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Physics Condensed Matter

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Wednesday 1 July

Materials Science

Double-pulse control of all optical magnetization reversal in Tb/Co multilayers

Recent experiments have shown that femtosecond laser pulse with a Gaussian intensity profile can induce magnetization reversal in Tb/Co multilayers with a ring-shaped switching pattern within the laser-irradiated area. Here, we investigate the ultrafast magnetization dynamics leading to such a ring-shaped switching by using double-pulse laser excitation. The laser pulses cause heat-induced quenching and subsequent recovery of the magnetic anisotropy in the multilayers and drive the precessional magnetization switching in the magnetic multilayers. By adjusting the delay between the two pump pulses, we demonstrate that the recovery process can be manipulated and show, experimentally and numerically, that this allows control over the final magnetic domain pattern.
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All authors Sheng Li, Dinar Khusyainov, Rein Liefferink, Lukas Körber, Quoc-Trung Trinh, Ricardo C. Sousa, Liliana D. Buda-Prejbeanu, Johan H. Mentink, Theo Rasing, Alexey V. Kimel

Superconductivity

Quench of chiral superconductivity by quantum phase fluctuations in twisted cuprate bilayers

Following theoretical proposals of chiral $d+id'$ superconductivity in twisted cuprate bilayers, experimental signatures of time-reversal symmetry breaking (TRSB) remain highly controversial. Here we demonstrate that quantum phase fluctuations fundamentally reshape the phase diagram of this proposed chiral state. Unlike regular superconducting orders, the chiral $d+id'$ state requires long-range coherence of an interlayer phase degree of freedom and is therefore intrinsically vulnerable to phase fluctuations. Incorporating these fluctuations nearly eliminates the chiral phase over most parts of the phase diagram, restricting it to a narrow twist-angle window and ultra-low temperatures. Phase fluctuations also strongly weaken Josephson phase locking near a twist angle of $45^\circ$. More broadly, our work establishes quantum phase fluctuations as a fundamental constraint on the emergence of TRSB phases in low-dimensional layered quantum materials.
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All authors Yin Shi, Mengxian Zhao, Fei Yang, Miao Liu, Sheng Meng

Mesoscale and Nanoscale Physics · Cross-listed from physics.optics

Evanescent absorption spectroscopy of transition metal dichalcogenide materials using guided photoluminescence in Si$_3$N$_4$ photonic waveguides

On-chip integration of two-dimensional transition metal dichalcogenides (TMDs) with photonic waveguides underpins a growing class of compact optoelectronic and sensing devices, whose performance depends on the optical absorption of the 2D material in this integrated environment. We demonstrate source-free, on-chip evanescent absorption spectroscopy of MoS$_2$ and WS$_2$ flakes integrated on Si$_3$N$_4$ waveguides, in which the broadband defect-related photoluminescence of the Si$_3$N$_4$ core itself acts as the internal probe. Light generated inside the core propagates under the TMD flake and is spectrally attenuated by evanescent interaction with the 2D material, and normalizing the transmitted spectrum to a reference waveguide without TMD yields the energy-dependent absorption response without any external illumination. The extracted guided absorption agrees with Raman and local micro-photoluminescence characterization and resolves differences between spatially uniform and non-uniform flakes. A complementary top-pumping scheme recovers guided WS$_2$ photoluminescence, whose spectral reshaping during propagation is quantitatively reproduced by the measured absorption. This source-free platform qualifies 2D materials in their integrated photonic environment and provides a direct route toward waveguide-integrated TMD photodetectors and sensors.
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All authors Victor Gonzalez-Morote, Marianna Sledzinska, Arkadiusz P. Gertych, Syed Hassan Abbas Jaffery, Mariusz Zdrojek, Daniel Navarro-Urrios

Materials Science

In vacuo synthesis of single-layer Ni3(HITP)2 on HOPG surface using metallo-organic precursor

Single-layer conjugated metal-organic frameworks (SL c-MOFs) are predicated theoretically to host rich quantum phases. To date, however, the experimental synthesis has largely resulted in SL c-MOFs on metal substrates, whose intrinsic properties are strongly screened due to substrate hybridization. To overcome this obstacle, here we develop a method to grow clean SL c-MOF Ni3(HITP)2 on a chemically inert substrate of highly oriented pyrolytic graphite (HOPG). By means of an ultra-high vacuum based multi-step protocol using nickel acetylacetonate [Ni(acac)2] precursor, we obtain continuous single-layer Ni3(HITP)2. Scanning tunneling microscopy reveals a well-defined hexagonal framework with a uniform azimuthal orientation rotated by approximately 30 degrees with respect to the underlying graphite lattice. Furthermore, we control the growth of bilayer Ni3(HITP)2 which features an unusual AA stacking configuration. This work establishes metallo-organic chemistry as an efficient route for integrating 2D c-MOFs onto inert substrates, which opens a new avenue for exploring the exotic quantum properties of SL c-MOFs.
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All authors Chuyu Song, Yifei Feng, Henan Chen, Nian Lin

Mesoscale and Nanoscale Physics

Robustness of Quantum Discord in Nonequilibrium Electronic Transport through Tunnel-Coupled Quantum Dots

Quantum discord captures quantum correlations beyond entanglement and can remain finite even when the entanglement vanishes. We investigate the transient nonequilibrium dynamics and steady-state behavior of quantum discord and classical correlations in a double quantum dot (DQD) system coupled to fermionic reservoirs. By employing a quantum Langevin equation formalism, we obtain the exact reduced density matrix of the system, enabling a comprehensive analysis of its quantum and classical correlations under nonequilibrium conditions. The influence of system-reservoir coupling strength, spectral bandwidth, thermal bias, and varying initial state on both the transient dynamics and steady-state correlations is systematically analyzed. Quantum discord remains finite in the nonequilibrium steady state over a broad parameter range. Although thermal gradients reduce the overall magnitude of correlations, quantum discord persists and exhibits greater resilience. These results demonstrate that nonequilibrium electronic transport, together with the environmental spectral properties and reservoir asymmetry, provides an effective means of controlling nonclassical correlations in mesoscopic systems and establishes quantum discord as a robust hallmark of open fermionic quantum devices.
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All authors Thingujam Yaiphalemba Meitei, Saikumar Krithivasan, Md. Manirul Ali, Arijit Sen

Materials Science

Entropy-Driven Structural Phase Transition in Nb$_3$Cl$_8$ via Density Functional Theory and an Effective Model

As a prototypical flat-band cluster Mott insulator on an effective triangular lattice, Nb$_3$Cl$_8$ is a potential candidate for hosting a quantum spin liquid (QSL) state. Nevertheless, a first-order structural phase transition around 90K transforms the high-temperature paramagnetic $\alpha$ phase into the low-temperature nonmagnetic $\beta$ phase, suppressing the candidate QSL regime of the $\alpha$ phase. To clarify the microscopic origin of this transition, we combine first-principles calculations with an extended Hubbard model to construct a unified free-energy framework. This framework reveals that the transition is jointly driven by phonon and spin entropy: the $\alpha$ phase is stabilized by softer phonons and larger paramagnetic spin entropy, whereas the $\beta$ phase is favored by interlayer dimerization, which hardens the phonons and quenches the spin entropy through singlet formation. Furthermore, by evaluating the pressure-dependent generalized enthalpy, we provide a thermodynamic explanation for the suppression of the transition under c-axis uniaxial pressure, where stabilizing the $\alpha$ phase may allow the candidate QSL regime of the $\alpha$ phase to be explored at low temperatures.
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All authors Chenjie Zhu, Shuai Zhang, Zhong Fang, Zhijun Wang, Quansheng Wu, Hongming Weng

Materials Science

A general-purpose atomic cluster expansion interatomic potential for niobium

Niobium, a body-centered cubic transition metal, poses a challenge for interatomic potentials, which struggle to capture its properties, such as phonons, high-pressure behavior, energy barriers to dislocation glide, and others. To tackle this challenge, we constructed a general-purpose atomic cluster expansion (ACE) potential for niobium. We trained our ACE on thousands of density functional theory (DFT) structures spanning a diversity of local environments. We validated it across a range of properties and compared it with existing empirical and machine learning (ML) potentials, including a novel universal ML potential. The resulting ACE balances accuracy, efficiency, and robustness, enabling large-scale exploration of niobium with near-DFT precision. Finally, our ACE held its own in a stringent test: a near-million-atom molecular dynamics simulation of fracture
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Strongly Correlated Electrons

Strongly frustrated 2D magnetism in a 3D hexagonal perovskite

Exotic quantum phenomena are often found to occur in spin systems that exhibit low-dimensional magnetism. By combining nuclear magnetic resonance, neutron scattering, and muon-spin spectroscopy ($\mu$SR) techniques, we report a rare instance of strongly frustrated two-dimensional (2D) magnetism in a three-dimensional (3D) hexagonal perovskite. Here, Ba$_2$La$_2$MnTe$_2$O$_{12}$, a triangular-lattice magnet, is shown to undergo a magnetic transition at $T_\mathrm{N} \approx$ 4.4 K, below which the manganese moments form a 120$^{\circ}$ AFM order within the $ab$-plane, while staying disordered along the $c$-axis. This exotic ground state, which exhibits ideal 2D magnetism, is highly consistent with the persistently strong spin fluctuations and the large internal field distributions revealed by zero-field $\mu$SR. Further, the 2D magnetism also leads to a significant frustration, much larger than that of most known magnetically-ordered frustrated systems. Our work on Ba$_2$La$_2$MnTe$_2$O$_{12}$ not only challenges the interpretations of magnetic order in other 3D hexagonal perovskites, but it also provides insight into how the dimensionality affects the exotic magnetic states.
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All authors Bocheng Yu, Otkur Omar, Songtai Lv, Long Ma, Zhengcai Xia, Jing Meng, Yanran Yang, Jie Ma, Yang Xu, Qingfeng Zhan, Vladimir Yu. Pomjakushin, Haiyuan Zou, Shang Gao, Toni Shiroka, Tian Shang

Materials Science

Effect of granules anisotropy on "double quantum" magnetic resonance excitation in nanogranular composites

Films of metal-insulator nanogranular composites (CoFeB)x(Al2O3)100-x with different contents of the metal ferromagnetic (FM) phase CoFeB (x ~ 15-50 at.%) are investigated by the method of electron spin resonance (ESR) in a wide range of frequencies (f = 7-80 GHz) and temperatures (T = 4.2-300 K). Besides the conventional FM resonance signal, the experimental spectra demonstrate an additional absorption peak with a double effective g-factor g ~ 4 which is explained within the quantum mechanical "giant spin" model by excitation of "double quantum" transitions in FM granules CoFeB. According to the theory, the intensity of this "double quantum" peak is a complex function of frequency and temperature, including as parameters the granule magnetic moment and anisotropy. Experimentally, the size and anisotropy of the granules can be varied either changing the nominal FM phase content x in the composites or annealing the samples at different temperatures. Here we study the effects of concentration x and thermal annealing of (CoFeB)x(Al2O3)100-x films on their ESR spectral parameters. The observed behavior of the "double quantum" peak intensity is well explained within the considered "giant spin" theoretical concept. In conclusion, we demonstrate the correlation between the size of FM granules in nanocomposites and their anisotropy, indicating the surface origin of this anisotropy.
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All authors A.B. Drovosekov, M.Yu. Dmitrieva, A.V. Sitnikov, S.N. Nikolaev, V.V. Rylkov

Mesoscale and Nanoscale Physics

Real-time dynamics of triplet-resonant tunneling driven by nonequilibrium phonons

Driven nonequilibrium systems can host emergent functionalities beyond equilibrium, but real-time access to excited-state dynamics remains limited. Here we report real-time measurements of phonon-driven charge and spin dynamics in excited states of a double quantum dot. Under phonon irradiation, resonant inter-dot tunneling emerges at triplet resonance. Time-resolved charge sensing reveals that the resonant inter-dot tunneling is strongly modified by spin blockade. For weaker inter-dot coupling, the nonequilibrium phonon environment generates a unidirectional transport cycle along the phonon density gradient.
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All authors Kazuyuki Kuroyama, Sasha R. Valentin, Arne Ludwig, Andreas D. Wieck, Yasuhiro Tokura, Seigo Tarucha, Sadashige Matsuo

Materials Science

Atom-selective spin-polarized transport in a charge-ordered altermagnet

Altermagnets provide a promising platform for spin-polarized transport without net magnetization, but their transport properties are usually discussed in terms of momentum-space spin splitting. Here, using first-principles calculations and quantum transport simulations, we show that the charge-ordered altermagnet $\alpha$-Fe$_2$PO$_5$ exhibits a distinct form of real-space spin selectivity despite weak altermagnetic spin splitting near the Fermi level. The charge order creates inequivalent Fe$^{2+}$ and Fe$^{3+}$ sites within each sublattice, while the puckered C-type antiferromagnetic stacking suppresses inter-sublattice transport. As a result, electron and hole doping activate spin-polarized transport predominantly through Fe$^{3+}$- and Fe$^{2+}$-based channels, respectively. These atom-selective channels carry opposite spin polarizations on the two antiferromagnetic sublattices, giving rise to a globally compensated charge current with hidden Néel spin character. We further propose an all-in-one $\alpha$-Fe$_2$PO$_5$ tunnel junction, where matching or mismatching atom-selective conduction channels yields orders-of-magnitude conductance modulation. Our findings establish a real-space design principle for atomically controlled spin functionality and spintronic devices.
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All authors Liu Yang, Yuan-Yuan Jiang, Xiao-Yan Guo, Yi-Dong Liu, Xian-Zhe Chen, Wen-Jian Lu, Yu-Ping Sun, Ming Li, Ding-Fu Shao

Strongly Correlated Electrons

Weak Ferromagnetism in NiS$_2$ under Nanocrystallization

Structurally well-ordered NiS$_2$ nanocrystals with an average diameter of $27.0 \pm 6.5$ nm retain the bulk-like two-step antiferromagnetic transitions, as shown by magnetization and heat-capacity measurements. Below the lower transition, the nanocrystals exhibit a hysteretic ferromagnetic response with large coercivity, exchange bias, and a vertical loop shift after field cooling, whereas the $M$-$H$ response just above the transition is nearly linear. These features are best explained by uncompensated surface moments generated where the low-temperature antiferromagnetic order terminates at the nanocrystal surface. The absence of a clear additional bulk-like weak-ferromagnetic component constrains homogeneous-canting models and indirectly favors a domain-wall scenario for the weak ferromagnetism of bulk NiS$_2$.
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All authors Hayato Miyazaki, Tomohiko Yoshinaga, Ojiro Miyazaki, Akira Matsuo, Koichi Kindo, Hirofumi Ishii, Tatsuya Kawae, Tetsuya Kida, Masashi Nantoh, Yoichi Ishiwata

Statistical Mechanics

Single-cell-level distributions and relationships can differentiate cell-division and growth models

Complex interactions among regulatory molecules determine the rules underlying cell growth and division in microbial cells. While the governing molecular network may not always be obvious, it is well known that correlations among certain physiological quantities measured in experiments, such as birth-size, division-size, division-time, and division-added-size, can differentiate among various cell-division models, such as Timer, Sizer, and Adder. Here we show that, apart from these correlations, which we extend for the case of stochastic single-cell growth and stochastic asymmetric partitioning, probability distributions of these quantities and statistical relationships between them can also be used to differentiate between these division models. Interestingly, we show that these quantities can not only differentiate the division models, but also distinguish among the single-cell growth paradigms, such as linear and exponential growth. We then demonstrate this differentiability among various division and growth models by comparing our analytical results with published experimental data. We further show that these results remain valid even when the growth rate of a cell is correlated with the growth rate of cells from previous generations in the lineage.
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Statistical Mechanics

Slow heat-driven flow in a gas of hard disks

We study a slow heat-driven flow in a gas of elastically colliding hard disks confined to a long channel. The initial state consists of two regions with large temperature and density contrasts but nearly equal pressures, leading to a low-Mach-number, nearly isobaric evolution. In the dilute limit, the corresponding isobaric hydrodynamic theory reduces to a previously known ideal-gas description. We extend this theory to finite densities by incorporating a non-ideal equation of state of a hard-disk fluid, and solve the resulting one-dimensional equations numerically. Finite-density effects produce appreciable deviations from the ideal-gas prediction. We then test the theory directly against event-driven molecular dynamics simulations of hard disks and find very good agreement in both the dilute and finite-density regimes. The results provide, to our knowledge, the first particle-level test of isobaric gas dynamics of a strongly inhomogeneous cooling flow.
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Superconductivity

Transforming Native Oxide into a Metallic Platinum–Niobium Alloy for Passivation of Superconducting Niobium Films

Dielectric losses at surfaces and interfaces remains a primary limitation to coherence in superconducting transmon qubits. Niobium (Nb), a widely used material in superconducting quantum circuits, readily forms native oxides under ambient conditions, leading to lossy dielectric interfaces that degrade device performance. Here, we demonstrate a novel fabrication strategy that chemically transforms the native dielectric oxide on Nb into a metallic Pt–Nb surface alloy through post-oxidation Pt deposition followed by thermal annealing, thereby stabilizing Nb surfaces against further oxidation, potentially including sidewall regions. High-purity Nb films were fabricated with bulk-like superconducting transition temperatures ($T_c = 9.30\pm0.10$~K). Spectroscopic and microscopic analyses confirm the conversion of the native oxide into a chemically stable, metallic alloy-dominated layer that suppresses subsequent oxide growth. Ab initio simulations elucidate the atomic-scale rearrangement and electronic structure evolution associated with Pt incorporation into native niobium oxide, providing insight into the mechanism underlying the oxide-to-metal transformation and stabilization of the alloyed surface.
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All authors Ananya Chattaraj, Conan Weiland, Bruce Ravel, Kim Kisslinger, Sooyeon Hwang, Xiao Tong, Ajith Pattammattel, Andrew M. Kiss, Steven L. Hulbert, Aswin kumar Anbalagan, Andrew L. Walter, Peter V. Sushko, Mingzhao Liu

Materials Science

Modulation of the Nernst Thermoelectrics by Regulating the Anomalous Hall and Nernst Angles

The large anomalous Nernst effect in magnetic Weyl semimetals is one of the most intriguing transport phenomena, which draws significant attention for its potential applications in topological thermoelectrics. Despite frequent reports of substantial anomalous Nernst conductivity (ANC), methods to optimize Nernst thermoelectrics remain limited. Our research reveals that the magnitude of the ANC is directly related to the sum of the anomalous Nernst and Hall angles. While the sign of the anomalous Hall angle is relatively stable in a certain material, the sign of the anomalous Nernst angle can be intrinsically tuned. Therefore, the ANC can be effectively optimized by regulating these angles to work in concert. This finding is verified by experimental modulation from iron-doped magnetic topological material Co3Sn2S2. Additionally, we observed a robust TlnT scaling law of the ANC over the temperature range of 40 to 140 K in all studied samples, suggesting an intrinsic origin of the ANC. Considering the common opposite sign of the anomalous Nernst and Hall angles in many magnetic topological materials, our research offers an applicable scheme for optimizing the Nernst thermoelectrics.
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All authors Meng Lyu, Junyan Liu, Jianlei Shen, Shen Zhang, Yang Liu, Jinying Yang, Yibo Wang, Yiting Feng, Binbin Wang, Hongxiang Wei, Enke Liu

Soft Condensed Matter · Cross-listed from physics.bio-ph

A bilayer cellular Potts model of epithelial docking

Fusion of two epithelial cell sheets brought together in a bilayer configuration is a common step in animal morphogenesis, yet, in contrast to other epithelial fusion processes such as wound healing in a monolayer of cells, it has not been a strong focus of modeling efforts. Here we consider a preliminary stage of bilayer fusion, recently termed "docking." In multiple instances of docking that span apical and basal varieties, cells appear to have a tendency to remodel so as to co-localize their bilateral junctions (match their edges) across the bilayer. Motivated by this observation, we introduce a bilayer cellular Potts model that couples two standard 2D area- and perimeter-elasticity models via short-range, out-of-plane interactions between cell edges. The new coupling involves a single adjustable parameter that minimally models the combined effect of dynamic cytoskeletal protrusions, cadherins, and other potential edge-associated adhesion molecules. Our model predicts that bilayer edge matching is maximized when the two monolayers are in their fluid-like regimes (average cell shape index greater than 4.6 in our implementation), and when the bilayer coupling strength strikes a balance between in-plane and out-of-plane energy scales. At higher coupling strengths, the system tends to get stuck in metastable states with sub-optimal edge matching. Exploration of the mechanisms of edge matching reveals that pairs and quadruplets of coordinated T1 transitions play a particularly important role. We also find numerous examples of emergent features we term "domain walls" - branching or unbranching curves that cross no matched edges, but that separate regions of nearly complete matching. These domain walls can be both system spanning and long lived. Finally, we extend our model to crudely account for bending of the two sheets, and study the distributions of docking front speeds that result.
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Strongly Correlated Electrons

Holographic Quantum Transformer: A Generalist Neuro-Symbolic Architecture for Solving Frustrated Systems via Generative Attention

Simulating two-dimensional frustrated quantum matter is a grand challenge due to the sign problem and exponential Hilbert space complexity. In this work, we introduce the Holographic Quantum Transformer (HQT), a physics-inspired generative architecture that leverages global self-attention to resolve non-local entanglement patterns. We validate HQT on the square lattice $J_1-J_2$ Heisenberg model. On the heavily frustrated $8 \times 8$ lattice at the quantum critical point ($J_2=0.5$), HQT reaches a ground-state energy per site ($E/N$) of $\mathbf{-0.5001(1)}$, consistent with the expected finite-size scaling trend. Beyond numerical accuracy, HQT exhibits intrinsic physical awareness, autonomously recovering the underlying $J_2$ interaction geometry through interpretable attention maps. Our central contribution is “Holographic Transfer", a zero-shot size-extrapolation protocol with rapid alignment: a model trained on $8 \times 8$ systems is directly projected onto larger $10 \times 10$ lattices via continuous positional-embedding interpolation and head re-initialization, achieving high-fidelity initialization and rapid convergence. This zero-shot protocol yields an energy of $E/N = \mathbf{-0.49782(3)}$, statistically consistent with the variational state of the art while requiring no from-scratch training on the target lattice. Our results establish generative attention as a scalable paradigm for transferable quantum simulation.
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All authors Xingran Guo, Tiaojie Xiao, Jie Liu, Keqin Li

Mesoscale and Nanoscale Physics

Modulation of anomalous Hall angle in a magnetic topological semimetal

The anomalous Hall angle ({\theta}A) is a measure of the efficiency of converting a longitudinal driving current to a transverse spin-polarized Hall current. For anomalous Hall sensing, a large anomalous Hall angle can improve the sensitivity of magnetic field detection. However, modulation of this angle is challenging and magnetic materials typically have low angles of 0.1 to 3{\deg}. Here, we report modulation of the anomalous Hall angle in the magnetic Weyl semimetal Co3Sn2S2. We propose that the angle parameter tan{\theta}A can be formulated as a function of the product of electrical resistivity and anomalous Hall conductivity. Our scheme was utilized to demonstrate the modulation of tan{\theta}A up to a magnitude of 0.46, corresponding to an angle of around 25{\deg}. Microfabricated anomalous Hall devices using Fe-doped Co3Sn2S2 single-crystalline nanoflakes exhibit a high Hall sensitivity of 7028 {\mu}{\Omega}ucm/T and a magnetic field detectability of 23.5 nT/Hz0.5 at 1 Hz.
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All authors Jinying Yang, Yanxing Shang, Xingchen Liu, Yibo Wang, Xuebin Dong, Qingqi Zeng, Meng Lv, Shen Zhang, Yang Liu, Binbin Wang, Hongxiang Wei, Yizheng Wu, Stuart Parkin, Gangqin Liu, Claudia Felser, Enke Liu, Baogen Shen

Statistical Mechanics · Cross-listed from quant-ph

Subsystem Thermalization and Work Statistical Characterizations of Floquet Dynamics

We study Floquet thermalization in a periodically driven quantum non-integrable Ising chain by combining two operational diagnostics: subsystem thermalization and work statistics. For generic interacting Floquet systems, stroboscopic dynamics lead to heating toward an infinite-temperature state at low driving frequencies, to a prethermal state during the crossover regime, and then to a finite-temperature state at high driving frequencies. We show that reduced density matrices of small subsystems provide a precise measure of local equilibration and clearly resolve prethermal plateaus. In parallel, we analyze the statistics of work performed over a Floquet cycle using both the characteristic function of work with and without the two-point measurements, and the related fluctuation theorem, which captures coherent contributions and deviations from thermal equilibrium. By comparing these two diagnostics within the same Floquet setting, we demonstrate that work statistics encode the same dynamical crossover that governs subsystem thermalization. Our results establish a unified and experimentally accessible framework for characterizing Floquet thermalization, prethermal regimes, and coherent energy absorption in interacting quantum systems.
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Mesoscale and Nanoscale Physics

Universal Scaling of the Spin Hall Effect

We study the spin Hall (SH) effect for the Dirac electrons in terms of the spin and magnetic-moment accumulation coefficients $-\Gamma^{00} g_{s(m)z}^{\phantom{s(m)z} xy}$. We take short-range nonmagnetic impurities into account within the self-consistent $T$-matrix approximation. Similarly to the universal scaling for the anomalous Hall (AH) effect, we find three disctinct regimes by changing the electric conductivity $\sigma^{yy}$; the superclean regime with $-\Gamma^{00} g_{s(m)z}^{\phantom{s(m)z} xy} \propto \sigma^{yy}$ owing to the skew scattering, moderately dirty regime with almost constant $-\Gamma^{00} g_{s(m)z}^{\phantom{s(m)z} xy}$, and dirty regime with a new scaling relation $-\Gamma^{00} g_{s(m)z}^{\phantom{s(m)z} xy} \propto (\sigma^{yy})^{0.6}$ whose exponent differs from that of the AH conductivity. Our results construct a unified theory of the SH effect without any ambiguity of spin current.
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Statistical Mechanics · Cross-listed from quant-ph

Coupling effect of nearest-neighbor interacting qubit chains to a single qubit system

This study establishes a theorem that provides sufficient criteria for identifying terms in any time-independent Hamiltonian that have no influence on local dynamics, local observables, or any local phenomena, without any approximation. The usefulness of this theorem is demonstrated by predicting the behavior of three systems. The first system consists of multiple qubit chains with Ising interactions. The second system is formed by a single qubit chain, differentiated by the substitution of Dzyalonshinskii-Moriya (DM) interaction for the last Ising interaction. The predictions were verified by analytically deriving the reduced dynamics of both systems. A third system was also considered, namely, a short qubit chain with a transverse magnetic field on the intermediary environment qubit. This transverse magnetic field signals that the commutation relation required by our theorem no longer holds. The third system's local dynamics were also derived analytically, demonstrating that all Hamiltonian constituents contributed to the reduced dynamics. The physical consequences of our theorem's inapplicability were also explored using this third system by analyzing the entanglement dynamics between the qubits that do not directly interact. The results showed that the entanglement is caused by an emergent coupling between the two non-directly interacting subsystems. This emergent coupling arises from the non-commutativity of the intermediate interactions connecting the two subsystems. When searching for these emergent couplings, our theorem can eliminate intermediate interactions that will not produce them.
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Tuesday 30 June

Materials Science · Cross-listed from physics.app-ph

Non-reciprocal heat transfer advances flexible thermoelectric devices

Complex heat dissipation assemblies, inferior performance, and limited flexibility are the primary constraints impeding the wide application and commercialization of conventional flexible thermoelectric devices in wearable electronics and other high-end cooling scenarios. In this work, we report a non-conventional design for flexible thermoelectric devices which can reduce the temperature to -7.03 at room temperature without external heat sink, achieving a cooling temperature drop of 29.25. The design is based on non-reciprocal heat transfer, integrated with thermally conductive composites and screen-printing technologies. This approach takes advantage of directional heat flow, thereby eliminating the need for complex heat sink networks, which extend the applications of flexible thermoelectric devices from personal thermal management to more broader fields such as home healthcare and emergency first aid.
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All authors Jinwen Yang, Wenmei Luo, Hongbin Xu, Fuqing Duan, Yafei Ding, Jie Chen, Guimei Zhu, Baowen Li

Mesoscale and Nanoscale Physics · Cross-listed from physics.chem-ph

Quantum Thermodynamics of Electron Transport along Chains of Redox Centers

Intramolecular electron transport in biological systems is typically described as a diffusive hopping process, according to the semi-classical rate theories of Marcus and Hopfield combined with classical Pauli-type master equations. However, the possibility that non-trivial quantum mechanical effects could play a functional role in the transport dynamics in certain biomolecular processes has attracted increasing attention. Here, we extend the quantum mechanical model of open system dynamics by the Lindblad equation to a key biological component, the long chains of redox centers based on iron-sulfur clusters or heme groups that are widespread in many biological organisms, where they realize the cellular respiration. This approach allows to explore a wide range of physical parameters, showing key features of electron transport in these multi-domain protein structures. We pay particular attention to heat and entropy transfer between the electrons and the protein bath, which constitutes a benchmark of physical realism for the models. Electron currents, average transfer times and relative efficiency of the transport process are also explicitly characterized.
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Other Condensed Matter

Valley-dependent electron optics using quantum dots in bilayer graphene

Electrostatically defined quantum dots (QDs) with layer-antisymmetric gating in Bernal-stacked bilayer graphene (BLG) open a local gap and generate a mass-like term with opposite sign in the two valleys, producing strongly valley-dependent scattering without magnetic fields, strain, or spin-orbit coupling. Building on this mechanism, we propose a tunable platform based on such QDs for valley-dependent electron optics in BLG. Using a four-band continuum model and a generalized multiple-scattering formalism, we analyze scattering of Gaussian electron beams from single- and multi-dot architectures and compute valley-resolved currents and angular profiles. A single dot produces distinct valley-dependent deflection, while multi-dot configurations enable enhanced control: identical-dot arrays act as valley splitters, whereas oppositely gated pairs function as valley filters. Combining these elements yields tunable generation, steering, and filtering of highly valley-polarized currents with strong suppression of forward transmission. The required energy scales, gate asymmetries, and device dimensions are within experimentally accessible regimes for dual-gated BLG, establishing quantum-dot arrays as a realistic platform for controllable valley-resolved electron optics.
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Statistical Mechanics · Cross-listed from q-bio.PE

Demographic senescence as multi-level selection in miniature

Multi-level selection and senescence do not at first sight have much in common. Here, we demonstrate that the emergent mortality patterns generated by demographic senescence can be understood as the product of multi-level selection. We formulate a two-level Moran type process and use its scaling limits to illustrate that a simple mathematical framework that models multi-level selection in group-structured populations also models damage accumulation patterns and resultant mortality curves in ageing organisms. To verbally make the connection, observe that defectors spread within a group consisting of cooperators and defectors; when groups compete against each other, defector-rich groups suffer, and between-group selection causes such groups to be systematically under-represented. Exactly analogously, senescing individuals accumulate damage to physiological sub-systems, and `damage begets damage'; individuals who are more damaged are more likely to die, hence damage-rich individuals are systematically under-represented in later age classes. Thus, emergent senescence patterns in complex, integrated organisms are formally equivalent to the patterns generated by a within-generation multi-level selection process in which intra-organismal sub-systems play the role of particles, organisms play the role of collectives, and selective disappearance plays the role of group selection.
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Materials Science

Anomalous bulk dealloying below the parting limit

Dealloying has been extensively studied both as a corrosion degradation mechanism in structural materials, including those used in nuclear, aerospace, or marine environments, and as a versatile method to fabricate porous materials for catalysts and other functional applications. Classical dealloying theory in aqueous environments predicts a critical reactive-element concentration (parting limit) for continuous selective dissolution at temperatures where bulk diffusion does not dominate; this threshold is commonly reported around 50~60 at.%. Yet recent studies show that molten salt environments can generate extensive bulk dealloying below this threshold. Despite the importance of this anomalous dealloying behavior in many energy systems and electrochemical applications, its fundamental origin remains elusive. Here, we address this critical gap, revealing a grain boundary (GB)-assisted bulk dealloying mechanism. Using three-dimensional (3D) reconstruction of the dealloyed regions correlated with crystallographic and elemental analyses, we directly map the 3D GB-void architecture and reveal that diffusion-induced recrystallization (DIR) generates a high-density GB network, which then promotes molten-salt infiltration and can drive bulk dealloying far-below the conventionally reported parting limit, producing a distinctive morphology reminiscent of discontinuous precipitation (DP). Understanding this dynamic GB-void interplay is crucial for the prediction and control of dealloying in complex electrochemical environments.
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All authors Weiyue Zhou, Hooman Gholamzadeh, Lei Ding, Kevin Daub, Mehdi Mosayebi, Travis Casagrande, Yingxin Zhu, Miaomiao Jin, Mark R. Daymond, Yang Yang, Michael P. Short, Suraj Y. Persaud

Materials Science

Dominant-pair free energies predict phase selection in high-entropy alloys

Phase selection in multicomponent alloys is governed by the competition between entropic stabilization of disordered solutions and enthalpic driving forces for chemical ordering. However, widely used parametric criteria reduce it to a single scalar, carrying no explicit free energy for any competing ordered phase. Herein, we develop a thermodynamic framework based on the semi-empirical macroscopic atom model and the Dinsdale lattice stability database to fill this gap. We show that a dominant-pair mechanism, in which the Al-transition-metal interaction family dominates the ordering enthalpy, enables the complex multicomponent B2-ordering problem to be reduced to an effective pseudo-binary system with an analytically evaluated Bragg-Williams free energy. Combined with a minimum-free-energy classifier, the framework predicts the lowest-energy phase as a function of composition and temperature. This provides continuous phase stability maps rather than the single-value predictions of conventional descriptors. Demonstrated on high-entropy alloys using a dataset of 269 experimentally characterized samples, the model outperforms widely used phase-selection criteria in the class-balanced macro-F1 metric and achieves 77.9% on the well-posed three-class task, outperforming the valence electron concentration criterion. The model is general by construction and computationally efficient for predicting phase stability in multicomponent alloys over a broad range of compositions and temperatures.
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Materials Science

Structure-Dependent Chemical Order Modification in Strained Alloy Nanoparticles

Alloy nanoparticles (nanoalloys) exhibit tuneable physicochemical properties that depend sensitively on their atomic arrangement, making control over chemical ordering a central challenge in nanomaterials design. While most theoretical studies consider nanoalloys in vacuum, practical systems are typically supported, where strong cluster-substrate interactions can introduce significant lattice strain. Here, we investigate strain as a control parameter for chemical ordering in bimetallic nanoalloys using atomistic molecular dynamics and Monte Carlo simulations. By imposing controlled tensile and compressive strain through an implicit anchored interface, we systematically probe the response of NiPt nanoparticles with distinct structural motifs. For truncated octahedral particles, we find that chemical ordering and segregation behaviour remain remarkably robust even under large strains, indicating that intrinsic thermodynamic preferences dominate. In contrast, icosahedral nanoparticles exhibit pronounced strain-induced chemical redistribution, with a significant increase in surface Ni concentration under tensile strain. This behaviour is attributed to the combined effects of intrinsic geometric frustration and a high fraction of undercoordinated sites in icosahedral structures. Our results demonstrate that strain can selectively modulate chemical ordering in nanoalloys in a structure-dependent manner, establishing a general framework for understanding strain-induced chemical ordering in nanoalloys.
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All authors Yue Wang, Zibo Chen, Evropi Toulkeridou, Joseph Kioseoglou, Panagiotis Grammatikopoulos

Quantum Gases · Cross-listed from quant-ph

A universal time-of-arrival signature of Bose–Einstein condensation

We show that Bose–Einstein condensation produces a cusp in the time-of-arrival (TOA) statistics of a harmonically trapped gas released into free fall. In the semiclassical long time-of-flight regime, with $\epsilon=\sigma_V/\sqrt{2gH}\ll1$, both the mean and standard deviation of the arrival time distribution, which are governed by the longitudinal velocity variance, remain continuous, but acquire a cusp whose one-sided slope ratio is universal within the ideal-gas far-field limit, $\mathcal{R}_\infty=2.5556\ldots$, and equals the trapped-gas specific-heat ratio $C(Tc^-)/C(Tc^+)$. Finite atom number rounds the cusp and weak interactions perturb it only weakly, leaving a measurable time-domain signature of condensation.
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