Atomic and Molecular Clusters · Cross-listed from cond-mat.mtrl-sci
Crystal Generation using the Fully Differentiable Pipeline and Latent Space Optimization
Osman Goni Ridwan, Gilles Frapper, Hongfei Xue et al. (+1 more)
We present a materials generation framework that couples a
symmetry-conditioned variational autoencoder (CVAE) with a differentiable SO(3) power spectrum objective to steer candidates toward a specified local environment under the crystallographic constraints. In particular, we implement a fully differentiable pipeline to enable batch-wise optimization on both direct and latent crystallographic representations. Using the GPU acceleration, this implementation achieves about fivefold speed compared to our previous CPU workflow, while yielding comparable outcomes. In addition, we introduce the optimization strategy that alternatively performs optimization on the direct and latent
crystal representations. This dual-level relaxation approach can effectively escape local minima defined by different objective gradients, thus increasing the success rate of generating complex structures satisfying the target local environments. This framework can be extended to systems consisting of multi-components and multi-environments, providing a scalable route to generate material structures with the target local environment.
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All authors Osman Goni Ridwan, Gilles Frapper, Hongfei Xue, Qiang Zhu
Chemical Physics · Cross-listed from quant-ph
Path Integral Lindblad Dynamics in Presence of Time-Dependent Fields
Amartya Bose
The path integral Lindblad dynamics (PILD) method [A. Bose, J. Phys. Chem. Lett. 15(12), 3363-3368 (2024)] had been introduced as a way of incorporating the impact of certain empirical processes like pumps and drains on the dynamics of
quantum systems interacting with thermal environments. The method being based on the time-translational invariance of the Nakajima-Zwanzig
memory kernel, however, was not able to account for time-dependent external fields. In this communication, we give an alternate, simpler formulation of PILD, that allows us to go beyond this limitation. It does not require the evaluation of the non-Markovian
memory kernel directly, and consequently can be applied to Floquet systems as well.
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Applied Physics
An Adaptive Power Division Strategy for Nonlinear Components in Rectification
Zhongqi He, Liping Yan and Changjun Liu
This letter presents a novel adaptive power division strategy, which uses two rectifying diodes with nonlinear impedance characteristics that are configured in parallel to function optimally at their individual power levels. Through the strategic adjustment of the input admittance, the conductance of the low-power diode decreases progressively with increasing power, while the conductance of the high-power diode increases correspondingly. This conductance-based power allocation method ensures that the power is rectified consistently by the most appropriate diode, regardless of the power level, and, thus, enables efficient rectification across an extended range. This letter presents a rectifier typology to substantiate the proposed strategy. Experimental results confirm the efficiency of the adaptive power division strategy, with the rectifier showing efficiency in excess of 60% from 5 to 29.5 dBm, giving a power dynamic range of 24.5 dB.
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Applied Physics
Reversible vertical positioning of acoustically levitated particle using a spiral reflector
Yusuke Koroyasu, Takayuki Hoshi, Yoshiki Nagatani et al. (+3 more)
Dynamic positioning in acoustic levitation typically depends on active control of the transducers phases, which necessitates complex driving electronics. While mechanically actuated reflectors offer a simpler alternative, achieving reversible transport along the vertical axis solely through mechanical actuation remains challenging. Here, we demonstrate vertical particle translation using a rotating spiral reflector with a half-wavelength pitch. With the rotation axis laterally offset relative to the acoustic focus, the spiral surface functions as a series of translating slopes. Experimental and numerical results confirm stable, bidirectional transport, yielding a vertical displacement of approximately $0.58\lambda$ per revolution and a maximum height of $3.18\lambda$, with radial confinement maintained within $0.24\lambda$. This approach provides a cost-effective solution for non-contact sample handling without active phase control.
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All authors Yusuke Koroyasu, Takayuki Hoshi, Yoshiki Nagatani, Daichi Tagami, Yoichi Ochiai, Tatsuki Fushimi
Fluid Dynamics
Low-wavenumber wall pressure fluctuations in turbulent flows within concentric annular ducts
Yaomin Zhao, Taiyang Wang and Benshuai Lyu
Compressible direct numerical simulations of turbulent channel flows in concentric annular ducts of height $2\delta$ are performed to study the low-wavenumber wall pressure fluctuations (WPF) over cylindrical walls at a bulk Mach number $M_b = 0.4$ and bulk Reynolds number $Re_b=3000$. The radius of the inner cylinder $R$ is varied between $0.2\delta$, $\delta$, $2\delta$ and $\infty$. As $R$ decreases, the one-point power spectral density of the WPF decreases at intermediate but increases at high frequencies. When $R$ decreases, the 1D (streamwise) wavenumber-frequency spectrum of the WPF decreases at high wavenumbers. At low wavenumbers, however, as $R$ reduces to $0.2\delta$ the 1D wavenumber-frequency spectrum exhibits multiple spectral peaks whose strengths increase with frequency. Examination of the 2D wavenumber-frequency spectra shows that these represent acoustic duct modes that closely match theoretical predictions. The acoustic modes of higher radial orders exhibit increasingly high amplitude on the inner than on the outer walls. The low-wavenumber components of the $0$th-order (azimuthal) 2D wavenumber-frequency spectrum are of great importance in practice, and their magnitude increases as $R$ reduces; this increase is increasingly pronounced at higher frequencies. Analytical modelling and numerical validation show that this increase appears to arise from the “
geometric” effects connected with the Green's function, and they are generated mainly by radial and azimuthal disturbances. Disturbances closer to the wall are shown to be increasingly important in WPF generation as $R$ reduces, which highlights a potential in WPF control using wall treatment on thin cylinders.
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Instrumentation and Detectors · Cross-listed from cond-mat.mtrl-sci
Spatial resolution(s) in atom probe tomography
Baptiste Gault, Frédéric De Geuser, Christoph Freysoldt et al. (+2 more)
Atom probe
tomography (APT) is often quoted to provide "atomic-scale" analysis of materials in three dimensions. Despite efforts to quantify APT's spatial resolution, misunderstanding remain regarding its true spatial performance. If the depth resolution was once reported to be 20 pm, quoting this value outside of its specific context is misleading and should be avoided. The resolution achievable in pure metals, at one specific location within one reconstructed
dataset, does not generally apply across materials or analysis conditions, or even throughout a single tomographic reconstruction. Here, we review various efforts at defining and measuring the spatial resolution in the study of single phase and single element materials - i.e. pure metals - in field-ion microscopy (FIM) and APT. We also report on the degradation of the resolution arising from ion optical devices used to improve the mass-resolution. We aim to offer some perspective as to how reported resolutions may be or may not be of any relevance to most of the materials characterisation efforts by APT, including cases of precipitates in a
matrix that emphasise the need to consider an effective resolution. Finally, we discuss concepts to improve the spatial accuracy of the technique in a relatively distant future.
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All authors Baptiste Gault, Frédéric De Geuser, Christoph Freysoldt, Benjamin Klaes, François Vurpillot
Classical Physics
On extracting momentum from supports: the bullet in the beam problem
Xiaoyu Zheng, Tianyi Guo and Peter Palffy-Muhoray
To gain insights into momentum transfer from the supporting environment, we consider the simple problem of a bullet, fired from below, into a wooden beam resting on two supports. The resulting upward velocity of the beam strongly depends on where the bullet enters the beam; this dependence is due to upward momentum extracted by the beam from its supports. Our simple example illustrates the momentum transfer mechanism exploited in the remarkable dynamics of the chain fountain.
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Physics and Society
Towards a Sociology of Sociology: Inequality, Elitism, and Prestige in the Sociological Enterprise From 1970 to the Present
Gavin Cook
There is a science of science and an informal economics of economics, but there is not a cohesive sociology of sociology. We turn the central findings and theoretical lenses of the sociological tradition and the sociological study of stratification inward on sociology itself to investigate how sociology has changed since the 1970s. We link two bibliometric databases to trace diachronic relationships between PhD training and publication outcomes, both of which are understudied in the science of science and sociology of science. All of sociology's top 3 journals remained biased against alum of less prestigious PhD programs, and while most forms of bias in elite sociological publishing have ameliorated over time, the house bias of the American Journal of Sociology in favor PhD alumnae of UChicago has intensified.
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Optics
Ultra-high performance microwave spectral filters using optical microcombs
David J. Moss
Microwave photonic (MWP) filters are essential components in microwave systems due to their wide bandwidth, low loss, and immunity to electromagnetic interference. A sharp transition band is critical for precise spectral shaping and interference suppression, yet conventional MWP filters face challenges in achieving both sharp transitions and high reconfigurability. Adaptive MWP filters with sharp transition based on a transversal filter structure using an optical microcomb source are demonstrated in this paper. Four different types of single-band MWP filters with roll-off rates up to ~32.6 dB/GHz and a minimum shape factor of ~1.15 are achieved. In addition, simply through designing tap coefficients, band-pass filters with tunable centre frequencies ranging from 5 GHz to 15 GHz and dual-band MWP filters with various filter response are demonstrated without changing any hardware, where sharp transition is also validated. The adaptive filters with sharp transition presented in this paper offer a stable and highly reconfigurable solution for applications requiring stringent spectral selectivity, such as next-generation wireless networks, high-resolution radar imaging, and advanced biomedical photonic sensing.
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Optics · Cross-listed from quant-ph
Increasing the secret key rates and point-to-multipoint extension for experimental coherent-one-way quantum key distribution protocol
Venkat Abhignan, Mohit Mittal, Aditi Das et al. (+1 more)
Using
quantum key distribution (QKD) protocols, a secret key is created between two distant users (transmitter and receiver) at a particular key rate.
Quantum technology can facilitate secure communication for cryptographic applications, combining QKD with one-time-pad (OTP) encryption. In order to ensure the continuous operation of QKD in real-world networks, efforts have been concentrated on optimizing the use of experimental components and effective QKD protocols to improve secret key rates and increase the transmission between multiple users. Generally, in experimental implementations, the secret key rates are limited by single-
photon detectors, which are used at the receivers of QKD and create a bottleneck due to their limited detection rates (detectors with low detection efficiency and high detector dead-time). We experimentally show that secret key rates can be increased by combining the time-bin information of two such detectors on the data line of the receiver for the coherent-one-way (COW) QKD protocol with a minimal increase in
quantum bit error rate (QBER, the proportion of erroneous bits). Further, we implement a point-to-multipoint COW QKD protocol, introducing an additional receiver module. The three users (one transmitter and two receivers) share the secret key in post-processing, relying on OTP encryption. Typically, the dual-receiver extension can improve the combined secret key rates of the system; however, one has to optimise the experimental parameters to achieve this within security margins. These methods are general and can be applied to any implementation of the COW protocol.
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All authors Venkat Abhignan, Mohit Mittal, Aditi Das, Megha Shrivastava
Fluid Dynamics
Numerical study on fast spectral evolution due to double resonance and applicability of generalized kinetic equation
Mitsuhiro Tanaka
It is known that for a two-layer fluid system, the kinetic equation governing the
evolution of the spectrum of the wave field given by the standard wave
turbulence theory (WTT) breaks down due to the existence of a "double resonance", and the spectrum can evolve on a time scale much faster than that predicted by the standard WTT. In this study, using a simplified model for a two-layer fluid system, the applicability of the generalized kinetic equation (GKE) for such a situation is examined numerically. It is shown that the GKE can reproduce the appearance of a sharp peak in the surface wave spectrum due to double resonance, but it overestimates the growth of the peak, consequently failing to quantitatively describe the temporal
evolution of the spectrum correctly, particularly near the double resonance point.
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Optics
Silicon photonic optical-electrical-optical converters based on load-resistor and current-injection operation
Masaya Arahata, Shota Kita, Akihiko Shinya et al. (+2 more)
Optical-electrical-optical (OEO) converters are key primitives for low-latency, energy-efficient photonic computing because they enable nonlinear activation and optical signal regeneration on chip. We report two monolithically integrated silicon-photonic OEO converters-load-resistor (high-speed variant) and current-injection (high-gain variant) types-fabricated at a silicon photonics foundry. Each device combines a germanium photodetector with a micro-ring modulator (MRM). The converters exhibit reconfigurable nonlinear transfer functions and measurable on-chip RF OEO gain. The RF OEO gain scales linearly with the MRM bias power, with slopes of 0.10 mW^-1 (load-resistor of 10 k{\Omega}) and 1.4 mW^-1 (current-injection), enabling a gain > 1 region at practical bias powers (~10 mW and ~1 mW, respectively). Eye diagrams confirm clear openings up to 4 Gb/s for a high-speed load-resistor variant with a 500-{\Omega} load. To the best of our knowledge, this is the first experimental demonstration of a monolithically integrated, foundry-fabricated silicon-photonic load-resistor type OEO converter exhibiting reconfigurable nonlinear transfer and on-chip RF OEO gain. In the carrier-injection device, the activation slope exceeds unity, yielding 3.9 dB extinction-ratio regeneration. Short-pulse measurements yield 3-dB bandwidths of 1.49 GHz, 160 MHz (load-resistor of 500 {\Omega} and 10 k{\Omega}), and 76 MHz (current-injection), consistent with the RF data. Energy analysis shows an energy-bandwidth trade-off (RC-limited for load-resistor vs. lifetime-limited for injection) and outline routes to sub-pJ/bit operation via reduced capacitance and improved EO efficiency. These results establish silicon-photonic OEO converters as compact, foundry-compatible building blocks for scalable optoelectronic computing and optical neural networks.
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All authors Masaya Arahata, Shota Kita, Akihiko Shinya, Hisashi Sumikura, Masaya Notomi
Fluid Dynamics
Impact force and spreading characteristics of droplet impact on cylindrical surfaces
Mengqi Ye, Tianyou Wang and Zhizhao Che
Droplet impact phenomena are ubiquitous in both nature and industry. Existing studies of droplet impact have focused on the kinematics of droplet impact on flat surfaces, whereas research on cylindrical surfaces remains relatively limited, particularly from a force-based perspective. Here, droplet impact on cylindrical surfaces is studied by numerical simulation, with particular
attention to the spreading behavior and impact force acting on the wall. In the deposition mode, a single peak appears in the impact force curve, which corresponds to the rapid transfer of the droplet's initial momentum. In the rebound mode, two distinct peaks are observed, and the second peak arises from the reaction force during the retraction process. Increasing the surface wettability causes the asymmetry coefficient, the ratio of the maximum spreading lengths in the azimuthal and axial directions of the cylinder, to first decrease and then gradually approach a constant, while the effect of the surface wettability on the initial impact force is negligible. As the Weber number We increases, the first dimensionless peak of the impact force $F_{p1}^{*}$ approaches a constant, and the relationship can be expressed as $F_{p1}^{*}={\beta}_1+{{\beta}_2}{{We}^{-1}}$ (where ${\beta }_1$ and ${\beta }_2$ are constants). The dimensionless maximum spreading area, dimensionless maximum spreading length, dimensionless maximum spreading angle, and asymmetry coefficient all exhibit power-law relationships with the Weber and Ohnesorge numbers. Furthermore, an increase in the diameter ratio of the cylinder and the droplet leads to a reduction in the asymmetry coefficient and an increase in the first dimensionless peak of the impact force.
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Optics
Self-heterodyne spectroscopy via a non-uniformly spaced frequency comb
Bofeng Zhang, Gang Zhao, Xiaobin Zhou et al. (+4 more)
Frequency comb spectroscopy has significantly advanced molecular spectroscopy across scientific research and diverse applications. Among its key performance metrics especially for time-resolved studies, sensitivity and measurement speed are paramount. However, a long-standing compromise between these parameters arises from the need for noise reduction. Here, we introduce a comb spectroscopy system that overcomes this limitation using a single frequency comb of non-uniformly spaced modes. The comb is generated using an extremely simple setup, composed of a continuous-wave (CW) fiber
laser and a single-sideband phase modulator (SSM). Our approach delivers optical-to-
radio-frequency conversion comparable to dual-comb spectroscopy (DCS) but through a simplified self-heterodyning architecture. By leveraging the intrinsic mutual coherence of the comb, this design achieves a noise-equivalent absorption coefficient (NEA) of 5.0*10^(-6) Hz^(-1/2)–an order-of-magnitude improvement over state-of-the-art DCS, coupled with long-term stability. The system resolves weak molecular overtone spectra on nanosecond timescales, in a single-shot measurement, at a signal-to-noise ratio of 128. This integration of high sensitivity, resolution, and speed resolves the core trade-off that has long constrained time-resolved spectroscopic analysis.
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All authors Bofeng Zhang, Gang Zhao, Xiaobin Zhou, Xiaojuan Yan, Jiaqi Yang, Weiguang Ma, Suotang Jia
Optics
Photonic Temporal Illusion
Grigorii Ptitcyn, Diego M. Solís, M. S. Mirmoosa et al. (+1 more)
Materials with unusual optical properties are central to advanced control of light. Yet, in nature, such materials may be exceedingly rare and often difficult to obtain. To overcome this limitation, here we introduce the concept of temporal illusion: A temporally dynamic framework in which carefully programmed temporal variations in effective parameters generate responses akin to those of, in principle, any arbitrary time-invariant structure. We theoretically demonstrate that proper modulation of the permittivity of a conventional dielectric in space and time replicates the optical behavior associated with exotic materials. Besides, we reveal that, beyond steady-state effects, temporal illusion also enables control over transient responses, for instance, by effectively lowering the time constant of high-quality-factor resonators, therefore, allowing faster energy accumulation. Moreover, by incorporating detuning between modulation and excitation, we show that the framework unlocks additional functionalities. The temporal illusion paradigm thus broadens the capabilities of space-time varying systems, offering a powerful route to synthesize material responses on demand and paving the way for new theoretical and experimental directions in optics and wave physics.
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All authors Grigorii Ptitcyn, Diego M. Solís, M. S. Mirmoosa, Nader Engheta