Mesoscale and Nanoscale Physics
Antisymmetric breathing in altermagnetic skyrmions
Yunxi Jiang, Chen Xuan, Xi Chen et al. (+3 more)
A skyrmion in an altermagnet with \(d\) wave
symmetry consists of two elliptical sublattice textures with perpendicular long axes. For each sublattice component $\eta=A,B$, we define an effective skyrmion radius $R_\eta=\sqrt{a_\eta b_\eta}$, where $a_\eta$ and $b_\eta$ are the distances from the skyrmion center to its boundary along $y$ and $x$, respectively. For the anisotropic exchange parameters studied, the
equilibrium radius at zero field is smaller than in a reference with parallel sublattice textures and otherwise identical parameters. A
magnetic field perpendicular to the film expands one sublattice skyrmion and contracts the other, generating a radius difference $\dR=R_A-R_B$ and a net
magnetic moment. The exchange modulation used to represent uniaxial strain also produces a nonzero radius difference at zero field. Because the strong and weak exchange directions are interchanged between the two sublattices, a common directional change of the exchange couplings increases one radius and decreases the other. Unlike the
magnetic coupling, this mechanism vanishes when the two sublattice exchange tensors become identical. The radius difference also supports an antisymmetric breathing mode. After a short field pulse, it oscillates in quadrature with the uniform helicity, the common rotation of the wall magnetization within the film plane, at \(49.5\,\mathrm{GHz}\) for the reference parameters.
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All authors Yunxi Jiang, Chen Xuan, Xi Chen, Zhikai Wang, Qinfeng Zhu, Hao Yu
Superconductivity
Hidden magnetic order within the pressure induced superconducting dome of UTe2
Kaixin Ye, Lubin Wang, Dengpeng Yuan et al. (+12 more)
Unconventional superconductivity typically occurs near
magnetic instabilities, and the corresponding
spin fluctuations are widely believed to play a crucial role in mediating electron pairing. UTe$_2$ is a promising candidate for exhibiting multiple
spin-triplet superconducting phases when tuning with applied pressure and
magnetic fields, but the nature of the magnetism driving these unconventional pairing states is undetermined. Our measurements of UTe$_2$ under applied pressures and
magnetic fields reveal the presence of a
magnetic order hidden within the pressure-induced superconducting dome, which vanishes together with the superconductivity once there is sufficiently high pressure to induce the three-dimensional antiferromagnetic phase. Extrapolation of the phase boundary of the hidden
magnetic order, which is most likely antiferromagnetic in nature, points to a zero-temperature
quantum critical point that coincides with the maximum transition temperature of the pressure-induced superconducting dome, suggesting that it could corresponds to the parent
magnetic phase of the critical antiferromagnetic
spin fluctuations driving the triplet superconductivity. These findings advance the understanding of the interplay of magnetism and superconductivity in an exemplar candidate triplet
superconductor, which is necessary for revealing the microscopic origin of the different unconventional superconducting phases.
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All authors Kaixin Ye, Lubin Wang, Dengpeng Yuan, Binbin Zhang, Yanan Zhang, Ye Chen, Yu Liu, Xin Lu, Chaofan Zhang, Qiuyun Chen, Shiyong Tan, Frank Steglich, Lin Jiao, Michael Smidman, Huiqiu Yuan
Statistical Mechanics
Amplified Memory and Finite-Time Regularity in Driven Non-Hermitian Systems
H. Yavartanoo, R. Jafari and Alireza Akbari
We study the roles of broken spectra and exceptional points in finite-time driven non-Hermitian fermionic dynamics. We compute the Nambu biorthogonal correlation
matrix for this purpose. The imbalanced-pairing Kitaev chain serves as our concrete realization. Transient passage through a broken-spectrum region amplifies preparation
memory. The effect survives when the final
Hamiltonian returns to a real-spectrum regime. Negative imbalance forces spectral nonpositivity in the static endpoint state. We isolate the genuine drive history by subtracting out this baseline, leaving an excess that is strictly controlled by the accumulated imaginary-energy action and persists over the entire post-ramp time window. A connected longitudinal correlation mirrors this physics. Its slow-ramp growth tracks the corresponding doubled action. Unstable sectors instead continue amplifying post-ramp if the drive halts inside the broken-spectrum region. Exceptional points yield distinct physics. The finite-time propagator and subsystem correlation
matrix remain entirely regular near an exceptional endpoint, even as the quasiparticle gap exhibits its characteristic square-root closing. This finite-time regularity reflects the analyticity of the
matrix evolution in the endpoint parameter; a diagonalizable endpoint is strictly not required. A diverging long-time crossover eventually reveals the exceptional scale. We halt the drive exactly at the exceptional point to find that the correlation projector and the connected longitudinal correlation share an identical ballisti front. The subsystem saturation length establishes a distinct but comparable spatial scale.
Memory and exceptional-endpoint scalings show no divergence across the tested negative-imbalance range.
Memory scaling is fixed by the drive and remains insensitive to the specific choice of real-spectrum final endpoint.
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Materials Science
Superconductivity and Band Topology in Functionalized 2D Hexagonal MBenes
Mohammad Keivanloo, Shashi B. Mishra, Amirreza Shariatmanesh et al. (+5 more)
Recently, two-dimensional transition-metal borides (MBenes) have attracted substantial interest due to their promising properties for electrocatalytic applications. Here, we explore their potential as novel two-dimensional
superconductors and topological materials through first-principles calculations on both pristine and surface-functionalized hexagonal MBenes. We conduct a thorough examination of the structural, electronic, phononic, superconducting, and topological properties of 36 compounds with formulas M$_{2}$B$_{2}$ and M$_{2}$B$_{2}$T$_{2}$ (M = Sc, Ti, V, Zr, Nb, Hf, Ta, Mo, W; T = F, O, OH). Our analysis identifies 21 superconducting MBenes, including four with critical temperatures (T$_{c}$) exceeding 10 K, with Ti$_{2}$B$_{2}$O$_{2}$ exhibiting the highest predicted T$_{c}$ of 24 K based on the McMillan formalism. For the two most promising compounds, Ti$_{2}$B$_{2}$O$_{2}$ and V$_{2}$B$_{2}$(OH)$_{2}$, we further solve the anisotropic Migdal-Eliashberg equations, obtaining zero-temperature superconducting gaps of 6.1 and 3.6 meV and anisotropic T$_{c}$ values of approximately 32 and 25 K, respectively.
Symmetry-indicator-based analysis further reveals nontrivial normal-state band
topology in several superconducting MBenes. These results indicate the coexistence of
phonon-mediated superconductivity and nontrivial normal-state band
topology within this material family, making MBenes promising platforms for future investigations of the possible emergence of topological superconductivity.
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All authors Mohammad Keivanloo, Shashi B. Mishra, Amirreza Shariatmanesh, Mohammad Sandoghchi, Kenta Hongo, Ryo Maezono, Elena R. Margine, Mohammad Khazaei
Mesoscale and Nanoscale Physics
Light-induced rectified orbital magnetization in electron-hole bilayers
Erlend Syljuåsen, Gabriel Cardoso, Esra Ilke Albar et al. (+3 more)
Circularly polarized light can rectify orbital motion into a static magnetization through the inverse Faraday effect (IFE), but in electron-hole bilayers the electron and hole contributions cancel exactly when their properties are equivalent. We show that electron-hole bilayers in transition-metal dichalcogenide platforms avoid this cancellation through effective-mass asymmetry alone, and that the surviving orbital IFE is sensitive to interlayer coupling. In the weak-coupling regime, a two-component Drude description yields an induced magnetization of order one Bohr magneton per carrier for representative terahertz driving. In the strong-coupling regime, where the carriers bind into interlayer
excitons, we treat the relative motion using a hydrogenic model with a Rytova-Keldysh interaction and obtain a reduced but finite response. We give closed-form expressions that allow estimates across a broad parameter range and identify where the response is largest.
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All authors Erlend Syljuåsen, Gabriel Cardoso, Esra Ilke Albar, Patrick J. Wong, Angel Rubio, Alexander V. Balatsky
Mesoscale and Nanoscale Physics
Nonequilibrium Dirac condensate in bosonic Kitaev chain
Kazuki Yamamoto and Youichi Yanase
We explore a nonequilibrium Bose-Einstein condensate (BEC) in a bosonic Kitaev chain. Within a mean-field framework, we show that bosonic superfluid order develops once the pairing strength exceeds a critical threshold. The condensate order parameter adopts an alternating phase between even and odd sites, giving rise to a spontaneous sublattice ordering. By mapping the emergent sublattice degrees of freedom onto a pseudospin, the elementary Bogoliubov excitation is described by a non-Hermitian Dirac
Hamiltonian, displaying two prominent features: a re-entrant bosonic Andreev bound state localized around boundaries, and a macroscopic degeneracy of exceptional Majorana
bosons at the critical point.
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Materials Science
Electric Current-Driven Microstructural Evolution in SrTiO3
Jingjing Yang and Jian Luo
Polycrystalline SrTiO3 is employed as a model system to investigate microstructural
evolution under applied electric currents. Under a substantial current density, well-aligned, elongated abnormal grains develop near the anode following a flash event, in contrast to previously reported cathode-side enhanced grain growth under negligible currents. The equivalent diameter of the abnormal grains increases linearly with time, deviating from classical parabolic grain growth kinetics. The applied current drives elemental redistribution near the anode, producing a Ti-rich region adjacent to a Sr-rich belt that migrates toward the cathode, from which the abnormal grains nucleate. Aberration-corrected scanning transmission electron microscopy and electron energy-loss spectroscopy reveal that the fast-moving grain boundaries (GBs) within the Ti-rich bulk region are Sr-enriched, O-depleted, and Ti-reduced. An analysis based on the Brouwer diagram suggests the formation of p-i-n regions under the applied electric field. Conversion between electronic and ionic currents at the p-i and i-n junctions, field-driven precipitation and dissolution of the Sr-rich Ruddlesden-Popper phase, and field-driven migration of Sr and O vacancies collectively explain the elemental redistribution and redox-modulated migration of the Sr-rich belt. Incomplete redox reactions at the moving junctions create the moving Sr-rich belt and generate a locally reducing environment, consequently producing fast-moving, Sr-rich, reduced GBs. These findings reveal new mechanisms of electric current-driven defect-mediated microstructural
evolution.
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Disordered Systems and Neural Networks
Perfect resonance and fragile localization suppression in correlated disordered chains
Zhixuan Zhao and Jun Li
Spatial correlations can suppress scattering in disordered chains and produce perfectly transmitting resonances. The practical value of this protection, however, depends not on the resonance peak itself but on the width of the surrounding transmission window and its sensitivity to local ordering errors. We show that a resonance can remain exactly transparent at its center while arbitrarily rare adjacent-swap errors restore an inverse localization length proportional to the square of the energy detuning. For lossless single-channel chains assembled from independent blocks of fixed length and composition, this positive quadratic term is guaranteed by a local scattering invariant and holds for every arrangement and every fixed swap probability between zero and one. With exact tuning and matched contacts, the central transmission remains unity. A microscopic
quantum chain exhibits both higher-order suppression of scattering in the ideal recursive arrangement and the predicted response to local exchanges. These results reveal a limitation of spatial ordering that is invisible to a measurement at the resonance alone: spatial ordering protects the resonance peak, not the transport around it. The effect can therefore be tested experimentally by measuring transmission spectra before and after exchanges, without identifying microscopic defects.
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Materials Science
Frustrated junctions in interfacial networks
Håkan Hallberg, Vasily V. Bulatov, Bryan W. Reed et al. (+1 more)
Networks of interfaces in materials and living systems evolve through motion and rearrangement of interfaces and junctions. Local
equilibrium at a junction requires interfacial force balance. We show that in three dimensions the classical Herring condition for triple lines is necessary but insufficient: four triple lines meeting at a quadruple node may each satisfy Herring
equilibrium, while the four conditions remain mutually incompatible. Such a frustrated node has no admissible local
equilibrium geometry. In the semi-isotropic limit, the six interfacial energies must form the edge lengths of a non-degenerate tetrahedron, with constructibility determined by the Cayley-Menger determinant. This hidden compatibility constraint arises from three-dimensional geometry and applies broadly to foams, polycrystals, tissues and other interfacial networks.
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All authors Håkan Hallberg, Vasily V. Bulatov, Bryan W. Reed, Mukul Kumar
Other Condensed Matter
Geometry-Induced Effective Tight-Binding Hamiltonians for Phononic Systems: Mode Conversion and SSH-Like Physics
José E. González and Carlos Ramírez
We present a framework that maps harmonic vibrational systems onto effective multi-orbital tight-binding
Hamiltonians, establishing a direct correspondence between phononic degrees of freedom and graph-based
lattice models. Within this mapping, the Cartesian displacement components of each mass become internal orbitals, while elastic interactions generate effective onsite energies and hopping amplitudes determined by the geometry of the system. This representation enables the application of numerical and conceptual tools originally developed for electronic transport to the study of phononic systems. The method is first applied to a monoatomic chain containing an angular bend. For this
benchmark system, analytical expressions for the polarization-resolved transmission and reflection probabilities are derived and compared against calculations performed using a recursive scattering-
matrix method within the mapped tight-binding representation. Excellent agreement is obtained, validating the mapping and demonstrating its ability to describe geometry-induced mode conversion and the influence of evanescent states. We then investigate zigzag chains, where alternating bond orientations generate effective dimerized
Hamiltonians reminiscent of the Su–Schrieffer–Heeger (SSH) model. Although the uniform zigzag chain develops a spectral gap, no localized edge states are observed. We show that modified boundary parameters generated by the phononic mapping suppress the edge-state formation expected from the ideal SSH picture. Introducing a
geometric domain wall restores localized domain-wall states inside the gap, which give rise to resonant transmission channels across an otherwise insulating frequency window. The resonance energies remain robust against system-size variations and the corresponding transmission approaches unity.
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Materials Science · Cross-listed from cs.LG
Growth-Inspired Graph Generation and Inverse Design of Mechanical Lattices via Dot Matrices Database Augmentation and GCNN
Weiyun Xu and Jiamu Liu
Natural load-bearing and transport networks are not assembled in a single step; they emerge through a temporally ordered process of growth, branching, reinforcement, and loop formation. Inspired by this developmental logic, this work introduces a morphogenetic graph-generation framework for mechanical
lattices in which a discrete dot
matrix provides potential nodes and the final architecture is created by sequential cross-layer and intra-layer growth. The same rule is visualized in two dimensions as a leaf-vein-like developmental sequence and implemented in three dimensions on a 3x3x3 nodal
matrix containing 27 candidate nodes. A
dataset of distinct three-dimensional
lattices was evaluated by beam-based finite element analysis and represented directly as graphs. A graph convolutional neural network (GCNN) with three graph-convolution layers and dual global pooling learns the
topology-property mapping and predicts effective compressive stiffness. Coupling the GCNN surrogate with rapid structural sampling enables inverse design: for a target stiffness of 1000 MPa, the selected design was predicted at 1042.43 MPa and validated by finite element analysis at 1027.49 MPa. Beyond straight members, the framework has also been extended to parameterized horseshoe-shaped curved beams made of nonlinear materials, enabling
topology-geometry design toward prescribed deformation shapes. Our work provides a paradigm for augmenting the database of mechanical metamaterials, and the resulting perspective links biological morphogenesis, graph learning, and nonlinear shape programming in a unified generative design framework for architected materials.
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Strongly Correlated Electrons
Exact selection of a toric-code vison crystal in a flux-conditioned Kitaev model
Jiucai Wang and Chuan Chen
We construct an exactly solvable extension of the
spin-$1/2$ Kitaev honeycomb model in which conserved $\mathbb{Z}_2$ fluxes determine not only the signs but also the connectivity of nearest-neighbor Majorana hopping. At a tuned loop point, hopping survives only across opposite-flux plaquettes, so every vertex has active degree zero or two and the matter
Hamiltonian fragments in each flux sector into independent Majorana rings and isolated zero modes. Exact ring spectra and bond counting then bound the matter energy over all local flux configurations and all four Wilson-loop sectors, and split it exactly into a frustrated triangular-
lattice Ising term, whose extensively degenerate ground states are the fully packed loop coverings, and a non-negative Majorana residual. On admissible commensurate
tori, the residual selects precisely the three translation-related $2/3$-vison
crystals, which saturate the bound, and an exact
fermion-parity identity shows that for antiferromagnetic coupling their
vacua also survive projection, making them rigorous ground states of the
spin model. Within a single
crystal, a depth-one local
unitary then maps the ground space onto that of a sheared square-
lattice toric code, giving fourfold topological degeneracy. The model thus realizes exact nonperturbative gauge-matter feedback: the flux fixes where the Majorana
fermions may move, and their zero-point energy selects in return a topologically ordered vison
crystal with spontaneously broken translation
symmetry.
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Materials Science
Generative crystallographic phasing through invariant relationships
Qi Li, Rui Jiao, Liming Wu et al. (+16 more)
Crystal structure determination requires the phases of scattered waves – yet diffraction measures only their intensities. Direct methods exploit phase invariants but become less reliable as diffraction information diminishes. Learned phase prediction has lowered the resolution barrier, yet remains primarily confined to centrosymmetric
crystals with binary phases. We introduce PhiGen, a generative reformulation of traditional direct methods that learns origin-independent phase relationships for binary and continuous phasing. Across 210 space groups, including groups absent from training, it recovered high-quality maps for 99.0% of centrosymmetric structures and invariant-consistent phases for 92.8% of non-centrosymmetric structures. From simulated 3 Å zeolite powder data, the network recovered framework maps for 84.2% of held-out structures, versus 1.0% for Superflip. For experimental ZSM-25 and TNU-9, generated phases seeded high-resolution phase extension. These results suggest a route to structure determination from low-resolution, incomplete, and overlapped diffraction data.
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All authors Qi Li, Rui Jiao, Liming Wu, Chang Chen, Tiannian Zhu, Bintang Wang, Qiuliang Liu, Zhonglong Peng, Munan Hao, YingPeng Yu, Lin Yao, Wei Ding, Mao Su, Lei Bai, Yang Liu, Hongming Weng, Wenbing Huang, Shifeng Jin, Xiaolong Chen
Materials Science
Beyond the Kagome Layer: Interlayer Origin of the Flat Band in FeSn
Shimin Zhang, Bipasa Samanta, Ho Viet Thang et al. (+1 more)
Kagome FeSn exhibits an occupied flat band at its terminated surface, whereas bulk FeSn adopts A-type antiferromagnetic order and does not display the same feature. Here, we combine density functional theory with primitive- and doubled-
cell analysis and a double-layer tight-binding model to determine how interlayer electronic coupling and
magnetic stacking control flat-band formation in FeSn. We identify an occupied Fe-$d_{z^2}$-derived flat-band
manifold in the ferromagnetic state that is consistent with the experimentally observed surface feature. Brillouin-zone folding reveals that its flat branch originates from the $k_z=\frac{\pi}{c}$ sector of the primitive
cell, demonstrating that it cannot be understood as an isolated kagome-layer state. Instead, the state depends on coupling between neighboring kagome layers and can be seen as a result of antibonding coupling between nearest neighbor kagome layers. A double-layer tight-binding analysis identifies interlayer Fe-Fe hopping as the dominant microscopic coupling responsible for this behavior, while a contrasting unoccupied flat-band-related
manifold is governed primarily by intralayer Fe-Sn hybridization. These results establish interlayer coupling and
magnetic stacking as key control parameters for kagome flat bands and highlight how coupling between layers can generate and tune extended correlated-electron states in
quantum materials.
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All authors Shimin Zhang, Bipasa Samanta, Ho Viet Thang, Alexandru B. Georgescu
Mesoscale and Nanoscale Physics
Zhi-Hai Liu, Jiang Zhang, Guilu Long et al. (+1 more)
Spin is typically traced out in the description of
quantum-dot-based Kitaev chains to simplify the construction of Majorana
fermions. Yet the intrinsic
spin structure of poor-man's Majorana modes in minimal Kitaev chains under finite Zeeman fields offers a natural interface for the Kitaev parity
qubit to interact with other spinful systems. Here, we establish such a platform to bridge the parity
qubit and a
quantum-dot
spin qubit, with the effective coupling governed by the
spin-dependent delocalization of the Majorana modes. Depending on whether the
spin qubit is coupled to one or two chains constituting the parity
qubit, the parity-
spin coupling exhibits distinct forms: an anisotropic parity-conserving exchange interaction or a nontrivial exchange tensor tunable via the interchain superconducting-phase bias. Leveraging fast
spin-
qubit manipulation, we further demonstrate universal parity-
qubit control, high-fidelity
qubit-state readout, and entangling operations between the parity and
spin qubits. These results turn the spinful structure of poor-man's Majoranas from a finite-field imperfection into a resource for hybrid
quantum control.
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All authors Zhi-Hai Liu, Jiang Zhang, Guilu Long, H. Q. Xu
Quantum Gases
Moiré droplet of ultracold Bose gases in a twisted-bilayer optical lattice
Tianqi Luo, Jing Zhang and Xiaoling Cui
We report the emergence of Moiré droplet in two-dimensional ultracold
bosons subjected to a
spin-dependent optical
lattice, effctively realizing a twisted-bilayer configuration. We show that the droplet formation dramatically enhances the visibility of Moiré pattern in the density profile, even for exceptionally weak
lattice potentials. The Moiré pattern can be enhanced similarly by increasing the
lattice depth, which, however, also induces droplet
diffusion characterized by a spreading density profile. Furthermore, we demonstrate a dynamical generation of Moiré pattern by dragging a small droplet through a moving
lattice. At appropriate velocities, the droplet undergoes bifurcation and exhibits pronounced Moiré pattern within periodic time intervals. Our results establish the ultracold droplet as a compelling platform for simulating interacting Moiré physics, particularly the interplay between Moiré
lattice and bound-state formation.
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Mesoscale and Nanoscale Physics
Conductance of silicon nanotube junctions in high magnetic fields
Teresa Kulka, Juan Alberto Canché-Martín, Irina V. Lebedeva et al. (+2 more)
We investigate coherent
quantum transport through silicon nanotube (SiNT) junctions in high
magnetic fields up to 60 T using a tight-binding model combined with the non-
equilibrium Green's function formalism, and
magnetic field included via Peierls substitution. We consider junctions of metallic nanotubes (6,0)+(6,0) and semiconducting ones (9,9)+(9,9), and examine the effects of the overlap length, inter-tube distance,
magnetic-field direction, and field strength on the electronic transmission. In contrast to carbon nanotube junctions, the SiNT systems exhibit irregular transmission oscillations and do not show the emergence of highly conductive gateway states. The transmission is substantially more sensitive to a
magnetic field perpendicular to the nanotube axis than to a parallel field, while increasing the field strength progressively modifies the transmission spectrum. Increasing the overlap length results in more frequent transmission oscillations, whereas increasing the inter-tube distance modifies their positions and amplitudes without changing their overall character. Generally, similar trends are observed for both types of junctions, involving metallic and semiconducting nanotubes. However, in the junction of semiconducting nanotubes, one observes peculiar additional field-dependent in-gap transmission features. These results demonstrate that the
magnetic-field response of SiNT junctions is strongly governed by their geometry and differs qualitatively from that of pristine carbon nanotube junctions.
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All authors Teresa Kulka, Juan Alberto Canché-Martín, Irina V. Lebedeva, Jacek A. Majewski, Karolina Z. Milowska
Materials Science
Influence of chemical vapor deposition conditions on N incorporation ratio on vicinal 4H-SiC(000-1) surface: Ab Initio-based approach
Wataru Ota, Akira Kusaba, Yoshihiro Kangawa et al. (+3 more)
In experimental studies, increasing the ratio of source gases (C3H8/SiH4; C/Si ratio) for chemical vapor deposition (CVD) causes the growth rate to increase monotonically, and nitrogen incorporation tends to decrease accordingly; however, a unique phenomenon has been observed in which nitrogen incorporation increases discontinuously in the range of C/Si ratio between 1.0 and 1.5. This phenomenon is specific to the vicinal 4H-SiC(000-1) C-face and is not observed on the vicinal 4H-SiC(0001) Si-face. In this study, N incorporation behavior on a vicinal C-face during CVD is investigated using an ab initio-based approach. The calculation results suggest that when C/Si ratio is less than 1.0, the Si-terminated step edge is stable, whereas when C/Si ratio exceeds 1.0, the existence probability of the C-H-terminated step edge, where the N substitution energy is lower than in the former case, increases sharply. This change in the step-edge state across C/Si = 1.0 is thought to be the cause of the discontinuous increase in N incorporation.
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All authors Wataru Ota, Akira Kusaba, Yoshihiro Kangawa, Keisuke Kurashima, Ichiro Mizushima, Kenji Shiraishi
Materials Science
Magnetostrictive properties in Fe$_{4-x}$Co$_{x}$N films: Insight from experiments and first-principles calculations
Huameng Yu, Keita Ito, Shoya Sakamoto et al. (+4 more)
The ferromagnetic nitride Fe$_{4}$N has attracted
attention for application in spintronic devices due to its high
spin polarization and large magnetostriction. We present a combined experimental and theoretical study on the magnetostriction of Fe$_{4-x}$Co$_{x}$N films across a wide composition range. The Fe$_{4-x}$Co$_{x}$N films were grown on SrTiO$_{3}$(001) substrates using molecular beam epitaxy, and the magnetostriction constants along the [100] direction (${\lambda}$$_{100}$) and [111] direction (${\lambda}$$_{111}$) were precisely evaluated using an optical cantilever method. The experimental results reveal that ${\lambda}$$_{111}$ remains positive in the whole composition range and shows a maximum value of +82 ppm around x = 0.9. The variation in ${\lambda}$$_{111}$ with x is much smaller than that in ${\lambda}$$_{100}$, for which giant tunability and sign reversal are observed. First-principles calculations show reasonable agreement with the experimental ${\lambda}$$_{111}$ for x ${\ge}$ 1.6, but give negative values at lower x, and an exceptionally large negative ${\lambda}$$_{111}$ is obtained at x = 0.8, where the Fermi level coincides with a pronounced minority-
spin peak in the density of states. The calculated ${\lambda}$$_{111}$ depends strongly on the smearing parameter, indicating that the rhombohedral magnetostriction is highly sensitive to the treatment of atomic disorder. The saturation magnetostriction constant (${\lambda}$$_{s}$) derived from ${\lambda}$$_{100}$ and ${\lambda}$$_{111}$ is also compared with the ${\lambda}$$_{s}$ measured for the (001)-oriented polycrystalline Fe$_{4-x}$Co$_{x}$N films, and a possible scenario for deviation between them is discussed. Our findings clarify the basic features of magnetostriction in the Fe$_{4-x}$Co$_{x}$N system, providing essential magnetoelastic parameters for designing nitride-based spintronic devices.
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All authors Huameng Yu, Keita Ito, Shoya Sakamoto, Ivan Kurniawan, Yoshio Miura, Yasushi Endo, Takeshi Seki