusivities, given by the Schmidt number Sc. We show that polymeric
turbulence is a less efficient mixer than the Newtonian one at small to moderate Sc numbers. Newtonian scalar
turbulence (NST) forms large islands of fluctuations with extended, contiguous fronts. In contrast, polymeric scalar
turbulence (PST) is marked by small, interspersed patches of strong but less intermittent fluctuations. These patches collectively comprise a larger volume fraction of strong fluctuations, indicating a less efficient mixing, alongwith smaller scalar gradients and therefore smaller average flux across their boundaries. Box counting dimensions reveal a smoother and more space filling nature of patch boundaries in PST compared to NST fronts. Finally, spatial changes of the scalar are stronger in PST, but with a slower self-similar growth and less intermittency as revealed by the kurtosis of scalar differences. Overall, these observations hint at reduced mixing in PST where fluctuations are typically stronger while the average scalar flux is smaller in a stationary state.
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Fluid Dynamics
LCS.jl: A High-Performance, Multi-Platform Computational Model in Julia for Turbulent Particle-Laden Flows
Taketo Tominaga and Ryo Onishi
Multiphase turbulent flow phenomena are observed not only in industrial devices but also in environmental flows, and direct numerical simulation (DNS) plays a key role in their investigation. Many numerical models have been developed; nevertheless, few models are highly optimized for GPU platforms, which represent the current mainstream in high-performance computing (HPC). In this study, we developed LCS.jl (Lagrangian Cloud Simulator in Julia), a single-source and multi-platform multiphase
turbulence simulation model implemented in Julia
language and KernelAbstractions.jl. Validation results confirmed that the present fluid and particle statistics agree well with those obtained in prior studies. A GPU-native particle communication
algorithm based on prefix-scan reduced the particle communication cost from approximately 78% (CPU-delegated) to 10% of total execution time. LCS.jl achieved computational performance equivalent to the Fortran implementation in many-processes computations. For GPUs, strong scaling efficiency was maintained above 85% (up to 256 GPUs) and weak scaling efficiency above 90% (up to 216 GPUs) on TSUBAME4.0 (a GPU supercomputer at the Institute of Science Tokyo). LCS.jl achieved a maximum speedup of 18.0x on GPUs over CPUs. A trial heterogeneous execution achieved a 72% reduction in execution time compared to the CPU-only configuration even in configurations where the GPU was not the primary compute device. These results demonstrate that LCS.jl is a multiphase
turbulence simulation platform that achieves both portability and scalability across a variety of computational resource configurations.
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Optics · Cross-listed from cond-mat.supr-con
Microscopic mechanism for resonant light-enhanced pair correlations in K$_3$C$_{60}$
Juan I. Aranzadi, Joseph Tindall, Paul Fadler et al. (+1 more)
Recent experiments on K3C60 revealed a
giant enhancement of the light-induced superconducting-like optical response for pump frequencies near 10 THz, with an efficiency roughly two orders of magnitude larger than for off resonant excitation. Here we show that a resonant enhancement of pair correlations arises naturally in a driven purely electronic model of K$_3$C$_{60}$ with ab initio parameters. The underlying mechanism is a
symmetry constrained two-
photon pathway: the first
photon drives the system from the even-parity ground state to an intermediate odd-parity
manifold, while the second
photon induces a transition to an even-parity excited state with enhanced pair correlations. Larger-cluster calculations show that the corresponding resonance energy is strongly renormalized downward with system size and connectivity, reflecting the kinetic-energy gain of delocalized photo-excited doublon-holon configurations. A simplified single-orbital model reproduces this scaling trend and reaches a 14-site fcc cluster, where the resonant peak is pushed to 30 THz, with a trend compatible with a further reduction toward the experimental 10 THz scale in larger systems. Varying the Hubbard coupling strength, we find that the resonance is lowest and the pairing enhancement strongest near intermediate couplings, where doublon-holon excitations are both well defined and mobile. Our results establish a purely electronic mechanism for resonant light-enhanced pair correlations in K$_3$C$_{60}$ and support the interpretation of the experimental 10 THz resonance as optical access to a paired many-body excited state rather than improved
metallicity. More broadly, they suggest that related resonant pathways may arise in other intermediate-coupling Hubbard materials.
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All authors Juan I. Aranzadi, Joseph Tindall, Paul Fadler, Michael A. Sentef
Chemical Physics · Cross-listed from cond-mat.mtrl-sci
opt-DDAP: Optimisable density-derived atomic point charges via automatic differentiation
Mohith H. and Sudarshan Vijay
Interatomic potentials which accurately describe long-range electrostatics require atom-centred charges. One such method to determine these atom-centred charges from density functional theory (DFT) calculations is the density-derived atomic point (DDAP) charge method. DDAP fits atom-centred Gaussians to the ground-state DFT charge density and preserves the multipole moments that govern long-range electrostatics. While these charges accurately predict long-range behaviour, in practice, they are limited by their reliance on fixed, heuristic parameters and a constrained solver that becomes numerically unstable for complex or covalent systems. In this work, we present opt-DDAP, which solves this limitation by reformulating the
algorithm as a differentiable computational graph. This reformulation allows for the optimisation of Gaussian basis parameters and the reciprocal-space cutoff using automatic differentiation. To ensure numerical robustness through this automatic differentiation process, we replace the conventional Lagrange-multiplier approach with a pseudo-inverse solution followed by charge renormalisation, maintaining stability even in the presence of ill-conditioned
matrices. We validate the framework on NaCl vacancy supercells and on MoS$_2$, demonstrating faithful reconstruction of both absolute and difference charge densities. The optimised charges are intended to serve as inputs to effective electrostatic models in machine-learning and empirical interatomic potentials that incorporate long-range interactions.
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Fluid Dynamics
Non-Monotonic Marangoni Suppression of Hydrodynamic Coarsening in Bicontinuous Liquid-Liquid Phase Separation
Tian Liu, Haohao Hao, Jiaxi Liu et al. (+3 more)
Hydrodynamic coarsening of bicontinuous domains is a central process in
liquid-
liquid phase separation, yet how soluble surfactants regulate this process remains poorly understood. Using a validated two-order-parameter phase-field model coupled to the incompressible Navier-Stokes equations, we show that hydrodynamic coarsening is suppressed primarily by surfactant-induced Marangoni stresses rather than by the reduction of mean interfacial tension alone. These stresses hinder interfacial coalescence, reorganize the local vortical flow, and thereby redirect the morphological
evolution of bicontinuous domains. A central result is that this suppression depends non-monotonically on the surfactant Péclet number, with the strongest inhibition occurring at an intermediate value, $Pe_\psi=10$, rather than at $Pe_\psi=1$ or 100. Analyses of force
evolution, interfacial surfactant statistics, and decomposed surfactant flux budgets show that this non-monotonicity arises from a competition between surfactant replenishment and gradient retention. At low $Pe_\psi$,
diffusion efficiently replenishes the interface but smooths interfacial concentration gradients; at high $Pe_\psi$, advection preserves interfacial heterogeneity but leaves the interface insufficiently supplied with surfactant. The strongest suppression therefore occurs when sufficient interfacial surfactant loading coexists with persistent concentration gradients. These results establish a transport-controlled mechanism by which soluble surfactants regulate bicontinuous hydrodynamic coarsening.
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All authors Tian Liu, Haohao Hao, Jiaxi Liu, Yongjie Zhou, Feiyu An, Huanshu Tan
Optics
Twist-Controlled Symmetry Breaking in Surface Phonon Polariton Moiré Metasurfaces
R. B. Iyer, S. H. Park, N. R. Sahoo et al. (+2 more)
Moire
lattices provide a powerful route for engineering emergent
symmetries and length scales through the relative rotation of periodic structures. However, their implementation in polaritonic systems remains relatively unexplored, and a general framework describing how twist modifies the interaction of optical modes in momentum space is still lacking. Here, we investigate how twist-induced moire periodicities can control
symmetry and momentum-space coupling in surface
phonon polariton (SPhP) metasurfaces. We fabricate twisted overlapping dual-grating metasurfaces on a polar dielectric substrate with dielectric overlayer and characterize their optical response using polarization-resolved
Fourier-transform infrared microscopy. Experimental measurements are combined with full-wave simulations and momentum-space analysis to identify the resonant SPhP and SPhP-like waveguide (WG) modes arising from both individual grating periodicities and emergent moire periodicities. The results reveal twist-controlled
symmetry breaking manifested as asymmetry between p to s and s to p polarization conversion, along with twist-dependent interactions between SPhP and SPhP-like WG modes. Our analysis reveals that the twist-engineered polarization-conversion asymmetry enables directional biasing of infrared radiative heat transfer. These findings establish twisted
phonon-polaritonic metasurfaces as a versatile platform for geometry-controlled
symmetry engineering in the mid-infrared. Future work may leverage such twist-programmable polaritonic interactions to enable directional thermal emission, polarization-selective detection, and reconfigurable infrared photonic devices.
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All authors R. B. Iyer, S. H. Park, N. R. Sahoo, T. Low, T. G. Folland
Geophysics · Cross-listed from cond-mat.stat-mech
Forecasting Return Time of Extreme Precipitation by Large Deviation Theory
Haotian Xie, Haoxian Liu, Jingfang Fan et al. (+1 more)
Forecasting extreme precipitation is essential yet challenging due to its rarity and complexity. We develop a large deviation framework to estimate the return times of extreme precipitation events. We first find that the Landau distribution, originally introduced in
plasma physics, accurately captures extreme precipitation at approximately 93% of global locations, outperforming conventional extreme value distributions with 76% matched locations under the same accuracy criterion. Enriching rare event samples by the fitted Landau distribution, we obtain more accurate estimates of large deviation rate functions and return times, enabling forecasts beyond historically observed precipitation intensities. Mapping historical return times to future projections from the Coupled Model Intercomparison Project Phase 6 (CMIP6), we show that return time curves under different emission scenarios collapse onto a unified relation, revealing a sharply increased lifetime exposure to extreme precipitation for 21st-century birth cohorts under most future emission scenarios.
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All authors Haotian Xie, Haoxian Liu, Jingfang Fan, Ying Tang
Optics
Ultrasensitive Nanoplastics Detection Leveraging Shrinking Surface Plasmonic Bubble
Yang Liu, Renzheng Zhang, Amartya Mandal et al. (+3 more)
Nanoplastics pose serious environmental and health risks due to their widespread presence in aquatic systems. Detecting trace amounts of nanoplastics is a challenging task, which currently requires sophisticated equipment and tedious sample preparation (e.g., ultrafiltration). In this work, we demonstrate an ultra-sensitive Shrinking Surface Bubble Deposition (SSBD) technique for nanoplastics detection. SSBD leverages plasmonic photothermal effects to generate a surface bubble and the resulting Marangoni flow to concentrate sparsely suspended nanoplastics onto the bubble surface. The collected nanoplastic particles are subsequently deposited on the substrate after the bubble shrinks and vanishes. To quantify the detection limit of SSBD for nanoplastics in water, core-shell gold plasmonic nanoparticles are mixed with the aqueous sample to enable photothermal bubble generation, while also supporting surface-enhanced Raman spectroscopy (SERS) for signal enhancement. Results show that the limits of detection are 10 ng/mL, 10-1 ng/mL and 10-3 ng/mL for polystyrene (PS) particles with diameters of 500 nm, 200 nm and 30 nm, respectively. We further used SSBD to detect plastics particles in real drinking water (e.g., bottled and fountain water) and found polyamides (PA) and polypropylene (PP) micro/nanoplastics, demonstrating the potential of the SSBD-SERS technique as a versatile and sensitive platform for detecting trace-level nanoplastic contamination and assessing human exposure risk.
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All authors Yang Liu, Renzheng Zhang, Amartya Mandal, Eungkyu Lee, Seunghyun Moon, Tengfei Luo