Papers

Optical atomic magnetometry is a powerful tool for continuous sensing applications, yet, in the absence of quantum correlations, its sensitivity is limited by the standard quantum limit (SQL) stemming from a trade-off between optical probe imprecision and quantum measurement backaction. Beyond-SQL sensitivity requires quantum correlations that modify these measurement noise sources. Here we demonstrate such sensitivity by using entangled state of the probe light and by engineering correlations between measurement imprecision and backaction. Having first explored SQL in a broad range of frequencies, we demonstrate overcoming the limit by combining variational readout with coupling the magnetometer to one mode of a bipartite entangled light state and conditioning the results on the other entangled mode. Tuning the detected light quadratures and combining the signals from the two measurement channels, we achieve sensitivity beyond the SQL in a broad range of acoustic frequencies which has so far remained inaccessible to quantum-noise-limited optical magnetometry.

We experimentally explore the absorption of a propagating wavepacket impinging upon a dissipative region in an engineered quantum system. We employ a 1D non-Hermitian synthetic lattice with an abrupt interface between dissipative and non-dissipative subchains, using the states of the electronic ground-state hyperfine manifold in a $^{87}$Rb Bose-Einstein condensate as sites. By tuning the dissipation rate, we observe a progression from ballistic propagation, to near-perfect absorption, to quantum Zeno reflection. Guided by numerical simulations, we identify that optimal absorption occurs when tunneling and dissipation are properly matched, and find qualitative agreement with an idealized semi-infinite model across all dissipation regimes. Our results establish synthetic lattices as a versatile Quantum simulation platform for dissipation-engineered quantum transport and highlight controlled dissipation as a resource for tailoring quantum dynamics.

Compact cesium beam clocks are major frequency references for deployable timing systems. However, further improvement of their short-term frequency stability is limited by the clock signal-to-noise ratio (SNR). Although two-laser optical pumping can increase the effective atomic utilization, the achievable clock SNR has long been limited by laser-induced frequency-to-amplitude noise conversion. Here, we demonstrate a compact dual-Faraday-laser-pumped (DFP) Cs beam clock enabled by a low-frequency-noise atom-referenced laser architecture. The intracavity Faraday anomalous dispersion optical filter provides inherent alignment to the Cs D$_2$ resonances, while modulation transfer spectroscopy offers suppressed frequency noise and drift. The resulting laser system supports robust turnkey operation with a Lorentzian linewidth of 2.12 kHz. The DFP Cs clock achieves a clock SNR of 46,365 in a 1-Hz bandwidth and a fractional Allan deviation of $7.7\times 10^{-13}/\sqrt\tau$ , with Hadamard deviation reaching $7.7\times 10^{-15}$ at 10,000 s. This work pushes the fractional frequency stability of a compact Cs beam clock into the $10^{-13}/\sqrt\tau$ regime, providing a pathway toward high-performance Cs frequency references for field-deployable precision timing, navigation, and synchronization.

We present a formulation and numerical results for positronium (Ps) laser cooling. The formulation is based on the Lindblad master equation and follows the time evolution of the density matrix of Ps atoms. It therefore accounts for atomic coherence, which is necessary to describe the interaction of Ps with the train of short laser pulses generated by the system developed by Shu $\textit{et al.}$ [K. Shu $\textit{et al.}$, Phys. Rev. A $\textbf{109}$, 043520 (2024)]. Using this formulation, we calculate the time evolution of the populations in each internal and momentum state and thereby quantitatively predict the momentum distribution after laser cooling. We present the representative time evolution of the internal-state populations and momentum distribution, together with a comprehensive scan of the laser parameters used to optimize the cooling efficiency. A prominent feature of the simulated distributions is sub-recoil cooling through velocity-selective coherent population trapping, a coherent effect captured by the quantum-mechanical treatment.

Cold heavy molecules are promising systems for exploring nuclear $\mathcal{P}$- and $\mathcal{CP}$-violating phenomena in search of new physics beyond the Standard Model. However, most proposed experimental strategies and their early realizations to date have been limited to proof-of-principle molecular species with effectively spin-zero nuclei that are not sensitive to nuclear symmetry-violating phenomena. Here, we introduce a comprehensive experimental toolbox that integrates cooling, trapping, coherent state manipulation, and a complete precision-measurement protocol that is applicable to molecules carrying relevant nuclear spins. Using ${}^{137}$Ba${}^{19}$F and nuclear-spin-dependent parity violation (NSD-PV) as representative species and benchmark application, respectively, our approach achieves a projected statistical sensitivity roughly two orders of magnitude beyond comparable molecular beams by combining techniques already demonstrated individually in current experiments. This level of precision could provide realistic experimental access not only to the enhanced NSD-PV signals arising from the heavy ${}^{137}$Ba nucleus within this molecule but also to the contributions from the lighter ${}^{19}$F nucleus, bringing direct benchmarks of nuclear ab initio theory within reach. We further identify a candidate magic wavelength as a route to second-scale rotational coherence in future experiments. The techniques developed here can be transferred to measurements of nuclear Schiff and magnetic quadrupole moments in molecules containing deformed nuclei, establishing a general platform for laboratory searches for nuclear symmetry violations.

We report the observation of large anomalous shifts, up to +7.5 G, of the positions of the 33.6 G and 39.9 G Feshbach resonances in potassium-39 atoms confined in a 1063.9 nm optical dipole trap (ODT) at temperatures up to around 35 {\mu}K and trap depths up to about 136 {\mu}K. When the atom cloud is cooled to lower temperatures, by reducing the trap depth of the ODT, the shifts decrease proportionally with trap depth and approach zero at zero depth. We show that the large observed shifts originate from a large differential ac Stark shift between the incoming pair of potassium-39 atoms and the weakly bound Feshbach molecule, which in turn originates from an unexpectedly large dynamic polarizability of the Feshbach molecule. The polarizabilities of the Feshbach molecules extracted from the measured shifts of the 33.6 G and 39.9 G resonances are about four to seven times the sum of the polarizabilities of the two incoming potassium-39 atoms, that is, about four to seven times larger than the usual polarizability of weakly bound Feshbach molecules. The large polarizabilities of the Feshbach molecules are attributed to a near-coincidence between the frequency of the 1063.9 nm ODT laser and the frequency of a molecular transition from the last vibrational level of the lowest triplet a3{\Sigma}+u potential to a vibrational level of the excited b3{\Sigma}+g potential. Other potassium-39 Feshbach resonances we have studied exhibit a zero or very small shift, corresponding to molecular polarizabilities close to the sum of the polarizabilities of the two incoming potassium-39 atoms.

Distributing entanglement between distant qubits is a crucial element of scalable quantum computing. Here, we describe a scalable quantum interconnect that generates remote entanglement at rates approaching those compatible with two-qubit gates of current neutral-atom quantum processors. The proposed approach exploits the strong dipole-dipole interactions between atomic Rydberg states to generate entanglement between stationary qubits and propagating photons, without the need for an optical cavity. We provide a thorough description of the optimal conditions for the developed entanglement-generation protocol for realistic experimental parameters and demonstrate that entanglement-generation rates $\gtrsim 3\times 10^5$ s$^{-1}$ can be achieved using Rydberg states of ytterbium atoms. Given the inherent scalability and design flexibility of the proposed interconnect, our results suggest a promising approach towards distributed networks based on neutral-atom quantum architectures.

Studies of anions are inherently more challenging than investigations of neutrals and cations because of the diffuse and weakly bound character of an anionic electron. Here, we present a comprehensive computational examination of ground-state diatomic molecular anions composed of alkali-metal (Li, Na, K, Rb, Cs, Fr) and alkaline-earth-metal (Be, Mg, Ca, Sr, Ba, Ra) atoms. We study 21 alkali-metal diatomic anions in the X$^{2}\Sigma^{+}$ electronic state and 36 alkali-metal–alkaline-earth-metal diatomic anions in the X$^{1}\Sigma^{+}$ electronic state. The calculations employ a hierarchy of the coupled cluster methods, combined with large Gaussian basis sets and small-core relativistic energy-consistent pseudopotentials for heavier elements. We compute potential energy curves, permanent electric dipole moments, and static polarizabilities, and we assess convergence and uncertainties of our results. Additionally, using the multireference configuration interaction and equation-of-motion electron-attachment coupled cluster methods, we investigate excited electronic states of alkali-metal molecular anions, including valence-bound and dipole-bound states. We predict crossings between ground neutral and excited anionic states, which may enhance resonant electron attachment and subsequent anion dissociation. This finding may be relevant for experiments with mixtures of ultracold ground-state alkali-metal molecules and Rydberg atoms.

Rydberg entangling gates in optical-tweezer arrays are commonly executed with the trapping light switched off, so every gate contains a release–and–recapture cycle that heats the atomic motion and can ultimately limit circuit depth. We develop a motional refocusing protocol that exactly removes this heating in the harmonic approximation using only programmable intensity switching of the trapping light. The protocol closes the release–and–recapture cycle for every matched harmonic mode, returning arbitrary motional populations and coherences exactly up to ordinary evolution under the static trap. We derive the recovery sequence in closed form for arbitrary catch depth and prove that, within the experimentally relevant regime, it is the unique globally time-optimal solution under bounded trap intensity. The harmonic theory is then extended in two directions. First, we construct exact common-intensity recovery sequences that simultaneously refocus several nondegenerate harmonic modes, including radial–axial and fully anisotropic three-dimensional traps. Second, we derive a composite sequence that suppresses the leading anharmonic correction of weakly anharmonic traps by canceling all first-order motional transitions induced by the quartic anharmonicity, changing the residual heating law from $U_0^{-2}$ to $U_0^{-4}$. Wave-packet simulations in realistic Gaussian tweezers validate the analytic theory and quantify the residual effects of anharmonicity, finite switching ramps, trap ellipticity, and control errors. Applied to representative cesium Rydberg gates, the protocol suppresses the dominant recapture heating to the anharmonic floor and prevents the associated motional Doppler contribution from increasing with circuit depth. The resulting framework provides a practical route toward heating-free trap-off neutral-atom gates using only trap-intensity modulation.

Deviations from both the ideal linear Paul trap (LPT) geometry as well as the ideal quadrupole driving scheme introduce imperfections to ion trapping potentials. We investigate the effects of these imperfections in a LPT operated in a conventional dipole-drive configuration. We demonstrate the trapping of the Li$^+$ ions along the axial direction with zero and negative end-cap voltages. This occurs due to the modified axial $a-q$ space resulting from radial-to-axial coupling of the electric field. The dipole drive configuration lifts the degeneracy of the radial trapping potentials, resulting in unequal radial secular frequencies, and this is demonstrated experimentally. The combined effects of dipole drive and trap dimensions are summarized in a two-dimensional map that quantifies deviations from ideal behaviour. Based on this map, we propose a geometric modification that significantly reduces radial-to-axial coupling of the potential.

Neurtal atoms in optical tweezer arrays constitute a highly promising platform for quantum computing and quantum simulation. Their operation relies on precise control of the Rydberg excitation, which is highly sensitive to background electric fields. Here, we identify a previously overlooked source of stray electric fields arising from trapped charges within the antireflection coating layers of glass vacuum cells. In contrast to the conventional approach of removing surface charges through ultraviolet-light-induced desorption, we compensate these clamped charges by generating additional charges via photo-ionization of a cold atomic ensemble. We verify the resulting suppression of stray electric fields through Rydberg excitation spectroscopy in an atomic array and further confirm that the residual electric field inside the vacuum cell is effectively eradicated with the aid of external electrodes. Our work identifies and mitigates a previously unrecognized source of residual electric field, providing a practical solution for improving the performance of neutral atomic quantum processors and other Rydberg-based quantum technologies, as well as surface-sensitive atomic systems.

Generalized squeezing interactions are foundational to quantum optics, and have recently come under experimental control in hybrid spin-oscillator quantum processors [O. Băzăvan, et al., Nat. Phys. 22, 757 (2026); S. Saner, et al., Phys. Rev. X 16, 021049 (2026)]. These interactions open the door for new applications in the processing of discrete- and continuous-variable quantum information, four of which we propose and investigate in this work: geometric phase gates mediated by spin-dependent generalized squeezing acting on two spins and a common oscillator; genuine N-body spin interactions mediated by individually addressed spin-dependent generalized squeezing; oscillator thermometry via spin readout; and the preparation of high-fidelity quantum states of the oscillator via spin-dependent generalized squeezing and mid-circuit measurement. A unifying feature of these applications is the geometric phase induced by generalized squeezing interactions, which is nonlinear in the Fock occupation of the oscillator and the interaction order of the generalized squeezing. This work provides a foundation for fast, high-fidelity discrete- and continuous-variable quantum computation and sensing in the hybrid spin-oscillator platform via generalized squeezing.

Quantum computational advantage is generally attributed to coherent interference and other non-classical resources, yet their respective roles remain difficult to disentangle in experimental platforms where multipartite entanglement is inherently present. High-dimensional quantum systems provide an attractive route for investigating these resources while simultaneously reducing hardware overhead for quantum information processing. Here we realize a programmable four-dimensional optical qudit encoded in a single trapped $^{138}\mathrm{Ba}^{+}$ ion and demonstrate universal coherent control through phase-programmable optical rotations. Using this platform, we implement an entanglement-free realization of Grover's quantum search algorithm, achieving target-state identification probabilities of up to $94.5\pm2.0\%$. Within the same processor, we further demonstrate state-dependent quantum contextuality through a Clauser–Horne–Shimony–Holt (CHSH)-type noncontextuality inequality, obtaining a maximum violation of $S = 2.816 \pm 0.082$, in close agreement with the Tsirelson bound. By integrating programmable quantum computation and contextuality measurements within a single multilevel trapped-ion platform, our work establishes a versatile architecture for investigating the relationship between coherent interference and contextuality in quantum information processing and provides a scalable route toward high-dimensional quantum technologies.

We present a theory of the collective tunnel effect in atomic systems subject to strong low-frequency laser fields. Using an analytic semi-classical method and numerical solution to the time-dependent Schrödinger equation we demonstrate the collective channel of the nonsequential double ionization in a model two-dimensional two-electron system with ionization potentials reproducing those of neutral xenon and of the negative bromine ion. Collective tunneling in the presence of the electron-electron repulsion comprises the joint sub-barrier motion of the two electrons along quantum trajectories transversely shifted in opposite directions with respect to the direction of the external electric field. Analytic results for the rates of collective tunneling allow indicating the intervals of laser intensity, where this effect can be expected to compete with sequential tunneling in helium, xenon, and negative bromine. Momentum distributions of the electron pairs carry clear signatures of the collective channel in the form of shoulders in the direction lateral to the field polarization.

Rare-earth ions in crystals are useful in precision measurements and quantum information science because of their exceptional optical and spin coherence properties. We show that the nuclear spin coherence time of $^{153}\mathrm{Eu}^{3+}$ ions doped into yttrium orthosilicate can be significantly enhanced by driving the $^{89}\mathrm{Y}$ nuclear spins in the host crystal. This improvement in spin coherence time opens up ways to improve the precision of measurements using rare-earth-doped crystals.

Rydberg atoms have emerged as a versatile platform for quantum optics due to their exaggerated properties, particularly their strong long-range interactions, which enable a new regime of light-matter interaction. By mapping the interactions between Rydberg atoms onto photons, effective photon-photon interactions can be realized at the single-photon level, thereby overcoming the intrinsic weakness of conventional optical nonlinearities. In this review, we first introduce the fundamental physical principles of Rydberg-mediated quantum optics, and then discuss some key developments, including single-photon engineering, photonic quantum gates, contactless nonlinear optics, and quantum entanglement, providing a comprehensive overview of the current state and prospects of this rapidly developing field.

We report precise measurements of inter-level interactions in a bosonic optical lattice clock based on $^{88}$Sr atoms. We observe a nonlinear density dependence of the clock shift, even without reaching quantum degeneracy. In a 2D lattice, the Rabi line shape exhibits an interaction sideband consistent with a collective spin model, while in a 1D lattice the shift is modified by density-induced dephasing. These findings, combined with a careful choice of interrogation detuning and atomic density, can enable operation at a net-zero systematic density shift in $^{88}$Sr lattice clocks. We discuss the implications of these findings in many-body physics, quantum simulation, and precision isotope shift measurements, which provide a powerful probe for new physics beyond the Standard Model.

In spite of recent advances, quantum computers are expected to be sufficiently noisy in the coming few years to the extent of limiting quantum chemical calculations to relatively small number of orbitals. However, even with reasonable quality single particle basis sets, small active spaces with limited orbitals can result in a significant fraction of correlation energy being lost, motivating the design of moderate quality qubit-efficient basis sets for quantum algorithms. We begin by reoptimizing the existing minimal basis sets using a genetic algorithm-inspired approach in conjunction with aggressive refinement strategies, and generate modified minimal basis sets (MSTO-kG basis; k = 2-11) for atoms from H through F. The ground state energies of H through F using our MSTO bases at FCI level of theory yield ground state energies that are comparable or sometimes even lower than those obtained using 6-31G basis sets. In the case of Li, the MSTO bases surpass the performance of cc-pVQZ bases. Thus, we obtain better atomic energies with same number of qubits relative to STO bases, and better/comparable energies with fewer qubits relative to higher quality bases. In the case of molecules, H2 performs poorly; a finding that is consistent with an earlier work in literature. For other molecules, Li2, C2, LiH, BeH and BeH2, the FCI results (except C2 for which we employ CISD) from our bases are comparable to/outperform those from 6-31G basis. Finally, we compare the resources required between different bases and find that MSTO bases yield better energies than the competing basis sets while incurring fewer qubits and two-qubit gates with VQE, QPE, and HHL. The logical T-gate counts are also found to be considerably lower for QPE and HHL respectively. Overall, our work paves way for more accurate yet less qubit-hungry quantum chemical calculations using near-term quantum computers.

We report a measurement of the optical frequency ratio between the $^2\mathrm{S}_{1/2}(F=0)$–${^2\mathrm{F}_{7/2}(F=3)}$ electric-octupole (E3) transition of $^{171}$Yb$^{+}$ and the $^1\mathrm{S}_0$–${^3\mathrm{P}_0}$ transition of $^{87}$Sr, $\nu_{\mathrm{Yb}^{+}}/\nu_\mathrm{Sr} = 1.495\,991\,618\,544\,900\,588\,1(65)$. Reaching a fractional uncertainty of $4.3 \times 10^{-18}$, this result improves upon the previous best by more than a factor of three and is among the few that meet the requirements for interspecies clock comparisons specified by the roadmap towards the redefinition of the SI second. The comparison is between a transportable optical lattice clock and a stationary single-ion clock. It spans a period of nearly two years, during which the transportable clock was intermittently operated off-campus. The ratio was reproducibly measured during four separate campaigns, which are consistent within their statistical uncertainties. The results demonstrate reproducible $10^{-18}$ level operation of the transportable clock and thus validate its application for chronometric geodesy and as a transfer standard for inter-institute clock comparisons, e.g., in the absence of optical fiber links.

Achieving joint quantum-enhanced precision in multiparameter sensing requires both high sensitivity and measurement compatibility. These two aspects are characterized by the quantum Fisher information matrix (QFIM) and the Uhlmann curvature matrix (UCM), respectively, with weak compatibility corresponding to the vanishing of the relevant UCM elements. Here, we develop a symmetry-projection framework that classifies phase generators into subspace-preserving and subspace-changing sectors. For probe states confined to a symmetry subspace, symmetry projection imposes a common block-diagonal structure on the QFIM and UCM, rendering cross-sector parameters simultaneously free from information cross-talk and measurement incompatibility. When the subspace-changing generators act as scalars within the occupied subspace, the corresponding QFIM block reduces to four times the symmetrized covariance matrix, even for mixed probe states. For parity-protected collective $\mathrm{SU}(2)$ systems, this structure singles out the transverse anti-squeezed quadrature and the longitudinal mean-spin direction as natural optimal sensing axes. Applied to a dissipative one-axis twisting model, the dynamically generated probe state exhibits identically vanishing UCM elements for transverse–longitudinal parameter pairs, while maintaining nearly balanced, Heisenberg-scaled QFIM components over a broad transient window. Our work opens a route to symmetry-protected, weakly compatible multiparameter sensing in interacting quantum many-body systems.

We introduce a validation process that harnesses engineered many-body relaxation to control and calibrate quantum hardware. On two independently developed neutral-atom processors, we realize the many-body quantum Mpemba effect in an open system for the first time. Initial-state engineering creates fast and slow relaxation pathways: the fast pathway opens access to unreachable mixed-state physics before hardware noise obscures the target dynamics, whereas the slow pathway amplifies hidden imperfections in preparation and control. Computational-basis measurements directly and independently benchmark dynamical reliability, revealing each processor's actual operating window as a many-body simulator. The processors are thus judged by the very dynamics they are built to reproduce. Complementary responses disentangle control errors and drive an adaptive, time-resolved scheme that supplies hardware developers directly actionable corrections, enhancing faithful reproduction of the target dynamics. These results establish many-body relaxation as a transferable validation and calibration tool for programmable quantum processors.