Materials Science
Altermagnetism and Room-Temperature Metal-to-Insulator Transition in CsCr$_2$S$_2$O
Yi Liu, Chen-Chao Xu, Jin-Ke Bao et al. (+14 more)
Metal-to-
insulator transitions (MITs), particularly near room temperature, have been extensively studied in nonmagnetic and conventional
ferromagnetic and
antiferromagnetic systems, yet the co-emergence of MIT and altermagnetism (AM) remains unexplored. Here, a layered chromium-based compound CsCr$_2$S$_2$O that realizes this coexistence was synthesized. It crystalizes in CeCr$_2$Si$_2$C-type structure with Cr moments orders in a C-type
antiferromagnetic configuration below $T_\mathrm{N}$ = 326 K, constituting a room-temperature d-wave altermagnet. In the altermagnetic state, a subsequent Verwey-type MIT appears at $T_\mathrm{MI}$ = 305 K, driven by a tetragonal-to-orthorhombic structural distortion and stripe charge ordering of Cr$^{+2}$/Cr$^{+3}$ ions, while maintaining its altermagnetic character. First-principles calculations show moment-dependent
spin-split electronic structures with maximum splitting energies of ~0.6 eV and ~0.3 eV in the metallic and insulating states, respectively. Our work links the two prominent phenomena, MIT and AM, in a single material, establishing a new platform for potential spintronic applications.
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All authors Yi Liu, Chen-Chao Xu, Jin-Ke Bao, Bai-Jiang Lv, Hao Li, Jing Li, Yi-Qiang Lin, Hua-Xun Li, Yi-Ming Lu, Xin-Yu Zhao, Wu-Zhang Yang, Zhen-Yi Zhang, Xian-Yan Chen, Wen-he Jiao, Ji-Yong Liu, Bai-Ren Zhu, Guang-Han Cao
Soft Condensed Matter
Dynamical mean-field theory of active, self-interacting heteropolymers
Andriy Goychuk
Analytical theories of
polymer dynamics typically focus on the linear response around some steady state obtained via perturbative calculations. The present study derives a dynamical, nonlinear mean-field theory that yields unified access to the
evolution of conformations, contact probabilities, and fluctuations of active
polymers within a single analytical framework. As in previous mean-field descriptions of passive
polymers, the object of interest is the two-point correlator, which is the lowest-order relevant observable in the general Langevin equation of a
polymer. In contrast, the present focus is on active
polymers driven by heterogeneous monomer-level kicks and spatially correlated active flows, while allowing nonreciprocal couplings, in the presence of hydrodynamic and contact interactions. Using a Gaussian closure to truncate higher-order correlations leads to a self-consistent
diffusion equation for the chain correlations. In some cases, this can be further simplified to the dynamics of pairwise squared separations in closed form. In the continuum limit, the theory reveals useful analogies to similar mean-field approximations for reaction-
diffusion systems, as well as fractional
diffusion in different scale-free regimes. Deriving asymptotic solutions in different parameter regimes of the continuum limit recovers the scalings of coiled, globular, and self-avoiding
polymers, thus validating the theory. Applied to hydrodynamically coupled active
polymers, such as chromatin, the framework predicts a sequence of crossover scalings between coiled, swollen, and hyper-compacted fractal states.
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Strongly Correlated Electrons · Cross-listed from hep-lat
Taste-splitting mass and edge modes in $3+1$ D staggered fermions
Tatsuhiro Misumi, Tetsuya Onogi and Tatsuya Yamaoka
We investigate the
symmetry structure of the $3+1$ D staggered
fermion Hamiltonian and its implications for anomalies. Since the
spin and
flavor degrees of freedom of Dirac
fermions are distributed over the
lattice, in addition to the standard on-site mass term, the staggered
fermion system also admits one-, two-, and three-link bilinear terms within a unit cube as local, charge conserving mass terms with different
spin and
flavor dependence. We identify the
spin flavor structures of all those bilinear mass terms and determine the
symmetries preserved by each of them. Among them, one of the one-link mass terms preserves a larger residual
symmetry associated with conserved charges that generate the Onsager
algebra. Motivated by this structure, we consider a kink profile of the one-link mass and analyze the resulting domain-wall system. In the low-energy limit, the $3+1$ D bulk becomes gapped, while two-
flavor massless Dirac
fermions appear as localized modes on the $2+1$ D domain wall. We show that the bulk conserved charges act on the wall as generators of a
flavor $\mathrm{SU}(2)$
symmetry, and that no symmetric mass gap is allowed for the boundary theory when this $\mathrm{SU}(2)$
symmetry and space reflection
symmetry are both imposed. This realizes the parity anomaly of the boundary theory and shows that the boundary
flavor symmetry and anomaly descend from the ultraviolet staggered-
fermion Hamiltonian rather than emerging only in the infrared.
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Quantum Gases · Cross-listed from gr-qc
Emergence of volume-law scaling for entanglement negativity from the Hawking radiation of analogue black holes
S. Mahesh Chandran and Uwe R. Fischer
The
quantum information content of Hawking radiation holds the key to understanding black-hole evaporation and the fate of unitarity. Motivated by recent advances in cold-atom experiments, we develop a
lattice-regularization approach aimed at simulating the coarse-grained
entanglement scaling of a
quantum field in a 1+1D analogue black-hole background. We provide the first concrete demonstration that logarithmic negativity – an
entanglement monotone that typically exhibits a UV-divergent log-scaling for the conformal
vacuum – acquires a UV-finite volume term from the nonlocal correlations seeded by Hawking radiation. We show that this volume term encodes the number density as well as the spatial distribution of entangled Hawking pairs along the black-hole interior and exterior. We highlight its prospective detection in currently realizable experiments and its implications beyond the analogue paradigm, in particular for black-hole thermodynamics.
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Mesoscale and Nanoscale Physics
Optimal skyrmion stability in antisymmetric ultrathin ferromagnetic bilayers
Anne Bernand-Mantel, Valeriy V. Slastikov and Cyrill B. Muratov
We demonstrate the stray-field-mediated skyrmion stabilizing capabilities of ultrathin exchange-decoupled antisymmetric
ferromagnetic bilayers based on conventional transition metal materials. Using an asymptotically exact micromagnetic model valid in the ultrathin film limit, we show that the antisymmetric tailoring of the
bilayer allows the Dzyaloshinskii-Moriya interaction and the dipolar interaction to act synergistically to stabilize skyrmions, in contrast to the monolayer case, in which these energies compete. To obtain optimal stability of these skyrmions against collapse and bursting – the two fundamental processes determining skyrmion lifetime, we carry out an asymptotic analysis of the saddle point solution that separates the skyrmion from the demagnetized state. The result is an optimal stability line for compact skyrmions in the non-dimensional parameter space of the effective Dzyaloshinskii-Moriya interaction strength and the effective film thickness. Our predictions are confirmed by extensive micromagnetic simulations of antisymmetric
bilayers, using
magnetic parameters of the conventional Pt/Co/AlO$_x$ systems. Our results provide a new pathway for experimental observations of 10 nm radius zero-field skyrmions with lifetimes compatible with information technology applications.
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Statistical Mechanics · Cross-listed from physics.soc-ph
Collective attention under digital exposure: A dynamical systems approach
Nuno Crokidakis
The widespread use of digital devices has raised growing concerns about its impact on sustained
attention at the population level. In this work, we propose a minimal dynamical framework to describe the collective
evolution of
attention under continuous exposure to screen-mediated environments. We introduce a macroscopic variable representing the population-level sustained
attention and model its dynamics as the result of competing mechanisms: intrinsic cognitive recovery and degradation induced by digital stimulation. The digital environment is treated as an external control parameter that continuously perturbs the system, leading to a relaxational dynamics. The proposed mechanisms are consistent with empirical findings on attentional dynamics under digital exposure. We first analyze a linear formulation, which provides an analytically tractable baseline, and then extend the model by incorporating a nonlinear degradation term that captures amplification effects under high-intensity stimulation. We derive an explicit expression for the stationary state and show that the
equilibrium attention level decreases monotonically with increasing exposure. An effective potential formulation is introduced, revealing that digital overstimulation progressively deforms the dynamical landscape, shifting the stable state toward regimes of reduced
attention without generating multiple
equilibria. Importantly, the model does not rely on social contagion or interaction-driven bistability, but instead describes a continuous displacement of the collective cognitive regime under environmental pressure. Our results suggest that the impact of digital technologies on
attention may be understood as a gradual macroscopic effect emerging from persistent external stimulation, rather than as a transition between competing behavioral states.
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Disordered Systems and Neural Networks · Cross-listed from q-bio.NC
Thermodynamic connectivity reveals functional specialization and multiplex organization of extrasynaptic signaling
Giridhar Sunil, Habib Benali and Elkaïoum M. Moutuou
Neural communication operates on both fast synaptic transmission and slower, diffusive extrasynaptic signaling, yet how these two modes jointly organize
brain function remains unclear. Here, using the complete synaptic and neuropeptidergic connectomes of Caenorhabditis elegans, we develop a unified multiplex framework linking anatomical wiring to functional communication. We infer structure-derived functional connectivity from the synaptic connectome using
equilibrium principles from statistical physics, yielding a probabilistic map of information flow across all synaptic pathways, and compare this functional layer directly with the extrasynaptic connectome. This reveals a principled functional specialization across four communication regimes: (i) a
topology-dependent layer that reinforces and stabilizes synaptic motor
circuits, (ii) a
topology-resilient modulatory layer supporting global regulation and behavioral state control, (iii) a purely extrasynaptic network sustaining survival and homeostasis, and (iv) a purely synaptic regime mediating rapid, low-latency sensorimotor processing. Together, these findings reveal that synaptic and extrasynaptic signaling form complementary architectures optimized for speed, modulation, robustness, and survival, and provide a general strategy for integrating structural and modulatory connectomes to understand how distinct communication modes cooperate to sustain coherent
brain function.
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Strongly Correlated Electrons · Cross-listed from physics.chem-ph
Efficient Auxiliary-Field Quantum Monte Carlo using Isometric Tensor Hypercontraction
Maxine Luo, Victor Chen, Yu Wang et al. (+1 more)
Auxiliary Field
Quantum Monte Carlo (AFQMC) has emerged as a powerful framework for treating strongly correlated electronic systems, offering a favorable balance between computational cost and accuracy. In this paper, we present a novel AFQMC method that uses the isometric tensor hypercontraction (ITHC) technique to diagonalize the two-body Coulomb interaction of molecular electronic
Hamiltonians by introducing additional fictitious fermionic modes. Our method shows reduced theoretical complexity and better practical performance for both propagation and local energy evaluation compared to the standard AFQMC method. We demonstrate the efficacy of this approach by computing the ground-state energies of a linear $\ce{H10}$-chain and the benzene molecule. Our results show that the extended-basis AFQMC recovers many-body correlations with a precision comparable to that of high-level wavefunction methods such as Coupled Clusters (CC) or Density
Matrix Renormalization Group (DMRG), while offering significantly improved scaling.
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All authors Maxine Luo, Victor Chen, Yu Wang, Christian B. Mendl
Strongly Correlated Electrons · Cross-listed from quant-ph
High-threshold decoding of non-Pauli codes for 2D universality
Julio C. Magdalena de la Fuente, Noa Feldman, Jens Eisert et al. (+1 more)
Topological codes have many desirable properties that allow fault-tolerant
quantum computation with relatively low overhead. A core challenge for these codes, however, is to achieve a low-overhead universal gate set with limited connectivity. In this work, we explore a non-Pauli stabilizer code that can be used to complete a universal gate set on topological toric and surface codes in strictly two dimensions. Fault-tolerant syndrome extraction for the non-Pauli code requires mid-
circuit $X$ corrections, a key difference to conventional Pauli codes. We construct and
benchmark a just-in-time (JIT) matching decoder to reliably decide these corrections. Under a phenomenological error model with equally likely physical and measurement errors, we find a high threshold of $\approx 2.5\,\%$, close to the $\approx 2.9\,\%$ of a decoder with access to the full syndrome history. We also perform a finite-size scaling analysis to estimate how the logical error rate scales below threshold and verify an exponential suppression in both physical error rate and in the system size. A second global decoding step for $Z$ errors is required and the non-Clifford gates in the
circuit reduce the threshold from $\approx 2.9\,\%$ to $\approx 1.8\,\%$ with a naive decoder. We show how $Z$ decoding can be improved using knowledge of the $X$ corrections, pushing the threshold to $\approx 2.2\,\%$. Our results suggest non-Clifford logic in 2D codes could perform comparably to 2D
quantum memory. Our formalism for efficient benchmarking and decoding directly generalizes to a broader family of CSS codes whose $X$ stabilizers are twisted by diagonal Clifford operators, and spacetime versions thereof, defined by CSS-like
circuits enriched by $CCZ$, $CS$, and $T$ gates.
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All authors Julio C. Magdalena de la Fuente, Noa Feldman, Jens Eisert, Andreas Bauer
Mesoscale and Nanoscale Physics · Cross-listed from quant-ph
Compact system development of efficient quantum-entangled photon sources towards deployable and industrial devices
Yared G. Zena, Moritz Langer, Ahmad Rahimi et al. (+9 more)
Entangled
photon pair sources are a key enabling technology for
quantum communication and networking, yet their deployment beyond laboratory environments is hindered by system-level complexity, limited operational stability, and insufficient industry compatibility. Here, we demonstrate a rack-based, mobile
quantum light source architecture based on a
semiconductor quantum dot emitter that directly addresses these challenges through modular system integration and automated operation. The source generates polarization-entangled
photon pairs with an
entanglement negativity 2n of up to $0.98(1)$, confirming near-maximal
entanglement quality. In continuous, hands-off operation over a six-hour time window, the system achieves an average single-
photon emission rate of $697(8)$ kHz and a maximum rate of $740(7)$ kHz, while maintaining 2n-value of more than $95$ $\%$. These results are enabled by the integration of optical excitation, collection, cryogenic operation, and control electronics within a standardized rack footprint, together with automated monitoring. By demonstrating simultaneously high
entanglement quality, sustained brightness, and long-term operational stability in an industry-aligned system architecture, this work advances
semiconductor quantum dot sources toward deployable entangled
photon sources for applied
quantum photonics.
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All authors Yared G. Zena, Moritz Langer, Ahmad Rahimi, Abhishikth Dhurjati, Pavel Ruchka, Sara Jakovljevic, Mandira Pal, Frank H. P. Fitzek, Harald Giessen, Juergen Czarske, Riccardo Bassoli, Caspar Hopfmann
Quantum Gases
Merging and oscillations of dipolar Bose-Einstein condensate droplets
Wojciech Orłowski and Bartłomiej Szafran
We investigate the dynamics of Bose-Einstein condensate droplets composed of $^{164}$Dy atoms formed in a double-well potential following removal of the interwell barrier. By solving the dipolar Gross-Pitaevskii equation, we determine phase diagrams of ground-state configurations as functions of the atom number confined in the double-well potential. For an interwell separation $2d=3\,\mu\mathrm{m}$, we consider the relative dipolar-to-contact interaction strengths $\varepsilon_{dd}=1.4$, $1.45$, and $1.5$.
Symmetry-broken lowest-energy configurations are found for $\varepsilon_{dd}=1.5$ and, over a reduced range of atom numbers, for $\varepsilon_{dd}=1.45$, whereas no
symmetry-broken states are found for $\varepsilon_{dd}=1.4$ up to $N=5\times10^4$. We analyze the subsequent time
evolution after removal of the central barrier, revealing both droplet oscillations and merger events leading to the formation of larger droplets. The oscillations are driven by the external potential and by the repulsive tails of the in-plane component of the dipolar interaction. For the two-droplet states at $\varepsilon_{dd}=1.5$ and $2d=3\,\mu\mathrm{m}$, merging is found for $N=8000$ and $8800$, whereas the droplets remain separated for the investigated cases with $N\geq9000$. Increasing the initial separation to $2d=5\,\mu\mathrm{m}$ shifts the approximate upper atom number for merging to $N\simeq1.65\times10^4$, demonstrating that the crossover is controlled by the competition between the post-quench excess energy and the repulsive inter-droplet barrier.
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Strongly Correlated Electrons
Moiré Mott correlated mosaics in twisted bilayer 1T-TaS$_2$
Ana Vera Montoto, Jose L. Lado and Adolfo O. Fumega
The tunability and twist engineering of van der Waals materials enable the emergence of electronic states not present in individual monolayers. Among them, monolayer 1T-TaS$_2$ is a well-known Mott insulating system, whose
star-of-David charge density wave reconstruction realizes an emergent triangular
lattice of local
magnetic moments. Interestingly, in its bulk form, the insulating gap is not correlation-driven, but stems from interlayer coupling. Here, we exploit the stacking-dependent nature of the insulating gap to show that in twisted 1T-TaS$_2$
bilayers, the spatially dependent competition between many-body and single-particle gaps creates Mott-trivial mosaic superlattices, featuring regions with local
magnetic moments and non-
magnetic insulating regions. We further demonstrate the tunability of the mosaic correlated state with an interlayer bias, giving rise to controllable charge transfer and quenching of correlations. Our results establish twisted 1T-TaS$_2$ as a flexible platform to engineer mixed spatially modulated correlated insulating phases, arising from the moiré profile.
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Statistical Mechanics
Resetting optimized competitive first-passage outcomes in non-Markovian systems
Suvam Pal, Rahul Das and Arnab Pal
We investigate the role of
stochastic resetting in non-Markovian systems, where
memory effects arise due to slow relaxation, rugged energy landscapes, disordered environments, and molecular crowding. Using the celebrated continuous-time random walk (CTRW) framework, we analyze first-passage processes with multiple competing outcomes and examine how resetting can selectively enhance desired events. We characterize the efficiency of resetting through conditional mean first-passage times (MFPTs) and demonstrate that its impact is highly sensitive to the underlying waiting-time statistics. Furthermore, we derive an inequality that quantifies how resetting controls fluctuations in conditional first-passage times (FPTs), revealing regimes where variability is significantly suppressed. Our results provide a systematic understanding of how long-term
memory influences competitive first-passage outcomes and establish resetting as a powerful control mechanism beyond the conventional Markovian setting.
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Other Condensed Matter
Relativistic Effects on Photoabsorption Cross Sections of Highly Charged Ions
Anvar Khujakulov and Caterina Cocchi
The study of highly charged ions offers a unique platform for probing the breakdown of non-relativistic theory under the influence of extreme electromagnetic environments. Here, we investigate the photoabsorption of highly charged ions within the dipole approximation using both the time-dependent Schrödinger equation (TDSE) and the time-dependent Dirac equation (TDDE), modelling the external field as an instantaneous broadband excitation. Nonrelativistic scaling relations with respect to the
nuclear charge are utilized as a diagnostic tool to systematically identify and quantify relativistic contributions. Within the purely nonrelativistic TDSE framework, these scaling relations hold exactly, allowing the absorption spectra of arbitrary highly charged ions to be inferred directly from a neutral hydrogenic reference. However, as the
nuclear charge increases, relativistic effects become dominant through a sizeable blue shift in the absorption cross section, due to the relativistic enhancement of the binding energy. We further evaluate semi-relativistic TDSE approximations by direct comparison with full TDDE simulations, assessing their predictive power and establishing the regimes where a full Dirac treatment is indispensable for quantitative accuracy.
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Statistical Mechanics · Cross-listed from physics.soc-ph
Hyperscaling of spatial fluctuations constrains the development of urban populations
Wout Merbis, Fernando A. N. Santos, Jay Armas et al. (+2 more)
Urban populations exhibit fractal organization and systematic scaling regularities, yet the scaling exponents reported across cities vary substantially, challenging existing theory. Using 100~m gridded population maps for 109 urban regions in the Netherlands (2000–2023) and 368 major world cities (1975–2020), we recursively coarse-grain each city and quantify how the mean and variance of inhabitants in square grid
cells of side length $\ell$ scale with $\ell$. This yields two exponents, $\beta$ from $\langle N_\ell\rangle\sim \ell^{\beta}$ and $\gamma$ from $\mathrm{Var}(N_\ell)\sim \ell^{\gamma}$, where in the small-$\ell$ limit $\beta$ equals the planar fractal dimension of populated space. Across cities within a given year, $\gamma$ depends linearly on $\beta$. Compiling $>$10,000 exponent estimates over five decades shows that this hyperscaling relation is robust yet non-universal: its slope and intercept vary across continents and drift systematically in time, trending toward the limiting form $\gamma\simeq 2+\beta$. A mean-field (independent-
cell) argument predicts a quadratic mean–variance mapping and cannot reproduce the observed $\beta$–$\gamma$ dependence, implying strong spatial correlations. We derive a correlation-aware variance decomposition in which $\gamma$ is controlled by a correlation dimension $D_c$; in the correlation-dominated regime $\gamma=2+D_c$. If large maturing cities, as are the ones selected in our
dataset, evolve to effective monofractal ($D_c\simeq \beta$) cities, the asymptotic prediction becomes $\gamma\simeq 2+\beta$, consistent with the observed temporal drift. This interdependence links urban geometry and fluctuations, provides an empirical constraint for mechanistic models of urban growth, and implies scaling predictions for spatial indicators built from local means and variances.
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All authors Wout Merbis, Fernando A. N. Santos, Jay Armas, Frank Pijpers, Mike Lees
Strongly Correlated Electrons
Hydrodynamic Backflow for Easing the Fermion Sign in Finite-Temperature Electron Path Integral Simulations
Ingvars Vitenburgs and Jarvist Moore Frost
Some notable technology systems, such as high-temperature
superconductors and materials for controlled
nuclear fusion, require an accurate description of finite-temperature
quantum matter.
Stochastic path integral methods are finite-temperature and numerically exact, but scale poorly with system size due the notorious
Fermion sign problem. To somewhat mitigate this, we use a hydrodynamical backflow coordinate transformation. Our first approach was a continuous normalizing flow machine learning optimisation. We found this to roughly halve the statistical uncertainty at medium sign severity. Numerical issues challenged training effectively. Thus, a semi-analytic analogue was developed to estimate the optimal parameters. We do this by using a derived expression dependent on a Bosonic observable. Hence, the calculation of these values does not have a sign problem. The resulting backflow transformations reduce the problem by multiple orders of magnitude in the specific case of a harmonically trapped, two-dimensional, electron gas at finite-temperature. The total energy of the system agrees with previous, backflow untransformed, studies and we calculate energies for up to 32 electrons. The limiting factor is found to be, primarily, the $O(N^3)$ calculation of the Jacobian, stemming from the coordinate transformation of the backflow. A more thorough implementation may further improve this scaling. Even without this, a route for simulating electron systems at currently unreachable regimes is obtained.
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Mesoscale and Nanoscale Physics
Quantum anomalous Hall conductivity in altermagnets under applied magnetic field
Meysam Bagheri Tagani, Amar Fakhredine and Carmine Autieri
We investigate the emergence of
quantum anomalous
Hall conductivity in a two-dimensional $d$-wave altermagnet on a Lieb
lattice under an external
magnetic field. Altermagnetic order induces momentum-dependent
spin splitting without net magnetization in the relativistic limit, producing distinct
spin-resolved bands at the $X$ and $Y$ valleys. The phase diagram features a normal
insulator and a
spin Chern
insulator separated by an accidental Dirac semimetal. The
magnetic field breaks rotational
symmetry between valleys while maintaining vanishing total magnetization, enabling independent valley contributions to
topology. One valley supports Chern numbers $C=-1$ or $0$, while the other hosts $C=0$ or $+1$, governed by field strength and bandwidth. This competition yields valley-dependent
topology. Berry
curvature analysis reveals fully gapped phases with total Chern numbers $C=\pm1$, separated by valley-selective gap closings. We uncover a mechanism for rapid
magnetic control of the
quantum anomalous
Hall effect near the semimetal phase and highlight key distinctions from ferro-valleytronic and
quantum spin Hall systems.
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Materials Science
Lead-free antiperovskite derivatives Ba$_3$MA$_3$ (M = P, As, Sb, Bi; A = Cl, Br, I): Next-gen materials for optoelectronics
Surajit Adhikari, Aftab Alam and Priya Johari
Antiperovskite derivatives have recently emerged as promising lead-free alternatives to halide perovskites for optoelectronic applications. Here, using a comprehensive first-principles calculations including density functional perturbation theory and many-body perturbation theory (involving GW and Bethe-Salpeter equation (BSE)), we investigate the stability, excitonic, polaronic, and optoelectronic properties of cubic Ba$_3$MA$_3$ (M = P, As, Sb, Bi; A = Cl, Br, I). These compounds are found to be dynamically and thermodynamically stable direct-gap
semiconductors with G$_0$W$_0$@PBE+SOC band gaps spanning 1.23-2.17 eV. BSE calculations reveal moderate
exciton binding energies (0.254-0.352 eV) and intermediate-radius
excitons, while Fröhlich polaron analysis indicates intermediate carrier-
phonon coupling and mobilities up to $\sim$ 75 cm$^{2}$V$^{-1}$s$^{-1}$. The resulting spectroscopic limited maximum efficiencies reach $\sim$ 19-32%, surpassing several lead-based perovskites. Our results establish Ba-based antiperovskite derivatives as a robust, eco-friendly platform for next-generation optoelectronic devices.
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Soft Condensed Matter
A Residence-Time Approach for Determining Position-Dependent Diffusivities from Biased Molecular Simulations
Rinto Thomas, Praveen Ranganath Prabhakar and Michael von Domaros
Position-dependent diffusivities are central parameters in reduced
stochastic descriptions of molecular transport in heterogeneous environments, but their reliable estimation from molecular dynamics simulations remains challenging. We present a residence-time approach (RTA) that extracts local diffusivities from first-exit statistics measured in biased simulations after compensation of the mean free-energy gradient. We apply the method to oxygen
diffusion across a hexadecane/water slab, water permeation across a POPC lipid
bilayer, and transport of water and volatile organic compounds through a model skin-barrier membrane. In the slab system, RTA diffusivities agree with independently determined bulk reference values. In the membrane systems, propagator predictions based on RTA-derived diffusivities reproduce unbiased molecular dynamics propagators over substantial lag-time ranges, while also revealing that, in some cases, no single lag-time-independent diffusivity profile captures the dynamics across all timescales. These results support residence-time statistics as a practical route for determining effective position-dependent diffusivities from biased molecular simulations.
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Statistical Mechanics · Cross-listed from cs.CL
How to measure the optimality of word or gesture order with respect to the principle of swap distance minimization
Ramon Ferrer-i-Cancho
The structure of all the permutations of a sequence can be represented as a permutohedron, a graph where vertices are permutations and two vertices are linked if a swap of adjacent elements in the permutation of one of the vertices produces the permutation of the other vertex. It has been hypothesized that word orders in
languages minimize the swap distance in the permutohedron: given a source order, word orders that are closer in the permutohedron should be less costly and thus more likely. Here we explain how to measure the degree of optimality of word order variation with respect to swap distance minimization. We illustrate the power of our novel mathematical framework by examining spontaneous gestures produced by speakers from four
languages (two SVO
languages and two VSO
languages, which represent two linguistic families). We show that crosslinguistic gestures are at least $77\%$ optimal. It is unlikely that the multiple times where crosslinguistic gestures hit optimality are due to chance. We establish the theoretical foundations for research on the optimality of word or gesture order with respect to swap distance minimization in communication systems. Finally, we introduce the quadratic assignment problem (QAP) into
language research as an umbrella for multiple optimization problems and, accordingly, postulate a general principle of optimal assignment that unifies various linguistic principles including swap distance minimization.
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Statistical Mechanics
Universal features of nonequilibrium Ising models in contact with two thermal reservoirs
Iago N. Mamede, Bart Cleuren and Carlos. E. Fiore
We derive generic properties of nonequilibrium phase transitions in all-to-all Ising models placed in contact with two thermal reservoirs, in which parameters (temperatures, interactions and field parameters) assume arbitrary values depending on the contact with each thermal bath. The presence of different kinds of external parameters leads to remarkably different sort of phase transitions. While continuous, discontinuous and even tricritical points are presented when external parameters are symmetric (e.g. the case of energetic barriers or different couplings between the system and thermal baths), the tricriticality is absent when external parameters are antisymmetric (e.g. the case of
magnetic fields or biased drivings) implying that solely critical or discontinuous are possible. In such latter case, the probability distribution acquires the Boltzmann-Gibbs like form, irrespectively the model parameters when the switching between thermal reservoirs is sufficiently fast. Our work sheds light about the differences between
equilibrium and nonequilibrium ingredients and theirs consequences upon phase transitions.
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Other Condensed Matter · Cross-listed from quant-ph
Critical timescales for chiral state conversion and irreversibility
Giorgos Pappas, Diego Bautista Avilés, Luis E. F. Foa Torres et al. (+1 more)
Non-Hermitian systems driven along slow parametric loops undergo non-adiabatic transitions whose outcome depends sensitively on the driving speed, yet no explicit formula has been available for the critical timescale $T_{\mathrm{cr}}$ at which these transitions develop. Using a $2\times 2$
Hamiltonian with circular parameter trajectories, we derive $T_{\mathrm{cr}} = \mathcal{G}\,\ln(1/|\Delta|)$ in closed form for non-encircling loops, phase-shifted loops, offset loops, and loops encircling exceptional points, where $\mathcal{G}$ is a geometry-dependent growth factor and $\Delta$ is the instability seed. This formula sharply separates the regime where the system remains in the averagely dominant eigenstate ($T< T_{\mathrm{cr}}$) from the superadiabatic regime where the instantaneous dominant eigenstate takes over ($T> T_{\mathrm{cr}}$), resolving the apparent tension between the previous literature. We identify two competing seeds: a
geometric Stokes multiplier and the finite-precision floor. When the
geometric seed vanishes, precision alone governs the transition, yielding $T_{\mathrm{cr}} \propto m\ln\beta$, linear in the number $m$ of digits in base $\beta$ (bits for $\beta=2$). For loops encircling an exceptional point, the Stokes seed only sets an intermediate plateau; the final transition is again seeded by the precision floor, and $T_{\mathrm{cr}}$ remains linear in $m$. This provides a purely forward-
evolution manifestation of precision-induced irreversibility [Phys. Rev. A 114, 012207 (2026)], demonstrating that the fundamental limit identified through echo protocols also controls the outcome of slow non-Hermitian dynamics without requiring time reversal. For PT-symmetric energy spectra, $T_{\mathrm{cr}}$ additionally determines the onset of chirality: the dynamics is non-
chiral for $T< T_{\mathrm{cr}}$ and
chiral for $T> T_{\mathrm{cr}}$.
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All authors Giorgos Pappas, Diego Bautista Avilés, Luis E. F. Foa Torres, Vassos Achilleos
Materials Science
Phonon Thermal Hall Effect in quartz and its absence in silica
Yu Ling, Benoît Fauqué and Kamran Behnia
The observation of a misalignment between the applied heat flux and the measured temperature gradient in insulating solids induced by
magnetic field has become a subject of experimental investigation, theoretical speculation, and unsettled controversy. To identify the origin of this
phonon thermal
Hall effect, we performed a comparative study of longitudinal and transverse heat transport in crystalline (quartz) and vitreous (silica) SiO$_2$ using identical experimental set-ups and thermometers. A finite signal was detected in the crystalline samples and none in the amorphous sample, within our resolution. The cleaner
crystal exhibited a larger thermal
Hall conductivity than the dirtier one, ruling out disorder as the driver of the effect. On the other hand, the amplitude of the transverse thermal resistivity is almost identical in the two crystalline samples (W$_{\perp}$/B$\approx 10^{-6}$ m.K.W$^{-1}$.T$^{-1}$). We show that in a
phonon gas, as in a molecular gas displaying the Senftleben-Beenakker effect, heat is conducted through two channels, and argue that a thermal
Hall response is unavoidable whenever these channels differ both in
entropy production and in their coupling to the
magnetic field. Under such conditions, the conserved energy current and the non-conserved
entropy current cease to be parallel. Finally, the magnitude of the transverse thermal resistivity can be accounted for by a surprisingly simple picture. The heat flux induces a tiny drift velocity of the
lattice nuclei, the
magnetic field exerts a transverse Berry force on this drift, and this force is balanced by an entropic restoring force.
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Superconductivity
Dissecting superconductivity in the Ruddlesden-Popper nickelates: The role of electron correlation and interlayer magnetic exchange
Xiaoyang Chen, Zezhong Li, Mei Xie et al. (+9 more)
The discovery of superconductivity in the Ruddlesden-Popper (RP) nickelates has opened a new chapter in the search for high superconducting transition temperatures ($T_\mathrm{c}$) materials. A central and puzzling feature of this family is the wide variation in $T_\mathrm{c}$ despite their common NiO$_2$ building blocks, as highlighted by the recent observation of superconductivity at $\sim$ 30 K in trilayer $\mathrm{La_4Ni_3O_{10}}$, significantly lower than 80 K reported in
bilayer $\mathrm{La_3Ni_2O_7}$. Understanding the factors that control $T_\mathrm{c}$ in this family is therefore of paramount importance. Here, we use resonant inelastic x-ray scattering (RIXS) to investigate the electronic and
magnetic excitations of $\mathrm{La_4Ni_3O_{10}}$ in direct comparison with its
bilayer counterpart. Our results reveal a markedly different landscape. $\mathrm{La_4Ni_3O_{10}}$ exhibits a more itinerant character, evidenced by broader Ni $dd$ orbital excitations and a strong Ni 3$d$ fluorescence continuum, suggesting weaker electronic correlations than in the
bilayer. Despite this, well-defined collective
spin excitations persist, including dispersive acoustic and optical
magnon branches alongside an incommensurate
spin density wave. Using linear
spin wave theory, we extract the interlayer superexchange interaction ($J_z$) to be $\sim$ 22 meV, much smaller than that in $\mathrm{La_3Ni_2O_7}$. The weaker correlation and reduced interlayer exchange together provide a consistent explanation for the substantially lower $T_\mathrm{c}$ in the trilayer compound. Our findings establish interlayer
magnetic coupling and electronic correlation as key parameters governing superconductivity in layered nickelates and offer critical constraints for understanding the pairing mechanism in this emerging family.
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All authors Xiaoyang Chen, Zezhong Li, Mei Xie, Deyuan Hu, Yiu-Fung Chiu, Stefano Agrestini, Wenliang Zhang, Yi Lu, Meng Wang, Mirian Garcia-Fernandez, Donglai Feng, Ke-Jin Zhou
Materials Science
Atomistic theory of the phonon angular momentum Hall effect
Daniel A. Bustamante Lopez, Verena Brehm and Dominik M. Juraschek
The
spin and orbital
Hall effects convert longitudinal charge currents into transverse flows of electronic angular momentum. Here we develop an atomistic theory of the recently proposed
lattice-vibrational analogue, in which a longitudinal heat current driven by a thermal gradient is converted into a transverse current of
phonon angular momentum. We derive a microscopic real-space expression for this current and show that it originates from thermally induced mixing of polarized vibrational motion, leading to a characteristic edge accumulation of
phonon angular momentum. We demonstrate the effect in minimal square- and honeycomb-
lattice models and compute the resulting
phonon angular momentum accumulations for a range of example materials using input from first-principles calculations. Our results confirm that the
phonon angular momentum
Hall effect is a universal response of crystalline solids and our framework is generically applicable to all materials.
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Materials Science
Xinyang Jiang, Jian Wu and Weiyi Pan
Antiferromagnetic (AFM) and
ferromagnetic (FM) skyrmions possess unique advantages for spintronic applications. AFM skyrmions eliminate the skyrmion
Hall effect and exhibit fast dynamics, whereas FM skyrmions are easier to nucleate and manipulate. However, realizing a transition between AFM and FM skyrmions within the same two-dimensional (2D) material has remained elusive. Here, using first-principles calculations and atomistic
spin simulations on the Janus monolayer Cr2Ge2Te3S3, we demonstrate that strain-driven modulation of
magnetic interactions enables switching between AFM and FM skyrmion phases. A compressive strain of $-3\%$ induces an AFM ground state hosting AFM skyrmions, while a tensile strain of $+2\%$ drives the system into a FM skyrmion phase. Moreover, under an out-of-plane
magnetic field, FM skyrmions are rapidly transformed into a uniform FM phase, while AFM skyrmions transform into AFM bimerons under stronger fields. These findings establish a framework for controllable transitions between topological
magnetic states in a single 2D material.
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Materials Science
Elastic softening and fracture in randomly perforated solids
Tero Mäkinen, Alessandro Taloni, Giulio Costantini et al. (+3 more)
We study the mechanical response of quasi-brittle polymethyl methacrylate (PMMA) specimens containing controlled random distributions of
laser-cut holes. Tensile tests combined with digital image correlation reveal a nearly linear decrease of the Young's modulus with porosity, but with a softening rate far exceeding classical effective medium theory and the Hashin-Shtrikman bound. The extrapolated critical porosity at which the modulus vanishes is well below the 2D percolation threshold, indicating that ideal cylindrical void models fail to capture the observed behavior. Microscopy shows irregular pore geometries and frequent coalescence, which effectively act as crack-like defects and strongly enhance compliance. The rupture stress distributions are well described by a Weibull model accounting for both load-bearing area reduction and stress concentration at hole edges. Digital image correlation reveals heterogeneous but non-localized deformation, with strain increasingly correlated with the hole pattern, indicating a growing influence of defect-induced stress concentrations. These results highlight the dominant role of defect morphology in governing stiffness degradation and fracture statistics in porous quasi-brittle materials.
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All authors Tero Mäkinen, Alessandro Taloni, Giulio Costantini, Davide Della Torre, Riccardo Donnini, Stefano Zapperi
Mesoscale and Nanoscale Physics
Z.Z. Alisultanov
We theoretically introduce a quasi-1D
magnetic heterostructure of alternating 2D topological and normal
insulator strips. Its low-energy physics is governed by a hybrid
Hamiltonian intertwining the Su-Schrieffer-Heeger and Shockley models, with
spin-momentum locking and local Zeeman splitting.
Symmetry analysis places it in class AIII, characterized by
chiral symmetry and a $\mathbb{Z}$ topological invariant. Computing the winding number from the block-off-diagonal structure of the
Hamiltonian reveals topological phases characterized by invariants $\nu = 0$, $1$, and $2$. Furthermore, a single
magnetic defect acts as a sensitive local probe, whose in-gap spectrum provides a spectroscopic fingerprint to distinguish topological phases. Extending the platform to a multilayer geometry uncovers a nonsymmorphic projective
symmetry that gives rise to Möbius band
topology, with the Brillouin zone compactifying into a Klein bottle. Our work establishes a platform for higher-order
topology via
heterostructure design and
magnetic patterning.
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Statistical Mechanics
Beyond dynamic scaling: rare events break universality
Ulysse Marquis, Riccardo Gallotti and Marc Barthelemy
Surface growth driven by non-monomeric deposition has remained largely unexplored. We investigate a model based on the deposition of blobs with a power-law size distribution $P(s)\sim s^{-\tau}$. We find that the critical exponents vary continuously with $\tau$, recovering Kardar–Parisi–Zhang behavior only for $\tau \ge 3$. For $\tau<3$, roughness scaling exhibits strong corrections and scale invariance breaks down. We show that this behavior originates from the emergence of a second dynamical length scale $\zeta$, corresponding to the linear size of the largest cluster, in addition to the usual correlation length $\xi$. The coexistence of these two relevant scales signals the breakdown of the usual Family–Vicsek scaling. These results point to a new phenomenology of surface growth beyond the standard scale-invariant paradigm.
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Strongly Correlated Electrons
Bond-Length-Driven Magnetic Transition in Quasi-One-Dimensional CrSb$X_3$ ($X$=S, Se)
Kang Lee, Hong-Suk Choi and K.-W. Lee
Using ab initio calculations, we investigate the
magnetic ground states of quasi-one-dimensional insulating CrSb$X_3$ ($X$ = S, Se) with infinite double-rutile chains. Within conventional band theory, without explicit Coulomb correlations ($U$), we obtain band gaps in close agreement with experiment. Remarkably, we find that the
magnetic order is highly sensitive to the Cr-Cr bond length $d_{\rm Cr-Cr}$: increasing the bond length induces a transition from
antiferromagnetic to
ferromagnetic order at a critical distance $d^c_{\rm Cr-Cr} \approx 3.53 (\pm 0.05)$ Å. Accordingly, CrSbS$_3$ lies near the transition boundary, whereas CrSbSe$_3$ is robustly
ferromagnetic, in good agreement with experiment. Analysis of the exchange interactions reveals that the first-order phase transition is dominated by a sign reversal of the intrachain nearest-neighbor superexchange $J_1$ mediated by chalcogen ions, while the intrachain direct exchange $J_2$ remains
ferromagnetic and changes only gradually. This behavior reflects an emergent Bethe-Slater-like behavior driven by competing exchange pathways in a quasi-1D transition-metal system, where the competition between $J_1$ and $J_2$ dictates the
magnetic ground state. Besides, the electronic structures of the ground states of each compound are investigated.
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