Strongly Correlated Electrons
Kagome lattice candidate URhSn: Measured Bragg diffraction patterns and theory for hexagonal and trigonal Sohncke phases
S. W. Lovesey and D. D. Khalyavin
Ternary intermetallics use a ZrNiAl-type chemical structure known as a kagome system. Complexity observed in the phase diagrams of these compounds is attributed to the
geometric frustration. The 5f-electron compound URhSn exhibits two phase transitions at 16 K and 54 K. No super-
lattice reflections in
neutron powder diffraction patterns are detected in the intermediate range of temperatures (16 K - 54 K). Recent resonant x-ray diffraction patterns for uranium ions in the intermediate phase suggest a chiral structure and a trigonal Sohncke space group. It is firmly established that a simple hexagonal space group describes the parent structure at room temperature. A ferroic order parameter that includes hexadecapoles is shown to characterize the trigonal Sohncke phase. Resonant x-ray diffraction by this phase is fully investigated with our
symmetry informed theory. It repairs
symmetry in the original data analysis by using a grey group, and it lifts an unjustified spatial condition on uranium positions. The theory uses axial atomic multipoles that satisfy sum-rules established in the first instance for x-ray dichroic signals. A confrontation between observed and calculated diffraction patterns lends support to a trigonal Sohncke phase, and exposes grounds for additional experimental work on an enigmatic compound.
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Soft Condensed Matter
Dynamical Anisotropy of a Colloidal Glass Under Pressure
Shengyun Shi, Li Tian and Bo Li
Pressure is a critical thermodynamic parameter that profoundly influences the physical properties of glasses. Pressure-induced densification and structural transformation endow glasses manufactured under such conditions with exceptional mechanical and optical properties. Although pressure-treated glasses have been characterized by ensemble-averaged methods such as X-ray diffraction and Raman spectroscopy, their microscopic dynamics have rarely been addressed, limiting our understanding of the coupling among structure, dynamics, and mechanics. Here, using a binary hard-sphere colloidal glass confined in cylindrical capillary tubes, we impose a constant pressure on the particles through the tangential component of
gravity. This approach enables the first investigation of pressure effects on colloidal glasses. We find that the dynamics are substantially frozen, whereas the structural change remains comparatively mild. At low pressure, spatial correlations among structural, dynamical, and local elastic heterogeneities are observed. Remarkably, dynamical anisotropy emerges in response to pressure, characterized by faster motion parallel to the pressure direction than perpendicular to it. This anisotropy is attributed to an instability induced by the strong pressure force. Concurrently, structural and dynamical heterogeneities are strongly suppressed under pressure. Our experiments characterize the microscopic dynamics of colloidal glasses under pressure and offer design principles for the manufacturing protocol of glass materials.
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Disordered Systems and Neural Networks
Anderson localization in periodic elastic systems with random perturbations
Xin Feng, Peijun Li and Wei Wu
This paper investigates Anderson localization in subwavelength elastic periodic systems with random perturbations. For the unperturbed system, we use layer potential techniques to reformulate the
eigenvalue problem as boundary integral equations, and derive asymptotic formulas for the subwavelength
eigenvalues. For perturbed systems, we apply the Floquet transform to obtain a periodic formulation and derive equations determining the resonant frequencies under general perturbations. Numerical experiments for perturbed periodic monomers and dimers agree with the theoretical predictions. We further demonstrate Anderson localization by increasing the strength and number of random perturbations. These results provide a mathematical foundation for understanding subwavelength localization in elastic metamaterials.
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Soft Condensed Matter
Avalanches can increase stored energy in a granular fault
A. Douin, E. Saurety, V. Levy dit Vehel et al. (+4 more)
Slowly sheared granular materials generally store mechanical energy and dilate between abrupt failures that release energy and compact the material. Here, simultaneous measurements of torque, layer thickness, acoustic emission, and photoelastic force networks reveal all four combinations of energy release or storage with contraction or dilation in a compressed granular fault. Most strikingly, some avalanches both dilate the layer and increase the elastic energy transmitted to the resisting boundary. These events reorganize force chains beyond the shear band and produce a distinct acoustic response. The results show that an avalanche need not relax a driven disordered material; it can instead redistribute stress into a more highly loaded configuration, a mechanism with potential relevance to the physics of both laboratory and natural faults.
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All authors A. Douin, E. Saurety, V. Levy dit Vehel, L. Combe, L. Vanel, O. Cochet-Escartin, O. Ramos
Strongly Correlated Electrons
Reservoir-conditioned virtual returns generate random Liouvillian skin localization in a reciprocal Mott insulator
Y. T. Wang, X. Z. Zhang and W. M. Liu
Directional dissipation can concentrate relaxation modes in space, but connecting this accumulation to controlled microscopic processes in correlated matter requires separating virtual charge motion from
spin coherence. We study this connection in a half-filled Hubbard chain with reciprocal hopping and number-conserving, direction-selective returns of virtual doublon–hole defects. Eliminating charge defects and then Mott coherences yields asymmetric
spin-exchange rates under an explicit separation of timescales, with full short-chain dynamics supporting the reduction on finite exchange times. Balanced random returns concentrate the stationary population and several low-lying right modes at sample-selected positions rather than a predetermined edge, producing random Liouvillian skin localization despite zero end-to-end logarithmic rate bias. The accumulated rate imbalance determines an exact finite-density hard-core stationary state and a one-particle activated relaxation scale governed by random barriers. This connection between locally calibrated return rates, many-body stationary weights and slow relaxation offers a means of controlling transport in constrained open
quantum matter without changing the reciprocal
Hamiltonian.
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Disordered Systems and Neural Networks · Cross-listed from math.DS
Phase Transitions and Modulation in Dense Oscillatory Associative Memories
Shurui Liu and Zhuchun Li
We introduce high-order Winfree models for oscillatory associative
memory. We characterize
memory performance through the local-stability dichotomy between stored and unstored patterns. Using this criterion, we show that crosstalk noise drives a cascade of ferromagnetic, mixed, and
spin-glass transitions as the
memory load increases. For both
polynomial and exponential Winfree models, we derive the phase boundaries and develop auxiliary-field modulation schemes adapted to the different phases. We further present corresponding
circuit designs and numerical simulations that support our theoretical predictions.
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Statistical Mechanics · Cross-listed from quant-ph
Quantum synchronization: A tutorial guide
Sourabh Lahiri and Shamik Gupta
Synchronization is a collective phenomenon in which interacting nonlinear oscillators develop a persistent relation between their phases and frequencies. In
quantum systems, its description requires connecting the classical dynamics of limit-cycle oscillators with
quantum fluctuations, dissipation, and the notion of phase. In this tutorial review, we offer a systematic framework for analyzing synchronization in classical and
quantum dynamical systems. Starting from amplitude-phase dynamics, we introduce successively topics of relevance, such as phase locking, the Adler equation, Arnold tongues, and the Kuramoto model, and use these concepts to analyze coupled oscillators and their stability. We then formulate the corresponding description for
quantum limit-cycle oscillators using Lindblad master equations and phase-space methods, with explicit examples of two and many coupled oscillators. We further discuss noise, synchronization measures, and the extreme
quantum regime, including synchronization in
spin systems. The emphasis throughout is on analytical derivations and a practical methodology for identifying synchronized states, determining their stability, and characterizing synchronization in
quantum systems. The review is designed as a self-contained guide from which we hope that students can learn the essential concepts and techniques, while researchers can readily find the analytical tools and methodological insights needed to approach new synchronization problems.
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Materials Science
4DMulti: automated multicomponent identification at complex material interfaces
Haoran Zhang, Zian Mao, Shufen Chu et al. (+6 more)
Mapping crystalline phases at heterogeneous interfaces is essential for understanding material performance and degradation. However, structural heterogeneity, phase overlap, and local disorder complicate diffraction interpretation, while growing data volumes make manual analysis increasingly impractical. We introduce 4DMulti, a physics-guided learning framework for automated multicomponent identification from large-scale four-dimensional scanning transmission electron microscopy (4D-STEM) data. The supporting diffraction data resource comprises over 6 million high-quality experimental patterns and labeled patterns generated by Sim2real. A
retrieval-conditioned latent
diffusion transformer (Sim2real) translates simulated patterns into experimental-style examples under constraints designed to preserve Bragg geometry, while a rotation-invariant coordinate convolutional network identifies phases across in-plane rotations. 4DMulti achieves 98.82% classification accuracy on a five-phase experimental nanoparticle
benchmark, with ablation studies supporting the complementary benefits of domain adaptation and rotation-invariant classification. We define diffraction-inferred structural complexity (DISC), a normalized predictive
entropy score that quantifies phase-assignment ambiguity within a specified candidate phase library. We apply 4DMulti to generate structural maps of superconducting
heterostructures, corroded
alloy surfaces, and degraded solid-state battery interfaces down to single-nanometer spatial resolution. 4DMulti connects simulation-derived crystallographic knowledge to automated experimental interpretation, establishing a foundation for scalable analysis of complex interfaces and data-driven discovery of interfacial design principles.
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All authors Haoran Zhang, Zian Mao, Shufen Chu, Xiaoya He, Yuyan Guan, Antong Yang, Mingze Li, Xiaoqin Zeng, Yujun Xie
Soft Condensed Matter · Cross-listed from nlin.PS
Extreme Events in an Active Fluid Medium
Joydeep Das, Abhishek Chaudhuri and Sudeshna Sinha
We observe the emergence of extreme events in an active fluid involving two distinct chemical species that regulate active stress. One species is slow diffusing and the other is fast diffusing, and the growth of the fast-diffusing species is modelled using a nonlinear logistic term. We demonstrate the presence of extreme events in the temporal
evolution of the concentrations, as well as in the spatial profile of the system,in regimes of merging-emerging
soliton-like dynamics and spatio-temporal chaos, through analysis of the time-series, bifurcation diagrams, probability distribution functions of the concentration of the two species, return maps and distributions of inter-event intervals. Interestingly, we also find evidence of pronounced bunching of extreme events and super-extreme events in the slow chemical species in the
soliton-like regime. We go on to systematically explore the dependence of the extreme event occurrences on the Péclet number and the strength of the nonlinear growth term, and find that the probability of extreme events increases after a critical Péclet number, while increasing the nonlinearity suppresses extreme events. Lastly, in order to gain further insight, we investigate a modified mode-truncated reduced order model comprising of coupled differential equations mimicking this active fluid system. We find that this reduced order model also exhibits extreme events whose emergence is correlated with a sudden expansion in attractor size due to a crisis arising from attractor collision.So these results demonstrate the existence of extreme events in an active fluid system, and are of potential relevance to biological phenomena where active transport plays an important role.
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Mesoscale and Nanoscale Physics
Spectral density of angular momentum transfer from a swift electron to a large spherical nanoparticle
Jorge Luis Briseño-Gómez and Alejandro Reyes-Coronado
Swift electrons in scanning transmission electron microscopy transfer both linear and angular momentum to nanoparticles, underlying electron-beam-driven nanoscale manipulation ("electron tweezers"). Prior theory relied either on the small-particle (dipolar) approximation, valid only well below experimentally relevant sizes, or on frequency-integrated multipolar calculations that leave the spectral structure of the interaction unresolved. Here we present a fully retarded, causal, multipole-converged electrodynamical methodology for the angular momentum transfer from a swift electron to an isolated spherical nanoparticle, based on a closed-surface Maxwell stress tensor formulation whose angular integrals reduce analytically to a small, material- and trajectory-independent set of irreducible integrals over associated Legendre functions. This lowers the cost of the double multipolar sum, enabling convergence up to l_max=51 for nanoparticles as large as a=50 nm, nearly four times the order of the largest previous calculation at this size and previously unreached for an optically complex, interband-dominated material. Applied to aluminum and gold nanoparticles up to a=50 nm, the method resolves the transfer spectral density across the full frequency domain, showing it is set by interference between the electron field and the field scattered by the nanoparticle, which dominates the scattered-scattered contribution at essentially every frequency; the electric contribution dominates at moderate speeds, but the
magnetic contribution, of the same sign, grows steadily in relative weight with electron speed, from a few percent of the total at v = 0.5c to between a quarter and a half of it at v = 0.95c for trajectories passing close to the nanoparticle surface.
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Materials Science
Interfacial Engineering Enabled High-Resolution Stretchable Metal-Level Conductive Lines and Transparent Conductor
Ke Chen, Eric Tianjiao Zhao, Weichen Wang et al. (+16 more)
As stretchable electronics advance toward higher integration density and finer feature sizes, stretchable conductors, which serve as the architectural backbone of these electronics, must be scaled down accordingly. However, achieving both high stretchability and high electrical conductivity at high resolution remains a challenge using existing conductive materials. Here, through material design and interfacial engineering, we develop a thiol-functionalized conducting
polymer/gold hybrid stack that can be patterned down to 4 micrometer linewidths using standard photolithography, while maintaining high stretchability, metal-like conductivity (>40,000 S/cm), and environmental stability. Leveraging this capability, we demonstrate grid-based stretchable transparent electrodes that surpass the figure-of-merit of indium tin oxide, as well as a 1000-pixel-per-inch image interconnected with stretchable lines. This work helps to broaden the scope of next-generation functional soft electronics, including e-skins and bioelectronics.
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All authors Ke Chen, Eric Tianjiao Zhao, Weichen Wang, Yepin Zhao, Kostas Parkatzidis, Lukas Michalek, Yuran Shi, Elizabeth Zhang, Tianyang Chen, Ruiheng Wu, Hao Lyu, Yating Yao, Yujia Yuan, Tianhao Chen, Ruby Rong Zhou, Shiyuan Wei, Junyi Zhao, Jeffrey B.-H. Tok, Zhenan Bao
Statistical Mechanics · Cross-listed from hep-th
Abhigyan Saha, Piotr Sułkowski and Tadashi Takayanagi
Pseudo
entropy extends
entanglement entropy from a single
quantum state to a pair of nonorthogonal states and is generally complex. Taking advantage of Cauchy-Riemann equations, Kramers-Kronig relations, and analytic continuation in state parameters, we show how and to what extent real and imaginary parts of pseudo
entropy can be derived from ordinary
entanglement entropy. For families with holomorphic coefficients in finite-dimensional
Hilbert spaces, the reduced transition
matrix equals the ordinary reduced density
matrix formula evaluated at complex parameters. Then a convergent Taylor series gives the real and imaginary parts of pseudo
entropy from even and odd derivatives of
entanglement entropy at the real midpoint. The
matrix identity also gives formulae for excess pseudo
entropy and Renyi
entropies, and interpolation formulae for families with
polynomial coefficients. We apply these results to boundary-state quenches and thermal states in conformal field theory, and to fermionic and bosonic Gaussian states and quenches. In conformal field theory, Kramers-Kronig relations give the first moment of the imaginary part in terms of the central charge and one-point functions for boundary states.
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Other Condensed Matter · Cross-listed from hep-th
Holographic Casimir Effect for Mixed Boundary Conditions and non-CFTs
Bing-Ji Ding, Hua-Chao Liu and Rong-Xin Miao
This paper investigates the holographic Casimir effect in AdS/BCFT with a brane-localized scalar field. The scalar field takes different values at the strip's two boundaries, leading to mixed boundary conditions. The massive brane-localized scalar field typically breaks the boundary conformal
symmetries, allowing us to study the holographic Casimir effect in non-CFTs. In two-dimensional spacetime, we apply the holographic g-
theorem to prove the holographic bound on the Casimir effect for general brane-localized matter fields. In higher dimensions, we find that the brane-localized scalar field reduces the Casimir amplitude when the mass squared \(m^2=0\), but can increase it when \(m^2 < 0\). Additionally, there is a no-hair
theorem for the cases where \(m^2>0\). These findings indicate that relevant boundary deformations can enhance the Casimir effect. As a byproduct, we obtain a gravitational dual of the repulsive Casimir force under mixed boundary conditions and argue that it aligns with the
cosmic censorship
conjecture.
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Materials Science
Time- and Frequency-Resolved Observation of Inverse Orbital Hall Effect in Gallium Nitride via Terahertz Polarimetry
Kota Aikyo, Tomohiro Fujimoto, Ami Mi Shirai et al. (+6 more)
Orbitronics has attracted significant
attention as a platform for information storage and processing that exploits the orbital angular momentum (OAM) of electrons without the need for
spin-orbit coupling. However, experimental evaluation of OAM-charge interconversion remains a challenge and the results are often controversial due to the coexistence of bulk and interfacial contributions and the complexity in sample structures. Here, using circularly polarized light pulses and terahertz (THz) polarimetry, we developed a non-contact method to observe the inverse orbital Hall effect as a bulk response within a single material without employing
heterostructure samples. In a
semiconductor GaN, we directly captured the OAM-to-charge current conversion of holes in the THz frequency range. By analyzing the sharp frequency dependence of the Hall conductivity, we disentangled the competing microscopic mechanisms and revealed the dominant role of extrinsic contributions to the orbital Hall effect in the dc limit. By contrast, the Hall conductivity at THz frequencies above the impurity scattering rate is attributed to the intrinsic Berry-
curvature mechanism,allowing a quantitative comparison with the microscopic theory. Furthermore, the ultrafast dynamics of the inverse orbital Hall signal directly revealed sub-picosecond OAM relaxation of holes, comparable to that of
phonon-mediated thermalization. The quantitative argument based on theoretical calculations suggested the existence of an even faster decay channel due to momentum redistribution by acoustic
phonons, suggesting a sub-nanometer-scale OAM relaxation length. Our results provide comprehensive and crucial insights into OAM transport and establish an ultrafast, contact-free approach for investigating OAM-to-charge conversion.
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All authors Kota Aikyo, Tomohiro Fujimoto, Ami Mi Shirai, Yuta Murotani, Mitsuru Funato, Shinji Miwa, Jun Yoshinobu, Yoichi Kawakami, Ryusuke Matsunaga
Materials Science
Cryothermal Measurements of Variable-Emittance Coatings with Lower Phase Transition Temperatures for Space Thermal Control
Chloe Stoops, Vishwa Krishna Rajan and Liping Wang
Space thermal control is critically important to ensure proper operation of on-board equipment in a regulated temperature range. Passive thermal control with variable-emittance coatings (VECs) could help save power consumption in a dynamically changing space thermal environment. Vanadium dioxide (VO2) based VECs have been studied for space thermal control but its intrinsic phase transition around 68{\deg}C limits its wider space applications where lower temperature ranges are expected. In this work, we experimentally demonstrate enhanced radiative heat dissipation in space-like thermal environment via cryothermal measurements with VECs of undoped and tungsten doped VO2. The fabricated undoped VEC exhibits a large emittance change of 0.6 across the phase transition, while the 1 at.% tungsten doped one shows an appreciable emittance variable of 0.4 with phase transition temperature lowered by 25{\deg}C. A
vacuum cryothermal setup is developed with a
liquid nitrogen cooled coldfinger to mimic cold space thermal background and a custom-designed sample mount suspended by nylon wires. After careful calibration and validation, greatly enhanced radiative heat dissipation upon VO2 phase transition up to 3.5 times with transition temperature lowered by 25{\deg}C from 1 at.% tungsten doping is clearly observed from the cryothermal tests. In the actual space thermal environment, radiative heat flux could further increase across phase transition from 160 W/m2 to 650 W/m2 with undoped VO2 coating from 55{\deg}C to 80{\deg}C, and from 175 W/m2 to 493 W/m2 with 1 at.% tungsten doped VEC from 30{\deg}C to 55{\deg}C.
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Disordered Systems and Neural Networks · Cross-listed from math.PR
Disorder transfer for the critical SK overlap law
Yan Ru Pei
We give a quantitative disorder comparison for the zero-field Sherrington–Kirkpatrick model at inverse temperature one. For any fixed number of replicas, replacing Gaussian couplings by independent couplings from a bounded symmetric variance-one law changes a bounded replica expectation by at most a constant times the Gaussian overlap second moment plus $N^{-1}$. A multiplicative comparison for nonnegative observables controls the tails. The proof uses Talagrand's positive-observable estimates and Yu-Ting Chen's fourth-order replica cancellation. Assuming the Gaussian critical overlap limit stated by Du and Huang, we obtain the same limit for the random quenched overlap measure in the iterated Wasserstein-2
topology. No separate moment assumption is needed for this transfer. Their additional exponential moment bound gives convergence of the rescaled
spin-glass susceptibility in every finite Wasserstein distance. The coupling class includes fair signs, uniform disorder, and signs thinned at any fixed positive density.
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Disordered Systems and Neural Networks · Cross-listed from q-bio.NC
Nonlinear dynamics of random neural networks with second-order synaptic motifs
Jun Yang and Hannah Choi
Classical theories of random neural networks typically assume independent connectivity, overlooking the local motif structures prevalent in biological
circuits. Here, we investigate how four second-order synaptic motifs (chain, reciprocal, convergent, and divergent) shape the dynamics of nonlinear firing-rate networks. While previous studies have established that chain correlations generate outlier
eigenvalues, we demonstrate that these motifs also jointly reshape the Jacobian
eigenvalue bulk. Using the path-integral formalism, we derive a dynamic mean-field theory which reveals that the chain motif acts as a retarded feedback of the ensemble-mean activity through the response kernel, producing a rich repertoire of dynamical regimes, including ferromagnetic states and limit cycles. At sufficiently large magnitude, negative chain correlations produce a glassy, multistable regime that was previously mainly associated with partially symmetric networks. Our theory also distinguishes convergent from divergent motifs: divergent correlations primarily rescale temporal noise, while convergent correlations suppress temporal chaos by converting nonzero mean activity into quenched heterogeneity. Finally, analyses of the Lyapunov spectrum and participation-ratio dimension show that motif structure changes the geometry of chaotic activity, reducing
entropy production and attractor dimensionality even when the effective spectral edge is held fixed. Together, these findings establish second-order motifs as a fundamental structural mechanism governing the dynamical regimes of local cortical
circuits.
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Mesoscale and Nanoscale Physics
The effect of light scattering in cavity electrodynamics: Fresnel equations with decoherence
Natalya A. Zimbovskaya and Abraham Nitzan
We consider the effect of light decoherence in a Fabri-Perot (FP) microcavity. We show that, when present, it may significantly change its linear response to the incident light.The optical properties of the bounding mirrors are described using the classical electrodynamics, and the light scattering causing the phase breaking is treated as a multichannel scattering problem employing a model introduced by Büttiker to describe dephasing in electron transport. We show that the dephasing causes a gradual erosion of the cavity
photon mode and thus impedes the formation of molecular polaritons. Consequently, the polaritons signatures in the transmission and absorption optical spectra of the microcavity are fading away as the scattering intensifies.
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Mesoscale and Nanoscale Physics · Cross-listed from quant-ph
An All-van-der-Waals Qubit
Sein Park, Sameia Zaman, Junghyun Kim et al. (+19 more)
Advances in solid-state physics, materials science, and device engineering have accelerated the development of superconducting
qubits. Among emerging platforms, van der Waals (vdW) materials and their
heterostructures are potentially attractive building blocks for
quantum devices, yet their realization in
qubit architectures remains largely underexplored. Here we report an all-vdW superconducting
qubit based on a NbSe$_2$-hBN-NbSe$_2$ junction, in which a thin hBN layer simultaneously provides Josephson coupling and capacitive shunting between two NbSe$_2$ islands, forming a "merged-element" transmon. Temporal characterization using
circuit quantum electrodynamics (cQED) techniques yields an average energy-relaxation time $T_{1,\mathrm{avg}} = 55 ~\mu s$, Hahn-echo coherence time $T_{2\mathrm{E},\mathrm{avg}} = 21 ~\mu s$, and Ramsey coherence time $T_{2\mathrm{R},\mathrm{avg}} = 1.9~\mu s$. The relatively low Ramsey time is primarily attributable to an enhanced sensitivity to charge noise consistent with the realized device parameters and not a fundamental limitation. These results show that lumped-element superconducting
qubits based on vdW
heterostructures can achieve coherence times comparable to those of conventional Al-AlO$_\mathrm{x}$-Al
qubits, while offering a reduced device footprint and suppressed stray capacitive coupling.
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All authors Sein Park, Sameia Zaman, Junghyun Kim, Junyoung An, Daniel Rodan-Legrain, Hung-Yu Tsao, Chia-Chin Tsai, Aranya Goswami, Réouven Assouly, William P. Banner, Gabriel D. Cutter, Kenji Watanabe, Takashi Taniguchi, Terry P. Orlando, Gil-Ho Lee, Kyle Serniak, Max Hays, Jeffrey A. Grover, Philip Kim, Pablo Jarillo-Herrero, Joel Î-j. Wang, William D. Oliver
Strongly Correlated Electrons
Vestigial altermagnetism
Peng Rao and Johannes Knolle
Interaction effects and fluctuations govern the phase diagram of systems with multiple competing phases. In particular, as individual phases are destroyed by increasing temperature, fluctuations can still produce a composite `vestigial' order given by a product of individual order parameters. Here, we describe vestigial Altermagnetism (AM) from the thermal melting of antiferromagnetic (AFM) and orbital orders (OO) on the square
lattice. The coexistence of AFM and OO can give rise to conventional AM with ordering wave vector $\mathbf{Q}=(\pi,\pi)$. We show that a distinct `vestigial AM' phase with $\mathbf{Q}=0$ can arise from thermal melting of AFM and OO, and investigate its generic phase diagram. We find that the transition from the high-temperature disordered phase into the vestigial AM phase can be either first or second order, depending on the AFM and OO bare susceptibilities and their interactions. We then investigate the unique experimental signatures by calculating the electron spectral function for a minimal two-orbital model. Despite the fact that the vestigial AM order parameter does not couple to electrons directly, fluctuations dominate the self-energy corrections giving rise to a
spin- and orbital-dependent quasi-particle lifetime with the AM
symmetry.
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Strongly Correlated Electrons
Emergence of Subdominant Quadrupolar Order in the 5$d^2$ Multipolar Mott Insulator Ba$_2$CaOsO$_6$
Ilija K. Nikolov, Giuseppe Allodi, Ginevra Corsale et al. (+5 more)
Relativistic $5d$ Mott
insulators host a rich variety of exotic hidden multipolar order, whose microscopic nature remains heavily debated. A broken local point-
symmetry (BLPS) phase followed by antiferromagnetism was previously observed in the doped compound Ba$_2$Na$_{0.1}$Ca$_{0.9}$OsO$_6$, where mixed Os valence places the system toward the $5d^2$ end of the $5d^1$-$5d^2$ regime. In contrast, pristine $5d^2$ Ba$_2$CaOsO$_6$ has shown a single octupolar transition with average cubic
symmetry, raising the question of whether BLPS arises from chemical disorder in the doped systems. Here, we discover the BLPS phase in pristine Ba$_2$CaOsO$_6$ emerging at $T^* \approx 50$ K, precisely coincident with the octupolar transition. Beyond standard ${}^{43}$Ca nuclear
magnetic resonance (NMR) spectral analysis, our
spin-echo nutation measurements detect a finite electric field gradient, demonstrating spontaneous
symmetry breaking despite the cubic average structure. While our NMR data support the previously identified octupolar order, the BLPS phase reveals a subdominant quadrupolar contribution, establishing that the hidden order in Ba$_2$CaOsO$_6$ is intrinsically multicomponent. Such mixed multipolar states lie beyond conventional theoretical descriptions of the $5d^2$ ground state. Our results establish local
symmetry breaking as an intrinsic property of the clean $5d^2$ limit and provide a new constraint on microscopic theories of strongly
spin-orbit-coupled Mott
insulators.
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All authors Ilija K. Nikolov, Giuseppe Allodi, Ginevra Corsale, Anshu Kataria, Cierra Foster, Patrick Woodward, Samuele Sanna, Vesna F. Mitrović
Statistical Mechanics · Cross-listed from math.PR
Correlation comparisons and critical curves for disordered XY models
Yan Ru Pei
We prove a lower comparison for disorder-averaged ferromagnetic XY correlations: independent nonnegative random couplings $K_e$ can be replaced by $-\frac12\log\mathbb{E}e^{-2K_e}$. Ginibre's inequality makes each normalized correlation convex in $1-e^{-2K_e}$, so conditional Jensen and thinning compare Bernoulli bond densities; two
star-wise Jensen passes handle site dilution on bipartite graphs. Together with the phase-existence
theorem of Dario and Garban, these comparisons give local Lipschitz regularity of both the averaged algebraic-phase and susceptibility-divergence thresholds throughout the supercritical density intervals on $\mathbb{Z}^2$. The clean finite-domain criterion of van Engelenburg and Lis also yields explicit finite-size susceptibility lower bounds in a weak-dilution region. For bounded centered bond noise, the possible suppression of the algebraic-phase temperature is at most quadratic in the noise amplitude. Finally, at finite positive thresholds we prove total-variation continuity for bounded iid coupling laws whose essential supremum equals the common support cap, with local Lipschitz control when the reference law has an atom at that cap.
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