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Physics Condensed Matter

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Wednesday 26 August

Strongly Correlated Electrons · Cross-listed from hep-th

Why Cooper pairs live in AdS2: a spectral analysis of the Yukawa-SYK model

We establish the spectral foundation of the geometric formulation of Cooper pairing in the Yukawa–Sachdev–Ye–Kitaev model. Starting from the large-$N$ bilocal effective action, we derive the Gaussian fluctuation kernel in the even-frequency spin-singlet Cooper channel. Following the construction of Maldacena and Stanford, we determine the kernel eigenvalue $k\left(h\right)$ analytically for arbitrary conformal weight $h$ and resolve the pairing fluctuations into the continuous and discrete sectors of the associated de-Sitter space Laplacian. We show that the superconducting instability and the universal low-energy fluctuations near it reside entirely in the continuous scattering sector, while the discrete modes remain non-critical. Expanding the kernel about the lowest continuum mode yields a Klein–Gordon action on ${\rm dS}_2$, restricted to the continuous spectral subspace. This is precisely the subspace on which the inverse Radon transform to ${\rm AdS}_2$ is well defined. The projected bilocal Cooper-pair field can therefore be mapped onto a scalar matter field propagating in ${\rm AdS}_2$, without requiring any further spectral restriction on the bulk theory. Our results provide the missing microscopic justification for the projection implicit in earlier holographic formulations and clarify how a local bulk field emerges from the bilocal pairing theory.
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Superconductivity

Exact pair density wave in topological moire flat bands and universal superfluid stiffness

Pair-density waves (PDWs) are unconventional superconducting states beyond the BCS paradigm, but identifying them unambiguously in microscopic lattice models is generally challenging due to various competing orders. In particular, an exact realization of PDW in interacting models with topological bands remains elusive. Here we construct an interacting model on a twisted bilayer checkerboard lattice (TBCB) featuring topological flat bands, and rigorously show that an exact PDW ground state can be induced by quantum geometric nesting (QGN), owing to its momentum-space nonsymmorphic symmetry. We further prove that the superfluid stiffness of any nondegenerate QGN superconductor (including the PDW studied here and uniform superconductor) obeys the universal relation $D_s=2N_{\rm flat}\nu(1-\nu)m_{\rm pair}^{-1}$, where $N_{\rm flat}$, $\nu$, and $m_{\rm pair}$ are the number of flat bands, flat band filling, and the two-particle effective mass, respectively. Our results reveal a rich interplay among PDW order, quantum geometry, and band topology.
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Statistical Mechanics · Cross-listed from quant-ph

Least Variable Quantum Counting Processes

Counting processes provide a fundamental description of stochastic events ranging from photon detection to clock ticks. A central question is how accurately such events can be timed when only finite memory resources are available. Here, we investigate this problem within a general framework of finite-dimensional classical and quantum counting processes. We derive a rigorous finite-memory variance bound obeyed by every classical $d$-state counting process, which is tight and saturated by a discrete Erlang-type ladder process. Through numerical optimization, we identify quantum counting processes that violate this classical bound, achieving smaller first-tick fluctuations than any classical process with the same memory size and mean tick time. For the qubit case, we further derive an analytical large-mean bound within a single-Kraus no-tick family, showing that the quantum advantage persists asymptotically within this class. The optimized quantum processes exhibit coherent conditioned dynamics and approach a continuous-time quantum-jump description as the mean increases. Our results establish a finite-memory quantum advantage in temporal precision and connect discrete-time counting processes with continuous-time quantum timekeeping.
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All authors Bita Olamaei, Florian Meier, Costantino Budroni, Pharnam Bakhshinezhad, Giuseppe Vitagliano

Materials Science

When chemical potential continuity fails: kinetic interface models for hydrogen isotope transport

Macroscopic hydrogen transport codes model material interfaces with local thermodynamic equilibrium (LTE), imposing continuity of chemical potential as a per-species constraint. Three assumptions hide in that condition: fast interfacial equilibration, a single exchange pathway between the two sides, and a carrier species known in advance on each side. The literature scrutinises the first, but the other two are the more consequential failures, and neither survives at a metal/molten-salt interface. We replace the constraint with reversible reaction channels at the interface that obey mass action, with detailed balance fixing each ratio of rate constants from the thermodynamic data that already parameterise LTE, and we implement the framework in festim. LTE is recovered as the fast-kinetics limit of a single channel, in both its Sieverts/Sieverts and its Sieverts/Henry form, so the framework generalises LTE and does not compete with it. A Damköhler number delimits validity within a channel, a branching ratio between channels. In a representative nickel/FLiBe system, hydrogen partitions kinetically between molecular and fluoride carriers. The apparent interfacial law then drifts between Sieverts and Henry with loading and salt redox state, and an LTE condition underestimates the steady permeating flux. The measured pressure exponent is set by the branching ratio, not by any fixed property of the salt; a redox sweep at fixed temperature should continuously shift it between 0.5 and 1. With two isotopes, two metal-side species feed five salt-side carriers, and a per-species LTE condition is ill-posed.
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Mesoscale and Nanoscale Physics

Multicomponent Magnetic Domain Walls in Rhombohedral Graphene

Spatial textures of magnetic order, such as domain walls and skyrmions, are fundamental objects in magnetism. In rhombohedral multilayer graphene, magnetic order involves spin and valley degrees of freedom, opening the possibility of qualitatively new spatial textures. Here, we explore this possibility through a microscopic study of a one-dimensional domain wall in the valley-imbalanced quarter-metal phase of rhombohedral graphene. We uncover two different classes of domain walls. One resembles a conventional magnetic domain wall, locally rotating between the two bulk states, whereas the other is intrinsically multicomponent and explores states that are not occupied in either bulk domain. Which texture is realized is controlled by the competition between intervalley Hund's coupling and spin-orbit coupling, and we identify experimental signatures to distinguish them. For a superconducting junction formed across the wall, we further show that the superconducting phase difference couples directly to the intervalley-coherent phase of the texture, allowing precession of this internal phase to generate a voltage. This mechanism provides an explanation for the resistive domain walls recently observed in chiral superconductors [arXiv2605.13303] and predicts accompanying magnetization oscillations that could be detected using GHz-frequency AC probes. Our theory establish a microscopic connection between multicomponent magnetic textures, their internal dynamics, and superconducting transport.
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Mesoscale and Nanoscale Physics

Viscochiral Transport: Chiral Selection of Hydrodynamic Vortices by Berry Curvature

We predict a new viscochiral regime of electronic transport in which spatially varying Hall viscosity selects vortical flow patterns. Although uniform Hall viscosity cannot alter incompressible bulk flow, its spatial gradient redistributes vorticity, amplifying vortices in one chamber while suppressing the vortex in the other. We further determine the underlying mechanism to be generic to recirculating flows and insensitive to the details of the device geometry. The paper maps the resulting phase diagram and shows that the regime is experimentally accessible in valley-polarized bilayer graphene.
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Quantum Gases

Exact quantum geometry from sublattice symmetry: Closed-form solution of the quarter-flux Harper-Hofstadter model

Quantum geometry has emerged as a guiding principle across atomic and condensed-matter physics, shaping the topological responses of Bloch bands and the stability of the correlated phases they host. Sublattice symmetry, though common among bipartite lattice models, has not yet been exploited to obtain closed-form quantum geometry in multiband systems. For this purpose, we derive a general expression for the QGT of sublattice-symmetric systems in terms of contributions from the individual sublattice sectors, and show that this symmetry renders the Bloch Hamiltonian of a paradigmatic four-band model, the quarter-flux Harper-Hofstadter model, anti-block-diagonal, analytically yielding the spectrum, eigenstates, and full quantum geometric tensor (QGT), including the Berry curvature and quantum metric, for all four bands. The model, describing charged particles on a two-dimensional square lattice subjected to a uniform magnetic field, has recently been realized experimentally with ultracold atoms, photons, and superconducting circuits. Finally, we evaluate fractional-Chern-insulator stability criteria analytically and quantify the lowest band of the quarter-flux Harper-Hofstadter model to be a nearly ideal Chern band. Our approach opens a route for studying also the quantum geometry of other sublattice-symmetric multiband systems.
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Statistical Mechanics · Cross-listed from quant-ph

Yang-Lee Criticality as a Dissipative Dynamical Phase Transition: Quantum Simulation of non-Hermitian Physics without Post-selection

We show that the $d+0$-dimensional Yang-Lee theory describing classical Ising spins in an imaginary magnetic field can be realized, without post-selection, within a $(d-1)+1$ open quantum system whose dynamics consist of local unitaries and engineered dissipation. Competition between the coherent unitary and dissipative dynamics drives a transition wherein the time-dependence of a particular class of linear observables changes from damped oscillatory "underdamped" to purely exponential "overdamped" decay. Our construction relies on an extensive number of weak-symmetries of the Lindbladian fixed by the choice of observable but is otherwise exact. Consequently, we show that the dynamics are described by the non-Hermitian generator of the Yang-Lee transfer matrix, leading to an effective Yang-Lee theory defined on the spacetime history of the open system. By locally modifying the dynamics, we directly measure spin correlation functions of the Yang-Lee theory as well as a related "Loschmidt Echo" correlator which we detail. We explicitly show that the required dissipation channels can be obtained through local $2$-qubit gates and discuss potential realization on near-term quantum simulator devices. Finally, we generalize our construction to embed arbitrary non-Hermitian Hamiltonians within an open quantum system under Lindbladian time-evolution without post-selection, drawing connections between unconditional open quantum dynamics, exceptional point physics, and non-unitary statistical mechanics.
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Materials Science · Cross-listed from cs.AI

SwarmWorld: Stigmergic technological evolution in societies of language-model agents

Collective intelligence can emerge when individuals coordinate through a shared environment, allowing local actions to accumulate into durable social organization. Language-model agents offer a new substrate for this process, yet most multi-agent systems rely on direct conversation, predefined roles, or centralized workflows. It remains unclear whether decentralized agents can build functional technologies and outperform independent search. Here, initially homogeneous LLM agents in SwarmWorld self-organize without assigned roles or recipes into evolving technological societies. Agents explore a spatial environment, process resources, test materials, construct persistent artifacts, and write executable controllers evaluated by a deterministic simulator under unseen disturbances after the agents are removed. SwarmWorld splits cognition from consequence: agents propose architectures and controllers within fixed action and material schemas, while the simulated world determines function. Shared societies develop broader, more resilient technological portfolios than a strong best-of-N isolated-search baseline, although isolated search remains competitive for the strongest artifact. Agents differentiate into exploration, construction, maintenance, and coordination behaviors, transitioning as the world matures. Technologies accumulate through collaborative construction, executable inheritance, and persistent agent-artifact networks, with most reuse beginning through physical observation rather than communication. Explicit cultural mechanisms amplify collaboration and organization, but functional benefits depend on outcome and timescale. Physical stigmergy alone supports capable societies, while interaction drives persistent technological ecologies rather than universally superior individual inventions.
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Strongly Correlated Electrons

Parity Anomaly as Modular Commutator with Massless Dirac Fermion

The modular commutator $J(A,B,C) = i\langle[K_{AB},K_{BC}]\rangle$ extracts the chiral central charge $c_-$ from a single bulk wavefunction of a gapped 2d state, where $3J/\pi=c_-$. Inspired by the recent developments in the field of gapless symmetry-protected topological phases, we ask: what does the modular commutator measure, if it is well-defined at all, when the 2d bulk becomes gapless? Several interesting new insights can already be obtained using the simple Haldane honeycomb model. For the critical point hosting an isolated Dirac node we find that $J$ remains sharp: it converges to a half-quantized value, with corrections that decay as a power law in the subsystem size rather than exponentially, mirroring the power-law correlations in gapless systems. We prove the half-quantization using an emergent reflection symmetry of the massless Dirac cone, and show that the half-quantized contribution comes from the other gapped cone (the massive partner of the massless one). This massive partner can be interpreted as the physical incarnation of the Pauli-Villars regulator, which is the origin of the parity-breaking level-$\frac{1}{2}$ Chern-Simons term (with half-quantized Hall conductance) and the parity anomaly. When protected chiral edge modes coexist with a bulk Dirac node we obtain $3J/\pi = c_-+\frac{1}{2}$. The half-quantization is also shown to be robust against tripartition deformation, tuning Dirac velocity and Dirac cone anisotropy. We further investigate other types of gaplessness—quadratic nodes (in contrast to linear Dirac) and the case with Fermi surface—and show that the robust half-quantization of $J$ is lost in such non-Dirac cases. These results generalize the modular commutator beyond gapped phases, and at the same time provide an information-theoretic measurement of the parity anomaly.
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Strongly Correlated Electrons

Incommensurate spin fluctuations in one-dimensional Kondo metal CeCo2Ga8

We present an experimental and numerical study of the spin fluctuations in 1D Kondo metal CeCo$_2$Ga$_8$. Using inelastic neutron spectroscopy, we measure highly one-dimensional magnetism with low-energy incommensurate short-ranged magnetic fluctuations. ARPES similarly shows a highly one-dimensional electronic band structure, confirming the one-dimensional nature of the system. We use density matrix renormalization group (DMRG) simulations of the 1D Kondo lattice model to interpret the measured spectrum, which successfully reproduce the neutron scattering features. We are thus able to place CeCo$_2$Ga$_8$ within the emergent incommensurate phase of the 1D Kondo lattice phase diagram, and demonstrate that the Kondo lattice simulated non-perturbatively is an accurate microscopic model for heavy fermion physics. This shows CeCo$_2$Ga$_8$ to be one-dimensional despite its complexities, and reveals a coexistence of low-energy Kondo and magnetic features in its inelastic spectrum.
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All authors Yixuan Huang, P. Murgatroyd, Yi Wu, M. Cook, P. F. S. Rosa, E. D. Bauer, Asish K. Kundu, A. Rajapitamahuni, E. Vescovo, S. Zhang, V. Anil, P. Piyawongwatthana, N. Murai, M. Kofu, K. M. Shen, F. Ronning, Jian-Xin Zhu, A. Scheie

Materials Science · Cross-listed from physics.geo-ph

Lab earthquakes confirm the theory of frictional slip pulses

Large natural earthquakes are typically mediated by frictional pulse-like rupture, which features a finite slipping zone. Recently, a comprehensive two-dimensional theory of frictional slip pulses has been developed. It predicts that pulses are categorically unstable rupture modes, whose evolution is intrinsically slow. Unsteady pulses satisfy an equation of motion expressed in terms of discrete observables, which is inherently related to their steady-state counterparts. The theory also predicts a transition from decaying to slowly growing pulses. Here, we perform extensive lab earthquake experiments to test the theory. The experiments confirm the theoretical predictions for pulse-like lab earthquakes over a range of prestress levels, rupture nucleation conditions and small-scale fault roughness amplitudes. Specifically, the predicted time-dependent dynamics are tested in a plane defined by the evolving pulse size and peak slip rate, along with measurements of the dimensionless growth rate of pulses, demonstrating their intrinsically slow unsteady nature. The predicted transition between decaying and growing pulses is also experimentally demonstrated. These results constitute major progress in understanding a dominant earthquake rupture mode.
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All authors Alina Shafir, Tom Gabrieli, Yuval Tal, Eran Bouchbinder

Mesoscale and Nanoscale Physics

Depth Control of Room-Temperature Quantum Emitters in Gallium Nitride

Bright quantum emitters are key components for quantum communication systems. Radiative point defects in gallium nitride (GaN) are promising candidates for room-temperature single-photon emission, operating from the visible to the telecom O-band. Despite their potential, their integration into photonic structures has remained limited in the literature, with experimental photon extraction efficiencies far below simulated predictions. To identify the origin of this limitation, we investigate visible and near-infrared quantum emitters in GaN epilayers grown on $c$-plane sapphire substrates exhibiting narrow linewidths ($\sim$4 nm), high photon count rates ($ > $2 MHz), and strong antibunching, reaching $g^{(2)}(0)$ values as low as 0.06 at room temperature. We find that these emitters are located near the GaN/substrate interface, explaining their limited coupling to optical modes. Building on this observation, we show that the insertion of a thin low-temperature GaN interlayer enables the formation of quantum emitters at arbitrary depths with sub-60 nm accuracy, independent of the substrate. The intentionally introduced emitters retain optical properties comparable to naturally occurring ones, including narrow linewidths ($\sim$6 nm), saturation count rates exceeding 1.5 MHz, high Debye-Waller factors (0.69-0.98), and strong antibunching. The resulting epilayer fully coalesces within less than 250 nm ensuring compatibility with GaN-based cavity fabrication and enabling emitter placement within intrinsic regions of p-i-n diode architectures. These results mark a decisive step toward efficient emitter-cavity coupling, enabling the realization of cavity-enhanced quantum emission in GaN.
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All authors Alexandros Bampis, Johann Stachurski, Anna Schwab, Jean-François Carlin, Raphaël Butté, Nicolas Grandjean

Statistical Mechanics

Topology of Fluctuation Bands in Chiral Active Crystals

While band topology is usually associated with the deterministic dynamics of a system, we show that it can instead reside in its fluctuations. Using a reciprocal lattice driven by nonequilibrium chiral active noise, we find that the displacement spectrum—which quantifies displacement fluctuations—admits bands with nonzero Chern numbers despite a Chern-trivial deterministic mechanics. A two-band valley theory captures the emergence of this topology through a Dirac mass inversion, a Haldane-type mechanism, or a quadratic band touching, depending on the relevant transition. Through the bulk–boundary correspondence, we find boundary-localized fluctuation modes that are distinct from the usual propagating mechanical edge states.
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Materials Science · Cross-listed from physics.plasm-ph

Experimental Characterization of Additively Manufactured Metallic Alloys for Electric Propulsion Applications

This work explores the sputtering of additively manufactured (AM) materials for use in gridded ion source applications. The first part of the paper uses 316L stainless steel as an example to demonstrate that additively manufactured material does not exhibit adverse sputtering behavior, such as higher sputter yield, compared with conventionally manufactured material. To this end, three additively manufactured 316L stainless steel samples were exposed to the beam of a KDC-40 electrostatic gridded ion source at three distinct energy levels of 400, 600, and 800 eV on each side of the sample for a duration of one hour. The samples were masked to create a distinct boundary between treated and untreated regions, identifiable using profilometry, and were biased to -18V for testing. Samples were then examined using a Bruker optical profilometer and further processed using the open-source software Gwyddion to evaluate the sputtering yield. The sputter yield varied in the range 0.2-2 atoms/ion for 400-800 eV ions and increased with ion energy. The measured sputtering yield was fairly consistent with predictions from analytical models developed in prior literature, while exhibiting some variations potentially due to added effects of increased temperature and oxide layers. The second part of the paper demonstrates feasibility of using an additively manufactured tungsten-rhenium grids in existing KDC-40 electrostatic gridded ion source.
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Superconductivity

Electrical manipulation of oxygen stoichiometry in multiterminal YBa$_2$Cu$_3$O$_{7-\delta}$ junctions

Local manipulation of oxygen stoichiometry offers a route to control the electronic properties of complex oxides, yet the selective modification of individual current-carrying branches through oxygen redistribution remains unexplored in multiterminal high-temperature superconducting junctions. In a YBa$_2$Cu$_3$O$_{7-\delta}$ Y-shaped three-terminal device, we demonstrate the possibility to electrically control oxygen vacancy migration on a hand-picked terminal while largely preserving the other two. Oxygen-depleted propagating fronts are directly visualized by the resulting change in optical reflectivity and they are linked to the evolution of the electrical response. The process is highly directional and determined by the polarity of the applied current, allowing for the creation of either a converging or a diverging propagating front from the central node of the Y-shaped device. The associated changes in resistance exhibit relaxation on a timescale of minutes, driven by the vacancy concentration gradient. Effects of oxygen migration are also mapped by Kelvin Probe Force Microscopy and Scanning Laser Microscopy, which probe work-function changes and spatially resolved variations in the superconducting transition, respectively. Notably, the Tc contrast revealed by the latter provides a quantitative handle on the underlying oxygen content, enabling direct visualization of oxygen redistribution. Finite-element modeling and nanoprobe X-ray diffraction qualitatively reproduce the observed vacancy redistribution. These results establish a post-fabrication route to locally tune properties of superconducting multiterminal devices such as nanocryotrons, yTron, and tunable weak links.
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All authors Daniel Stoffels, Caio C. Quaglio-Gomes, Nicolas Lejeune, Emile Fourneau, Pedro Schio, Huidong Li, Lourdes Fabrega, Anna Palau, Maycon Motta, Alejandro V. Silhanek

Soft Condensed Matter · Cross-listed from physics.flu-dyn

A Scalable OpenLB LAMMPS Framework for Fully Resolved Simulations of Hindered Settling of Arbitrary Non-Spherical Particles

Hindered settling of non spherical particles remains significantly less understood than spherical particles due to the computational challenges in resolving the complex contact mechanics and hydrodynamic interactions. In this paper, we present a scaleable fluid structure interaction (FSI) framework coupling the open-source LBM software in OpenLB with the Discrete Element Method (DEM) implemented in LAMMPS to simulate arbitrary shaped rigid bodies in a fluid. Particle contacts are captured using a multi-sphere "clump" representation in DEM, while particle geometries are resolved on the fluid grid via voxelization. We validate our model against single and multi-particle benchmarks, and proceed to study the hindered setttling of cubes in systems containing upto 100,000 cubes. Our simulations show distinct differences between the settling of cubes and sphere, as cubes form pronounced coordination shells without face-parallel contact, in contrast to the contact-dominated clustering observed in spheres. Our results find that correlation length in velocity fluctuations scale with system size even for the largest system studied. These findings highlight the role of particle morphology in suspension dynamics and demonstrate a robust framework for simulating large-scale geotechnical and particulate flows.
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All authors Varghese Babu, Adrian Kummerländer, Mathias J. Krause, Santosh Ansumali, Dilip Gersappe

Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

Immittance formulas for exact blackbox quantization and divergence-free effective models in circuit QED

Building on the first-order circuit quantization method [arXiv:2304.12252, arXiv:2401.09120], we provide simple formulas to construct exact Hamiltonians for Josephson-junction-based superconducting qudits capacitively, inductively, or galvanically coupled to passive linear environments. These environments may be multiport, multimode, discrete or continuous, reciprocal or nonreciprocal, and are characterized directly by their impedance or admittance matrices. In the weak-coupling regime, we further derive divergence-free dispersive Hamiltonians for mode-resolved environments and transition-resolved weak-coupling master equations for dissipative continua. Mode structure, frequency renormalizations, environment-mediated interactions, decay rates, and directional cross couplings then follow from the same causal immittance response, while spurious Lamb-shift divergences arising from uncontrolled approximations in previous treatments are made explicit and avoided. We apply the theory to a set of illustrative circuits comprising a discrete resonator filter, finite-band metamaterial environments, nonreciprocal waveguide-QED systems, and superconducting giant atoms, for which analytical response matrices can be obtained, although the method is particularly well suited to numerical responses from electromagnetic solvers or experimental characterization. We thereby extend the black-box quantization framework to multiport, dissipative, and nonreciprocal settings, establishing a simple and scalable route toward optimized and automated electromagnetic design of large-scale superconducting quantum hardware.
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Materials Science

Electron spin resonance driven photogalvanic effect in graphene-based structures

We report an electron-spin-resonance-driven linear photogalvanic effect (LPGE) in unbiased monolayer graphene and WSe_2/graphene heterostructures. Under linearly polarized 45–75 GHz radiation, the photovoltage exhibits pronounced resonant features in both Faraday and Voigt geometries. Multiple resonances associated with the electron spin resonance in graphene are observed for both out-of-plane and in-plane magnetic-field orientations. Their magnetic-field positions vary linearly with frequency, their amplitudes reverse sign across the charge-neutrality point, and the resonant contribution has the opposite sign to the nonresonant Drude photogalvanic background. We develop a microscopic theory in which radiation-induced momentum alignment followed by skew scattering generates both contributions. Their opposite signs originate from the orthogonal momentum alignments produced by indirect Drude absorption and direct spin-resonant transitions. The theory describes well the main features of the observed resonant photocurrent and provides a microscopic description of ESR-induced LPGE in two-dimensional systems. These results establish the photogalvanic response as a probe of ESR in unbiased micron-scale graphene-based devices.
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All authors C. Bray, I. Yahniuk, L. E. Golub, M. Marocko, C. Consejo, B. Benhamou-Bui, Ziyang Gan, A. George, A. Turchanin, P. Sadovyi, K. Watanabe, T. Taniguchi, J. Eroms, J. Fabian, F. Teppe, S. D. Ganichev

Materials Science

Oxidation-resilient structural modifications in Nickel-functionalized 3D-graphene for hydrogen storage applications

Porous materials represent a versatile solution for several applications. Indeed, the recent development of a new material, named 3D-Graphene, which combines the exceptional characteristics of graphene with a three-dimensional structure, opens perspectives for applications where a high surface-to-volume ratio is beneficial. In this study, we explore the functionalization of 3D-Graphene with nickel (Ni)-nanoparticles as a strategy to enhance hydrogen storage capabilities, and we assess the influence of the NPs on hydrogen uptake and oxidation resilience. The morphology and structural properties of pristine and Ni-functionalized samples were characterized using Scanning Electron Microscopy. Additionally, X-ray Photoelectron Spectroscopy was employed to analyze the surface chemical composition of the functionalized samples. Samples have been hydrogenated supplying molecular or atomic hydrogen, and hydrogen storage performance was assessed through Thermal Desorption Spectroscopy. Afterwards, oxidation effects were systematically studied by exposing the samples to atmospheric oxygen, followed by further hydrogenation experiments. Our results indicate that Ni functionalization influences both hydrogen adsorption and oxidation behavior, with potential implications for improving the stability of the material, especially for hydrogen storage applications.
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All authors Filippo Fincato, Ylea Vlamidis, Markus Leitgeb, Georg Pfusterschmied, Ulrich Schmid, Valentina Zannier, Silvia Rubini, Stefan Heun, Stefano Veronesi

Strongly Correlated Electrons

Rare-earth oxysulfides RE$_2$O$_2$S as model mixed-anion frustrated magnets

The study of low-dimensional and anisotropic magnetism is a promising avenue for the discovery of novel quantum phenomena. Mixed-anion materials, defined by the coordination of metal cations by two or more distinct anionic species, provide an intrinsically anisotropic platform for the tuning of structural, magnetic, and electronic properties. In this work, we report the synthesis and characterization of a family of rare-earth oxysulfide (RE$_2$O$_2$S) antiferromagnets (AFM) possessing a triangular-bilayer slab lattice geometry. Long-range AFM order is observed for the majority of compositions, with several (RE = Ce, Pr, Nd, Sm) having been previously unreported. Although assumed to form stoichiometrically, pair distribution function (PDF) analysis provides evidence for significant, synthesis-dependent interslab structural disorder as RE$_2$O$_{2+x}$S$_{1-x}$, resulting in significant variability in the bulk magnetic response of the Nd member. This work highlights the tunability of frustrated magnetic ground states in rare-earth-based mixed-anion materials, and the importance of thorough structural characterization in the discovery of new mixed-anion magnets.
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All authors Austin M. Ferrenti, Ksenia Khoroshun, Mohamed Oudah, Graham King, Jonathan Gaudet, Alannah M. Hallas

Superconductivity

Symmetry Origins of the Field-Free Superconducting Diode Effect in the Kagome Superconductor CsV$_3$Sb$_5$

Field-free superconducting diode effects require both inversion-symmetry breaking and an internal time-reversal-symmetry (TRS) breaking field, making them sensitive probes of hidden order in superconductors. In centrosymmetric kagome AV$_3$Sb$_5$, the inversion symmetry generally should generally preclude the observation of the superconducting diode effect. Furthermore, though TRS breaking has been reported in the superconducting regime of CsV$_3$Sb$_5$, whether it is generated by superconductivity or inherited from charge-density-wave (CDW) order remains unresolved. Here we show that pristine CsV$_3$Sb$_5$ devices exhibit no intrinsic field-free superconducting diode effect, whereas surface oxidation or asymmetric etching activates a large nonreciprocal supercurrent. Moreover, the response is stochastic, with sweep-dependent polarity and magnitude, indicating metastable TRS-breaking domain configurations. Small out-of-plane magnetic fields stabilize the superconducting diode response, consistent with field selection of such domains. Finally, when long-range CDW order is suppressed by Ti doping, the SDE disappears. Our results establish the symmetry requirements for the field-free SDE in CsV$_3$Sb$_5$, reveal its stochastic domain-controlled character, and link superconducting-state TRS breaking to CDW-related order.
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All authors Xin-Jie Liu, Shengbiao Sun, Ke-Fan Song, Jia-Peng Peng, Xilin Feng, Lang Xiao, Tong Liu, Qilin Han, Ya-Qing Bie, Ning Kang, Xiaosong Wu, Yanfei Wu, Shouguo Wang, Kam Tuen Law, Shuo Wang, Dapeng Yu, Ben-Chuan Lin

Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

The Gain-Engineered Transmon

The interaction between a qubit and its environment can be engineered such that one error channel dominates over all others, resulting in noise bias. This property enables error correction codes to focus on the dominant error type, thereby significantly reducing the number of physical systems required for fault-tolerant quantum computation. However, engineering noise bias typically introduces complexity at the physical system level, which decreases its usefulness by limiting scalability. Here, we introduce and experimentally realize a noise-biased qubit in a standard transmon-readout resonator circuit, one of the most common superconducting architectures, by only adding a single microwave tone. We encode the qubit in the transmon $|\mathrm{g}\rangle$- and $|\mathrm{f}\rangle$-states, and engineer a frequency-selective gain channel that counteracts single-photon loss errors between the computational states. We demonstrate an order-of-magnitude enhancement in relaxation time compared to the $|\mathrm{g}\rangle-|\mathrm{e}\rangle$ encoding, conceding only a factor-of-two decrease in the echo-coherence time. Furthermore, we show that this qubit is compatible with fast, high-fidelity operations. Our results open a path towards using this system as a simple building-block for hardware-efficient quantum error detection and correction schemes.
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All authors Ian Yang, Francesco Adinolfi, Alessandro Bruno, Venus Hasanuzzaman Kamrul, Daniel Z. Haxell, Alexander Grimm

Materials Science

Bayesian Optimization for Self-Driving Materials Laboratories: From Algorithms to Physics-Informed Workflows

Self-driving laboratories (SDLs) are transforming materials research by closing the loop among synthesis, characterization, data analysis and experimental decision making. Bayesian optimization (BO) is a decision engine for these loops because it can select experiments from scarce and noisy data while balancing exploitation and exploration. Yet real materials campaigns often depart from the standard black-box setting, involving failed or missing experiments, noise and drift, mixed variables, constraints, multiple objectives, variable cost and fidelity, transfer from historical data, batch or asynchronous operation, and prior physics knowledge. This review presents BO for materials SDLs through the lens of these practical challenges. We summarize Gaussian-process-based BO and the formulation of materials goals as quantitative objectives, then discuss major choices in surrogate modelling and acquisition. Particular emphasis is placed on physics-informed Bayesian optimization (PIBO), in which domain knowledge enters through representations, priors, kernels, acquisition functions, and constraints. We survey achievements enabled by BO and related active-learning approaches across semiconductors, catalysis, chemical reactions, batteries, alloys, functional materials and quantum materials, highlighting advances beyond parameter optimization, including new materials and synthesis routes, improved functional performance, and reusable scientific knowledge. We conclude by outlining open problems for BO-driven materials SDLs, including nonstationarity, multimodal observations, adaptive problem formulation, and scientific reasoning by humans, large language models and research agents. Addressing these challenges may advance SDLs beyond efficient optimization toward interpretable and knowledge-generating experimentation.
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Materials Science

Watching a GaN Transistor Switch: Real-Time Nanoscale Strain and Heat Dynamics

Digital and energy technologies depend on microelectromechanical and power electronic components whose performance is critically impacted by rapid, cyclic deformations. Real-time information on their operation has remained inaccessible due to the need for nanosecond and nanometer resolution in fully integrated devices. We break this limitation by imaging the complete switching cycle of an industrial GaN high electron mobility transistor through stroboscopic dark field X ray microscopy at a fourth-generation synchrotron, resolving electromechanical and thermal micro strain fields across the entire device and correlating them with time dependent voltage characteristics. Coupled simulations benchmarked against the measurements reproduce electric field evolution and transient thermal hotspots. This combined approach provides direct insight into device physics and informs design strategies for next generation energy and information processing technologies.
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All authors C. Corley-Wiciak, N. T. Sammler, B. Butej, M. Petersmann, A.A. Corley-Wiciak, L. Neumann, Juan M. Carrillo-Larrea, P. Schmiedeke, M. Strätgen, P. A. Douissard, S. J. Leake, P. Boesecke, M. Sievers, P. Imrich, M. Nelhiebel, M. Glavanovics, D. Pogany, M. Reisinger, T.U. Schulli

Other Condensed Matter

Landau Theory for Commensurate Charge-Density Waves Coupled to Uniform Lattice Deformation

We formulate a minimal Landau theory for a charge-density wave (CDW) whose commensurability is defined with respect to a deformed lattice. The motivation is provided by recent observations on an isolated single NbS$_3$ chain, which exhibits a commensurate CDW state accompanied by a $6\%$ shrinkage of the lattice constant. A uniform stretch $a_0\to a_0(1+\varepsilon)$ changes the reciprocal lattice wave number to $G(\varepsilon)=G_0/(1+\varepsilon)$, so that an $N$-fold commensurate CDW has the wave number $Q_\mathrm{C}(\varepsilon)=G(\varepsilon)/N$, whereas the wave number $Q_\mathrm{IC}$ favored by the incommensurate instability remains fixed. We propose an amplitude-strain free energy for both $N=3$ and $N=4$, in which the CDW induces a finite uniform strain by relieving the mismatch between $Q_\mathrm{C}(\varepsilon)$ and $Q_\mathrm{IC}$. The mismatch is shared between the CDW and the lattice in a proportion set by their stiffness ratio; since the CDW stiffness grows with the CDW amplitude, the lattice takes up an increasing share of the mismatch as the CDW develops. Our results suggest a reexamination of lock-in theories and of strain-tuning experiments on density-wave systems.
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Superconductivity

Fluxtube Bouquets and Type-1.5 Clustering in Superfluid Neutron Star Cores

We study mesoscopic configurations of a neutron superfluid coupled to a proton superconductor in the outer core of a neutron star. The condensates are described by a two-component Ginzburg-Landau free energy with local couplings, neglecting genuine phase-gradient entrainment. In two spatial dimensions, we minimize the free energy using quasi-periodic boundary conditions and constrained phase-imprinting calculations to study vortex-fluxtube and fluxtube-fluxtube interactions. We find that, for locally attractive couplings in the free energy, vortex-fluxtube overlap is energetically favoured and several pre-existing proton fluxtubes can bind around a neutron vortex, forming finite vortex-centred aggregates that we call fluxtube bouquets. These bouquet configurations may become so dense that a vortex can effectively accommodate several quanta of magnetic flux. We also confirm the possible presence of a type-1.5-like regime and find that it survives in the zero-entrainment regime considered here. In this type-1.5 regime, the fluxtube-fluxtube interaction is repulsive at short distances and attractive at intermediate distances, leading to self-assembled clusters while the individual fluxtubes remain topologically distinct. Possible implications for dissipative coupling and transport in neutron stars are discussed.
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Mesoscale and Nanoscale Physics

Size and Impurity Effects on Scattering of Valley Hall Modes in Gate-Defined Bilayer Graphene Superlattices

In the present paper we perform a tight-binding simulation of gate-defined islands in Bernal bilayer graphene (BLG). The inversion of the gap sign on the boundaries of the islands creates topologically-protected valley Hall modes. We focus on the specific questions of whether the valley Hall modes around such islands could serve as a host for quantum walks or simulate weakly coupled systems, and how their tunneling is affected by in-gap impurities. In addition, we discuss the effect of misalignment of top and bottom gate patterns on the tunneling properties between islands. Our main results show that resonant tunneling via an impurity enhances overlap between superlattice islands, while misalignment does not break topological protection over a wide parameter regime. In addition, we study the two-island geometry and show that it is possible to leverage suppressed scattering to place islands more densely on a single sample.
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Strongly Correlated Electrons · Cross-listed from quant-ph

Magic of Kitaev spin liquids

Quantum spin liquids (QSLs) are long-range entangled phases of matter and a natural setting for exploring how quantum correlations generate quantum complexity. Motivated by the emergence of magic, or nonstabilizerness, as a diagnostic of many-body complexity beyond entanglement, we study magic of QSLs by computing the stabilizer Rényi entropy (SRE) of the Kitaev honeycomb model. We derive a correspondence between Pauli strings and products of itinerant Majorana operators in the model's free-fermion description; this enables the sampling of SRE using an optimized algorithm for Gaussian states in systems with thousands of spins. Our results show that magic is largest in the gapless phase, where subleading volume-law corrections indicate nonlocal contributions, while in the gapped phases, SRE decreases in quantitative agreement with a perturbative expansion that we develop in the anisotropic limit. At the topological phase transition, SRE exhibits universal scaling dictated by critical exponents.
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All authors Eleonora Lamma, Tim Bauer, Marcello Dalmonte, Mario Collura

Statistical Mechanics

Current fluctuations in a gas of active Ornstein-Uhlenbeck particles

We investigate the statistics of the time-integrated current in an infinite one-dimensional gas of independent active Ornstein–Uhlenbeck particles, as a model system for studying an active generalisation of the corresponding passive (diffusive) phenomenology. Unlike the latter, where current fluctuations exhibit universal sub-diffusive scaling, active systems display diffusive, super-diffusive, and sub-diffusive regimes over different time scales. We fully characterise the distribution of current in terms of large-deviation asymptotics, showing that all of these scaling regimes are described by a single scaled cumulant generating function. Moreover, the statistics retain a dependence on the initial condition even at large times, revealing a persistent memory of the initial state. We further obtain the joint large-deviation statistics of currents measured at two distinct times, characterising temporal correlations. Our analytical predictions are verified using rare-event importance sampling, which resolves probabilities as small as $10^{-1000}$.
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All authors Sandeep Jangid, Aman Kumbhakar, Juliane U. Klamser, Tridib Sadhu