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Physics Condensed Matter

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Friday 15 May

Statistical Mechanics

Short-time critical dynamics in the classical cubic dimer model

The classical dimer model on the cubic lattice hosts a columnar ordered phase and a disordered Coulomb phase, separated by a continuous phase transition that lies beyond the conventional Landau-Ginzburg-Wilson paradigm. While its equilibrium critical properties have been extensively studied, the nonequilibrium critical dynamics of this model–particularly in the short-time regime–remains largely unexplored. In this work, we investigate the short-time critical dynamics near the transition using large-scale Monte Carlo simulations. By quenching the system from both ordered and disordered initial states with vanishing initial correlation length, we analyze the scaling behaviors of the order parameter and its time correlation function in the short-time stage. From these scaling behaviors, we accurately determine the critical temperature $T_c = 0.672(1)$ and the static critical exponent $\beta/\nu = 0.581(5)$ according to the scaling theory of the short-time dynamics. These results are in excellent agreement with previous equilibrium studies. Moreover, we extract the dynamic critical exponent $z = 1.92(1)$ and, notably, find a negative critical initial slip exponent $\theta = -1.052(5)$. This unusual negative value contrasts sharply with the positive $\theta$ typically observed in conventional critical dynamics. We attribute this anomalous behavior to the combined effects of the emergent SO(5) symmetry at criticality and the local U(1) gauge constraint (Gauss law), which enforces a conserved diffusive dynamics and enhances fluctuations in the short-time regime. Our results provide the first comprehensive characterization of nonequilibrium short-time criticality in the three-dimensional dimer model, shedding new light on the universal dynamical features of phase transitions beyond the Landau-Ginzburg-Wilson framework.
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Mesoscale and Nanoscale Physics · Cross-listed from physics.optics

Nonlocal Optical Response and Surface Susceptibilities: A Systematic Derivation via Spatial Moment Expansion

We present a systematic theory connecting the nonlocal response kernel of a homogeneous medium to its effective surface susceptibilities for an arbitrary curved interface. Starting from the most general tensorial nonlocal constitutive relation and combining a spatial moment expansion with a distributional thin-layer limit, we show that the full complexity of the interfacial response condenses, at leading order, into a single scalar: the surface susceptibility $\chi^s$, equal for the tangential and normal components of the electric field. These quantities provide a constructive generalization of the Feibelman $d$-parameters to interfaces of arbitrary curvature, and the curvature corrections, proportional to the geometric invariants $H$ (mean curvature) and $K$ (Gaussian curvature), are derived explicitly. The formalism is illustrated on a comprehensive set of analytically tractable cases (planar, spherical, cylindrical, and ellipsoidal interfaces) for several kernel choices (Gaussian, Yukawa, tensorial Lorentz). Generalized Maxwell boundary conditions are established and compared with the classical Fresnel results.
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Superconductivity

Observation of flat-bottom U-shaped energy gap in high-Tc nickelate (La,Pr)3Ni2O7 thin films

The discovery of high transition temperature (high-Tc) superconductivity in Ruddlesden-Popper (R-P) bilayer nickelates under high pressure has stimulated extensive work to understand the underlying mechanism and search for superconductors with higher Tc. The recent realization of superconductivity in R-P bilayer nickelate thin films with onset Tc above 40 K at ambient-pressure enables the use of a wide array of powerful experimental tools to investigate the unconventional high-Tc superconductivity in bilayer nickelates. Here, using ultra-low temperature scanning tunneling microscopy/spectroscopy (STM/S) and electrical transport study, we report the first successful observation of an energy-symmetric, flat-bottom U-shaped gap with zero residual density of states around the Fermi level in the high-Tc nickelate (La,Pr)3Ni2O7 thin film grown on SrLaAlO4 substrate. Before and after STM/S studies, transport measurements on the same sample reveal consistent superconducting behaviors showing zero resistance, with an onset Tc above 40 K and zero resistance Tc above 20 K. The tunneling spectra exhibit highly unconventional temperature evolution, characterized by a rapid filling of the U-shaped energy gap to a V-shaped gap as the temperature increases. Furthermore, the U-shaped energy gap is reduced under a c-axis magnetic field of 14 T. The energy-symmetric U-shaped gap, taken together with its dependence on magnetic field and temperature, is consistent with the behavior of a superconducting gap, suggesting a nodeless gap function at ultra-low temperatures. Our findings shed new lights on the nature of high-Tc superconductivity and provide an encouraging and thought-provoking hint for a local superconductivity with Tc above liquid nitrogen boiling temperature in nickelate superconductors at ambient or zero pressure.
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All authors Zhen Liang, Tianheng Wei, Wei Ren, Haoran Ji, Zheyuan Xie, Yanzhao Liu, Ziqiang Wang, Jian Wang

Statistical Mechanics

A Finite-State Gibbs Construction from a Recognition Cost

On a finite outcome space, the canonical Gibbs distribution is usually obtained by maximizing Shannon entropy at fixed mean of an externally supplied energy functional. This paper studies the finite-state consequences of a ratio-cost construction instead: after adopting the normalized d'Alembert degree-two closure called the Recognition Composition Law (RCL), with unit log-curvature calibration at the reference ratio, the continuous nontrivial positive branch is $J(x)=\tfrac12(x+x^{-1})-1=\cosh(\log x)-1$. Given the induced cost vector $X_\omega=J(r_\omega)$, multinomial counting and convex duality recover the finite-state Gibbs weights and the identity $F_{\mathrm{R}}(q)-F_{\mathrm{R}}(p)=T_{\mathrm{R}}\,D_{\mathrm{KL}}(q\Vert p)$; the entropy-maximization steps are classical once the cost is fixed. New technical content includes a non-asymptotic Stirling bound and soft-shell constrained-type theorems for real-valued costs. A three-state example compares the Gibbs law to squared-log, affinity-as-energy, and Tsallis alternatives at the same cost vector and mean-cost constraint, with sample-size power calculations at fixed RCL ground truth. The framework is conditional on axioms (A1)–(A3) and restricted to finite outcome spaces with strictly positive weights; it does not derive the composition law from a more primitive principle.
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Materials Science · Cross-listed from math-ph

Thermodynamic Invariants of Coupled Channels: A Many-Channel Tolman-Ehrenfest Effect

When multiple thermodynamic channels are coupled, single-channel equilibrium conditions fail. Extending the Tolman–Ehrenfest effect to the entropy manifold, we derive the unique $n$-channel invariant $\zeta_i T_i = C$, where $\zeta_i$ is the holonomy of the Ruppeiner connection. For the granular volume–stress ensemble, Rowe's dilatancy ratio and energy restriction emerge as geometric consequences of the off-diagonal curvature $g_{V\sigma}$, and the 60-year puzzle of state-dependent $K_\mu$ is resolved: the correction $\zeta_V$ reaches $O(1)$ near jamming. The prediction $\zeta_V\chi=\mathrm{const}$ across a shear band is experimentally testable.
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Mesoscale and Nanoscale Physics

Topological property of graphene with triangular array of nanoholes

The nontrivial band topology for graphene with regular arrays of nanoholes with $C_{6v}$ symmetry is investigated theoretically. For the case of $3\sqrt{3} \times 3\sqrt{3}$ triangular array of nanoholes, we find an energy gap at $\Gamma$ point around the Fermi level associated with a band inversion which induces change in parity indices, whereas deep below the Fermi level there are a bunch of valence bands characterized as obstructed atomic limit (OAL) which also accommodate imbalance in parity indices. This band structure renders the gap at the Fermi level topologically trivial and carrying no edge states, while the nontrivial band topology of the OAL manifests in two flat bands in the ribbon structure associated with localized electronic states at ribbon edges. The present results exhibit rich topological behaviors in graphene derivatives waiting for explorations.
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Statistical Mechanics · Cross-listed from physics.chem-ph

Reweighting free energy profiles between universal machine learning interatomic potentials for fast consensus building

Free energy profiles serve as a fundamental bridge between microscopic atomic fluctuations and macroscopic thermodynamic observables. Estimating the free energy profile along a reaction coordinate, referred to as the potential of mean force (PMF), with density functional theory (DFT) accuracy is computationally expensive. Universal machine learning interatomic potentials (MLIPs) drastically reduce this cost, but their accuracy is strongly determined by their training data and hence can be uncertain for a given system. In this work, we present a systematic and scalable framework for reweighting PMFs, initially sampled with a single 'source' MLIP, across a representative suite of target MLIPs. Because traditional direct exponential reweighting fails for large system sizes due to low phase-space overlap between potentials, we deploy robust analytical corrections. Applying this to a complex 601-atom system of Li$^+$ transport in a nanoconfined electrolyte, we demonstrate that a mean energy-gap approximation effectively bypasses statistical collapse, producing a highly stable PMF matching the target PMF. Using this approach, we recover high-fidelity target thermodynamics across multiple DFT reference levels (PBE+D3, PBE-sol, r$^2$SCAN,r$^2$SCAN-D4) at a fraction of the computational cost of full simulations. Furthermore, thermodynamic analysis reveals that the studied MLIPs partition into two distinct clusters driven by their training data. Our reweighting framework successfully recovers target thermodynamic properties–specifically, reaction and activation free energies–even when the phase-space overlap between potentials is critically low. Ultimately, this approach establishes a vital diagnostic protocol to achieve affordable cross-model consensus on materials chemistry properties without redundant, resource-intensive simulations.
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All authors Sauradeep Majumdar, Miguel Steiner, Johannes C. B. Dietschreit, Swagata Roy, Daniel Willimetz, Lukaš Grajciar, Rafael Gómez-Bombarelli

Soft Condensed Matter · Cross-listed from cs.AI

ColPackAgent: Agent-Skill-Guided Hard-Particle Monte Carlo Workflows for Colloidal Packing

We introduce ColPackAgent, an agent framework that autonomously runs Monte Carlo simulations of colloidal packing through a Model Context Protocol (MCP) tool server and an agent skill, whether as a standalone agent or inside an existing agent system. By harnessing the MCP server and agent skill, ColPackAgent executes a structured workflow for colloidal packing simulations, which are central to studies of phase behavior, self-assembly, and materials design. Without dedicated simulation tools and workflow instructions, general-purpose Large Language Model (LLM) agents tend to describe such workflows rather than execute them reliably. The MCP server exposes a custom-built colpack Python package that wraps HOOMD-blue hard-particle Monte Carlo, and the skill encodes a four-stage workflow contract. ColPackAgent can carry out the workflow interactively with human feedback, autonomously from an end-to-end prompt, or as autoresearch following a provided program file. We demonstrate the system in different modes with several colloidal packing simulation examples such as cube particles in 3D, a binary system of disks and capsules in 2D, and the 2D hard-disk freezing transition using autoresearch. We also compare model performance on this workflow across a panel of LLMs with 17 stage-specific prompts. This benchmark provides a stage-level check of how reliably different models follow the setup, planning, and analysis workflow. Together, these results show that pairing a domain Python package with MCP tools and a portable agent skill provides a practical route for turning a simulation toolkit into an agent-assisted research workflow.
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Superconductivity

Non-Relativistic Spin-Orbit Interaction in Triplet Superconductors: Edelstein Effect and Spin Pumping by Electric Fields

Non-relativistic momentum-dependent spin splitting, as observed in collinear altermagnets and non-collinear $p$-wave magnets, provides exciting avenues for controlling spin dynamics. Here, we reveal a distinct form of non-relativistic “spin-orbit coupling" in triplet superconductors by demonstrating that the triplet order parameter induces a wave-vector-dependent spin texture of Bogoliubov quasiparticles, thereby entangling their orbital and spin motions. Even in the absence of relativistic spin-orbit coupling, this intertwining of spin and orbital motion allows an electric field to generate spin polarization in a $p$-wave superconductor – that is, an Edelstein effect. Building on this mechanism, we propose an efficient scheme for the nonlinear generation of a DC spin current via electric near fields, driven by AC spin polarization and electron velocity. This general principle offers a powerful route for generating and manipulating spin currents in unconventional superconductors.
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All authors Ping Li, G. A. Bobkov, I. V. Bobkova, Tao Yu

Materials Science

Local distortions as a source of piezoelectric/stiffness decoupling in B-doped AlScN

We present a first-principles analysis of the wurtzite pseudo-ternary (Al,Sc,B)N to elucidate the structural origin of a decoupling between stiffness $C_{33}$ and piezoelectric response $e_{33}$ upon boron incorporation, using DFT-relaxed 100-atom special quasirandom structures across a broad composition range. Pair distribution function analysis reveals interstitial threefold-coordinated boron atoms that have displaced from the tetrahedral cation site. Direct structural analysis establishes their preferential orientation along the $c$-axis and identifies a scandium-activated creation mechanism. The vertical coordination asymmetry of each cation is quantified through a site-specific axial asymmetry ratio (AAR), showing that boron incorporation progressively symmetrizes the Sc environment. Correlation with Born effective charges demonstrates that this symmetrization is the mechanism behind the piezoelectric enhancement.
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Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

Interface Piezoelectric Loss in Superconducting Qubits

Dissipation remains a central obstacle to improving superconducting quantum circuits, yet the microscopic origins of loss in widely used materials platforms are not fully understood. Here, we report the observation of interface piezoelectricity-induced dissipation in superconducting qubits fabricated on high-resistivity silicon. Our devices use a transmon qubit with a shunt capacitor that simultaneously serves as an interdigital transducer embedded in a surface acoustic wave resonator. By tuning the qubit transition into resonance with discrete mechanical modes, we observe up to a factor-of-two reduction in qubit lifetime, consistent with energy exchange between the qubit and mechanical modes mediated by piezoelectric coupling at the aluminum-silicon interface. Our findings provide direct evidence for interface piezoelectricity as a distinct loss channel in superconducting qubits. Combined with multiphysics simulations, these findings suggest that interface piezoelectric loss can dominate over loss from two-level systems at sufficiently high frequencies.
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All authors Haoxin Zhou, Kangdi Yu, Yashwanth Balaji, Sanjit Shirol, Leo Sementilli, Zi-Huai Zhang, Adam Schwartzberg, Alp Sipahigil

Materials Science

p-Wave Orbital Angular Momentum Texture in a Chiral Crystal

The spin and orbital angular momentum (SAM and OAM) are conceptually analogous, yet their roles in condensed matter systems have not been often treated on equal footing. While SAM has been extensively explored, OAM has long been regarded as quenched in crystalline environments and thus largely overlooked. Recent experimental and theoretical advances, however, have demonstrated that OAM can drive a variety of novel electronic phenomena, highlighting the importance of probing OAM textures in the electronic band structure. Here, we investigate the momentum-space OAM texture of (TaSe4)2I, a one-dimensional chiral crystal. Using circular-dichroism angle-resolved photoemission spectroscopy (CD-ARPES), we uncover a p-wave OAM texture accompanied by OAM dipole structures. This orbital p-wave texture is intimately connected to, and thus controllable by the chirality of the host lattice. Complementary spin-resolved ARPES measurements and first-principles calculations reveal that the OAM polarization overwhelmingly dominates the low-energy electronic properties of (TaSe4)2I, far exceeding the SAM polarization. These observations represent the experimental verification of a new type of OAM texture in crystalline materials. Most importantly, these findings underscore a promising material platform for spinless orbitronics applications and lay the foundation for realizing multipolar OAM textures-orbital counterparts of the spin texture in unconventional magnets.
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All authors Dongjin Oh, Chiara Pacella, Xiangyu Luo, Chris Jozwiak, Aaron Bostwick, Eli Rotenberg, Mats Leandersson, Craig Polley, Angel Rubio, Domenico Di Sante, Riccardo Comin

Mesoscale and Nanoscale Physics

Quantum Geometry-Driven Nonlinear Spin Currents in Floquet Non-Hermitian Altermagnets

Altermagnets are rapidly emerging as a highly promising platform for spintronics, yet dynamically controlling their spin responses remains a fundamental challenge. In this work, we demonstrate that introducing periodic optical driving and non-Hermiticity provides a powerful route to achieve tunable control over these systems. We derive a general analytical expression for nonlinear spin currents in non-Hermitian phases with a spectral line gap, revealing that the intrinsic response cleanly separates into quantum metric, Berry curvature, and Berry connection dipole contributions. Applying this formalism to a Floquet non-Hermitian $d$-wave altermagnet, we uncover that the nonlinear spin conductivity is overwhelmingly dominated by the bare quantum metric. Furthermore, we show that the optical field's polarization can actively tune – and even strictly reverse – the direction of both longitudinal and transverse spin currents. Our work establishes a quantum geometric framework for the optical manipulation of nonlinear spin transport in advanced magnetic materials.
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Mesoscale and Nanoscale Physics

Entropy Production from Spin–Vibrational Coupling in Endohedral-Fullerene Qubits Encapsulated in Suspended Carbon Nanotubes

Hybrid carbon nanotube-fullerene architectures provide a controllable platform for studying irreversibility and information flow in structured quantum environments. We analyze entropy generation in a system where paramagnetic endohedral fullerenes, such as N@C$_{60}$ and P@C$_{60}$, are encapsulated inside a suspended carbon nanotube (CNT) resonator, with selected multi-level fullerene spin states forming an effective qubit coupled to quantized CNT flexural modes. Building on prior work on fullerene-filled CNTs, spin-phonon control in suspended nanotubes, and phase-space propagators for damped driven oscillators, we develop a hybrid open-system model combining driven quantum Brownian motion of the CNT with an effective Jaynes-Cummings spin-vibrational interaction. The resonator dynamics are represented by a Wigner function whose evolution is written analytically in terms of the initial Wigner distribution and a Gaussian propagator. This phase-space description separates drive-induced displacement, diffusion, and damping, and connects these processes directly to entropy flow. The coupled spin-mechanical dynamics are embedded in a Lindblad master equation including mechanical damping, spin relaxation, pure dephasing, and thermally activated excitation. Within this framework we derive the entropy balance, identify entropy flux and non-negative entropy production, and examine how spin-vibrational hybridization redistributes irreversibility between coherent exchange and dissipative channels. We show that magnetic-gradient-enhanced spin-phonon coupling, resonant driving, and moderate thermal occupation produce crossovers between oscillator-dominated and spin-dominated entropy-production regimes. The framework provides a basis for using CNT-PEF hybrids as nanoscale platforms to study nonequilibrium quantum thermodynamics, decoherence, and information loss in vibrational environments.
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Strongly Correlated Electrons

Itinerant antiferromagnetism in the antagonistic pair compound Y$_4$Co$_3$Ag

Low dimensional crystallographic motifs have long been associated with desirable physical properties. The confinement of electrons to low dimensions is thought to enhance quantum fluctuations and may promote correlated phenomena. Here, using the antagonistic pair concept, we add Y to the immiscible Co-Ag pair to discover Y$_4$Co$_3$Ag. This compound adopts a monoclinic $I$2/$m$ structure consisting of Y channels that are filled by one-dimensional zigzag and hexagonal Co chains, which extend along the crystallographic $b$-axis with no nearest neighbor contacts between Co and Ag atoms. Transport, magnetic, and specific heat measurements reveal that Y$_4$Co$_3$Ag orders antiferromagnetically at $T_N=14.9$ K with an effective magnetic moment $\mu_{\text{eff}}$ = 1.4 $\mu_{\text{B}}$/Co. Specific heat measurements show only a small entropy loss on the order of $0.1\,R\ln2$ associated with magnetic order, and magnetization isotherms, in DC fields up to 70 kOe at 1.8 K and in pulsed fields up to 600 kOe at 500 mK, indicate a small ordered moment of less than 0.2 $\mu_B$/Co. Taken together, our results imply the presence of small, itinerant moments and strong fluctuations in Y$_4$Co$_3$Ag, suggesting that Y$_4$Co$_3$Ag may be a promising candidate material to investigate itinerant magnetic interactions in a quasi-one dimensional system.
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All authors Rafaela F. S. Penacchio, Nao Furukawa, Joanna M. Blawat, John Singleton, Zhouqi Li, Raquel A. Ribeiro, Sérgio L. Morelhão, Sergey L. Bud'ko, Paul C. Canfield, Tyler J. Slade

Thursday 14 May

Statistical Mechanics

Thermodynamic and statistical properties of a multifractional modified dispersion relation via the grand-canonical ensemble

We study the thermodynamic and statistical properties of a gas governed by a multifractional modified dispersion relation of the form $\omega^{2}=k^{2}+4E_{*}^{-1/2}k^{5/2}$, where $E_{*}$ sets the characteristic scale of the multifractional correction. Working within the grand-canonical ensemble, we derive the modified density of states, the grand potential, the partition function, and the main thermodynamic quantities for both bosonic and fermionic sectors. The deformation changes the available phase-space distribution and produces nonstandard thermal scalings controlled by the ratio $T/E_{*}$. In the infrared regime, the usual relativistic gas behavior is recovered with leading corrections proportional to powers of $(T/E_{*})^{1/2}$. In the ultraviolet regime, the density of states scales as $\varrho(\omega)\propto \omega^{7/5}$, corresponding to an effective density-of-states dimension $d_{\mathrm{eff}}=12/5$. As a consequence, the Stefan-Boltzmann law is deformed from $u\propto T^{4}$ to $u\propto E_{*}^{3/5}T^{17/5}$, while the equation-of-state parameter approaches $w=5/12$ instead of the standard radiation value $w=1/3$. We also analyze thermal stability, particle number and energy fluctuations, Bose-Einstein condensation, and the degenerate Fermi gas limit. The multifractional correction increases the critical temperature of a conserved bosonic gas and modifies the Fermi energy, pressure, sound speed, and low-temperature heat capacity of degenerate fermions. A direct fit to the COBE/FIRAS monopole spectrum yields $E_{*}>0.36\,\mathrm{MeV}$ at $95\%$ CL, while the conservative GWTC–3 propagation constraint gives $E_{*}>1.18\times10^{19}\,\mathrm{GeV}$ at $90\%$ credibility when the dispersion relation is assumed to be universal.
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Mesoscale and Nanoscale Physics

Multifractal and Ergodic Properties of Conductance Fluctuations under Strong Disorder

Understanding the stochastic properties of conductance fluctuations in disordered mesoscopic systems is fundamental to quantum transport. In this work, we investigate the multifractal and ergodic properties of the fictitious time series of conductance in two-dimensional tight-binding models under varying Anderson disorder. Using standard multifractal analysis, we show that conductance fluctuations exhibit a transition from non-ergodic to ergodic behavior as the disorder strength increases, as evidenced by the decay of the conductance correlation function. Remarkably, multifractality persists in both regimes; however, it becomes insensitive to shuffling in the strong-disorder (ergodic) regime, suggesting that distributional effects dominate temporal organization. On the contrary, in the weakly disordered (non-ergodic) regime, long-range correlations play a significant role. These findings are robust against changes in lead geometry (asymmetric vs. symmetric). Our results provide new insights into the interplay between ergodicity, multifractality, and rare events in disordered quantum transport.
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All authors Marcos A. A. de Sousa, Heitor R. Publio, Henrique A. de Lima, Adauto J. F. de Souza, Fernando A. Oliveira, Anderson L. R. Barbosa

Statistical Mechanics

Fractal signatures of strong universality in the disordered Ising model

Disordered systems are very rich laboratories for exploring complex systems. In particular, disordered magnetic systems have been extremely important in the last five decades for understanding a wide range of phenomena. In this work, we use the Edwards-Anderson Hamiltonian to obtain the thermodynamic properties of disordered magnetic systems. In this way, we conduct a systematic investigation of magnetization, correlation functions, order parameter, and fractal dimensions, in function of disorder. In this context, the autocorrelation function for order–parameter fluctuations, introduced by Fisher ( Journal of Mathematical Physics 5, 944322 (1964)), provides an important mathematical framework for understanding the second-order phase transition at equilibrium. However, his analysis is restricted to a Euclidean space of dimension $d$, and an exponent $\eta$ is introduced to correct the spatial behavior of the correlation function at $T=T_c$. In recent work, Lima et al ( Phys. Rev. E 110, L062107 (2024)) demonstrated that at $T_c$ a fractal analysis is necessary for a complete description of the correlation function. We use Monte Carlo simulations to validate analytical results and to show how disorder alters critical exponents , giving rise to different universality classes. On the other hand, there is a subgroup of critical exponents and fractal dimensions that are invariant with disorder. This subgroup heralds a strong universality class.
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All authors Henrique A Lima, Kaue Hermann, Ismael S. S. Carrasco, Jairo R. L. de Almeida, Fernando A. Oliveira

Mesoscale and Nanoscale Physics

Radio-frequency reflectometry in silicon carbide large-area transistors

Radio-frequency (RF) reflectometry is widely used for high-bandwidth readout of semiconductor quantum devices at cryogenic temperatures, but its application has mainly been limited to nanoscale structures with relatively small capacitances. Here, we investigate RF readout in a different regime by applying gate-based reflectometry to a large-area silicon carbide transistor with parasitic capacitances orders of magnitude larger than those of typical quantum devices, conditions normally expected to hinder RF readout. We observe a gate-dependent RF response which degrades and eventually vanishes as temperature is lowered, although MOSFET operation in DC transport is maintained down to deep cryogenic temperatures. We attribute this behaviour to impedance changes introduced by carrier freeze-out in the transistor drift region, and propose a modified circuit configuration designed to restore sensitivity under these conditions. These results establish how parasitic pathways and device geometry can limit RF readout, providing insight into the design of scalable cryogenic-CMOS quantum systems.
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All authors Alexander Zotov, Conor McGeough, Megan Powell, Alessandro Rossi

Materials Science

Reversible nanoscale patterning of WTe$_2$ with a scanning tunneling microscope

Manipulating the lattice structure of ferroelectric quantum materials enables their use in low-power electronic devices, including field-effect transistors. WTe$_2$ is a Weyl-semimetal candidate and ferroelectric, both properties arising from the reduced crystal symmetry of its T$_\mathrm{d}$ ground state. The T$_\mathrm{d}$ crystal phase results from a Peierls distortion of the 1T parent structure and an interlayer shift. While experiments in WTe$_2$ have established ferroelectric switching and transient control of the predicted topological phase via ultrafast excitations, persistent electronic changes on the nanometer scale remain elusive. Here, we demonstrate that current pulses applied via scanning tunneling microscopy can both write and erase persistent nanometer-scale patterns on the surface of WTe$_2$. These patterns consist of apparent picometer in-plane and out-of-plane atomic displacements, accompanied by changes to the local density of states. The out-of-plane displacements further modulate the Peierls-like distortion present in WTe$_2$, while the in-plane displacements are indicative of ferroelectric switching. The induced patterns can be repositioned and erased, suggesting a nanoscale handle on the ferroelectric properties of WTe$_2$.
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All authors Kevin Hauser, Danyang Liu, Berk Zengin, Jens Oppliger, Samuel Mañas-Valero, Catherine Witteveen, Fabian O. von Rohr, Jennifer E. Hoffman, Fabian D. Natterer

Materials Science

Chemical Origins of Non-Bonded Interactions Within and Between Solids

Non-bonded interactions govern structure, stability, and function across a wide range of solid-state materials, yet their chemical origins are often difficult to resolve from total energies alone. Here we generalize absolutely localized molecular orbital energy decomposition analysis to quantify and interpret non-bonded interactions within and between solids at the density functional theory level. Across molecular crystals, moiré heterobilayers, and layered perovskite heterostructures, this framework separates lattice-formation energies, interlayer binding energies, and band-structure changes into chemically intuitive contributions from frozen interactions, polarization, and charge transfer. The analysis reveals how dispersion controls polymorph stability in pharmaceutical crystals, how local stacking modulates interlayer coupling in MoS2/WSe2, and how alkali-cation substitution switches the quantum-well character of layered perovskite heterostructures. By connecting emergent solid-state properties to microscopic interaction mechanisms, this framework provides a chemically transparent basis for understanding and designing complex materials.
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All authors Paul J. Robinson, Adam Rettig, Hieu Q. Dinh, Anton Z. Ni, Joonho Lee

Materials Science

Disorder-driven symmetry suppression by van der Waals planar defects in a magnetic topological insulator

Magnetic topological insulators offer a platform to control electronic topology through magnetic order, yet reliable routes to tune their properties remain limited. Here, we show that ion irradiation allows to modify the magnetic properties and the anomalous Hall response of the van der Waals magnetic topological insulator MnBi$_2$Te$_4$. Using noble gas ion beams, intrinsic defects are introduced via collision cascades without chemical doping. We identify two distinct regimes. At low fluence, cation antisite disorder leads to a near-complete redistribution of Bi over cation sites while preserving long-range crystallographic order, accompanied by a transition from $p$-type to $n$-type transport. At high fluence, cation-anion intermixing drives the formation of a previously unreported layer-disordered phase characterized by a high density of van der Waals-specific planar defects, including swapped bilayers. Despite significant structural disorder, the system retains partial periodic order up to high displacement levels. Magnetometry and X-ray spectroscopy show that the Mn high-spin state and intralayer antiferromagnetic interactions likely persist, while macroscopic magnetic anisotropy is strongly reduced. At the same time, the magnitude of the anomalous Hall conductivity is reduced by an order of magnitude, far exceeding the change in magnetization, and its sign is modified. The observations are consistent with a suppression of the Berry curvature of the occupied states. These results establish ion irradiation as a means to tune anomalous Hall conductivity in topological insulators through defect engineering and reveal a disorder-driven approach to control symmetry and electronic structure in van der Waals magnetic materials.
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All authors Rikkie Joris, Heyi Xia, Ana Beatriz Pedro Fontes, Sara Bey, Seul-Ki Bac, Jiaqi Zhou, Zviadi Zarkua, Ahmed Samir Lotfy, Muhammad Saad, Philippe Ohresser, Bence G. Márkus, László Forró, Margriet van Bael, Clement Merckling, Xinyu Liu, Francisco Molina-Lopez, Jean-Christophe Charlier, Jin Won Seo, Badih A. Assaf, Lino M. C. Pereira

Other Condensed Matter

Zitterbewegung velocity in semiclassical electron dynamics

Zitterbewegung plays a major role in electron dynamics in solids, yet is not captured in conventional semiclassical treatments. Here, starting from the quantum Liouville equation, I identify a new Zitterbewegung velocity, which involves the symmetric and antisymmetric components of the quantum geometric tensor oscillating out of phase. The Zitterbewegung velocity resolves the position-shift paradox, recovering the field-induced shift in an electron's position by integrating the semiclassical equations, and is directly related to the famous minimum conductivity of massless Dirac fermions.
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Disordered Systems and Neural Networks

Stochastic Safety Limits and Scale-Dependent Power Fluctuations in Nuclear Reactors: A Critical Scaling Approach

Applying boundary functionals of random risk processes to various physical problems makes it possible to determine many important characteristics of these problems. For example, a special case of boundary functionals is the time to first reach a level, which is widely and successfully applied to a variety of problems. We consider the application of boundary functionals to solving nuclear safety problems. In situations such as reactor startup, as well as for certain types of reactors, neutron behavior changes. Neutron clustering begins to play an important role, and the distributions characterizing neutron behavior change. The normal Gaussian distribution is replaced by stable limiting, distributions to which the sums of random variables converge. Boundary functionals allow us to accurately calculate the statistics of random events, determine the behavior of reactor power peaks, the probabilities of catastrophic power surges, and other quantities important for reactor safety, providing a mathematical bridge between the abstract theory of directed percolation and engineering calculations of protection parameters. This article examines the first-passage time to reach a certain level.
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Strongly Correlated Electrons

Unveiling Magnetic Frustration via the Elastocaloric Effect

Motivated by experimental progress in pressure and strain tuning of quantum materials, we examine the thermodynamic response of frustrated magnets to uniaxial strain. Specifically, we study Ising and Heisenberg models on spatially anisotropic triangular (and, for the Ising model, also kagome) lattices. We determine the entropy as a function of temperature and strain, and use it to compute the elastic Grüneisen ratio $\eta$. The Ising models can be strain-tuned into and out of classical spin-liquid phases, and we show that $\eta$ can become arbitrarily large at low temperature $T$ near the point of maximal frustration, a universal hallmark of an extensive ground-state entropy. In contrast, the spin-$1/2$ Heisenberg model is moderately frustrated and displays multiple $T=0$ phase transitions. These transitions dominate $\eta$ at low $T$ while the intermediate-$T$ behavior is similar to that of the Ising model. We discuss the extent to which the elastic Grüneisen ratio can be used to deduce the phase diagram, and we connect our results to recent experiments on triangular-lattice magnets.
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Statistical Mechanics · Cross-listed from quant-ph

Mixed-State Long-Range Entanglement from Dimensional Constraints

We present a new mechanism for long-range entanglement (LRE) in strongly symmetric many-body mixed states that does not rely on symmetry anomalies or long-range correlations. Our primary example is the maximally mixed state in the translation-invariant subspace on a one-dimensional ring. This state is LRE because translationally symmetric short-range entangled states span a subspace whose dimension grows only polynomially with system size, whereas the full translation-invariant subspace grows exponentially. We further discuss certain unconventional properties of this state, including logarithmically growing conditional mutual information, strong-to-weak spontaneous symmetry-breaking, and Rényi-index-dependent operator-space entanglement. We also construct a geometrically non-local Lindbladian to stabilize this state as the steady state. Our results identify dimensional mismatch as a novel route to LRE that is intrinsic to many-body mixed states.
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Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

Translation symmetry-enforced long-range entanglement in mixed states

We show by a counting argument that even though translation symmetry admits symmetric short-range entangled (SRE) eigenstates, there are not enough such SRE eigenstates to span the zero momentum sector. This means that the fixed point strong-to-weak spontaneous symmetry breaking state of translation symmetry is long-range entangled: it cannot be written as a mixture of SRE states. This is a subtle form of long-range entanglement in mixed states that cannot be detected by long-range connected correlation functions.
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Strongly Correlated Electrons

Non-Invertible Symmetries on Tensor-Product Hilbert Spaces and Quantum Cellular Automata

We investigate realizations of (1+1)-dimensional fusion category symmetries on tensor-product Hilbert spaces, allowing for mixing with quantum cellular automata (QCAs). It was argued recently that any such realizable symmetry must be weakly integral. We develop a systematic analysis of QCA-refined realizations of fusion categories and prove two statements. First, we show that, under certain physical assumptions on defects, any QCA-refined realization has QCA and symmetry-operator indices determined by the categorical data, up to the freedom of redefining the symmetry operators. Second, we construct a lattice model that provides a QCA-refined realization for any weakly integral fusion category symmetry on a tensor product Hilbert space. We also compute indices of the QCAs in our lattice model and show agreement with the first result. As an application of the general construction, we give an explicit QCA-refined realization of general Tambara-Yamagami categorical symmetries.
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Soft Condensed Matter

From Coffee Rings to Self-Driven Assembly: Active Matter Enabled Design of Drying Droplets

Evaporating colloidal droplets have long been used as model systems to understand capillarity, interfacial transport, and particle assembly, most prominently through the coffee ring effect. In classical descriptions, suspended particles are treated as passive tracers carried by evaporation-driven capillary flow, with additional influence from Marangoni stresses, wettability, and contact line pinning. More recent studies, however, show that this picture changes significantly when the particles themselves are active. Systems containing motile microorganisms, chemically active colloids, or externally driven particles can continuously inject energy or generate gradients within the droplet, leading to self-driven flows, modified interfacial stresses, and dynamic contact line behavior. In this Perspective, we bring together these developments, identify the key mechanisms governing active droplets, highlight the role of bubble-mediated flows, and outline strategies for controlled deposition and functional interface design.
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Statistical Mechanics · Cross-listed from quant-ph

Universal quantum resource distillation via composite generalised quantum Stein's lemma

The performance of quantum resource manipulation protocols, including key examples such as distillation of quantum entanglement, is measured in terms of the rate at which desired target states can be produced from a given noisy state. However, to achieve optimal rates, known protocols require precise tailoring to the quantum state in question, demanding a perfect knowledge of the input and allowing no errors in its preparation. Here we show that distillation of quantum resources in the framework of resource non-generating operations can be performed universally: optimal rates of distillation can be achieved with no knowledge of the input state whatsoever, certifying the robustness of quantum resource distillation. The findings apply in particular to the purification of quantum entanglement under non-entangling maps, where the optimal rates are governed by the regularised relative entropy of entanglement. Our result relies on an extension of the generalised quantum Stein's lemma in quantum hypothesis testing to a composite setting where the null hypothesis is no longer a fixed quantum state, but is rather composed of i.i.d. copies of an unknown state. The solution of this asymptotic problem is made possible through new developments in one-shot quantum information and a refinement of the blurring technique from [Lami, arXiv:2408.06410].
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