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Physics Condensed Matter

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Saturday 23 May

Strongly Correlated Electrons

1/9 Magnetization Plateau in a Classical Kagome Ising Ferromagnet with Competing Further-Neighbor Interactions

The two-dimensional kagome lattice is a paradigmatic platform for exploring geometrically frustrated magnetism. While the nearest-neighbor ferromagnetic Ising model on this lattice is theoretically trivial, competing further-neighbor interactions can reintroduce severe frustration. In this work, we systematically investigate a classical kagome Ising model with ferromagnetic nearest-neighbor (J1) and antiferromagnetic second- (J2) and third-neighbor (J3) couplings using simulated annealing Monte Carlo methods. We demonstrate that while J2 couplings merely suppress the conventional ferromagnetic order, the inclusion of J3 fundamentally reconstructs the low-temperature phase diagram. This extended geometric frustration stabilizes a novel ordered phase characterized by a robust 1/9 magnetization plateau and a massively enlarged 3 by 3 magnetic supercell. Crucially, this fractional ordered phase manifests as a stability plateau in the phase diagram, where its critical temperature becomes nearly independent of the coupling strength J3. We also calculate the corresponding static spin structure factor, revealing a distinct Z6-symmetric reciprocal-space signature for experimental identification. Our findings reveal that complex fractional magnetic orders can emerge purely from classical geometric frustration induced by competing extended interactions, providing a distinct mechanism for understanding fractionally ordered states in real frustrated magnets.
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Statistical Mechanics

Thermodynamics of classifiers

The rise of artificial intelligence has led to a growing demand for computational power. In this situation, energy-efficient computing methods are being actively investigated, which raises a fundamental question: what is the relationship between computational error and thermodynamic cost? Here, we derive the error-cost trade-off in the binary classifier by considering classification based on nonequilibrium thermodynamics. We derive trade-off relations showing that classification error cannot be lower than fundamental bounds set by thermodynamic quantities: entropy production, which measures irreversibility, and dynamical activity, which quantifies the activity of the system. Our results show that when entropy production or dynamical activity vanishes, the classification error reaches $1/2$, equivalent to random guessing, whereas greater thermodynamic costs enable lower error. The results establish a quantitative trade-off in physical information processing, potentially leading to the development of energy-efficient computing devices.
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Superconductivity

Helical Rashba-exchange gauge field drives a uniaxial pair density wave in EuRbFe$_4$As$_4$

The recent discovery of an intrinsic, zero-field pair density wave (PDW) in the iron-pnictide superconductor EuRbFe$_4$As$_4$ poses a fundamental puzzle: how does a unidirectional, nanometer-scale superconducting modulation arise spontaneously below the magnetic ordering temperature? Here we show that the interplay of Rashba spin-orbit coupling – induced by the locally non-centrosymmetric FeAs layers – and the period-four helical Eu$^{2+}$ exchange field generates a layer-rotating effective $U(1)$ gauge field for the Cooper pairs. Because this gauge field shares the symmetry of the Fe $3d_{xz}/3d_{yz}$ orbital doublet, it drives an orbital-selective, finite-momentum pairing instability. Using a Ginzburg-Landau theory on the magnetic unit cell, we demonstrate that this mechanism naturally stabilizes a strictly uniaxial Bloch superconducting state at the experimentally observed wavelength, accompanied by spontaneous interlayer loop currents accessible to muon-spin relaxation or scanning SQUID microscopy.
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Statistical Mechanics · Cross-listed from quant-ph

Local Impurity Induced Growth and Scrambling in Clean Free Fermions

We study impurity-induced particle growth and scrambling in clean one-dimensional free-fermion systems. We show that a single local impurity can act as a branching source: particle or operator weight propagates coherently into the free bulk, returns to the impurity, and is locally converted into additional degrees of freedom. We develop this branching picture in three complementary settings: a monitored free-fermion model with feedback, a fully unitary interacting particle model, and Heisenberg operator dynamics with an interacting impurity. In the monitored model, we find a feedback-driven transition for both boundary and bulk impurities. In the unitary particle and operator models, a boundary impurity gives rise to an analogous transition from saturation to sustained growth and scrambling. These results reveal how a single impurity can generate complex many-body dynamics in an otherwise clean and free quantum system.
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Materials Science

Systematic comparison of approximations and functionals in first-principle calculations of aluminum-based III-V ferroelectric nitrides

We revisit first-principles predictions of structural, ferroelectric, and electronic properties in aluminum-based III-V nitride alloys, focusing on Al1-xScxN and Al1-xBxN. Using density functional theory within a unified 48-atom supercell framework, we systematically assess the role of chemical disorder and exchange-correlation approximations by comparing the virtual crystal approximation (VCA) and special quasirandom structures (SQS), as well as PBE, PBESol, SCAN, and SCAN+rVV10 functionals. We demonstrate that, even amongst the similar PBE and PBESol functionals, big quantitative and qualitative differences emerge. In particular, the VCA or SQS PBESol (a popular functional) strongly underestimate the stability domain of the ferroelectric wurtzite phase in Al1-xScxN compared to SQS PBE or SQS SCAN. We demonstrate that the 5-fold coordinated hexagonal phase predicted in 2002 by Farrer and Bellaiche [Phys. Rev. B 66, 201203] is a low-energy metastable state between the four-fold coordinated ferroelectric wurtzite phase and the six-fold coordinated rocksalt phase near the transition point upon increasing the Sc content. In contrast, Al1-xBxN shows a much faster destabilization of the wurtzite ferroelectric phase, with bond breaking which strongly distorts the wurtzite structure (with enhanced polarization) and eventually favor a zincblende phase and a threefold coordinated hexagonal layer phase. Our analysis highlights the critical importance of both local disorder and exchange-correlation treatment in predicting the functional properties of III-V nitride ferroelectrics. Overall, SQS combined with SCAN provides the most consistent theoretical framework for understanding and optimizing emerging nitride-based ferroelectric materials.
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All authors Alejandro Mercado Tejerina, Peng Chen, Keisuke Yazawa, Andriy Zakutayev, Laurent Bellaiche, Charles Paillard

Materials Science

Ultrafast Magneto-optical Fingerprints of Altermagnetism in MnTe

Recently identified altermagnets exhibit a distinctive dual-space nature: they possess spin-split electronic bands akin to ferromagnets in momentum space while maintaining the fully compensated magnetization of antiferromagnets in real space. This inherent duality, originating from the same crystal symmetry, gives rise to various intriguing physical phenomena unique to altermagnets. Consequently, a robust and efficient experimental signature capable of revealing this dual character is critically needed. The magneto-optical Kerr and Voigt effects, given their high sensitivity to ferromagnetism and antiferromagnetism, respectively, are ideally suited to probe this duality. Here, using time-resolved pump-probe magneto-optical measurements, we report the coexistence of pronounced Kerr and Voigt effects in the altermagnet MnTe. Combining the magnetization measurement and first-principles calculations, we demonstrate that the Kerr effect originates from the intrinsic Berry curvature of altermagnetism distribution in momentum space, while the Voigt effect arises from an anisotropic permittivity induced by the in-plane Néel order in real space, directly revealing the dual-space nature of altermagnets. Furthermore, the transient Kerr signal exhibits faster relaxation dynamics than the transient Voigt signal, underscoring their distinct origins in Berry curvature and Néel order, respectively. These findings establish transient magneto-optical responses as distinctive fingerprints of altermagnetism and position altermagnets as promising platforms for manipulating magneto-optical phenomena in ultrafast spin optoelectronics.
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All authors Xu Yang, Xingkai Cheng, Zhuo Deng, Yu-Han Gao, Qing-Lin Yang, Zheng Chang, Peng-Tao Yang, Hong-Mei Feng, Xiang-Qun Zhang, Wei He, Junwei Liu, Zhao-Hua Cheng

Friday 22 May

Soft Condensed Matter

Resonances in Overdamped Odd Materials

Odd viscoelasticity arises in parity-violating nonequilibrium materials, where it leads to unconventional mechanical responses and oscillatory relaxation even in overdamped systems. While many living and active chiral materials present promising candidates to exhibit odd viscoelasticity, there is currently no approach that allows for a rheological inference of the large number of elastic and viscous moduli that even a minimal isotropic odd viscoelastic material can depend on. Generalizing the century-old Papkovich-Neuber ansatz to active materials, our work introduces an odd Papkovich-Neuber (OPN) solution – an analytic solution for any isotropic linear odd fluid or solid, each described by up to 6 independent moduli – that enable us to study the boundary-driven response in geometries that mimic common rheology methods. OPN solutions reveal three physically distinct resonances in odd viscoelastic solids that are characteristic of the underlying material moduli and can all be interpreted within a single geometric framework. Underlying this unification is an equivalent description of overdamped odd viscoelastic materials in terms of damped harmonic oscillators. Resonances appear as the effective damping coefficients of these oscillators vanish, which is facilitated by the activity that powers odd material properties.
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Statistical Mechanics

Streaming Molecular Dynamics Simulation Data for On-the-fly Processing and Analysis

Only a small fraction of the data generated in state-of-the-art all-atom multi-microsecond molecular dynamics (MD) simulations is typically analyzed. With femtosecond integration steps, microsecond simulations generate billions of time steps containing atomic positions, velocities, and forces, often corresponding to petabytes of data. Since this exceeds practical storage capacities, only a subset of frames is usually written to trajectory files at intervals of 10-100 ps. While sufficient for ensemble averages and slow dynamics, this approach discards information on fast processes such as molecular vibrations, solvent dynamics, short-lived transition states, and transport phenomena that are directly related to macroscopic properties and experimental observables. Here, we introduce a streaming framework for MD simulations that provides direct access to all data generated during a running simulation. Instead of writing high-frequency output to disk, the framework enables user-defined analysis and processing routines to access simulation data in real time. To achieve this, we extend the Interactive Molecular Dynamics (IMD) protocol and implement an enhanced version, termed IMDv3, in the MD packages GROMACS, NAMD, and LAMMPS. We further introduce the Python package imdclient, which receives IMDv3 data streams and exposes them to external applications. To maximize usability, we add an imdclient-based reader to the MDAnalysis package, enabling streamed simulation data to be analyzed alongside conventional trajectory files. Benchmark results show that streaming can improve performance compared to simulations with high-frequency trajectory output. Example applications include live monitoring of custom variables, evaluation of velocity time-correlation functions with fast fluctuations, and real-time analysis of membrane pore currents.
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All authors Amruthesh Thirumalaiswamy, Lawson J. Woods, Heekun Cho, Hugo MacDermott-Opeskin, Jennifer Clark, Irfan Alibay, Yuxuan Zhuang, Oliver Beckstein, Matthias Heyden

Statistical Mechanics

Resonant interactions in the $\alpha$-FPUT lattice with site-dependent coefficients

The wave turbulence framework has proven to be an effective tool for analyzing certain features of nonlinear energy transfer in one-dimensional nonlinear chains. In this work, we extend this approach to the $\alpha$-FPUT problem when the spring stiffness $\chi$ and the nonlinear coefficient $\alpha$ are site-dependent. Although three-wave interactions are non-resonant for constant coefficients, their spatial modulation gives rise to a non-trivial resonant manifold. In this framework, we derive a new kinetic equation that suggests the possibility of substantially faster thermalization with respect to the constant coefficient case. The new kinetic equation includes also an extra term that can be associated to the Bragg-scattering mechanism, which promotes the isotropization of the wave-action spectral density function. We corroborate these results with direct numerical simulations, confirming the radically faster thermalization pathway in the presence of random coefficients.
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All authors Lorenzo Migliorelli, Giovanni Dematteis, Sergio Chibbaro, Miguel Onorato

Materials Science

ChatMOSP: A Chemistry-Grounded Mobile Agent for Working-State Catalyst Simulations

Catalytic nanoparticles restructure dynamically under reaction conditions, so their working morphology and activity are governed by temperature, pressure, and gas composition. However, converting experimentally specified environments into physically meaningful morphology-performance simulations remains difficult because the translation of reaction conditions into model-specific energetic, kinetic, and execution parameters requires the specialized knowledge in computational catalysis. Here we report ChatMOSP, a chemistry-grounded mobile scientific agent that translates natural-language and voice-expressed catalytic requests into parameter-validated simulations using the Multi-scale Operando Simulation Package. ChatMOSP maps catalyst identity, temperature, pressure, gas composition, and target observables onto multiscale structure reconstruction and kinetic Monte Carlo tasks, retrieves database parameters or constructs missing inputs from an online literature-retrieval workflow, and executes validated MOSP workflows. Using CO oxidation on Pd nanoparticles as an example, we verify the ChatMOSP simulations capture the temperature-induced transition from faceted to rounded morphologies observed by in-situ TEM experiments either by built-in database or from web-retrieved literature information when the parameters are absent. Moreover, we demonstrate the capability of ChatMOSP to perform end-to-end study at mobile devices to simulate a pressure-coverage-morphology-activity feedback cycle for Pt CO oxidation to interpret the oscillatory CO conversion. These results establish ChatMOSP as a physically constrained mobile agent for accessible and interpretable catalyst working-state simulations.
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All authors Sanyang Ye, Rui Qi, Beien Zhu, Yi Gao

Materials Science

The structure of a melt: The case of liquid bismuth

Molecular Dynamics (MD) is performed on supercells of 216 atoms of bismuth, going from 300 K to 573 K in 100 steps and maintaining it in the liquid state, at 573 K, during 500 steps using the Materials Studio (MS) suite of codes. The Pair Distribution Functions (PDFs) and the Plane Angle Distributions (PADs) of the last 1, 10, 25 and 100 steps of the MD have been obtained. Averaging the last 100 steps, as representative of the liquid, Reverse Monte Carlo (RMC) was applied to obtain 4 atomic structures, one for each set of initial random velocities. Then, a detailed structural study of liquid bismuth at 573 K was undertaken; PDFs and PADs are calculated and reported. Two noticeable peaks appear for the PDFs, at 3.25 and 6.55 Å, along with a pseudo peak (shoulder) at 4.6 Å. This shoulder (after the first peak) of the PDFs is found to be related to the third and fourth neighbor peaks of the crystalline Wyckoff structure and also to the diagonal distances in deformed squares in the liquid structure. For completeness J(r)s are also reported. Two prominent peaks in the MS PADs are observed: 53{\deg} and 85{\deg}; and two for the RMC PADs: 58{\deg} and 90{\deg}, suggesting the existence of deformed triangles and squares. Less abundant are higher-order geometrical structures.
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All authors Flor B. Quiroga, Isaías Rodríguez, David Hinojosa, Alexander Valladares, Renela M. Valladares, Ariel A. Valladares

Materials Science

AB2X4 spinel structures: similarity and difference between the centrosymmetric, Fd-3m, and non-centrosymmetric, F4132, space groups

Many compounds belonging to the spinel AB2X4 structure play an important role due to their wide range of practical applications. Most of them are traditionally assigned to the centrosymmetric space group Fd-3m. However, the physical properties of some spinels are incompatible with centrosymmetry. This discrepancy is often accounted for by reducing the symmetry to the non-centrosymmetric space group F-43m, allowing thus small atomic displacements from their original position in Fd-3m. In this work, we demonstrate that the loss of the inversion symmetry can occur without any atomic displacements, since the centrosymmetric Fd-3m and non-centrosymmetric F4132 space groups are equivalent for structure determination and refinement based on X-ray diffraction data. If consistent with experiment, only the use of an anharmonic model of atomic displacements can distinguish these space groups. This study aims to clarify certain misconceptions regarding the structural symmetry and physical properties of spinel type compounds.
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Mesoscale and Nanoscale Physics

Quantized thermal current vortices

The thermal Hall effect has emerged as a fundamental tool for probing exotic quasiparticles and topological order, particularly in magnetic insulators where electronic conduction is suppressed. Much like skyrmions, which are characterized by their topologically protected spin configurations, the thermal Hall effect is deeply rooted in the geometric properties of the underlying physical space. Although the effect is a well-established experimental phenomenon, current research points toward the existence of its quantum analogue: the quantized thermal Hall effect. In this paper, we provide a theoretical framework for this quantum version based on Sommerfeld's flux quantization. Furthermore, we demonstrate the potential existence of dissipationless thermal current vortices. We suggest that these vortices may play a crucial role in the stability and dynamics of other topological structures, such as skyrmion lattices, offering a new perspective on the interplay between heat transport and magnetic textures.
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Strongly Correlated Electrons

Charge density wave in a band insulator

Charge density wave (CDW) implies a periodic modulation of the charge density. Typically observed in metallic systems, CDWs arise from Fermi surface instabilities, resulting in the total or partial gapping of the Fermi surface. Here, we present experimental evidence for a CDW state emerging in a band insulator which has no Fermi surface. The bulk and surface of our material platform, Bi4Br4, is gapped over the entire Brillouin zone. Through topographic and spectroscopic imaging at low temperatures, we unveil an unexpected unidirectional charge modulation in Bi4Br4, breaking the lattice translation symmetry. The CDW develops at temperatures below 40 K and adds an energy gap atop the existing insulating gap of Bi4Br4. Furthermore, our transport measurements reveal nonlinear electrical conduction, a phenomenon conventionally associated with the sliding or phason mode of incommensurate CDWs. These highly unusual observations represent a new type of CDW and demand a new theoretical framework for CDWs.
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All authors Md Shafayat Hossain, Wenhao Liu, Yuqi Zhang, Qi Zhang, Chao Lei, Nana Shumiya, Kouta Dagnino, Maksim Litskevich, Yu-Xiao Jiang, Jia-Xin Yin, Nikhil Dhale, Zi-Jia Cheng, Byunghoon Kim, Yongkai Li, Tyler A. Cochran, Xian P. Yang, Fan Zhang, Yugui Yao, Zhiwei Wang, Bing Lv, Titus Neupert, Luis Balicas, M. Zahid Hasan

Strongly Correlated Electrons

Signature of spin liquid state in a frustrated 3D antiferromagnet

Frustrated pyrochlore lattices in transition-metal oxides provide an ideal platform for realizing exotic quantum states, including spin liquids with unconventional low-energy excitations arising from the macroscopic ground-state degeneracy of corner-sharing tetrahedral networks. Here, we report the synthesis and comprehensive characterization of ZnCrGaO$4$, a frustrated three-dimensional pyrochlore-like magnet in which intrinsic cation ordering gives rise to unavoidable atomic-site disorder. A Curie–Weiss analysis of the high-temperature magnetic susceptibility yields a large negative Curie–Weiss temperature, $\theta{\mathrm{CW}} \approx -205$ K, indicating dominant antiferromagnetic exchange interactions ($J/k_{\mathrm{B}} \sim 55$ K) between Cr$^{3+}$ ($S = 3/2$) moments. Despite the presence of strong antiferromagnetic interactions, no signature of long-range magnetic ordering is observed down to 125 mK, as evidenced by specific-heat and ac-susceptibility measurements. Furthermore, the absence of bifurcation between zero-field-cooled and field-cooled dc magnetic susceptibilities measured at 0.01 T indicates the absence of spin freezing, which is further supported by the frequency-independent ac susceptibility down to 250 mK. The presence of broad maxima in the magnetic specific heat and ac susceptibility at low temperatures suggests the development of short-range spin correlations within a dynamic magnetic state. In addition, the low-temperature specific heat follows a power-law behavior below 1 K, indicating the presence of unconventional low-energy excitations and algebraic spin correlations. These results provide compelling evidence for a dynamic correlated ground state in ZnCrGaO$_4$, establishing it as a promising platform for exploring highly frustrated $S > 1/2$ three-dimensional quantum magnets and potential spin-liquid behavior.
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All authors Satish Kumar, U. Jena, A. Bandhopadhay, G. B. G. Stenning, D. T. Adroja, S. Petit, P. Khuntia

Disordered Systems and Neural Networks

Anderson Localization: A Floquet operator Krylov space perspective

The problem of Anderson localization, as well as the single particle localization-delocalizaton transition of the Aubry-André model, is studied employing operator Krylov space methods. It is shown that even when the dynamics is generated by a Hamiltonian, studying the dynamics at stroboscopic rather than continuous times has its advantages. In particular, mapping the dynamics to an effective Floquet problem results in an operator Krylov space description where quantities such as the spectral function can be computed with fewer computational resources, while a moment method exists that allows for the extraction of Krylov parameters directly from the discrete time autocorrelation function. For stroboscopic dynamics, the operator Krylov space corresponds to the dynamics of an edge operator of an inhomogeneous Floquet transverse field Ising model, with the parameters of this effective model generated recursively. The Krylov parameters show disorder-averaged renormalization with their distribution narrowing as the recursion step increases. It is shown that a more physical spectral function is obtained from the Krylov parameters obtained from the disorder-averaged autocorrelation function, rather than the disorder-averaged Krylov parameters. The delocalized (localized) phase is shown to correspond to the appearance (absence) of a Porter-Thomas distribution, a ballistically propagating (localized) wavefront in operator Krylov space, and a smooth (discrete) Berstein-Szegö power-spectrum. The localization-delocalization transition is also demonstrated in operator Krylov space. A Porter-Thomas distribution is also observed at the critical point. The long-time dynamics and the inverse participation ratio at the critical point is shown to exhibit behavior consistent with a multi-fractal scaling with system size.
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Statistical Mechanics

Theory of supercooled water

We introduce a model of water contemplating true supercooled-liquid states that, as such, are metastable with respect to the crystalline-solid ones. Its numerical solutions reproduce from Speedy-Angell's stability-limit picture to Poole et al.'s metastable liquid–liquid criticality. The real existence of a liquid–liquid critical point is found to gain significant theoretical plausibility from a hitherto unnoticed analogy with the “inversion thermodynamics” of Joule-Thomson gas throttling process and, by extension, with the equivalent phenomenology exhibited by black holes.
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Disordered Systems and Neural Networks · Cross-listed from quant-ph

Dynamical self-dual criticality in Fibonacci-monitored quantum Ising chains

For the quantum phase transition in the transverse-field Ising chain, Kramers-Wannier duality not only protects its critical properties but also pinpoints the location of the phase transition. Its role in out-of-equilibrium, monitored dynamics, however, remains largely unexplored beyond time-periodic Floquet protocols where self-duality turns into a statistical average symmetry. Here we explore the emergence of dynamical self-duality in the absence of time-translation symmetry by investigating the monitored dynamics of one-dimensional Ising/Majorana chains where measurements are arranged in a quasiperiodic Fibonacci sequence. We find that the dynamical extension of this non-invertible symmetry to an out-of-equilibrium setting allows one to organize the dynamical phase diagram of entangled phases, both predicting the transition locations and protecting universal critical behavior. Analytically and numerically, we identify two distinct critical lines, both related to the golden ratio, for Born-rule weak measurements and for random Clifford projective measurements. The latter coincides with the transition of a pure imaginary-time evolution, which can be viewed as a post-selected trajectory. The universality classes of the long-time critical steady states at Fibonacci times are determined, while the transient dynamics between Fibonacci times is deformed by measurements, realizing dynamical measurement-altered quantum criticality in real time.
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All authors Finn Eckstein, Harald Schmid, Quinten Preiss, Simon Trebst, Felix von Oppen, Guo-Yi Zhu

Mesoscale and Nanoscale Physics

Electrostatically stabilized surface flat bands in rhombohedral graphite at zero displacement field

Rhombohedral (ABC-stacked) multilayer graphene hosts interaction-driven phases enabled by surface flat bands at large displacement fields. In thick flakes, however, strong screening suppresses internal electric fields, raising the question of whether a flat-band regime is accessible within the same experimental paradigm. Here, we show that self-consistent, nonlinear electrostatics provides a robust alternative mechanism: even in the absence of a displacement field, a nonuniform near-surface potential flattens the surface-band dispersion and enhances the density of states. In the strong-coupling limit, electrostatics drives the system toward uniform half-filling at each momentum, yielding an asymptotically flat surface band without any gating. At realistic interaction strengths, surface-band flatness is tuned by the proximal gate, with maximal flatness achieved at hole doping when the band is empty. Combining analytic arguments with fully self-consistent calculations in a realistic model, we map the resulting low-field regime and connect to finite $N\!\sim\! 6-15$ layered samples, providing a framework for analyzing the symmetry-broken phases observed in these systems. Our results motivate future experiments in large-$N$ devices and establish a low-field regime for exploring electrostatically induced flat-band physics.
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Mesoscale and Nanoscale Physics

Controlling spin-$\frac 12$ antiferromagnetic interaction strength in nanographene dimers

We demonstrate that the effective spin-exchange coupling $J$ in open-shell nanographene dimers can be precisely tuned via tip-induced dehydrogenation of selected carbon atoms. Using the double ionization potential equation-of-motion coupled-cluster singles and doubles (DIP-EOM-CCSD) method, we accurately compute the singlet-triplet gaps, which correspond directly to the exchange coupling $J$. We show that the position of the dehydrogenated (or hydrogen-passivated) site in triangulene dimers strongly modulates the singlet-triplet splitting, allowing $J$ to be tuned over a wide range - from a few meV to several tens of meV. This strategy provides a simple yet powerful route for designing tailored spin models with alternating or spatially patterned spin-exchange couplings.
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Quantum Gases

Pressure and Size Dependence of Roton Emission and Vortex Creation by Moving Objects in He~II in $T \to 0$ Limit: Generalized Nonlocal Gross-Pitaevskii Model

In the framework of generalized, nonlocal Gross-Pitaevskii (GP) model, we study numerically the pressure- and size-dependent mechanisms of roton emission and vortex nucleation by objects moving in superfluid $^4$He. As far as the authors are aware, this is the first attempt to analyze the pressure dependence of these mechanisms and the associated critical velocities within a single theoretical framework. For each of several pressures in the range from 0 to the solidification pressure of $\approx25$~bar, we chose the parameters of the interatomic interaction potential such that the resulting excitation spectrum for the generalized, nonlocal GP equation approximates fairly accurately the pressure-dependent dispersion curve determined experimentally by Godfrin et al., Phys. Rev. B 103, 104516 (2021). In the two-dimensional approximation, for circular obstacles (disks) moving in quiescent $^4$He, we calculated two critical velocities – one corresponding to the roton emission and the other to the nucleation of quantized vortices – as functions of pressure and the obstacle's size. We also comment briefly on three-dimensional simulations of the roton emission and vortex nucleation by moving spherical obstacles.
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All authors Nicolás Pablo Müller, Ladislav Skrbek, Yuri A. Sergeev, Giorgio Krstulovic

Statistical Mechanics

Universal classification of continuous phase transitions with two order parameters

The continuous phase transition, indicated by the macroscopic order parameter and the occurrence of the spontaneous symmetry breaking, is well illustrated based on the Ginzburg-Landau's paradigm. In systems described by one order parameter, the phase diagram is only composed of the normal phase and the ordered phase. However, in systems with two or more order parameters, much richer phase diagrams and critical phenomena may emerge. According to coupling terms of the free energy, we classify the systems with two order parameters into several categories, featuring different patterns of phase diagrams and critical scalings respectively. Our work propose the new avenue to studying and evaluating the complex systems only based on the coupling terms in expressions of free energy.
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Quantum Gases

Time crystals in cavity-BEC systems

The understanding of light-induced dynamical states continues to be a challenging and fruitful pursuit of science. This pursuit is supported by quantum simulation of dynamical phenomena, e.g., in ultracold atom systems. Typically, ultracold atom dynamics are read out destructively, via time-of-flight imaging, limiting a detailed analysis. However, atom-cavity systems provide a real-time readout of the photonic state via photon emission from the cavity, making the system ideally suited for the simulation of dynamical phenomena. Here, we review three distinct time crystalline states, predicted and realized in a cavity-BEC system. We give an example for each of them, based on minimal few-mode models. We characterize the time crystalline states via correlation functions of the cavity mode, and characteristic momentum modes of the condensate. This supports a clear distinction between these time crystals. More generally, the sequence of studies reviewed here, serves as a blueprint for setting up minimal models and their characterization, for dynamical phenomena.
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Materials Science

Photoluminescent Tetragonal Tb-doped Pb2P2O7

In this study, we report the synthesis and characterization of a novel tetragonal polymorph of Tb-doped Pb2P2O7. Single-crystal X-ray diffraction confirms the stabilization of the P41 and P43 enantiomorphs at room temperature due to the incorporation of Tb3+ ions. Optical investigations reveal green photoluminescence from the characteristic 5D4 -> 7Fj (J = 1-5) transitions of Tb3+, with each emission split due to the crystal field effect, indicating the presence of Tb3+ in multiple coordination environments. The power dependence of the PL intensity follows a linear power-law behavior, suggesting a one-photon excitation process. Temperature-dependent PL measurements show an initial increase in intensity up to 125C, attributed to energy transfer from structural defects, followed by thermal quenching above this temperature. Structural stability at elevated temperatures is confirmed via high-temperature X-ray diffraction (XRD), showing no phase transitions before melting at approximately 800C. These findings highlight the potential of tetragonal Tb-doped Pb2P2O7 as a new class of photoluminescent material.
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All authors Yong Liu, Wenhua Bi, Alla Arakcheeva, Arnaud Magrez

Statistical Mechanics · Cross-listed from quant-ph

Quantum Quenches that Resemble Operator Growth

We study growth quenches, which are local quenches that may gradually destabilize a false vacuum in certain kinetic constrained quantum lattice models, such as the East-West model. We point out a formal analogy with the dynamics of a local operator in the Heisenberg picture. Exploiting this analogy, we obtain several results on growth quenches by adapting operator-dynamics concepts and methods. First, applying the Krylov approach (recursion method), we conjecture the linear growth of Lanzcos coefficients in generic quenches, $a_m \sim \nu m$ (diagonal), and $b_m \sim \alpha m$ (off-diagonal), extending an operator growth hypothesis. We show that the growth quench dynamics is localized in both Krylov and Fock spaces when $|\nu| > 2 \alpha$, and derive a bound for the growth quench analogue of Lyapunov exponent $\lambda_L \le \sqrt{4 \alpha^2 - \nu^2}$ when $|\nu| < 2 \alpha$. Second, we realize the Fock localization in large $N$ solvable growth quenches inspired by Sachdev-Ye-Kitaev (SYK) models. The bound on Lyapunov exponent is saturated in large-$q$ SYK grow quench. By contrast, the growth quench is almost always Fock localized in a nonrandom all-to-all growth quench amenable to semiclassics. Finally, in the 1D East-West model, we interpret Fock space cage states as the existence of a conserved charge. We show that the latter has ballistic transport due to current conservation. Moreover, adding hopping with a fine-tuned amplitude induces a partial localization due to a flat band. Our work suggest growth quenches as a promising approach to realize non-equilibrium coherent phenomena in many-body systems.
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Quantum Gases · Cross-listed from quant-ph

Coherent dynamics in chaotic spin chains via interference-protected subspaces

Generic quantum many-body systems are expected to thermalize, scrambling initial coherence while local observables relax to equilibrium values. Weak ergodicity breaking, often associated with quantum many-body scarring of homogeneous states, provides rare exceptions with long-lived coherence. We introduce a family of local spin-1/2 chains with a structured subspace that hosts a much broader range of nonthermal phenomena, such as scars, chirally propagating quasiparticles or approximate topological edge modes. These nonthermal phenomena happening at high energy densities can be understood via structured subspaces that are protected by destructive interference. We develop a quantitative leakage theory predicting which states retain coherence and suggest ways to improve the stability by inducing fast oscillations in the complement subspace. Our framework connects asymptotic scars, quantum cages, and parent-Hamiltonian constructions, and shows that weak ergodicity breaking in chaotic systems extends well beyond revivals of homogeneous initial states.
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Materials Science

Phase-dependent electronic structure of two-dimensional Ag layers at the graphene/SiC interface

Intercalation at the graphene/SiC interface provides a controlled route to stabilize atomically thin layers with properties distinct from their bulk counterparts. In this platform, the structure and stability of the intercalated phase depend sensitively on the defect landscape of the starting substrate. For intercalated two-dimensional silver at the graphene/SiC interface, two phases have been observed: a phase epitaxial to the SiC lattice, Ag$_{(1)}$, readily obtained following the conventional intercalation method under ultra-high-vacuum conditions and extensively characterized, and a more densely packed phase, called Ag$_{(2)}$, which has remained largely unexplored. Here we report an in situ ultra-high-vacuum preparation method of the second phase intercalated at the graphene/SiC interface; this phase previously was prepared via high-pressure confinement heteroepitaxy. Low-energy electron diffraction shows that Ag$_{(2)}$ is rotated by 30 degree relative to the SiC lattice and forms supercells, in contrast to the $(1\times 1)$ epitaxial relation of Ag$_{(1)}$ with SiC. High-resolution angle-resolved photoemission spectroscopy reveals a more rich Ag$_{(2)}$ band dispersion compared to the Ag$_{(1)}$. In density functional theory calculations, by defining the unfolding entropy which, in a quantified way, finds that the band structure of Ag$_{(2)}$ is more suitable to be unfolded to the SiC primitive cell, and the resulting unfolded band dispersion is in great agreement with the experimental data. We further show that the different intercalated Ag phases tune the electronic properties of the overlying quasi-free-standing graphene layer differently: compared with Ag$_{(1)}$, Ag$_{(2)}$ yields an $\sim$1.75 times higher charge carrier density and modifies the charge-plasmon interaction of the graphene layer, indicating a change in effective screening at the interface.
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All authors Sawani Datta, Boyang Zheng, Arpit Jain, Kathrin Küster, Joshua A. Robinson, Vincent H. Crespi, Ulrich Starke

Quantum Gases · Cross-listed from hep-th

On the Ising/tricritical-Ising interface: From ${W}_3$ symmetry to Rydberg atoms

We consider interfaces between critical spin-chains in different universality classes, described in the continuum limit by defect/interface conformal field theory (DCFT/ICFT). We focus on a conformal interface between the Tricritical Ising (TIM) and the Ising CFT exploring the possibility of its experimental realizations in the context of Rydberg atom arrays. Our analysis emphasizes non-invertible symmetries and consistency under modular transformations, and uses defect couplings and the defect spectrum – including in the case of mixed boundary conditions – to make sharp experimental predictions. The structure of the observables hinges on a newly discovered pattern of emergent ${W}_3$ chiral symmetry for the Tricritical-Ising/Ising interface.
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Superconductivity

Quantum critical collapse of a pinned vortex glass in high-field superconducting resonators

The interplay between disorder and vortex–vortex interactions in strongly disordered superconductors in a magnetic field can stabilize a vortex-glass state, characterized by strong pinning and the absence of positional order. Yet its role in the destruction of superconductivity at the field-driven superconductor–insulator transition has remained unresolved. Here we use plasmonic microwave spectroscopy of superconducting resonators patterned from amorphous indium oxide thin films to directly track the superfluid density up to the critical field $B_c$. We find an unexpected resilience of the superfluid density, which decreases only logarithmically over nearly three orders of magnitude in field, in stark contrast to the rapid power-law suppression expected for vortex lattices. We attribute this anomalously slow decay to a collective vortex-pinning mechanism counterintuitively enhanced by vortex–vortex interactions. The superfluid density then vanishes linearly at $B_c$, where independent magnetoresistance measurements identify a continuous quantum critical point, unlike the abrupt transition observed at zero field. We further uncover an exceptionally large nonlinear electromagnetic response of the vortex glass, manifested as a pronounced positive-Kerr effect with potential for quantum sensing. These results show how disorder controls the critical magnetic field and identify the vortex glass as the key intermediate state governing the magnetic-field-induced superconductor–insulator transition.
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All authors David Perconte, Thibault Charpentier, Nikolaos Koutsopoulos, Kalpajit Roy, Nadjib Benchabane, Xiaoli Peng, Florent Blondelle, Frédéric Gay, Mikhail Feigel'man, Viktor Kabanov, Benjamin Sacépé

Mesoscale and Nanoscale Physics

Orbital Selective Dirac-like States in EuAgAs Revealed by Polarization Dependent ARPES and DFT

Magnetic topological semimetals provide a promising platform for emergent quantum phenomena driven by the interplay between magnetism and relativistic fermions, including anomalous transport effects and tunable topological phases. Here, we investigate the electronic structure and orbital character of EuAgAs, a magnetic topological Dirac semimetal candidate, using density functional theory (DFT) and polarization dependent angle resolved photoemission spectroscopy (ARPES). Fermi surface mapping and constant energy contours measured at 9 eV reveal ring like features that systematically expand with increasing binding energy, consistent with nearly linear low energy Dirac like dispersion. ARPES measurements at different photon energies hint at the presence of a van Hove singularity predicted by DFT calculations. Furthermore, this indicates that the photoemission matrix elements are highly sensitive to the excitation energy, allowing different photon energies to selectively probe distinct orbital characters. Polarization dependent ARPES measurements performed in s- and p-polarized geometries exhibit pronounced variations in spectral intensity, indicating symmetry selective orbital contributions to electronic states. These matrix element driven intensity modulations are well reproduced by DFT calculations. Furthermore, the observed Dirac like states remain nearly unchanged over the temperature range from 9 K to 30 K, suggesting that the magnetic ordering has minimal influence on the electronic structure. Our combined experimental and theoretical results provide detailed insight into the orbital selective electronic structure of EuAgAs and its implications for magnetic topological quantum states.
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All authors Mohit Mudgal, Suman Nandi, Mohamed El Gazzah, Masashi Arita, Shin-ichiro Ideta, Nirmal J. Ghimire, Kenya Shimada, Anup Pradhan Sakhya