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Monday 31 August

Optics

Robust bistable vortex light bullets in graded-index multimode fibers

We explore theoretically the formation and evolution of spatiotemporal vortex bullets, pulses confined in both space and time while carrying orbital angular momentum, inside a graded-index multimode fiber. Through a two-fold approach, combining variational analysis with full numerical simulations, we establish the existence of a bistable vortex soliton family, characterized by distinct radial and azimuthal quantum numbers. These wave packets exhibit a Laguerre-Gaussian multi-ring topology in their spatiotemporal structure. We identify the experimental conditions necessary for the generation of such structured states of light. A stability analysis based on Vakhitov-Kolokolov criteria reveals an upper limit for the propagation constant, below which vortex bullets are found to be stable. Stationary and non-stationary dynamics of vortex bullets with different topological charges are analyzed fully, exploiting analytical techniques that are supported by full numerical simulations. These results enhance our understanding of self-trapped, spatiotemporal vortex solitons in a graded-index medium and may lead to potential applications in the area of classical and quantum information processing.
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All authors Ashis Paul, Anuj P. Lara, Govind P. Agrawal, Samudra Roy

Optics · Cross-listed from cond-mat.mes-hall

Coexistence of polariton bound states in the continuum and 2D radiative excitons

Bound states in the continuum (BICs) enable optical modes with ideally infinite radiative lifetimes despite lying within the radiation continuum. Radiation-matter interaction in periodically patterned planar waveguides embedding two-dimensional (2D) optically active excitations can be described quantum mechanically by diagonalizing a non-Hermitian operator, known as the Hopfield matrix, which can be generalized to incorporate independent photonic and excitonic losses into the polaritonic states. However, since 2D excitons undergo intrinsic wavevector-dependent radiative decay within the light cone, whether the Hopfield formalism can consistently account for this process while preserving polariton BICs has remained an open question. Here we show that a non-Hermitian Hopfield formalism incorporating excitonic radiative losses correctly captures the existence of genuine $k=0$ polariton BICs with diverging radiative lifetimes. The theory provides a unified microscopic framework for radiative excitons and polariton BICs, and an efficient predictive tool for designing photonic-crystal platforms coupled to quantum wells, transition-metal dichalcogenides, and other 2D excitonic materials.
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All authors Simone Zanotti, Marco Liscidini, Dario Gerace, Lucio C. Andreani

Optics

Complex-gate all-optical frequency-resolved optical gating for ultrabroadband isolated attosecond pulse characterization

We experimentally demonstrate all-optical frequency-resolved optical gating (AO-FROG) for the characterization of ultrabroadband isolated attosecond pulses (IAPs) generated by a mid-infrared sub-cycle laser field. By extending the AO-FROG framework beyond the conventional phase-only modulation approximation, we develop a strong-field approximation (SFA)-based theoretical framework and show that the weak perturbing field induces both phase and amplitude modulations during high-order harmonic generation. A complex-valued gate function is therefore required for accurate pulse reconstruction. Using a 2.26-$\mu$m sub-cycle driving laser, we characterize IAPs spanning 100-180 eV in argon. The measured AO-FROG traces exhibit delay-dependent spectral modulations arising from perturbation-induced modifications of the electron trajectories and ionization probability. SFA simulations reproduce the experimental observations and confirm the importance of including ionization-induced amplitude modulation. The reconstructed temporal and spectral properties reveal an IAP duration of approximately 300 as and its spectral phase, providing access to the attosecond chirp of the generated pulses. Our results establish AO-FROG as a promising approach for temporal characterization of ultrabroadband attosecond sources driven by long-wavelength infrared fields.
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All authors Minshuang Xia, Kaito Nishimiya, Dianhong Dong, Yuxi Fu, Eiji J. Takahashi

Optics · Cross-listed from eess.SP

Leveraging Bayesian Optimization for Array Shape Self-Calibration in Underwater DoA Estimation

Flexible sensing arrays are commonly used in underwater acoustic networks, but suppressed by unpredictable geometric deformations. Existing array shape self-calibration methods often estimate individual element positions separately, leading to a high dimensional optimization problem over long arrays. To address this problem, this paper proposes a Bayesian Optimization-assisted Geometry Estimation (BOGE) strategy operating with a hierarchical optimization process and a physics-informed parametric model for array geometry correction. BOGE formulates array shape self-calibration as an optimization problem, where candidate geometries are evaluated by the noise subspace residual. We perform Bayesian optimization to configure the physics-informed parametric model and then refine the selected geometry through numerical optimization. Empirical results show that BOGE achieves lower mean geometric root mean square error (RMSE) than the benchmark methods across a wide range of noise levels. On the public SWellEx-96 dataset, BOGE achieves a geometric RMSE of $0.659$ meters at $166$ Hz. A lake trial further shows that BOGE provides fixed source localization and moving target tracking performance comparable to the comparison methods.
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All authors Xin Gui, Tianang Li, Changjia Wang, Bowen Han, Yunchuan Zhang, Zhengying Li

Optics

Ghost infrared spectroscopy with bright twin beams

Frequency-correlated light offers a route to mid-infrared (MIR) spectroscopy without direct spectral detection in the MIR. Previous MIR ghost spectroscopy has mainly relied on low-gain spontaneous parametric down-conversion (SPDC) and photon-pair coincidence measurements, where the limited photon flux has restricted acquisition times to longer than one minute. Here, we demonstrate ghost infrared spectroscopy using bright twin beams generated by high-gain parametric down-conversion (PDC). High-gain PDC amplifies vacuum fluctuations, producing a different pair of frequency-correlated random spectra in each pump pulse. This pulse-resolved stochastic emission is naturally matched to time-stretch detection, which records the spectrum of the correlated near-infrared telecom signal for every pulse, while the MIR idler is measured by bucket detection. Consequently, each pump pulse yields one paired projection measurement comprising a spectrally resolved reference and the corresponding bucket value. We reconstruct the transmission spectrum of a structured optical filter and the molecular vibrational absorption spectrum of liquid benzene near 3.3 um with millisecond-scale acquisition, in good agreement with Fourier-transform infrared spectroscopy. This reduces the acquisition time by four to five orders of magnitude compared with previous MIR ghost spectroscopy demonstrations. These results transform ghost spectroscopy from coincidence-based photon counting to high-flux analog correlation spectroscopy, establishing a practical architecture for high-speed computational infrared spectroscopy driven by a narrowband semiconductor laser.
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All authors Akira Kawai, Makoto Shoshin, Kazuki Hashimoto, Takuro Ideguchi

Optics

Spatially or temporally resolved phase-based optoretinography with actively-tracked point-scanning optical coherence tomography

Optoretinography is a promising approach to measure visual function but its clinical translation has remained confined to research settings due to demanding hardware requirements. Here, we demonstrate that high-quality phase-based optoretinography can be performed using conventional point-scanning spectral-domain optical coherence tomography. We show that the need for high imaging speed can be circumvented by accurate sampling of phase changes at consistent spatial location. Light-evoked outer-segment expansion could be temporally resolved in B-scan series acquired at a fixed position when filtering off-location B-scans, and spatially resolved in volumes acquired at rates as low as 1~Hz. These results indicate that the technical barrier for phase-based optoretinography is substantially lower than previously assumed and pave the way toward broad clinical translation.
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All authors Léo Puyo, Jonas Franke, Felix Zeisberger, Roland Rocholz, Gereon Hüttmann

Optics · Cross-listed from quant-ph

Quantum-interference metrology of dissipative Kerr solitons

Dissipative Kerr solitons in optical microresonators underpin chip-scale frequency combs with applications ranging from coherent telecommunications to precision spectroscopy. Yet the characterization of their intrinsic femtosecond temporal structure remains challenging, as the low pulse energy and broad spectral bandwidth necessitate optical amplification and careful dispersion compensation in conventional ultrafast diagnostics, both of which can significantly distort the waveform. Here we demonstrate a quantum-interference metrology of microcomb solitons based on Hong-Ou-Mandel interference. By attenuating the soliton stream to the single-photon level and measuring fourth-order interference, we directly retrieve near transform-limited pulse durations without amplification or dispersion management, remaining accurate even after propagation through 25 km of standard fiber. The same interferogram also provides direct access to the temporal separations in multi-soliton states by converting inter-soliton separations into additional interference dips at corresponding delays, enabling sub-picosecond characterization of their intracavity temporal structure. This quantum-inspired paradigm introduces a fundamentally new metrological approach that is immune to amplification and dispersion distortions, offering a powerful tool for the characterization of complex soliton physics.
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All authors Yun-Ru Fan, Yong Geng, Ji Liu, Yong-Jun Huang, Hai-Zhi Song, Hao Li, Li-Xing You, Heng Zhou, Kun Qiu, Kai Guo, Guang-Can Guo, Qiang Zhou

Optics

Sensitivity Comparison of Microwave-Frequency and Optical Fibre Interferometry Based on State-of-the-Art Components

We compare the sensitivity of fibre interferometers to vibrations using microwave oscillators and state of the art lasers over distances up to 70 km. High spectral purity lasers outperform only above 10 Hz, highlighting microwave advantages at low frequencies and the potential of hybrid microwave optical interferometry systems
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All authors Georgios Aias Karydis, Marco Fasano, Paola Parolari, Pierpaolo Boffi, Charis Mesaritakis, Adonis Bogris

Optics

Revealing antenna-molecule coupling using virtual gain from synthetic complex frequency analysis

Synthetic complex frequency waves (CFWs) enhance spectral and spatial resolution by compensating loss through virtual gain. This approach is particularly useful in nano-photonics where loss is intrinsically linked to strong field confinement and system size. Here, we apply CFWs to metasurfaces composed of Fano-resonant plasmonic antennas with lithographically tunable coupling between the weak and strong coupling regimes and where loss may be reduced to the Drude damping limit. We quantitatively assess the impact of the virtual gain to find that, while reducing loss, internal coupling rates remain invariant. While the exceptional point associated with strong light-matter coupling is invariant under virtual gain, the cooperativity of Fano interference is enhanced. When the metasurfaces are functionalised with a molecular monolayer, CFWs are thus able to reveal a molecule's vibrational modes, even when obscured by loss, and allow direct extraction of the plasmon-molecule coupling strength. We thus use CFW analysis as a quantitative tool for revealing and assessing light matter-coupling.
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All authors Toby Severs Millard, Xiaofei Xiao, Mayela Romero-Gómez, Tom Aktaş-Vincent, Nathaniel J. Huáng, Chris C. Phillips, Stefan A. Maier, Olga Kazakova, Rupert F. Oulton

Optics

All-optical reconstruction of valley polarization through helicity-resolved high-harmonic generation

We theoretically investigate valley-resolved high-order harmonic generation in gapped graphene driven by elliptically polarized laser fields. Using two-band density-matrix simulations and an electron-hole recombination trajectory model, we find that the two inequivalent valleys emit harmonics with opposite helicities. Under an elliptically polarized field, these emissions occur predominantly in different half cycles of the laser field. Time-dependent density functional theory calculations for monolayer MoS$_2$ show the same temporal separation of harmonic emissions with opposite helicities, supporting the generality of this valley-dependent chiral response. We further propose an all-optical scheme to reconstruct valley polarization from helicity-resolved harmonic signals. A circularly polarized pulse first prepares a valley population imbalance. A subsequent elliptically polarized laser induces different changes in the harmonic intensities of opposite helicities through Pauli blocking. The ratio of these intensity changes provides a direct measure of the valley polarization. Our results demonstrate that chiral high-harmonic emission can serve as an all-optical probe of ultrafast valley-dependent carrier dynamics.
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All authors Xiaoyu Bu, Yan Meng, Xiaohui Zhao, Rongxiang Zhang, Fulong Dong

Sunday 30 August

Optics · Cross-listed from cond-mat.soft

Birefringent-colored optical profiling of wood presenting the 3D cellulose microfibril architecture

Wood slices under a polarized optical microscope show a spectrum of interference colors, such as cyan, blue, magenta, yellow, and bluish gray because of the birefringent cellulose in the microfibrils. An optical model is established to simulate the birefringent-colored micrograph of wood. Five typical cell wall architectures, line, helix, ring, crossed helix, and twisted helix, are considered. With a retardation wave plate to distinguish fibrils of different orientations, each structure displays its unique birefringent-colored texture, presenting its underlying 3D structure with the vivid colors. Cross sections of the trunk and twig of Eucalyptus grandis presented birefringent-colored profiles. Three identification methods were compared: visible fibril trends, birefringent-colored optical textures, and the simulated look-up library. The three methods gave consistent results, proving that the birefringent-color tags are efficient and accurate. Electron and atomic force microscopy are unable to resolve cellulose microfibrils embedded in the lignin and hemicellulose matrix. Polarized optical microscopy overcomes this by selectively detecting birefringent cellulose, enabling accurate identification of complex helical structures. This method enables statistical and spatial analysis of complex biomaterial compositions. Capable of profiling dozens of cells simultaneously, this high-throughput optical method provides a potentially fully automated analysis framework for plant science, biomechanics, and bioinspired cellulose materials.
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Optics · Cross-listed from cond-mat.soft

Chiral cellulose fibril organization in a plant cell wall as liquid crystal confined in a cylindrical boundary

The order of cellulose microfibrils in xylem cell walls is identified using polarized optical microscopy. The line, helix, ring, crossed helix, and twisted helix organizations in a cylindrical shell are the equilibrium states of balanced elastic deformation and surface anchoring. A computational model of the five organizations is established to simulate their birefringent-colored profiles. These five textures present unique optical textures, which are clearly recognized in the cross sections of Eucalyptus grandis. The libriform fiber cell for support has a twisted helical cell wall. The vessel cell for high-speed water uptake consists of a helical layer covered by a layer of vortex array. The ray cell for radial transportation is crossed helical. The microfibril angles versus the radius of the cell wall were measured utilizing the distribution of birefringence colors. In fiber cell walls, the MFA is significantly correlated with the curvature, bending, and surface anchoring, respectively. In vessel cell walls, the vortex array includes focal conic domains of chiral order and topological defects of nematic order, suggesting that the phase transition of cellulose fibrils leads to pattern formation. Liquid crystal phases and patterns in the cell walls reveal how the cell wall thickens and how cells differentiate. Out of the frustration of long, stiff, twisting fibrils packed in slender tubes, trees generate the helical channel networks, transforming the brittle lamina into an elastic, tear-resistant, self-healing tissue.
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All authors Jieh-Wen Tsung, Bo-Hsien Wu, Li-Yan Hung, Yu-Chieh Huang, Yueh-Ching Huang, Shao-Chun Hsieh

Optics

Controlling the Coupling Strengths in Nanophotonic Networks using Modified Yagi-Uda Nanoplasmonic Antennas

On-chip communication in optical neural networks is commonly done via waveguides which results in large system footprints. A compact alternative is to broadcast light signals between nano-optoelectronic components in free space and tailor the light field distribution using sub-wavelength nanophotonics. We propose and simulate nanoplasmonic metal structures in combination with III-V nanowire emitters and receivers to create an optical network in which the shape and position of these nanostructures create varying weights between the nano-optoelectronic nodes. Using Finite Difference Time Domain modelling, we investigate systems of experimentally verified nanowire optoelectronics combined with nanoplasmonic structures that can be made in the same fabrication step as electrical contacts powering the nanowires. We investigate both individual nanowire/antenna devices as well as networks corresponding to two layers in a neural network. We show that directed communication from a nanowire node can be significantly altered using Yagi-Uda antennas. Modifying the antenna with an asymmetric director component enables the directing of light several different angular directions simultaneously. We find that highly variable complex weight distribution between the connections in two seven node layers can be achieved depending on the combined geometry of the antenna components. The possible weight distributions in compact layers of nanowire nodes could be used for creating a variety of neural networks with complex connectivity. The concepts can be generalized to other types of nanoscale emitter/receiver systems.
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Optics

Magneto-optical intensity effect in a transparent perforated all-dielectric metasurface with an anapole state

We numerically study a perforated all-dielectric metasurface based on the magnetic semiconductor GaMnAs. Near the anapole state, the structure combines high transmittance with a moderate magneto-optical intensity effect. The absolute transmission modulation is enhanced by about a factor of five compared with a smooth film, while the metasurface transmittance reaches 81%. The enhancement is associated with strong field localization in the magneto-optically active material and suppression of the electric-dipole radiation channel in the anapole regime.
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All authors Polina V. Zorina, Andrey N. Kalish, Vladimir I. Belotelov, Venu Gopal Achanta, Daria O. Ignatyeva

Optics

Localization in microcavities revealed by phase-space non-Hermitian skin effect

Contrary to the semiclassical expectation for fully chaotic systems, localization of resonances is found to be a common feature in open microcavities. In spiral-shaped dielectric microcavities, a substantial fraction of resonances localize on polygonal patterns in real space, are chiral, and their momentum distributions accumulate near the critical line for total internal reflection. Despite the extensive investigation, the physical mechanism responsible for their remarkable abundance has remained a long-standing question. Addressing this, we reveal a physical correspondence between an inhomogeneous-loss Hatano-Nelson model and the dielectric phase space of a spiral microcavity. We show that the combination of geometry-induced momentum drift and refractive escape yields a generalized non-Hermitian skin effect in the phase space momentum. We identify this mechanism as the origin of the critical-line localization of resonances in open chaotic spiral microcavities, extending the skin-effect concept beyond nonreciprocal lattices to phase space and to open chaotic wave systems.
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All authors Jung-Wan Ryu, Yong-Hoon Lee, Muhan Choi, Chang-Hwan Yi, Martina Hentschel

Optics · Cross-listed from physics.ins-det

A high-speed anamorphic pupil-conjugate slit spectrograph for rapid, self-luminous sources

We present a slit imaging spectrograph whose wavelength registration is a property of the instrument rather than of the pointing of the fore-optic or the position of the source. An internal telecentric 4f relay places the system stop within the instrument while a cylindrical lens places the slit aperture at a plane where transverse position encodes source angle only (an $A = 0$ conjugate in the ABCD matrix formulation). As a result, the lateral motion of the source or the pointing of the fore-optic does not cause the spectral image illuminating the sensor to wander, thus eliminating any non-physical registration of chemical species not present in the event and the need for on-the-fly recalibration. Additionally, the use of a high-speed CMOS camera eliminates temporally averaged spectral lines and aliasing noise. We characterize wavelength calibration (He discharge lamp, quadratic fit, RMS residual 0.12 nm, verified with Ne discharge lamp, same calibration, RMS residual 0.13 nm), spectral resolution (R $\approx$ 639, FWHM 0.92 nm at the optimal slit width setting, R $\approx$ 783, FWHM 0.75 nm at the instrument profile floor), and pointing invariance (He 587.6 nm line wander 0.29 nm RMS, 1.03 nm peak-to-peak, a nearly 100x reduction relative to the same instrument with the aperture stop at the fore-optic pupil). We perform combustion spectroscopy on ignited nitrocellulose at 10 kHz, 99 $\mu$s exposure time, identifying Na, K, Ca, CaOH, and Rb chemical species using the unchanged wavelength calibration transferred from the helium discharge lamp.
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Optics · Cross-listed from physics.comp-ph

Characteristic Mode Analysis of Composite Nanostructures using a Coupled System of Volume Integral and Hydrodynamic Equations

Full-structure and sub-structure characteristic mode analysis (CMA) formulations are developed for composite metallic–dielectric nanostructures based on a coupled system of volume integral equations (VIE) and the hydrodynamic equation (HDE). In the full-structure CMA, the generalized eigenvalue equation (GEE) is constructed from the matrix of the complete coupled system, and the resulting characteristic currents describe the response of the entire composite nanostructure. In the sub-structure CMA, the GEE is constructed from a reduced system, derived from the coupled system by eliminating the dielectric-region unknowns, so that it is expressed only in terms of the metallic-region currents. This isolates the resonances of the metallic region while still incorporating the effect of the dielectric region through the reduced system. Because the reduced system has a smaller dimension, the sub-structure CMA is computationally more efficient than the full-structure CMA and, when the dielectric does not resonate in the frequency range of interest, identifies the same resonances. Both formulations are validated against extinction cross-section (ECS) results and are used to characterize how a dielectric environment reshapes the metallic resonances, including substrate-induced red-shifts and, for high-contrast substrates in direct contact, hybridized modal responses.
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All authors Meruyert Khamitova, Ran Zhao, Doolos Aibek Uulu, Sebastian Celis Sierra, Hakan Bagci

Optics · Cross-listed from quant-ph

Thresholdless dynamical instability in transverse $\mathcal{PT}$-symmetric scattering systems: The hidden role of bound states in the continuum

The stationary scattering properties of transverse parity-time ($\mathcal{PT}$) symmetric systems have been extensively studied, yet their dynamical stability, a prerequisite for any stationary description, remains largely unexplored. Here we uncover a thresholdless dynamical instability in such systems, driven by symmetry-protected bound states in the continuum (BICs). Without gain and loss, the up-down mirror symmetry of the transverse geometry generically protects a BIC, which manifests as the coalescence of an $S$-matrix pole and zero on the real axis of the complex wave-number plane. A Hermitian symmetry-breaking perturbation shifts the poles into the lower half-plane, converting the BIC into a resonance with a Fermi-golden-rule decay width. An anti-Hermitian $\mathcal{PT}$-symmetric perturbation instead reverses the sign of the second-order energy shift, driving the poles into the upper half-plane and producing a time-growing bound state with $\operatorname{Im}E=\gamma^{2}\Gamma_{V}/2+O(\gamma^{3})$, where $\gamma$ is the gain-loss strength and $\Gamma_{V}$ is the golden-rule coupling of the BIC to the continuum. The instability therefore sets in at arbitrarily small $\gamma$ whenever $\Gamma_{V}>0$. We confirm this mechanism in a three-site side-coupled model that is unstable despite possessing a unitary scattering matrix, and in a four-site rhombic model where transverse and longitudinal gain-loss placements yield vanishing and finite thresholds, respectively. These results establish a microscopic stability criterion and a design principle for stable $\mathcal{PT}$-symmetric scattering devices.
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Optics

Programmable generation of optical skyrmions on a silicon photonic chip

Optical skyrmions, characterized by topologically stable and spatially varying polarization textures, show immense potential for robust optical communications and metrology. However, conventional methods for generating optical Stokes skyrmions rely on bulky free-space optics, strictly constraining both system miniaturization and dynamic reconfigurability. Here, we demonstrate the efficient and programmable generation of optical skyrmions and bimerons using a compact silicon photonic chip. By integrating a programmable Mach–Zehnder interferometer mesh with a multi-dimensional grating emitter, we dynamically control the amplitudes, phases, and polarizations of emitted fundamental and orbital angular momentum modes. This architecture allows on-demand electrical switching among a complete library of optical quasi-particle states, including Néel, Bloch, intermediate, and anti-type skyrmions and bimerons. Experimental full-Stokes polarimetry confirms high-fidelity polarization textures with near-unity skyrmion numbers. Our foundry-compatible platform translates complex topological light generation into simple voltage controls, paving the way for next-generation communication and sensing systems based on optical skyrmions.
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All authors Mingyuan Zhang, Xiaofu Pan, Wu Zhou, Wenzhang Tian, Zengqi Chen, Yiou Cui, Yijie Shen, Yeyu Tong, Jianqi Hu

Saturday 29 August

Optics

Reliable iToF Depth Sensing via Sensor-Intrinsic Uncertainty Modeling and State-Space Restoration

Indirect time-of-flight (iToF) cameras provide compact and cost-effective dense depth measurements, but their ranging accuracy is often degraded by sensor-intrinsic uncertainty under practical imaging conditions. Spatially uniform or range-only Gaussian perturbations cannot accurately reproduce the range-dependent and signal-dependent noise characteristics of real iToF measurements, leading to a synthetic-to-real gap for learning-based restoration. To address this problem, we propose a joint depth-uncertainty modeling and restoration framework for reliable iToF sensing. A sensor-intrinsic depth-uncertainty model is first developed from calibrated tap responses, returned-signal levels, and sensor noise statistics through a depth-oriented weighted least-squares formulation. The resulting pixel-wise uncertainty is used for heteroscedastic depth synthesis and uncertainty-aware restoration supervision. Based on this heteroscedastic data synthesis, we further develop a U-shaped restoration network with Depth Visual State Space (DVSS) blocks, which combine long-range state-space modeling with convolutional spatial-channel refinement for structure-preserving depth recovery. Experiments on synthetic data and measurements captured by an in-house iToF prototype validate the proposed uncertainty model under varying range and returned-signal conditions. Controlled comparisons with fixed and range-aware Gaussian noise, together with evaluations on U-Net, Restormer, and DVSS, further demonstrate that the proposed synthesis consistently benefits different restoration backbones. The complete framework achieves 40.85~dB PSNR and 2.54 mm MAE on the synthetic test set, and 35.42 dB PSNR and 4.87 mm MAE on real iToF measurements.
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All authors Yansong Du, Yutong Deng, Yuting Zhou, Zhancong Xu, Yingjia Lu, Mengdi Wang, Feiyu Jiao, Bangyao Wang, Zhaoxiang Jiang, Xun Guan

Optics

Artificial Intelligence in a Photonic Temporal Processor

Optical neural networks (ONNs) promise high-throughput and energy-efficient artificial intelligence, yet essentially all implementations so far encode information across space either in free-space arrays or in integrated waveguide meshes, tying the number of neurons to the number of physical components and fixes the routing topology at fabrication. Here we show that moving the computation into time decouples computational dimension from hardware dimension. Exploiting space-time duality, we implement optical diffraction and interference entirely in time domain, using thin-film lithium niobate modulators as time lenses and temporal masks, with chromatic dispersion providing the coupling between successive temporal neurons. We experimentally verify high-order, complex-valued matrix-matrix multiplications using just a single optical input/output port, scaling the computational dimensions far beyond the channel count. By incorporating optical feedback, we extend this platform into versatile neural networks, where the network layers, neuron numbers, and synaptic connections are fully programmable and in-situ trainable. Our temporal diffractive neural networks are successfully validated on various classification benchmarks, alongside image and video generation tasks. Notably, using this platform we demonstrate an all-analogue generative pipeline in which the latent variable is drawn directly from amplified spontaneous emission, so that no digital sampling or electronic modulation appears anywhere in the generative path. Furthermore, high-resolution images and videos are generated at high frame rates, outperforming state-of-the-art modulator-refresh-limited optical generative systems. These results establish a unified photonic temporal computing framework, providing a scalable and deployable pathway toward next-generation machine intelligence.
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All authors Youlve Chen, Jinlong Xiang, Yimin Hu, Yuchen Yin, Chaojun Xu, Zhengshun Lei, Xin Wang, Yufeng Zhang, Yixiao Zhu, Qunbi Zhuge, Junwen Zhang, Wei Chu, Tao Lin, Yikai Su, Zhipei Sun, Xuhan Guo

Optics · Cross-listed from physics.app-ph

Advancing Lead-Free FASnI3 Perovskite Solar Cells via Cu-Doped NiOx HTL Engineering: An Optoelectronic Analysis

Efficient lead-free perovskite solar cells remain limited by inefficient charge transport and significant recombination losses. In this work, copper (Cu) doped nickel oxide (NiOx) is employed as the hole transport layer (HTL) in a formamidinium tin iodide (FASnI3) perovskite solar cell to improve hole extraction and suppress carrier losses. The optoelectronic response of the proposed device architecture is evaluated through a coupled numerical framework combining finite-difference time-domain (FDTD) optical simulations with finite element method (FEM)-based electrical modeling. Electrical analysis solves the Poisson equation together with the drift-diffusion and carrier continuity equations, while accounting for radiative, non-adiative, and interfacial recombination mechanisms. Systematic optimization of the thicknesses and doping concentrations of the constituent layers was performed to establish a high-performance device configuration. Following optimization of layer dimensions and carrier densities, the device achieved a power conversion efficiency (PCE) of 24.71%. Integrating an anti-reflection coating (ARC) effectively suppressed reflection losses, yielding a 5.47% relative enhancement in PCE. Consequently, the optimized device achieved a peak PCE of 26.06%, with a short-circuit current density (Jsc) of 28.98 mA/cm2, an open-circuit voltage (Voc) of 1.051 V, and a fill factor (FF) of 85.64%. These findings demonstrate that Cu-doped NiOx functions as a highly promising HTL to boost charge collection and maximize overall efficiency in lead-free FASnI3 solar cells.
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All authors Md. Faiaad Rahman, Jabed Hasan, Md. Ashaduzzaman Niloy, Ahmed Zubair

Optics · Cross-listed from cond-mat.mes-hall

Quantitative Disentanglement of Terahertz Spin and Orbital Pumping in 3d Ferromagnetic Heterostructures

Spin and orbital pumping - the injection of spin and orbital angular momentum from a driven ferromagnet into an adjacent nonmagnetic layer - are fundamental processes underlying angular-momentum generation and transport in magnetic heterostructures. Femtosecond optical excitation extends these phenomena into the ultrafast regime, where spintronic terahertz emission spectroscopy (STES) detects picosecond angular-momentum currents in a contact-free manner through spin-to-charge and orbital-to-charge conversion. Microscopic theory predicts that orbital-pumping efficiency increases from Fe to Ni across the 3d series, yet whether these predictions hold under ultrafast excitation remains unclear. A central challenge is that spin and orbital currents are generated simultaneously and contribute additively to the same terahertz emission, preventing their quantitative separation. Here, we overcome this limitation by combining STES with wedge-sample thickness control in heterostructures whose nonmagnetic layers (Ta, W, and Nb) have spin Hall and orbital Hall angles of opposite signs. The two angular-momentum channels therefore exhibit distinct emission polarities and thickness dependences, enabling their quantitative decomposition. Systematic measurements on Fe, Co, and Ni heterostructures reveal that the orbital-pumping contribution increases progressively toward Ni, reaching several tens of percent of the spin-current contribution - far exceeding theoretical predictions. Even Fe generates a non-negligible orbital current that becomes essential in the thin-nonmagnetic-layer regime. The extracted orbital diffusion lengths are consistently shorter than spin diffusion lengths and increase with decreasing spin-orbit coupling strength of the nonmagnetic layer. These results establish a quantitative framework for ultrafast spin and orbital pumping in magnetic heterostructures.
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All authors Tongyang Guan, Jiahao Liu, Yuxiao Mo, Liangliang Zhu, Yizheng Wu, Zhensheng Tao

Friday 28 August

Optics

First-return statistics and the point-spread function of a Henyey-Greenstein random walk - a far-field stable law

A particle launched normally into a half space, scattering by the Henyey-Greenstein (HG) phase function, exits after a first-return time whose count of flights n approaches the distribution-free Sparre Andersen exponent, f(n) ~ n^{-3/2}, with an amplitude fixed by the launch rather than by the theorem. Conditioned on n, and past a correlation-set transient, the lateral exit position is Gaussian with variance proportional to n, a scaling we test directly. Subordinating that Gaussian displacement to the one-sided 1/2-stable first-return time gives, in the diffusion limit, an isotropic 1-stable scaling limit: the far tail of the point-spread function (PSF) for a normally incident pencil beam is the two-dimensional Cauchy tail p(r) ~ r^{-3}, the large-radius limit of the half-space Poisson kernel. The index alpha = 1 is the product of the central limit theorem and the distribution-free first-return exponent, so no phase function admitting the same diffusion limit - finite step variance, short-range angular correlation - can move it. Absorption weights each path by exp(-mu_a L) in its total length L, truncating the subordinator and producing the screened radial structure (mu_eff + 1/r) exp(-mu_eff r)/r^2 carried by each source term of the Farrell-Patterson-Wilson (1992) diffusion dipole; the finite-depth two-source dipole is not derived here. Keeping the launch-depth factor that the tail calculation discards continues the same kernel into a finite core of radius 1.7 l*, with no additional fitted parameter. A scale-dependent index alpha_eff from the empirical characteristic function tracks the similarity parameter gamma, separating phase functions matched in g_1 by 0.15-0.22 near one transport mean free path. Results are Monte Carlo at g = 0 to 0.9 with up to 10^6 walkers.
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Optics

Defects encode high-dimensional topological information

In polarization fields, Stokes skyrmions are continuous vectorial textures that encode integer-valued topological invariants across real space, enabling robust optical information encoding under complex perturbations. This topological resilience, however, fails when singular points occur where the Stokes vector has no unique limiting value, placing a fundamental constraint on skyrmion-based information manipulation. Here, we show, paradoxically, that the very defects that destroy conventional resilience can become the carriers of topological information. We introduce the resulting structures as Stokes defect skyrmions, in which singular Stokes responses constitute measurable topological degrees of freedom with theoretically minimal size. We design and realize one class of them using all-dielectric metasurfaces that combine arbitrarily controlled distinguished fast-axis singularities with customized retardance profiles. The resulting fields are then described by high-dimensional integer-valued topological tuples, providing theoretically unbounded information capacity at the nanoscale. As a proof-of-concept demonstration, selected tuple components are mapped to represent predefined alphabetic symbols, realizing controlled high-dimensional information representation within a single optical field. Our results establish Stokes defects as functional units for higher-dimensional topological encoding, expanding the role of defects from failure points to engineerable carriers of optical information.
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All authors Yunqi Zhang, Fengjun Li, Runchen Zhang, Zi-Lan Deng, Liangyu Deng, Zhikai Zhou, Ruofu Liu, Zimo Zhao, Yifei Ma, Yuanzhe Xu, Zixuan Wang, Yixuan Zhao, Jize Yan, Honghui He, Xiangping Li, Chao He

Optics

HALO: A Physics-Aware LLM Agent Framework for Nanophotonic Design

Language models have recently been applied to nanophotonic design, but it remains unclear whether they can reliably translate optical objectives into simulation-ready designs, execute electromagnetic analysis, and revise decisions from numerical feedback. We introduce HALO, a physics-aware framework that couples language-model planners with typed design specifications, electromagnetic simulation, diagnostic evaluation, and optional reuse of prior failure trajectories in an iterative design loop. We further introduce HALO-Bench, a 52-task benchmark spanning lab-derived, paper-derived, and open-ended nanophotonic design tasks under a shared evaluation protocol. We compare three planner configurations: a Fixed Structured Workflow, an Autonomous Structured Agent using the same simulation interface, and an Autonomous Coding Agent that directly writes and executes simulation code. The Fixed Structured Workflow is the most token-efficient and exhibits no observed code- or path-level failures, while autonomous coding can achieve higher task success with stronger models at the cost of additional operational failures. We also study reuse of prior failed trajectories. On targeted multi-round tasks, retrieved failure feedback reduces both iterations to first success and total token use. These results clarify the tradeoffs between explicit interfaces, autonomous execution, and reusable design experience in scientific agents.
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All authors Yubo Zhang, Jinlin Xiang, Zijun Zhao, Yang Zhao, Eli Shlizerman, Arka Majumdar

Optics

Intracavity Dual-Resonance Stimulated Raman Spectroscopy with Cavity Ringdown Readout for Resolving Hydrogen Rotational Raman Transitions

Gas-phase rotational Raman lineshape metrology of hydrogen (H2) is challenging due to its weak Raman scattering cross-sections and intrinsically narrow linewidths. We report the first measurement of the complete Dicke-narrowing evolution of the H2 rotational Raman transitions S0(1) and S0(0), enabled by intracavity dual-resonance stimulated Raman spectroscopy with cavity ringdown readout and kHz-level spectral resolution. Our results establish a benchmark for gas-phase Raman lineshape measurements and provide stringent constraints for regime-based pressure-dependent linewidth models.
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All authors Qinxue Nie, Guanda Lyu, Yue Yan, Wei Ren

Optics · Cross-listed from quant-ph

How Long-Range Tails Reshape Non-Hermitian Spectra

Exponentially decaying long-range hoppings are ubiquitous in realistic tight-binding models and are often truncated to obtain a finite-range description. We show that this approximation can fail dramatically in non-Hermitian systems under open boundary conditions: an infinitesimal long-range hopping can nonperturbatively reconstruct the spectrum and eigenstates of a short-range non-Hermitian system. The mechanism is controlled by a competition between the decay length of infinitesimal long-range hoppings and the localization length of non-Hermitian skin modes, leading to a sharp transition as the decay rate is tuned. In one dimension, we show that a squeezed generalized Brillouin zone (GBZ) replaces the original GBZ of the short-ranged Hamiltonian, yielding the reconstructed open-boundary spectrum. In two or higher dimensions, we formulate a squeezed amoeba formulation describing the reconstructed spectral density. We further show that long-range hoppings can qualitatively reshape Green's function, which can be readily detected in experiments.
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All authors Ding Gu, Zhanpeng Fu, Yu-Min Hu, Zhong Wang

Optics · Cross-listed from cond-mat.mtrl-sci

Modifying van der Waals Materials via Cavity Vacuum Fluctuations

In the field of cavity quantum materials, vacuum fluctuations of optical cavities are used for modifying ground-state properties of quantum materials without external driving. Here, one example is the van der Waals (vdW)/dispersion interaction in layered 2D vdW materials, where non-additive long-range correlations can dominate the interlayer binding. While cavity-induced changes of such interactions have been predicted and described using ab initio methods for molecular systems, no efficient description exists yet for extended materials. In this Letter, we close this gap by introducing a periodic formulation of the photon many-body dispersion (pMBD) functional within quantum electrodynamical density-functional theory (QEDFT). Applying this method with efficient $\textbf{q}$-point sampling to bilayer hBN and graphene, we predict cavity-modified stacking, increased equilibrium interlayer distances, and softened layer breathing modes with increasing light-matter coupling strength. Our results establish cavity vacuum fluctuations as a tuning knob for the structural properties of vdW materials.
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All authors Mohammad Hassan, Cankut Tasci, Leon Orlov-Sullivan, Leonardo A. Cunha, Johannes Flick

Optics · Cross-listed from quant-ph

Langevin Theory of Non-Markovian Quantum Dynamics: Application to Delayed Coherent Feedback and the Laser Linewidth

Phase-space methods are powerful tools for the treatment of Markovian open quantum systems: they map the reduced dynamics of a system S, in interaction with an environment E, exactly onto Langevin equations for c-number stochastic variables, as opposed to Heisenberg-Langevin equations for operators. Langevin equations provide analytical insight in key regimes and excel at handling strong nonlinearities and couplings, where other methods often falter. Extending phase-space methods to non-Markovian dynamics, however, has remained a long-standing challenge. Here we address this gap by applying phase-space representations to the full S+E system; integrating out the environmental degrees of freedom then yields a general Langevin framework for S that incorporates both deterministic and stochastic contributions from E. Normally ordered representations, such as the Glauber-Sudarshan P representation and its positive variant due to Drummond and Gardiner, lead to Langevin equations in which (i) non-Markovian effects emerge exclusively in the deterministic terms, via a memory kernel, and (ii) noise contributions vanish when E is initially in the vacuum state. To demonstrate the power of this framework, we address the paradigmatic problem of delayed coherent feedback, in which the system is driven by its own past state, and study its impact on the laser linewidth: we recover the narrowing observed well above threshold and predict an enhanced narrowing just above it. Crucially, the number of stochastic variables scales linearly with the system size, making the framework suitable for problems ranging from a few degrees of freedom to genuinely many-body systems. This opens the way to the systematic study of non-Markovian driven-dissipative quantum systems using the same analytical and numerical tools that have long made phase-space methods so successful in the Markovian regime.
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All authors Marc Cuenca-Laràs, Ming Li, Carlos Navarrete-Benlloch, Germán J. de Valcárcel