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Physics Condensed Matter

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Tuesday 29 September

Soft Condensed Matter

Tactile Perception through Fluid-Solid Interaction

Soft tactile sensors elevate robotic touch through enhanced flexibility and adaptability, yet most existing designs depend on embedded electronics that are susceptible to interference and environmental limitations. In this work, we leverage fluid-solid interactions to develop a class of soft tactile sensors that operate entirely without electronics at the sensing site. The sensor comprises a fluid-filled elastomeric channel connected to only two external pressure sensors. Touching different regions of the elastomeric surface displaces the viscous fluid, producing distinct pressure patterns that encode both touch position and force. These signals are decoded through a machine learning framework that integrates feature extraction, soft clustering, and adaptive neuro-fuzzy inference to achieve accurate localization and force estimation. We validate this concept through single-point touch localization and force estimation in a linear (1D) sensor and extend the same sensing principle to 2D tactile mapping by routing the channel across the surface using space-filling curves, while maintaining the same minimal hardware setup. This simple approach remains effective in environments where conventional electronic sensors often fail, such as underwater or in the presence of magnetic interference.
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All authors Arman Goshtasbi, Minke Berghuis, Aida Parvaresh, Saravana Prashanth Murali Babu, Robert W. Style, Ahmad Rafsanjani

Mesoscale and Nanoscale Physics

From Dirac surface response to Casimir forces in Bumblebee-CFJ electrodynamics

We examine the Casimir interaction between planar massive Dirac materials coupled to a Lorentz-violating Bumblebee-CFJ vector sector. The standard renormalized one-loop polarization tensor of the Dirac quasiparticles is used as the nonlocal surface response in the Lifshitz scattering formalism. For the normally oriented Lorentz-violating background, the surface response remains parity-even. Hence, the repulsive regimes do not originate from a Hall-like conductivity. Instead, they arise from the CFJ-induced mixing of TE and TM bulk modes, combined with the spatially dispersive response of the Dirac sheets. Furthermore, we show that the Dirac mass suppresses the interaction and changes its large-distance scaling, whereas the CFJ parameter drives transitions between attractive and repulsive regimes.
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Superconductivity

Reply to "Comment on 'Topography of Fermi arcs in t-PtBi2 using high-resolution angle-resolved photoemission spectroscopy'"

In a recent work [1] we demonstrated that the Fermi arcs in t-PtBi2 are indeed disconnected segments of the Fermi surface. We showed that the surface state band crosses EF between Weyl points and is has finite band gap at all other momenta until it merges with bulk bands. We did not find evidence of a superconducting gap in the spectra down to 3K. In recent Comment, Sergey Borisenko reanalyzed data from repository posted with our paper and concluded that a superconducting gap with i-wave symmetry is present in our data up to temperatures of 19K. We argue that this claim arises from incorrect identification of the location of Fermi arc and confusion between band gap and superconducting gap. This error was compounded by the fact that Author of the Comment analyzed data from interpolated images used for mapping the Fermi surface that are not suitable for extraction of energy gap on meV scale. This fact was previously communicated to the Author of the Comment during e-mail exchange. We maintain that our conclusion of absence of a superconducting gap above 3 K are valid and consistent with recent STM measurements performed on the same samples, which found surface superconductivity with Tc = 3K, below the temperature at which the data for our ARPES paper was measured.
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Materials Science

Thermodynamic origins of multimode spinodal decomposition in multicomponent alloys

In a binary alloy, spinodal decomposition has one composition direction in which the free energy can fall. A multicomponent alloy has more directions available, yet its elements usually separate together in a single, pseudobinary mode. Why does this happen, and what would allow two independent directions to become unstable? We examine these questions using binary interaction parameters and the composition-constrained curvature of the regular-solution free energy. Across equimolar BCC quaternaries, one unstable mode is the most common outcome at 500 K, while 15.2% have at least two. The tendency of unlike elements to mix helps explain the preference for one mode. We then show how particular arrangements of interactions, including a balanced repulsive triangle and an attractive-repulsive pair, guarantee two downhill directions. When those directions have similar strengths, simplified phase-field models produce a broad texture of locally different solid solutions rather than two chemical blocks. A phase-specific screen identifies five provisional alloys with nearly balanced modes, with Cu-In-Ir-Ti providing an example of this possibility. Thus, we establish a theoretical framework for engineering microstructures via spinodal decomposition derived from basic binary interaction tendencies.
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Mesoscale and Nanoscale Physics

From Quantized Hall Plateaus to Topological Surfaces: Quantum Capacitance as a Unifying Probe

The quantum Hall effect, topological insulators and quantum capacitance are usually treated as distinct topics, yet they share a common thread. Bulk topology determines a protected boundary state, and quantum capacitance is one of the few electrostatic methods able to detect the density of states. This paper examines that connection. The integer quantum Hall effect showed that quantised boundary transport has a topological origin given by the Chern number, later extended to zero field in Z2 topological insulators with helical edge and Dirac surface states. Quantum capacitance, developed for two-dimensional electron gases, has since become a key technique for mapping the Landau level density of states underlying the quantum Hall effect and the linear Dirac density of states of topological surface states. This picture is complicated by self-consistent screening theory, which shows that the quantum Hall bulk splits into compressible and incompressible regions that shift with field. Local quantum capacitance measurements confirm that the bulk is not uniformly insulating across a quantised plateau, even though the plateau stays quantised. The paper argues that quantum capacitance is not a secondary feature of these phenomena but one of the clearest windows into the boundary density of states that topology imposes, and that it reveals the local, field-dependent nature of the insulating bulk assumption underlying the analogy between the quantum Hall effect and topological insulators.
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Mesoscale and Nanoscale Physics

Interior contacts in a narrow quantum Hall bar: a two-dimensional self-consistent screening calculation of the current distribution

We present fully two-dimensional self-consistent calculations of the electron density, local filling factor and current distribution in a six-terminal GaAs/AlGaAs Hall bar of width W = 3 micrometers with two additional square contacts, A and B, placed on the channel axis and connected to the outside by air bridges, following the interior-contact experiment of Kendirlik et al. [Nat. Commun. 8, 14082 (2017)]. Within the screening theory of the integer quantized Hall effect, the Thomas-Fermi-Poisson equations are solved on the full device plane, including the probe arms and the depletion regions around the interior contacts, and the current is obtained from a local Ohm's law with a filling-factor dependent conductivity tensor, for source-drain and interior-contact excitation separately. Across the nu = 2 plateau the interior contacts pass through three regimes as the field is lowered: galvanically connected to the current path in a compressible bulk, floating in the Hall potential of a fully incompressible bulk, and isolated from both the bulk and the edge strips by closed incompressible rings encircling each contact. In the floating and isolated regimes the two-terminal resistance between the interior contacts rises by orders of magnitude. The isolation interval lies within the Hall plateau and ends before its low-field edge; its high-field end is sharply set by the disappearance of the incompressible bulk, while its low-field end shrinks with temperature and Landau-level broadening. The resistance between an interior contact and a perimeter probe approaches one half of the quantized Hall resistance across the plateau. The topology of the incompressible regions and the boundaries of the isolation interval are insensitive to the regularization of the local conductivity, to the grid and to moderate disorder, whereas the magnitude of the isolation resistance is not.
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Strongly Correlated Electrons

Causality violations in cluster GW+DMFT: Exact Lehmann moments and the necessity of non-local vertex corrections

The $GW$ approximation is known to violate causality, yielding self-energies with unphysical poles in the upper half of the complex frequency plane. The combined $GW$+DMFT approach attempts to cure this by injecting the exact local self-energy. Using exact diagonalization on minimal Hubbard clusters, we rigorously benchmark the analytic structure of the $GW$ and $GW$+DMFT self-energies. We demonstrate a “dimer anomaly”: on the two-site dimer, inversion symmetry forces the non-local self-energy to be purely real, masking the causality violation. Moving to the non-bipartite three-site Hubbard ring, where hopping frustration yields a finite imaginary part in the non-local self-energy, we prove that both $GW$ and $GW$+DMFT violate the Matsubara causality condition. By analytically evaluating the exact Lehmann moments, we derive a closed-form expression for the high-frequency tail of the self-energy, $C = U^2\,\mathrm{Var}(d)\,I$, and show that standard methods fail to capture the exact equal-time two-particle correlators required to enforce it. The equal-time correlators that govern this tail are precisely those encoded in the high-frequency asymptotics of the fully irreducible vertex $\Lambda$; nevertheless, our intermediate-frequency analysis demonstrates that the local-only truncation of $\Lambda$ in $GW$+DMFT leaves non-local RPA resonances uncorrected. The two diagnostics are logically independent: $GW$+DMFT satisfies the necessary high-frequency condition $C\succeq0$ yet still violates the Matsubara sign condition at finite frequencies. Taking the interpolation-free real-axis evaluation of the exact self-energy as the primary causality certificate, with rational continuation as supporting evidence, we establish a rigorous benchmark demonstrating that local self-energy corrections are insufficient to guarantee a causal analytic structure on frustrated clusters.
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Soft Condensed Matter · Cross-listed from q-bio.BM

Ca$^{2+}$-tunable mechanics and recoil in reconstituted Tcb2 networks

Tetrahymena calcium-binding protein (Tcb2) forms Ca$^{2+}$-responsive networks that exhibit contractile behavior, yet how Ca$^{2+}$ concentration controls their local mechanical response remains poorly understood. Here, we use optical tweezers to perform active microrheology on reconstituted Tcb2 networks inside a microfluidic device that enables precise control of Ca$^{2+}$ concentration, allowing systematic tuning of network structure and mechanics. We find that increasing Ca$^{2+}$ from 1 to 100~mM enhances the effective stiffness by nearly two orders of magnitude, from $\sim$1$\times$10$^{-3}$ to $\sim$7$\times$10$^{-2}$~pN/nm, corresponding to a transition from a viscosity-dominated to a more elastic and mechanically robust network. Recoil assays further reveal rapid release of stored elastic energy following deformation. After two orthogonal pulls, the bead recoils along the diagonal rather than retracing the loading path, indicating that stresses from different directions combine to produce a resultant restoring response. These results establish Tcb2 networks as a minimal, tunable system for probing chemomechanical coupling and viscoelasticity in Ca$^{2+}$-regulated protein networks.
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All authors Xiangting Lei, K. R. Prathyusha, Carlos Floyd, Jerry Honts, Saad Bhamla

Soft Condensed Matter · Cross-listed from physics.flu-dyn

Directional Control of Droplet Motion via Geometric Gating

We explore new methods for inducing the movement of water droplets on elastomeric substrates, such as polydimethylsiloxane (PDMS). Our approach builds upon the well-known phenomenon that water droplets move easily across these substrates when swelled w,ith silicone oil. While designing shallow open channels and traps on a PDMS film offers a simple way to control a droplet's trajectory by tilting the substrate in two orthogonal directions, this method is poorly suited for manipulating multiple droplets simultaneously. To address this limitation, we introduce two new methods. The first method utilizes a plano-concave PDMS platform with a radius of curvature significantly larger than the size of the droplet and its translation distance. When the system's configuration is altered, this curved substrate consistently guides the droplet along a curved geodesic. The second method incorporates diode-like gates on the PDMS. These gates are created on either flat or plano-concave PDMS films by embedding thin, rigid plates into the elastomer prior to crosslinking, followed by swelling in silicone oil. This process generates sigmoidal steps that restrict droplet motion to a single direction. Finally, we demonstrate how combining these two strategies enables various forms of directed motion for both single and multiple droplets.
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Mesoscale and Nanoscale Physics

Three-Dimensional Shankar Skyrmions in Frustrated Antiferromagnets

We formulate a continuum theory for three-dimensional (3D) Shankar skyrmions in frustrated chiral antiferromagnets (AFs) and derive the conditions for metastable finite-size $\pi_3(SO(3))$ solitons. A Derrick–Hobart scaling analysis shows that exchange, Dzyaloshinskii–Moriya interaction (DMI), anisotropy, and frustration can balance to set a finite equilibrium size. We identify two microscopic routes to this common topological and stabilization framework: intrinsic rotation-frame order in noncollinear AFs and an $\mathbb{S}^3$ extension of an amplitude-softened Néel field. In the latter, the smooth four-component texture projects onto a Néel field containing a spatially separated pair of oppositely charged Bloch points. Numerical minimization yields metastable monopole textures, while the effective dynamics identifies coherent breathing oscillations as their characteristic finite-frequency collective mode. Our results provide a microscopic framework for the statics and dynamics of Shankar skyrmions and identify frustrated chiral AFs as promising hosts of 3D non-Abelian topological textures.
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All authors Vladyslav M. Kuchkin, Ricardo Rama-Eiroa, Carlos Saji, Alvaro S. Nunez, Roberto E. Troncoso

Strongly Correlated Electrons

Theory of criticality-enabled $U(1)$ symmetry breaking in a class of 1+1D systems

We develop an analytic theory of the recently proposed $U(1)$ symmetry breaking at interacting 1+1D Lifshitz quantum critical points. The low-energy theory contains two compact fields, $\theta$ and $\phi$, coupled by a Berry term that makes $\theta$ canonically conjugate to the conserved density $\partial_x\phi$. Within a controlled large-$N$ limit, we establish long-range order (LRO) of $e^{i\beta\theta}$ and stretched-exponential decay of the conjugate vertex, $\log\langle e^{i\beta\phi(x)}e^{-i\beta\phi(0)}\rangle\propto-|\beta|^{4/3}|x|^{2/3}$. Beyond large $N$, we argue that $U(1)$ LRO follows if the dynamical exponent satisfies $z\neq1$, consistent with existing calculations. Using finite-size and infinite-system DMRG, we study an itinerant-electron chain with $U(1)\rtimes\mathbb{Z}_2$ symmetry, whose spin sector realizes this theory at a ferromagnetic quantum critical point. We find spin-nematic LRO in $S_i^+S_{i+1}^+$ and stretched-exponential electron Green's functions, revealing distinctive non-Gaussian signatures of criticality-enabled order.
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All authors E. S. Andriyakhina, A. S. Shankar, T. Senthil, Z. D. Shi

Strongly Correlated Electrons · Cross-listed from nucl-th

Effective Contact Theory for Exotic Loosely Bound States in Strongly Interacting Expanding Matter

Short-distance correlations generate universal relations that can be independent of microscopic details. Tan's contact is a prominent example, connecting close pairs, high-momentum constituents, and bound-state formation across atomic, condensed-matter, and nuclear systems. Whether an analogous universality governs the nonequilibrium freeze-out of relativistic QCD matter is an open question. We develop an effective contact theory that relates the production of loosely bound states to continuum two-particle correlations in heavy-ion collisions. The construction replaces the hard relative-momentum cutoff of conventional coalescence by a regulated Bethe–Peierls kernel: freeze-out localization fixes its momentum scale, while the composite yield fixes its contact residue. Bound and continuum observables then become projections of a common two-particle density matrix rather than independent phenomena. Coulomb-bound $K\mu$ atoms provide an ideal realization because their atomic, production, and source scales are widely separated. A contact-theory analysis of STAR $d\Lambda$ correlations supplies a first bound–continuum consistency test and demonstrates how inferred near-threshold parameters can depend on the finite expanding source. The framework establishes a general strategy for relating coalescence, correlations, and exotic bound states in strongly interacting expanding matter.
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All authors Xiaofeng Wang, Zebo Tang, Zhangbu Xu, Chi Yang, Wangmei Zha

Materials Science

Enabling Domain-Specific Atomistic Models: A Machine Learning Potential for the Solid Acid Family

Machine-learned interatomic potentials trained across the periodic table have made atomistic simulation broadly accessible, and specializing them to a single compound class is widely expected to improve accuracy. Yet examples remain scarce, and fewer still surpass universal models in speed or reach a higher level of electronic-structure theory. Here we present a potential that is universal within the class of water-free solid-state hydrogen-bond network mediated proton conductors rather than across chemistry and a database of 4.4 million first-principles configurations spanning 55 materials. It surpasses leading general-purpose potentials across this domain, recovering measured activation energies and the ordering of anion rotational dynamics that those models miss; agreement on static structure does not imply agreement on transport. Accuracy falls for compositions far from the training set but stays competitive for close structural relatives, and a higher level of electronic-structure theory is reached with a few hundred additional configurations per material. We further introduce a compact variant carrying a fifth of the parameters, faster still and yet more accurate than every general-purpose model tested. It sustains more than a quarter of a million atoms on a single graphics processor, placing grain boundaries and the transition into the highly conducting phase within reach, and making a quantum treatment of the protons affordable. Reference accuracy and accessible system size thus become largely independent, offering a template for other compound classes.
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Materials Science

Single-particle detection of the Néel transition in LaCrO$_3$ microcrystals via widefield nitrogen-vacancy center magnetic imaging

Rare-earth orthochromites exhibit rich, chemically tunable magnetic behavior, making them attractive for temperature sensing and temperature-dependent switching applications. Realizing this potential requires understanding how synthesis conditions and particle morphology influence the underlying Cr$^{3+}$ magnetic ordering. Orthochromite magnetism has traditionally been characterized by ensemble techniques such as neutron diffraction and SQUID magnetometry, which report only averaged magnetic properties and cannot access particle-level information. Here we use widefield nitrogen-vacancy (NV) magnetometry to image the stray magnetic fields of individual LaCrO$_3$ microcrystals produced via molten salt synthesis, resolving the antiferromagnetic Néel transition in single particles. Of the 18 particles measured between 278 and 298 K, five show a clear onset of magnetization near the ensemble Néel temperature, four show no measurable magnetic signal, and nine display temperature-independent signatures consistent with localized magnetic impurities undetected by ensemble measurements. Below the Néel temperature, particle magnetization remains fixed under a rotating in-plane field, consistent with canted antiferromagnetic ordering rather than paramagnetism, while repeated thermal cycling shows that the magnetic field pattern varies between cooldowns with certain features recurring at the same locations, consistent with micron-scale structurally pinned antiferromagnetic domains in which the sign of the weak ferromagnetic moment is set independently each time they pass through the Néel transition. These results establish single-particle NV magnetometry as a sensitive probe of magnetic ordering and domain structure in individual microcrystals, a key step toward correlating individual particle morphology and defect structure with magnetic ordering in orthochromites.
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All authors Carson O. Patterson, Ethan Q. Williams, Eden Tzanetopoulos, Benjamin C. Li, Rachel T. Smith, Matthew Chang, Hideyuki Watanabe, Daniel R. Gamelin, Kai-Mei C. Fu

Soft Condensed Matter

Modeling density variations in two-dimensional microtubule-based active nematics

A dense two-dimensional layer of aligned microtubules (MTs), powered by molecular motors, is a canonical laboratory model of active materials and a synthetic analog of biological systems such as bacterial turbulence, mitotic spindles, and morphogenesis. This material exhibits nematic ordering and associated topological defects, which display complex emergent dynamics, including the creation and annihilation of defects and the braiding of defects around one another in a complicated chaotic dance. Despite its prominent role in research, the MT-based active nematic material lacks a well established theoretical model that accurately captures the rich density variations prominently seen in experiments—density variations that are, in fact, the experimental signature of the nematic structure itself. The MT-system is typically modeled using two fields: the Q-tensor (encoding the order and orientation of the nematic phase) and the fluid velocity; critically, the microtubule density is assumed to be constant. This traditional model is adopted from classical Landau-de Gennes liquid crystal theory. Here, we present a fundamentally different approach to modeling MT-based active nematics that explicitly incorporates density variations, producing simulations that strongly resemble experimental videos, including the characteristic striation patterns. It also reproduces important behavior of the system confined to a circular well—behavior seen experimentally, but not captured by current theory. In crafting our model, we present an alternative to Landau-de Gennes theory for the creation and annihilation of topological defects that does not rely on the classic isotropic-nematic phase transition.
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All authors Kevin A. Mitchell, Sean Ricarte, Md Mainul Hasan Sabbir, Brandon Klein, Daniel A. Beller

Soft Condensed Matter

Measures of Chaotic Advection in Simulations of Active Nematics

Active nematics are non-equilibrium fluids composed of rod-like self-propelled units that collectively generate large-scale coherent flows. Here, we focus on a canonical experimental system: an active nematic fluid in $2D$ driven by ATP, composed of densely packed, extended microtubule (MT) bundles cross-linked by kinesin motors. An intriguing feature of this system is the creation and annihilation of topological defects with topological charge $\pm1/2$, due to the fracturing of the material. Experiments confirm that the positive ($+1/2$) defects serve as "virtual stirring rods" that move around each other in a complex braiding pattern. This collective braiding motion of positive defects stretches and folds the fluid itself, i.e., produces macroscale chaotic advection. The degree of self-mixing due to the chaotic advection can be measured using topological entropy and the Lyapunov exponent. Our goal is to determine whether continuum models of MT-based active nematic fluid can reproduce these measurements. To this end, we use two continuum models: the traditional Beris-Edwards (BE) model and the more recently developed Beris-Edwards model with enhanced nematic locking (BENL). The difference between the two models is the adoption of the "nematic locking principle", which states that an individual MT bundle cannot rotate independently of its neighbors due to steric interactions among elongated dense MT bundles. This principle holds in the BENL model except in small localized areas of the material domain where the material fractures, specifically near the creation and annihilation of topological defects. We employ several numerical methods to estimate measures of chaotic advection using both models. Our study shows that the BENL model more accurately reproduces experimental measures of self-mixing driven by chaotic advection in MT-based active nematic fluids.
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All authors Md Mainul Hasan Sabbir, Brandon Klein, Daniel A. Beller, Kevin A. Mitchell

Materials Science

Results of Classical and Nonclassical theories of nucleation for ordering transition in barium titanate

Results of classical and nonclassical approach to nucleation at the ordering phase transition in barium titanate are presented. A nonclassical nucleation model is applied to the first-order paraelectric cubic phase to ferroelectric tetragonal phase transition in barium titanate is considered.
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Materials Science

Stress-based structure optimization for a range-separated hybrid van der Waals density functional

Complex matter, often partly soft and pliable, is the generic form of material systems. We must therefore generally call on density functional theory (DFT) to first predict the atomic structure before we can use it to also characterize (expected) properties. A recent range-separated hybrid (RSH) van Waals density functional (vdW-DF), `vdW-DF2-ahbr' (abbreviated AHBR) [PRX 12, 041003 (2022)], shows promise as a high-accuracy predictor of both binding energies and structure, from molecules to solids. However, the present implementation in Quantum Espresso (QE) does not, in our experience, support robust stress-based unit-cell optimization of RSHs. Here we document and illustrate work enabling practical AHBR-based complex-matter discovery: We port the AHBR XC functional to the Vienna Ab Initio Simulation Package (VASP) where use of stress-based DFT optimization is already stable also for RSHs. We test the implementation by comparing high-accuracy AHBR-QE and AHBR-VASP predictions of non-covalent molecular interactions and for structure and cohesion of simple bulk structures. We also illustrate and test the use of the new AHBR-VASP implementation to predict and understand (atomic and anti-ferromagnetic) structure in distorted-rocksalt metal monoxides. Finally, we illustrate use for complex-soft-matter discovery by predicting motifs for layer stacking in the C2N covalent-organic framework (COF) system [Nat. Commun. 6, 6486 (2015)].
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All authors Per Hyldgaard, Yunqi Shao, Raul Quintero-Monsebaiz, Lars Öhrström

Soft Condensed Matter · Cross-listed from physics.flu-dyn

Stable and Interpretable Multi-Mode Rheological Universal Differential Equations (mmRUDEs) for Data-Driven Constitutive Modeling

The Rheological Universal Differential Equation (RUDE) framework embeds neural networks within a frame-indifferent tensorial constitutive backbone and so enables data-driven discovery of complex material rheological behavior. However, the flexibility that makes the RUDE framework attractive also makes it difficult to deploy: the learned neural network correction can make the constitutive equation numerically stiff during training, distribute corrections across non-unique combinations of tensor-basis terms, and extrapolate poorly with increasing nonlinearity, especially for industrially relevant materials with broad relaxation spectra. We develop a stability- and reliability-focused multi-mode RUDE framework that addresses three key challenges: thermodynamic admissibility, out-of-distribution prediction, and interpretability. Logarithmic compression of the input invariants and a split-network architecture improve numerical conditioning during training, while a differentiable projection layer enforces the Clausius–Duhem inequality at every time step. We illustrate the framework with both synthetic (a multi-mode Giesekus model) and experimental data on an entangled silicone polymer melt. Both models were trained on LAOS; they remain stable and accurate under unseen flow conditions, including steady shear, transient stress growth, and extensional flows, for which the unconstrained models may diverge numerically. To aid in interpretation of the contributions of each learned correction to the rheological behavior, we introduce the rheome, a compact way of representing the dominant weighted tensor-basis contributions to the overall rheological behavior. These improvements to the RUDE framework lead to stable and interpretable trained models, paving the way for implementation in computational fluid dynamics simulations and for guiding the rational design of soft material processing operations.
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All authors Mohua Das, Nicholas King, Navid Azizan, Gareth H. McKinley

Soft Condensed Matter

Morphodynamics of lipid vesicles under osmotic forcing

We investigate the dynamics of spherical lipid vesicles subjected to an osmotic shock using continuum simulations of a permeable, area-incompressible fluid membrane with bending elasticity and surface viscosity. The dynamics are governed by a single dimensionless parameter $\varGamma$, which measures the relative strength of osmotic pressure and bending forces. Osmotic forcing drives a three-stage evolution comprising rapid buckling and collapse, smoothing of the resulting wrinkles and ridges, and slow folding into an invaginated morphology resembling the precursor to experimentally observed vesicle-in-vesicle structures. Linear stability analysis predicts the wavelength and growth rate of the initial buckling instability and shows that the dimensionless buckling time scales as $\varGamma^{-2}$, in quantitative agreement with simulations. At longer times, the energy budget reveals a reversal in elastic energy transfer: bending energy accumulated during buckling is released during relaxation and dissipated by membrane viscosity. A scaling analysis of the folding dynamics predicts that the dimensionless folding time scales as $\varGamma^{-2/3}$, again in excellent agreement with simulations. These results provide a continuum description of the mechanisms and widely separated timescales governing osmotically driven membrane collapse and invagination.
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Materials Science

Ab initio calculated diamagnetic and paramagnetic susceptibility of carbonate minerals

The anisotropy of magnetic susceptibility (AMS) is a widely used tool to infer rock fabrics, yet quantitative interpretation is limited by sparse single-crystal magnetic properties for rock-forming minerals and by the difficulty of separating intrinsic diamagnetism from impurity-related magnetism. Here we use density-functional theory (DFT) combined with perturbation theory to compute the diamagnetic susceptibility and AMS of calcite-group carbonates (calcite, magnesite, and dolomite) and to quantify the additional paramagnetic contribution from transition-metal doping. For pure calcite, the calculated susceptibility and its anisotropy are in good agreement with published single-crystal measurements, validating the ab initio approach for diamagnetic phases. We provide improved intrinsic diamagnetic reference values for magnesite and dolomite, for which experimental susceptibilities are commonly affected by magnetic impurities. To address impurity effects explicitly, we model Fe and Mn substitution in calcite using supercells. The computed spin moments reproduce expected high-spin states (Fe$^{2+}$, $S=2$; Mn$^{2+}$, $S=5/2$) and yield a susceptibility anisotropy per Fe concentration that matches the experimental slope. The strong anisotropy is primarily governed by an orbital contribution tied to the crystallographic $c$-axis rather than by spin-orbit coupling, highlighting orbital magnetisation as a key but numerically challenging ingredient for modelling of paramagnetic AMS in carbonates.
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All authors Jaroslav Hamrle, Matěj Machek, Vladimír K. Kusbach, Zuzana Roxerová

Soft Condensed Matter · Cross-listed from physics.bio-ph

Packaged DNA genome sets the long-range electrostatic anisotropy of a virus

Viruses are among the most highly charged objects in biology, and electrostatic interactions permeate nearly every stage of their life cycle. At the same time, an empty icosahedral capsid is almost isotropic as far as the surrounding electrolyte is concerned—its charge distribution is anisotropic only at high multipole order, and electrostatic screening removes such anisotropy long before it can be probed at a distance. Here, we show that the packaged genome of a filled virus imparts a long-range electrostatic anisotropy that extends throughout the surrounding medium, which is not present for empty capsids. We support these findings with a novel Poisson–Boltzmann continuum theory where the orientational order of dsDNA enters through an anisotropic dielectric tensor and an inhomogeneous volume-charge distribution, which is coupled to a charge-regulating shell containing ionizable amino acid residues of the capsid proteins. The resulting electrostatic potential profiles show that DNA packed in an inverse-spool geometry imprints a highly inhomogeneous potential distribution on the outer capsid surface, whose angular structure is a direct result of the DNA-free axial void. At high salinity, the multipole spectrum of this distribution persists at large distances, whereas at low salt concentration, higher-order multipoles decay more rapidly away from the surface. The surviving quadrupole renders virus–wall and virus–virus interactions orientation dependent at the $k_\mathrm{B}T$ level, with a preferred orientation controlled by the sign of the external charge and the pH. Using phage $\lambda$ as a model system and checking robustness of our results on two other phages, we find the same behavior across a range of pH and ionic strengths. This identifies the packaged genome, rather than the symmetry of the capsid, as the origin of the long-range electrostatic anisotropy of a filled virus.
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Materials Science

Energy-Efficient Non-Volatile Photonic Switching via Composition-Engineered Sn-Doped GST

Integrated phase-change photonics allows non-volatile optical switching with no static power draw, but the electrical energy needed to reversibly switch the material's state limits practical scaling. Efforts to improve energy efficiency have mostly focused on device optimization, such as redesigning the integrated microheater or waveguide. Here, we take a different, materials-centered approach by alloying Sn to Ge$_2$Sb$_2$Te$_5$ (GST) without altering the device structure or CMOS compatibility. We explore Sn concentrations ranging from 0 at.% to 20 at.% on waveguide-integrated PN and PIN heaters and observe a reduction in both the amorphization and crystallization energies in the 5–10 at.% range. At higher Sn content this trend reverses and the switching energy increases, which is suggestive of phase segregation when combined with TEM compositional analysis. A 10 at.% Sn device continues to switch over 1000 cycles, with observable degradation in the extinction ratio from 4.5 $\pm$ 0.3 dB to 2.4 $\pm$ 0.3 dB. Post-cycling imaging shows PCM migration and void formation which we believe can be further improved by enhanced encapsulation. Overall, Sn alloying offers a route to lower programming energy in integrated phase-change photonics without negatively affecting the switching speed relative to un-doped GST.
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All authors Xingyu Zhang, Daniel Vaz, Chi-Yi Kao, Marcus Tamura, Xiong Feng, Carlos A. Rios Ocampo, Bhavin J. Shastri, Nathan Youngblood

Soft Condensed Matter

Geometry and Mechanics of Ribbon Gridshells

Mechanical metamaterials exhibit anomalous properties induced from non-trivial mesoscopic constituents. Inspired from architectural and industrial structures, we introduce arrangements of long, narrow ribbons intersecting at prescribed angles as a model thin-sheet metamaterial. These ribbon gridshells are shown to display highly non-linear behavior driven by the geometric constraints, nonetheless unlike most complex mechanical systems, we are able to explicitly write out the coarse-grained governing equations and to classify their solutions in terms of the intersection patterns of the ribbons. It is shown that the structure can assume arbitrary, tunable Gaussian curvature distributions, allowing us to formulate an inverse design problem, solvable under a suitably defined local condition. An analysis of the soft modes, confirmed by experiment and numerics, reveals rich mechanics which may exhibit both a rigid and an anomalously soft behaviors.
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All authors Daniel Castro, Joo-Won Hong, Étienne Reyssat, José Bico, Benoît Roman, Hillel Aharoni

Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

Interferometric Readout of Momentum-Space Topology in a Programmable Dissipative Photonic Circuit

Topology under non-Hermitian dynamics is encoded in the phase of the bulk evolution, yet strong dissipation suppresses the amplitudes carrying it. We resolve this using a programmable photonic integrated circuit that implements such dynamics in synthetic momentum space through unitary dilation, with the phase recovered by phase-shifted interferometry. For the non-Hermitian Su-Schrieffer-Heeger model, the method distinguishes trivial and non-trivial Zak phases and yields a coherence winding $q=\pm 1$ induced by an exceptional point. Extending to a synthetic torus via a Rice-Mele pump gives the first Chern number $\mathrm{Ch}_1=0,1$ for trivial and non-trivial cycles, showing a programmable route to momentum-space topology under strongly dissipative non-Hermitian dynamics.
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All authors Andrea Cataldo, Emil J. Bergholtz, Daniel Leykam, Jun Gao, Ali W. Elshaari

Statistical Mechanics · Cross-listed from quant-ph

Collective Dynamics in Spin Chains with Constrained Dissipation: Classically Fragile but Quantum Robust

Collective non-equilibrium phenomena in many-body systems are strongly influenced by fluctuations, particularly in the vicinity of phase transitions, where the interplay between classical and quantum effects can alter cooperative behavior. Here, we investigate this classical-quantum competition in a kinetically constrained spin chain, the dissipative far-East model. In absence of fluctuations, the system exhibits emergent collective dynamics, resulting in phase coexistence. We find that this phenomenon is robust to quantum fluctuations, which further stabilize it, whereas classical fluctuations suppress phase coexistence at long times. We map out the steady-state phase diagram using a cluster mean-field approach and characterize the dynamics with stochastic tensor-network methods. Within the bistable phase we identify signatures of dynamical heterogeneity in both the local magnetization and the entanglement dynamics. This highlights how competing quantum fluctuations and classical kinetic constraints shape the relaxation dynamics and the phase structure of many-body systems.
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All authors Pietro Brighi, Gianluca Frazzei, Igor Lesanovsky, Juan P. Garrahan, Alberto Biella

Statistical Mechanics · Cross-listed from hep-th

Energy Transmission Across Holographic Conformal Interfaces in General Dimensions

Energy transport across conformal interfaces is universal in two spacetime dimensions, but its higher-dimensional counterpart has remained largely unexplored. In higher dimensions, scattering can depend on additional kinematic data, such as the angle of incidence, and conformal symmetry is far less restrictive. We use gravitational holography to study this problem. For a broad class of AdS$_d$-sliced domain-wall geometries, we derive a closed-form expression for the energy transmission coefficient in terms of the bulk warp factor. Our formula reproduces known two-dimensional holographic results and extends them to arbitrary dimension. Within this class, we establish different aspects of higher-dimensional universality. In particular, we show that the transmission is independent of the incidence angle and of the profile of the incident perturbation. We also derive bounds on transmission controlled by central-charge-like quantities characterizing the number of degrees of freedom of the theories on the two sides of the interface. This provides the first explicit result for reflection and transmission across conformal interfaces in higher dimensions, where no CFT-based results are currently available.
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All authors Igal Arav, Theodore Bertrand, Shira Chapman, Giuseppe Policastro, Sebastian Waeber

Mesoscale and Nanoscale Physics

Hidden Angular Momentum Loop Currents in Symmetric Crystals

Loop-current order has been invoked to explain unconventional electronic phases, with the crystal lattice usually regarded as a passive host for the underlying collective dynamics. Here we show that circulating currents can originate in the lattice itself, sustained by quantum and thermal fluctuations. We develop a microscopic description of angular momentum exchange that separates transfer between sites from crystalline restoring torques and reveals how circulation can emerge in a symmetry-preserving equilibrium state. In a two-dimensional elastic lattice preserving time-reversal, inversion, and fourfold rotational symmetries, we uncover opposite current loops on neighboring plaquettes while the mean angular momentum vanishes at every site. These currents are sustained by zero-point fluctuations in the phonon vacuum and persist at finite temperature. We trace their origin to directional elastic interactions in locally symmetry-lowered environments, with the higher crystal symmetry organizing the resulting currents into a compensated pattern of circulation. Our results extend the physics of equilibrium loop currents to lattice dynamics, revealing that elastic geometry can organize fluctuations into persistent angular momentum circulation without electronic or magnetic order, external driving, or spontaneous symmetry breaking.
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Statistical Mechanics · Cross-listed from quant-ph

Exact Operator Complexity Measures from Random Matchgate Unitaries

Matchgate circuits describe classically tractable dynamics in a physically relevant setting while nonetheless exhibiting features characteristic of complex quantum systems, such as high amounts of magic. This invites the broader question: to what extent are typical complexity measures saturated under trivial dynamics? Here, we address this by studying the behaviour of different Heisenberg-picture complexity measures in random matchgate ensembles. Our main technical contribution is a tractable and generalisible free-fermionic unitary Weingarten calculus formulated entirely in the Majorana basis. This method is tailored to computing moments of operators, and simplifies to a combinatorics problem which depends on the boundary conditions prescribed by a given operator functional. Using this framework, we derive closed-form expressions for the typical local-operator entanglement, operator stabiliser entropy, and higher-order out-of-time-ordered correlators. For extensive initial Majorana strings, both operator entanglement and stabiliser entropy obey volume laws, even though the underlying circuits remain classically simulable. Out-of-time-ordered correlators can likewise become exponentially small, showing that their late-time saturation value alone does not witness computational hardness and constituting a classically tractable example of emergent free independence. Finally, we relate these separations to operator resource theories, showing how operator entanglement beyond the Gaussian baseline lower-bounds the number of non-Gaussian gates in doped matchgate circuits. Our results present a practical toolbox for computing exact averages over random matchgates, while clarifying the distinction between quantum resources versus simulation complexity, and their dependence on the representation being exploited.
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Statistical Mechanics · Cross-listed from physics.soc-ph

Multiscale Renormalization of Weighted Networks

Recent progress in network renormalization has identified various ways to transform network representations consistently across resolution levels. In particular, the renormalization flow describing how random graph models transform under node aggregation has identified a fixed point corresponding to an aggregation-invariant model that preserves the form of the connection probability across arbitrary scales. While this probabilistic multiscale approach has successfully been used to model real-world networks, construct latent-space node embeddings, and reconstruct finer-grained versions of aggregate network data in a principled resolution-invariant way, it has so far been restricted to binary graphs. Here we reformulate multiscale network renormalization for weighted random graphs. Via a generating-function approach, we identify a weighted multiscale model whose full probability law, encoding both link creation and weight assignment, has an invariant compound-Poisson form under arbitrary node aggregation. The renormalization rules that transform parameters across aggregation levels allow the ensemble to be calibrated at one level and applied at another, enabling consistent modeling and reconstruction of weighted networks across arbitrary scales.
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