Optics · Cross-listed from quant-ph
Papers
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Monday 10 August
Silicon T centers are promising spin-photon interfaces in solid-state platforms for telecom-compatible, scalable quantum information technologies. A major challenge for T centers in nanophotonics is spectral diffusion, where fluctuations in the local electric-field environment from surface and bulk charge states broaden the optical transition and reduce photon indistinguishability. Strategies that directly suppress spectral diffusion are therefore critical for improving T-center-based quantum photonic devices. Here, we use atomic-layer-deposited Al2O3 to passivate the silicon surface and demonstrate a systematic narrowing of T center optical linewidths. Across our measurements, Al2O3 passivation reduces the T center emission linewidth by up to 57%. Complementary above-bandgap illumination and spectral hole burning measurements show that the remaining linewidth contains a significant spectral-diffusion component caused by adjacent charge traps, while placing an upper bound of approximately 75 MHz on the homogeneous linewidth. This work provides a CMOS-compatible path toward generating indistinguishable photons from silicon T centers for scalable quantum photonic applications.
Optics
A fully integrated dispersion-managed femtosecond mode-locked laser
Femtosecond lasers underpin applications ranging from material processing to corneal surgery, while their regular pulse trains form optical frequency combs that have revolutionized timekeeping, spectroscopy, and metrology. On-chip optical frequency combs, such as Kerr microcombs, have enabled high-repetition-rate applications in optical communications and microwave photonics. However, integrated chip-scale sources operating at low repetition rates (100 MHz to 1 GHz), crucial for high peak intensities, remain elusive, as existing devices typically operate well beyond 10 GHz. Here, we demonstrate a self-starting, photonic integrated mode-locked laser based on a dispersion-managed architecture that accesses this regime. The laser combines erbium-implanted silicon nitride gain waveguides, integrated chirped Bragg gratings, and a semiconductor saturable absorber mirror to generate optical pulses with repetition rates from 0.5 to 1.2 GHz, pulse durations as short as 300 fs, and mode-locking thresholds down to 27.3 mW. The output forms a passively stable optical frequency comb with a comb-line drift below 1% of the repetition rate, surpassing the stability of commercial fiber lasers by two orders of magnitude. Leveraging this ultra-low threshold, we achieve complete hybrid integration by co-packaging the laser with a telecom-grade 980-nm III-V pump diode chip inside a compact photonic module. The resulting electrical-in/optical-out module delivers turnkey, stable mode-locked pulses, providing a compact, low-power, and vibration-insensitive foundry-compatible platform for field-deployable optical metrology and precision sensing.
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Optics
Scalable laser micro- and nanostructuring of mould inserts for functional injection-moulded polymer surfaces
Functional polymer surfaces with tailored wettability, antibacterial and adhesion properties are increasingly required in medical, packaging and consumer applications. Laser structuring of steel mould inserts followed by injection moulding offers a scalable manufacturing route, but conventional single-beam texturing has limited throughput. Here, we present a selective acceleration strategy that applies different laser techniques to micro- and nanostructuring. Deep microhole drilling was accelerated up to 20-fold by operating an ultrashort-pulse fibre laser at a repetition rate of 1 MHz in single-beam mode. For laser-induced periodic surface structures (LIPSS), line-beam shaping with a spatial light modulator increased productivity by 35-fold, reaching processing speeds above 100 cm$^2$ min$^{-1}$ while retaining sub-micrometre fidelity. Replication experiments with polypropylene (PP), PA66 and ABS confirmed successful transfer of micro- and nanostructures, with PP showing the highest fidelity. Vacuum-assisted injection moulding increased replicated feature height by 56–283 percent. All laser-textured PP surfaces showed higher static water contact angles than the untreated reference, reaching approximately $134^\circ$ in the Wenzel regime. Structured PA66 surfaces reduced bacterial retention by up to 99.8 percent for E. coli and approximately 90 percent for S. aureus. Laser texturing also increased the shear strength of PP joints bonded with a non-optimised adhesive by up to 30-fold. This approach provides a practical, coating-free route to functional polymer components and helps bridge the gap between laboratory laser texturing and industrial injection moulding.
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Optics
In-situ integrated nonlocal Huygens metasurfaces enable robust vortex beams from multimode fibers
A fundamental hurdle for multimode fiber (MMF) integrated photonics is achieving robust and deterministic wavefront shaping against fiber perturbation, which induces random modal interference and scrambles the real-space output into speckle patterns. Existing wavefront shaping methods typically rely on pixelated phase or polarization pre-compensation, rendering them highly sensitive to fiber deformation. Here, we show that in-situ integration of a silicon nonlocal metasurface onto an MMF end facet enables direct conversion of arbitrary speckle patterns into optical vortex beams without pre-compensation. The metasurface supports overlapped Mie resonances and nonlocal bound states in the continuum (BICs), yielding high-transmission bands by satisfying the generalized nonlocal Huygens condition. Through momentum-space coupling between MMF modes and Huygens-BICs with topological polarization-vortex nature, the output maintains doughnut-shaped profiles under static and dynamic perturbations, demonstrating exceptional robustness against fiber deformation. This approach provides a compact, alignment-tolerant platform for robust structured light generation in MMFs for endoscopy, optical trapping and communications.
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Optics · Cross-listed from physics.atom-ph
Resonant photoionization dynamics during optical trapping of lithium atoms
Photoionization induced by trapping and auxiliary laser fields is an inherent feature of many laser-cooling and optical trapping experiments, yet its microscopic dynamics are rarely investigated directly. In this work, we employ a reaction microscope implementing an event-by-event photoionization time retrieval technique to extend momentum-resolved photoelectron spectroscopy to continuous-wave laser–atom interactions. We investigate low-intensity multicolor photoionization of laser-cooled lithium atoms confined in an all-optical trap. Complete three-dimensional electron momentum distributions and kinetic-energy spectra recorded for different laser wavelengths and polarization configurations identify resonant excitation of the $5p$ and $5f$ states and reveal an additional ionization channel following spontaneous decay from the $5f$ to the $4d$ state. A pronounced polarization dependence of the photoionization yield is explained by magnetic-sublevel selection rules and the coherent interference of different virtual excitation pathways. These results demonstrate that reaction microscopy combined with event-by-event time reconstruction provides a powerful approach for investigating microscopic electronic dynamics in laser-cooled atomic systems and offers new insight into photoionization processes occurring during optical trapping.
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Optics
Direct Laser Interference Patterning of Functional Metal Surfaces: From Written Geometry to Functional Interfaces
Direct laser interference patterning (DLIP) generates periodic micro- and nanoscale structures with increasing precision and throughput, yet similar geometries can produce fundamentally different functional responses. This review examines why morphology alone cannot predict friction, wetting and ice adhesion, bacterial response, cell behaviour, optical performance or electrochemical and photovoltaic function. DLIP is treated as a model system in which the optically prescribed geometry can be distinguished from the interface realised during processing. The written period is separated from relief depth, aspect ratio, hierarchical topography, surface chemistry, ageing and process history. Functional response is interpreted as a two-stage process: geometry creates the opportunity for interaction with an external agent, while the realised interface determines how that interaction becomes measurable performance under a specific interfacial state. A curated, metals-centred evidence base spanning tribology, wetting and anti-icing, antibacterial and biomedical surfaces, optics, electrochemistry, energy devices and manufacturing shows that period-depth coordinates alone rarely predict function across domains. Geometry remains highly transferable in optical systems and controlled mechanical contacts, whereas biological, state-dependent and device-level functions also depend on surface state, operating conditions and system architecture. The framework reconciles conflicting observations and identifies which variables are transferable and which remain context-dependent. Predictive DLIP surface engineering therefore requires identification of the interacting agent, separation of written geometry from the realised interface, isolation of variables governing interfacial coupling and evaluation through direct, mechanism-specific endpoints.
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Optics
Femtosecond Engineering of PolyMethylPentene(PMP) Nonlinearity via NA, Spin/orbital angular momentum (OAM), and In-Situ SC Diagnostics
While femtosecond vortex beams are widely studied for photonic fabrication, how OAM affects third-order susceptibility, energy deposition, and structural symmetry in transparent polymers remains unclear. To address this gap, we investigate femtosecond vortex beam interactions with polymethylpentene (PMP) to establish OAM control over beam shaping and energy deposition in laser micromachining. A 775 nm femtosecond laser is frequency-doubled to 387.5 nm and phase-shaped by a reflective liquid crystal-spatial light modulator, with OAM imprinted via computer-generated holograms and independently controlled spin via a quarter-wave plate. Theoretical modeling of the tensorial nonlinear polarization, combined with systematic experiments on low-NA filamentation, supercontinuum spectroscopy using an advanced spectrometer, and high-NA inscription with NA = 0.4 and 0.7, reveals that the same $\chi^{(3)}$ tensor components govern all regimes. The transition from perturbative to dissipative behavior is determined solely by whether the local intensity exceeds the plasma formation threshold. Through an analytical framework based on the isotropic material model, the key innovation lies in identifying that $\chi_{1122}$ governs the energy deposition and plasma threshold, whereas $\chi_{1221}$ mediates the transverse nonlinear current and helicity-dependent asymmetry, thereby converting phase topology into permanent chiral structures. This enables OAM-controlled structuring with sub-micrometer feature sizes (approximately 0.43 $\mu$m diameter and approximately 200 nm$^2$ area) and localized intensities reaching $10^{14}$–$10^{15}$ W/cm$^2$, providing an engineering framework for deterministic fabrication of chiral waveguides and photonic devices through precise control of topological charge and focusing conditions.
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Optics
Impact of Terminal Noise on Polarization Rotation Vector for Sensing Applications
State-of-Polarization sensing with coherent transponders enables wide-area geophysical monitoring over existing submarine cables, but its performance is limited by polarization noise from both the fiber and terminal hardware. This work investigates how terminal noise affects polarization rotation estimates derived from receiver equalizer coefficients and how it can obscure stochastic polarization drift used for sensing. We analyze Jones-matrix time series from two deployed receivers in the Sparkle Mediterranean link MedNautilus (approximately 2000 km and 450 km) and compare them with a laboratory back-to-back reference. Power Spectral Density (PSD) analysis reveals a low-frequency random-walk regime and a high-frequency white-noise floor, separated by a link-dependent corner frequency. The rotation innovation variance increases with link length, while the longest field link also shows elevated white noise consistent with accumulated amplifier and terminal contributions. Additionally, harmonic spectral components are observed, indicating a transponder-related artifact that should be considered in practical sensing applications.
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Optics
A Collective Propagation Law of Optical Vortex Constellations and Longitudinal Sensing
Optical vortices are ubiquitous phenomena naturally appearing in wave physics, yet higher-order charges inherently split into constellations of lowest-order singularities at the smallest deviation from an ideal situation. While these constellations are common phenomena in real-world scenarios, characterizing their longitudinal evolution typically relies on exhaustive full-field descriptions or the ambiguous, sequential tracking of individual singularities. Here, we reveal and experimentally demonstrate a simple deterministic law describing the paraxial longitudinal propagation of an arbitrary constellation of optical vortices in standard Gaussian backgrounds. By mapping the constituting singularity coordinates to their elementary symmetric polynomials (ESPs), we capture the holistic evolution of the constellation during propagation, completely bypassing the practical need to sequentially track indistinguishable vortices. We further show that such complex ESPs provide a useful metrological tool for the estimation of longitudinal displacements. Our results reveal a previously unrecognized compact description of collective vortex dynamics, introducing a new route to longitudinal sensing through singularimetry.
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Optics · Cross-listed from quant-ph
Evidence for Counterfactual Violation of Local Conservation Laws in Quantum Events
Physical conservation laws, such as those of energy and momentum, are generally believed to hold exactly and locally in spacetime, including in quantum phenomena. Yet Aharonov, Popescu, and Rohrlich (APR) recently argued, on the basis of a thought experiment, that individual quantum events, unlike ensemble averages, may occasionally violate local conservation laws. Their argument relies on the wave phenomenon known as "superoscillations", which APR themselves discovered more than 30 years ago. Here we provide experimental evidence for such a violation. We extract photons from a small superoscillatory region near the core of an optical vortex and show that their mean transverse momentum is statistically incompatible with a general bound implied by local momentum conservation. The derivation of this bound requires only the theoretically well-supported assumption that the extraction mechanism does not alter the photons' mean transverse momentum. We also detect photons with high transverse momentum at a rate significantly exceeding that predicted by a model assuming local momentum conservation. Because this violation can be established only counterfactually and through postselection, it does not conflict with relativistic causality. Our results may represent the first example of a distinct form of quantum nonlocality that does not explicitly rely on entanglement.
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Optics
High-speed volumetric amplitude-spectrum dynamic optical coherence tomography by neural network with multi-burst scanning
Dynamic optical coherence tomography (DOCT) enables label-free, three-dimensional (3D) assessment of tissue dynamics. However, it suffers from long acquisition times because conventional time-spectrum DOCT requires hundreds of repeated OCT frames per location. Here we present a neural network (NN) framework integrated with a non-uniform-time scanning protocol (multi-burst scan) to accelerate amplitude-spectrum DOCT (AS-DOCT). Combining 3D convolutional and long-short term memory (LSTM) layers with dual inputs (the temporal OCT sequence and its pseudo-amplitude spectrum), the model generates AS-DOCT images from only 16 frames per location. Validated on 29 cancer spheroids, the proposed method resolved distinct functional domain structures with high fidelity (structural similarity index metric (SSIM) > 0.8) and enabled full volumetric AS-DOCT acquisition in 26.2 seconds. This method will enable high-throughput 3D dynamic tissue screening.
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Optics
Population-inversion map of the mesospheric sodium ladder: continuous-wave and pulsed pumping schemes for directed emission
Directed mirrorless lasing from the mesospheric sodium layer has been proposed as a way to overcome the isotropy of laser guide star fluorescence, with demonstrated cell-scale analogues and a demonstrated stand-off magnetometry application. Several transition paths on the Na ladder compete for the same pump photons. We build a ten-level rate-equation model of the ladder from NIST transition probabilities and evaluate every electric-dipole line under four continuous-wave pumping schemes, both in a Doppler-averaged treatment and in a velocity-selective treatment appropriate for the collision-poor mesosphere. Three design-relevant results emerge. At practically accessible continuous-wave irradiances the column-gain exponents remain far below unity, consistent with published feasibility estimates; the value of the classification is to identify which lines, schemes, and pulse formats merit further study.
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Optics
Dispersion-managed octave soliton microcombs in heterostructured microresonators
Controlling group velocity dispersion is of fundamental importance in ultrafast optics, particularly for supercontinuum generation and optical frequency comb synthesis. However, the simultaneous, independent tailoring of multiple dispersion coefficients over an ultra-broad bandwidth remains a formidable challenge in conventional nanophotonic platforms. Here, we demonstrate a robust strategy for broadband dispersion management using heterostructured microresonators comprised of adiabatically concatenated waveguides with distinct geometries. By meticulously engineering the local dispersion profiles, we can flexibly synthesize the global effective dispersion coefficients of different orders, effectively expanding design degrees of freedom beyond conventional limits. As a benchmarking demonstration, we fabricate heterostructured silicon nitride microresonators using a commercial foundry process and successfully generate octave-spanning soliton microcombs with a repetition rate as low as 118 GHz. These microcombs feature deterministically tunable dispersive waves operating across the 290-310 THz range. Such octave-spanning microcombs with detectable repetition rates and carrier-envelope offset frequencies are readily applicable to f-2f self-referencing in optical clocks and frequency synthesizers. The proposed heterostructured architecture establishes a versatile paradigm for generating ultrawideband soliton microcombs with tailorable spectral profiles.
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Optics
Wafer-scale monolithic integration of Ce:YIG films and magneto-optical isolators on silicon
Silicon integrated cerium doped yttrium iron garnet (Ce:YIG) thin films are promising candidates for integrated nonreciprocal photonic devices, cryogenic photonic modulators and optical computing applications. However, previously reported Ce:YIG thin film on silicon is limited to milimeter sizes. Wafer-scale integration and non-destructive characterization of high quality Ce:YIG thin films on silicon has been elusive. Here, we report growth of 4-inch wafer-scale Ce:YIG thin films on silicon substrates by radio-frequency magnetron sputtering. Strong Faraday effect of 2318 deg/cm, low propagation loss of 80 dB/cm and excellent thickness uniformity of 3.5% is demonstrated across the 4-inch silicon wafer. Furthermore, a custom designed wafer-scale, non-destructive magneto-ellipsometry was established to characterize the film thickness, optical constants and magneto-optical constants across the wafer. Wafer-scale integration of ring resonator type magneto-optical isolators are also demonstrated. Our work demonstrates a step forward toward wafer-scale heterogeneous integration and characterization of magneto-optical thin films on silicon, providing material candidates for non-reciprocal photonic device arrays, magneto-optical in-memory computing networks and integrated magneto-optic magnetometers.
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Sunday 9 August
Optics
Multimode Quantum Effects of Optical-Axis Misalignment in Gravitational-Wave Interferometers
We develop a multimode quantum model of optical-axis misalignment in a simplified representation of the differential mode of an Advanced LIGO interferometer. The system is described as two coupled optical resonators corresponding to the signal extraction cavity and the arm cavity. Analytical expressions for the mode-mixing coefficients are derived, establishing a direct connection between geometrical perturbations of optical elements and multimode optical dynamics. Using the developed formalism, we investigate the influence of optical-axis misalignment on quantum-noise-limited sensitivity and injected squeezed states. We show that misalignment between the signal extraction cavity and the arm cavity leads to significant sensitivity degradation, frequency-dependent rotation of the squeezing ellipse, and a reduction of the observable squeezing in the fundamental spatial mode. At the same time, the injected squeezing is not destroyed but redistributed among coupled spatial modes. The resulting mode coupling generates quantum correlations between the fundamental and higher-order modes and leads to spatial-mode entanglement verified using the positive partial transpose criterion. Our results demonstrate that optical-axis misalignment should be treated as a coherent multimode quantum process rather than as a simple optical loss mechanism.
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Optics
Nonresonant optomechanical control of structural phases
Optical tweezers demonstrate how light can exert forces to trap, repel, and manipulate microscopic particles without absorption. Recent theory has suggested that such forces can extend beyond particle manipulation to drive structural phase transitions in solids. Here we apply this optomechanical principle to tin selenide (SnSe), a material where proximity to several different structural phases gives rise to its high thermoelectric figure of merit and makes it a candidate for a switchable topological crystalline insulator. Whereas the force for standard optical tweezers arises from a gradient in the intensity of a light field, the optomechanical force is mediated by a gradient in the dielectric constant as a function of phonon coordinate. Unlike conventional methods that rely on resonant excitation and absorption through the imaginary part of the dielectric function, this approach operates dispersively through the real part and can be directly driven by Raman processes, enabling selective transitions with reduced energy cost and ultrafast response. Using time-domain Raman scattering, we show that above a critical mid-infrared field strength the $A_g$ Raman modes disappear abruptly without softening, signaling the formation of a new structural phase. This phase, distinct from those induced by heating or carrier excitation, exhibits large-amplitude and long-lived modulations in its optical response. Complementing this observation, we show also evidence for an equivalent DC-field-driven structural phase transformation to a higher symmetry phase, as observed by atom probe tomography. Our study demonstrates the concept of nonresonant optomechanical phase control and defines novel opportunities for synthesizing hidden structural phases with unique functional properties.
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Optics
Low optical loss electrical isolation for multi-section monolithic GaSb-based photonic circuits
Monolithic photonic integrated circuits (PICs) platforms exploiting III-V materials combine passive and active waveguide structures in multi-section optoelectronic device architectures. Their operation requires high electrical isolation between adjacent functional sections without compromising the optical signal. This fundamental requirement is addressed for GaSb-based waveguides, which are known to exhibit high conductivity of p-type layers reducing the electrical isolation capability. To this end, a co-designed electrical-optical isolation strategy based on using deeply etched strip waveguides combined with adiabatic ridge-to-strip waveguide tapers in GaSb-based multiple-quantum-well heterostructures is proposed. While deep etching alone enables isolation resistances of up to 40 k-ohm, it severely degrades optical propagation. By introducing optimized adiabatic tapers, we demonstrate good optical performance as single-mode continuous-wave lasing in a two-section device with integrated absorber, while maintaining an isolation resistance of 17.3 k-ohm; this corresponds to an approximately 17-fold improvement over previously reported GaSb two-section devices. The approach establishes a critical building block for the development of monolithic GaSb-based PICs operating above 2 um.
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Optics
Degenerate four-wave mixing in a CPT-symmetric coupler with intermodal dispersion
Four-wave mixing provides a simple setting in which dispersion, nonlinearity, and non-Hermiticity compete to select resonant energy-transfer channels. We study degenerate four-wave mixing in a Kerr dual-core coupler with balanced gain and loss and frequency-dependent intercore coupling. The dispersive coupling changes the symmetry from conventional $\mathcal{PT}$ symmetry to a combined $\mathcal{CPT}$ symmetry and reshapes the two-branch linear spectrum. We determine the unbroken-$\mathcal{CPT}$ domain and classify the branch configurations that can satisfy the degenerate phase-matching condition. In the parameter ranges examined, three resonant channels persist over broad regions, whereas a same-branch channel appears only close to the symmetry-breaking threshold. In this near-threshold regime, a single pump can simultaneously satisfy two distinct nonzero sideband resonances. Direct pulse simulations confirm the predicted resonances and reveal secondary-wave generation and multifrequency cascades near eigenmode coalescence. A reduced three-wave model captures the initial dynamics away from the exceptional point but loses accuracy as the modal basis becomes ill-conditioned. These results show how dispersive coupling reorganizes resonances, group-velocity mismatch, and nonlinear energy exchange in a non-Hermitian wave system, and they identify the exceptional-point region as a regime where a few-mode description can break down.
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Optics
Geometric phase-space nonseparability triggers giant optical shifts
Nonseparability among multiple degrees of freedom has enabled fundamental advances in structured light and related applications. Here we unveil a previously overlooked form of nonseparability in phase space, which we term geometric phase-space nonseparability. The latter arises solely from the wavefront curvature of a conventional wave packet, such as a fundamental Gaussian beam. This phase-space structure manifests as a position-dependent transverse-momentum distribution across the beam profile leading to the giant spatial and angular beam shifts upon reflection at a planar interface that we predict analytically and observe experimentally. Remarkably, the curvature-induced phase-space correlation remains robust against spatial-coherence degradation, allowing the giant shifts to persist even in the nearly incoherent regime. Our results establish wavefront curvature as a general mechanism for engineering beam shifts across optical, acoustic, and matter-wave systems.
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Optics
Quasi-Sinusoidal Single Diamond Structure in Royal Jewel Butterfly: An Angle-Independent Photonic Structure
Structural colouration with narrow spectral photonic bandwidth and high reflectivity is of critical importance for modern optical applications, including displays, laser systems, and optical sensing, etc. Achieving such angle independent colouration typically relies on polycrystalline or inherent structural disorder. However, balancing angular uniformity with high brightness and strong colour contrast remains challenging. Herein, we uncover the structural origin of the spectacular bright, angle-independent blue colouration of Hypochrysops polycletus, a sapphire-like Royal Jewel butterfly. Three-dimensional (3D) electron microscopy reveals that the dorsal wing scale has a single diamond structure, a 3D photonic crystal previously documented only in beetles and weevils. The crystal domains form an extraordinary quasi sinusoidal surface geometry with a distinct template morphology-guided arrangement. Unlike typically thicker biophotonic structures that support multiple high symmetry stopbands, this design contains only 3-4 unit cells in the propagation direction. Its optical response is dominated by the fundamental stopband, with two dominant scattering mechanisms: specular reflection at the {111} inclined sidewalls of the hierarchical structure, and funnelling into localised quasi-normal modes enabled by a strongly anisotropic Bloch transport. By mimicking these features with two-photon polymerisation, we artificially reproduced the optical response in the infrared region. The study opens a pathway towards bioinspired brilliant diffuse colouration and angle-robust photonic devices.
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Optics
Fundamental limits of hot-carrier and photothermal plasmonic solar chemistry
Plasmonic catalysts convert sunlight through direct metal–adsorbate excitation, nonequilibrium hot carriers and photothermal heating, yet these channels lack a common efficiency limit analogous to the Shockley-Queisser (SQ) limit. Here, we formulate a channel-resolved detailed-balance theory for plasmonic solar chemistry. The theory enforces exclusive partition of absorbed power, microscopic reversibility, non-negative entropy production, electromagnetic passivity and causality, and one physical nanostructure shared by all wavelengths and operating states. A reduced tightly coupled cycle obeys a chemical diode law with closed-form stall and maximum-power free energies. It recovers a 33.68% single-threshold radiative limit and the 30.58% ideal single-junction water-splitting limit at a 1.23-eV chemical load, whereas a Fowler hot-carrier kernel lowers the limit to 8.53%. Finite one-structure benchmarks show that independent wavelength optimization overestimates shared-geometry performance by 6.6-33.8%, while cross-frequency correlations tighten semidefinite upper bounds by 21-56%. An exact multi-electron network yields a universal arrival-storage criterion and the low-flux scaling J_n\sim g^n\tau^{n-1}. A source-conditioned gold/p-type gallium nitride case study and a bias- and separation-complete ledger then distinguish enhanced product formation from net solar-energy conversion. The resulting framework provides a thermodynamically closed benchmark for hot-carrier and photothermal plasmonic chemistry.
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Optics
Simulating optical microcavities by inverting the thermal transfer function
I present a reduced-order approach for incorporating distributed thermal dynamics into nonlinear optical-microcavity simulations without repeatedly solving the time-dependent heat equation. A harmonic finite-element heat solve is used to obtain the thermal transfer function, which is introduced into the time domain through either a rational approximation or an impulse-response convolution. The method is validated against heat-equation-coupled finite-element simulations for prescribed TE1-mode heating and for nonlinear silicon microcavity dynamics. For the feed-forward TE1 tests up to 100 MHz and simplified cavity dynamics, the error remains below 4%. The reduced models reproduce the local self-pulsation dynamics, although long-time phase alignment is sensitive to the spatial definition of the thermal transfer function and to impulse-response truncation. These results establish a physics-based route for retaining multi-timescale thermal memory while substantially reducing the cost of coupled optical–thermal simulations.
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Optics
Broadly Tunable Compact Non-Coplanar X-Ray Cavity for Cavity-Based Free-Electron Lasers
Cavity-based x-ray free-electron lasers (CBXFELs) require tunable x-ray cavities to broaden their practical utility and enable access to a wider range of scientific applications. We propose and analyze a compact tunable non-coplanar x-ray cavity based on six Bragg-reflecting crystals arranged as two three-crystal backscattering units. The three-dimensional geometry provides a substantially larger tuning range than planar bowtie cavities while maintaining a compact transverse footprint. We derive analytical expressions for the cavity geometry, crystal kinematics, and polarization-dependent Bragg reflectivity both in the intrinsic and eigenpolarization bases. For a given Bragg reflection, the ultimate photon-energy tuning range is 100%, from $E=E_{_{H}}$ at backscattering to $E=2E_{_{H}}$ at Bragg angle $\theta=\pi/6$. Practical geometrical and polarization constraints reduce the directly usable range to approximately 45%, while operation in the cavity eigenpolarization basis can extend it to approximately 65%. By combining fundamental and harmonic diamond reflections, and using reflections from different crystallographic families, the accessible photon-energy range can be extended from about 3~keV to approximately 20~keV. These results establish non-coplanar multi-crystal cavities as a viable route toward compact, broadly tunable x-ray resonators for future CBXFELs.
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Saturday 8 August
Optics · Cross-listed from cond-mat.stat-mech
A Shared Observation Shields Collective Fluctuations while Preserving Local Independence
As a liquid approaches its glass transition, its dynamics turns heterogeneous: mobile and immobile regions coexist, and the four-point susceptibility $\chi_4$ that quantifies this heterogeneity grows sharply. Interpreting that growth is subtle, because the collective signals experiments record, such as a tagged particle's trajectory, an overlap function, or a mean field, are generated by the same particles they describe. Here we compute exactly what conditioning on such a shared record does to the population that produced it, for a broad class of stochastically observed systems; the guiding example is a tagged particle and the cage of $z$ neighbors that drives its force history. Using a Girsanov path transformation, we prove that the conditioning multiplies the independent joint law of the $z$ trajectories by exactly one term: a centered-square penalty along the single collective direction the record can see. Any fixed pair of particles stays nearly independent, with covariance falling as $O(z^{-1})$ and mutual information as $O(z^{-2})$, the property known as propagation of chaos, yet the $z(z-1)$ weak pair correlations add coherently into a finite suppression of collective fluctuations, the Schur shield $D - C = -C^2(aI + C)^{-1} \preceq 0$. An exactly solvable Brownian model calibrates the construction. The physical consequence is a calculable baseline for dynamical heterogeneity: conditioning itself contributes a computable, nonpositive amount to the susceptibility of a conditioned ensemble, so the genuine cooperative signal is the excess of the measured $\chi_4$ over this baseline rather than over zero, a comparison that existing simulation data can already perform.
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Optics
Fisher-Information Design of Ridge-Loaded Subwavelength Slits
We present an information theoretic framework for extraordinary optical transmission through a subwavelength slit containing symmetric internal ridges. Full wave finite element spectra are interpreted with a reduced Fabry Perot model in which the ridge interfaces introduce a reactive discontinuity phase associated with modal impedance mismatch and evanescent field loading. Fisher information is used to quantify how reliably resonance positions and geometric parameters can be inferred from transmission measurements. For an isolated Lorentzian resonance under white Gaussian noise, the Fisher information for the resonance center scales linearly with the quality factor when amplitude, sampling, and noise are fixed. We also extend the formulation to correlated Gaussian noise and Poisson shot noise, showing why the resonance with the highest Q is not necessarily the most informative under realistic experimental conditions. The framework clarifies the interpretation of ridge induced effective cavity corrections and provides a reduced order route toward Fisher information driven inverse design of subwavelength resonators.
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Optics · Cross-listed from quant-ph
Millisecond optical coherence and strong collective coupling in an integrated telecom rare-earth photonic platform
Long-range quantum network nodes require the combination of strong light-matter coupling, long coherence times and in situ spectral control at telecom wavelengths. The coherence of erbium in integrated devices is held back by its hosts, which do not simultaneously provide the weakly magnetic nuclear-spin environment and the well-defined substitutional sites found in coherence-optimised bulk crystals. Here we bring such an optimised crystal onto a photonic chip, by bonding an Er${^{3+}}$:CaWO${_{4}}$ host without an adhesive interlayer to a high-${Q}$ electro-optically tuneable thin-film lithium niobate microring resonator. At an effective temperature of ${75}$ mK and a field of only ${0.2}$ T, the bonded ensemble retains an effective homogeneous linewidth of ${289\pm34}$ Hz (${T_\text{M}=1.10\pm0.13}$ ms), with spectral diffusion proceeding at ${86\pm18}$ Hz and saturating at ${1.5\pm0.2}$ kHz. Electro-optically tuning the resonator through the erbium optical transition resolves an avoided crossing with a collective cooperativity of ${C=6.7\pm0.4}$. Exploiting superhyperfine coupling to the host's ${^{183}}$W nuclear spins, we store and retrieve optical phase information over ${5}$ s with a visibility of ${0.935\pm0.015}$. Strong collective coupling, millisecond coherence and in situ spectral tuning in a single device thus establish heterogeneous integration leveraging coherence-optimised hosts as a route to scalable telecom quantum networks.
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Optics
Epsilon-Near-Zero Materials based Photonic Architectures for Absorption and Emission Control
Engineering optical responses at surfaces, including reflection, absorption, transmission, and emission, is crucial for advanced photonic, energy, thermal-management, and optoelectronic applications. This thesis investigates epsilon-near-zero (ENZ) materials, particularly indium tin oxide (ITO) and titanium nitride (TiN), for controlling light-matter interactions through engineered optical coatings and nanostructures. It also explores the enhancement of optical absorption and emission in two-dimensional (2D) materials such as monolayer molybdenum disulphide (MoS2), whose atomic-scale thickness inherently limits light interaction. The research integrates theoretical analysis, finite-element simulations, nanofabrication, and experimental characterization to develop and validate ENZ-based optical platforms. An ITO-based multilayer coating is demonstrated to provide step-function-like reflectivity, with low reflectance in the visible-to-near-infrared range and high reflectance beyond a tunable cut-in wavelength, offering potential for spectrally selective energy management. Building on this, an ITO-based grating structure is developed to achieve broadband and angularly robust near-infrared absorption, demonstrating its potential for thermal-emission applications. TiN thin films are further demonstrated as an effective platform for enhancing the absorption and emission of monolayer MoS2 without complex nanostructuring. Complementary studies investigate substrate-induced strain and ion-irradiation-induced defects as approaches for tailoring the electronic and optical properties of MoS2. Overall, this work establishes ENZ materials based engineered surfaces as versatile platforms for spectral and light-matter interaction control, contributing to efficient, tunable, thermally stable, and scalable solutions for energy, thermal management, and 2D-material-based optoelectronic applications.
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Optics
Spectral Mixing, Skin Localization, and Linear Optical Response in Dissipative Photonic Lattices
We study the linear optical response of a finite dissipative Hatano–Nelson photonic lattice. The response between selected input and output ports is resolved into a phase-coherent intensity and an incoherent modal-weight contribution using the biorthogonal Green function. Their comparison isolates interference among non-Hermitian modal residues, while a response-weight entropy and the associated participation number $\Neff$ quantify how broadly the measured signal is distributed over the complex modes. The numerical results show that loss broadens the modal distribution, periodic-boundary spectral winding increases modal participation, and onsite disorder reduces it. Time-domain quantum-walk dynamics independently display the drift and right-edge accumulation produced by non-reciprocal hopping under open boundaries. A parameter map in the $(g,W)$ plane, supplemented by disorder-ensemble averages, identifies a finite-size crossover in which $\Neff$ responds to disorder before the response-weighted center is displaced from the skin boundary. The analysis applies to coupled waveguides, microring arrays, driven cavity lattices, and other linear photonic platforms with loss, gain, or non-reciprocal coupling.
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Optics
Sub-Rayleigh Imaging of Unequal-Intensity Sources: Near-Quantum-Limit Multiparameter Estimation
In optical imaging, diffraction strongly degrades the performance of conventional intensity-based estimation once the separation between two sources is below the Rayleigh-Abbe limit. Recent developments showed that this limitation can be surpassed using spatial-mode demultiplexing (SPADE), and this was demonstrated in several experiments for two equal-intensity spots of unknown separation. When there are multiple unknown parameters, as in the case of several unequal sources with unknown intensities and unknown separation, cross-talk among the parameters makes the multi-parameter estimation problem significantly more challenging. In this paper, we adapt super-resolved position localization by inversion of coherence along an edge (SPLICE) to estimate both the separation and relative intensity of two incoherent sources simultaneously. We demonstrate a clear advantage over direct imaging (DI), achieving a root mean squared error (RMSE) approximately $50 \%$ larger than the quantum limit and a sixfold improvement over DI within the range of parameters we tested. This improvement can be even greater for smaller separations and larger intensity imbalances when crosstalk is suppressed.
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Friday 7 August
Optics
Design of a Compact Monolithic Catadioptric Lens for CubeSat Hyperspectral Imaging Payloads
Monolithic catadioptric lenses have emerged as a novel class of compact long-focal-length lenses. Fabricated from a single fused silica substrate with distinct optical prescriptions across annular zones, these systems fold the optical path within the substrate, achieving long effective focal lengths at a fraction of the track length of refractive equivalents. The monolithic architecture and low coefficient of thermal expansion provide inherent athermal performance and preserve optical alignment under the thermal and vibrational loads of nanosatellite launch and orbital operation. Despite these advantages, commercial offerings of monolithic catadioptric lenses are limited and no comprehensive optical design literature review has been published for this lens class. We survey of monolithic catadioptric design variants, including Schmidt-Cassegrain-derived, annular folded, and gradient-index configurations. Building on this design space, we also present a novel monolithic catadioptric objective lens optimized for a CubeSat pushbroom hyperspectral Earth imaging payload. Pushbroom hyperspectral imagers require a precision entrance slit at the focal plane of the objective lens, and maintaining slit-to-focal-plane alignment under launch shock and thermal cycling is a significant optomechanical challenge. The proposed design places the focal plane coincident with the back surface of the substrate, enabling the slit to be lithographically etched directly onto that surface. This approach eliminates the slit-to-objective alignment degree of freedom, yielding an integrated, mechanically robust, and thermally stable objective-slit module for pushbroom imaging. We present the completed optical design of a near-diffraction-limited F/3 f=100mm VSWIR monolithic catadioptric lens, assess imaging performance, and discuss preliminary fabrication and tolerancing considerations.