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Physics Condensed Matter

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Monday 8 December

Strongly Correlated Electrons · Cross-listed from hep-th

Grand Canonical vs Canonical Krylov Complexity in Double-Scaled Complex SYK Model

We consider the complex SYK model in the double-scaling limit. We obtain the transfer matrix for the grand canonical ensemble and symmetrize it. In the (n,Q)- basis of chord states, the grand canonical transfer matrix is block diagonal, where each block is the canonical transfer matrix for the respective charge sector. We therefore conclude that the Krylov complexity for the grand canonical ensemble is given by the sum of the complexities in the charge sectors weighted by a probability function that depends on the chemical potential. Finally, we compute the Krylov complexity analytically in the limit of early and late time in the charge sector and numerically for both canonical and grand canonical ensemble.
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Mesoscale and Nanoscale Physics

Temporal magnetic interfaces reveal damping-induced spin-wave amplification near the stripe-domain transition in ultrathin films with DMI

Using micromagnetic simulations and analytical theory, we study temporal magnetic interfaces in ultrathin CoFeB films with perpendicular magnetic anisotropy and interfacial Dzyaloshinskii–Moriya interaction. We show that time refraction and reflection are governed by precession ellipticity, acting as a magnonic temporal impedance, while smooth field ramps suppress temporal reflections. Near the transition from a uniform state to stripe domains, the exceptional-point and critical fields delimit damping, slow-instability, and strong-instability regimes. In the slow-instability window, Gilbert damping counterintuitively drives spin-wave growth with a rate proportional to the damping parameter. Micromagnetic simulations confirm that a temporal-slab protocol exploiting this regime achieves up to 175-fold frequency-preserving amplitude amplification without continuous power injection. Energy analysis indicates that the field ramp stores energy in the metastable uniform state below the stripe-domain transition, later released into growing spin-wave excitations, consistent with the antimagnonic framework. These results establish temporal field modulation as a route to reconfigurable spin-wave gain.
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Mesoscale and Nanoscale Physics

Index-theoretic route to the subgap Andreev bands and topological response in Josephson junctions

We demonstrate that the subgap Andreev bound states in a transparent Josephson junction, comprising of either chiral or non-chiral superconductors, can be viewed as a consequence of the index theorem in supersymmetric quantum mechanics. We provide an exact solution for these states starting from the Bogoliubov-de Gennes (BdG) equations describing quasiparticles in such junctions. We demonstrate that the dispersion of these subgap states depends only on the asymptotic properties of the pair-potential and not on its local spatial variation. Our study reveals the crucial distinction between junctions of non-chiral $p$-wave superconductors and those of $s$-wave or chiral superconductors by analyzing the wavefunction of their subgap bound states. We find a stable topological response leading to the well-known $4\pi$ periodic Josephson effect protected against weak disorder potential for the non-chiral $p$-wave junctions; no such protection is found for junctions of $s$-wave or chiral superconductors. We supplement our analytic results with numerical computation of the Josephson currents in such junctions using exact numerical Green functions and starting from a lattice model of an itinerant altermagnet which is expected to host triplet $p$-wave superconductivity with equal-spin-pairing. We also discuss the implications of our results for Josephson junctions away from the transparent limit.
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All authors Sinchan Ghosh, Srinjoy Ghosh, Arijit Kundu, K. Sengupta

Strongly Correlated Electrons

Extreme Strain Controlled Correlated Metal-Insulator Transition in the Altermagnet CrSb

Correlated flat bands and altermagnetism are two important directions in quantum materials, centred respectively on interaction-dominated phases and symmetry-enforced spin-textured states, yet both derive from lattice symmetry and orbital hybridization. This common origin implies that extreme crystal distortion, by narrowing bandwidths, enhancing correlations and reshaping the symmetries of altermagnetic spin splittings, could unify flat-band and altermagnetic physics in a single material; in practice, however, achieving such large distortions in a crystalline altermagnet is a formidable challenge. Here we combine a dedicated strain device with a tailored single-crystal mounting scheme to impose a highly tensile strain gradient in bulk CrSb, a prototypical altermagnet, creating a near-surface layer in which the in-plane lattice is strongly distorted relative to the weakly strained bulk, while the average bulk distortion remains small. Angle-resolved photoemission reveals a reversible regime at moderate strain, where a deeper flat-band feature, attributed to a strain-gradient-driven suppression of Cr-Sb hybridization, coexists with a correlation-enhanced Cr 3d flat band, and an irreversible regime at larger strain where partial bond decoupling drives a predominantly insulating spectral response. Density-functional calculations show that an orbital-selective altermagnetic spin texture persists across this correlated regime despite strong bandwidth renormalisation. These results define a strain-symmetry-correlation map for CrSb and establish extreme tensile strain as a route to co-engineer flat-band tendencies and spin-textured, zero-net-moment correlated states in altermagnets, pointing toward strain-adaptive, spin-selective Mott filtering and related device concepts.
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All authors Cong Li, Mengli Hu, Jianfeng Zhang, Magnus H. Berntsen, Francesco Scali, Dibya Phuyal, Chun Lin, Wanyu Chen, Johan Chang, Oliver J. Clark, Timur K. Kim, Jacek Osiecki, Craig Polley, Balasubramanian Thiagarajan, Zhilin Li, Tao Xiang, Oscar Tjernberg

Quantum Gases

Multicomponent condensates: a flexible platform for soliton physics

We present a series of experimental investigations on binary mixtures of Bose-Einstein condensates. Our focus lies on the regime where the interaction parameters place the system at the threshold of miscibility. We demonstrate that the dynamics of such mixtures can be effectively reduced to a single nonlinear equation. This framework is illustrated through the discussion of stable solitonic solutions in one and two dimensions. Furthermore, we show that employing a binary mixture enables exploration beyond the dynamics governed by the nonlinear Schrödinger equation, allowing us to address other fundamental equations in nonlinear physics, such as the Landau-Lifshitz equation describing the motion of spin chains in ferromagnetic materials.
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All authors Franco Rabec, Jérôme Beugnon, Jean Dalibard, Sylvain Nascimbene

Materials Science

Network of localized magnetic textures revealed using a saddle-point search framework

A computational framework is presented for the exploration of energy surfaces of magnetic systems via systematic identification of first-order saddle points that connect local energy minima representing possible states of the system. The saddle points characterize the mechanism of transitions between states and, together with the energy of the local minima, provide estimates of the transition rates within harmonic transition state theory or Kramers/Langer theory. The calculations involve four stages: (1) the symmetry of a given energy-minimum configuration is identified and used to define subsystems whose eigenmodes provide relevant deformation directions. (2) These modes are then used to guide the system toward the neighborhoods of the various saddle points on the energy rim surrounding the given energy minimum. (3) Next, the geodesic minimum mode following method is employed to efficiently converge onto the saddle points. (4) Finally, the identified saddle points are embedded into the network describing the connectivity of the states of the system. This methodology is applied in a study of the metastable textures of two-dimensional chiral magnets described by a lattice Hamiltonian, where a hierarchy of transition mechanisms for the nucleation, annihilation, and rearrangement of various localized magnetic textures are identified, such as skyrmions, antiskyrmions, skyrmion bags, chiral droplet, etc. Transitions corresponding to homotopies that preserve the topological charge as well as transformations that change it are identified. By scaling the interaction parameters, the distinct behavior of these two classes is obtained as the continuum limit is approached. For some transitions, the topological charge changes during the transition even though it is the same for the initial and final states.
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All authors Hendrik Schrautzer, Tim Drevelow, Hannes Jónsson, Pavel F. Bessarab

Statistical Mechanics

Geometric Characterization of Anisotropic Correlations via Mutual Information Tomography

Characterizing anisotropic correlations in quantum and statistical systems requires a coordinate-invariant framework. We introduce a geometric map based on the local informational line element, calibrated by the Euclidean benchmark scale $C_{\mathrm{vac}}$: $ds^{2} = C_{\mathrm{vac}}/I(x,x+\epsilon)$. We prove that this map yields a smooth Riemannian structure $g_{ij}$ if and only if the short-distance mutual information (MI) follows the anisotropic inverse-quadratic law (local exponent $X_{\text{loc}}=2$). A key insight is that anisotropy is necessary to activate tensor geometry; isotropic MI forces conformal flatness $g_{ij} \propto \delta_{ij}$, suppressing shear degrees of freedom. We employ a parameterization-invariant unimodular split $g_{ij} = V^{2/D}\gamma_{ij}$, which rigorously separates local density fluctuations (volume $V$) from directional anisotropy (shape/shear $\gamma_{ij}$). We introduce “MI Tomography,” an operational protocol to reconstruct these geometric components from finite directional measurements. The protocol is validated using the equal-time ground state of an anisotropic 2D quantum harmonic lattice (massless relativistic scalar) on a torus, where the reconstructed shape tensor $\gamma_{ij}$ quantitatively recovers the physical coupling anisotropy. We work strictly in the local, fixed-coarse-graining $X_{\text{loc}}=2$ branch; the line element is used solely to extract the local kinematic structure (the local metric tensor), deferring global distance claims.
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Superconductivity

Robustness of flat band superconductivity against disorder in a two-dimensional Lieb lattice model

Recently, the possibility of high-temperature superconductivity (SC) in flat-band (FB) systems has been the focus of a great deal of activity. This study reveals that unlike conventional intra-band SC for which disorder has a dramatic impact, that associated with FBs is surprisingly robust to disorder-induced fluctuations and quasi-particle localization. In particular, for weak off-diagonal disorder, the critical temperature decreases linearly with disorder amplitude for conventional SC, whereas it is only quadratic in the case of SC in FBs. Our findings could have a major impact on the research and development of new compounds whose high purity will no longer be a critical barrier to their synthesis.
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Materials Science

Computational Studies on O2-P2 Phase-Transition Dynamics in Layered-Oxide Sodium-Ion Cathode Materials

Sodium-ion batteries have gained much interest over the past years and especially layered oxides are highly considered as cathodes for the next generation of batteries. However, there are still significant challenges to overcome in these materials for practical applications mainly related to capacity degradation and voltage fading. A key influence factor for these challenges are phase transitions that occur by gliding of layers during operation of these materials. Until now there is limited atomistic-level understanding on such transitions as simulations of these processes are computationally demanding. In this work, we trained a classical pairwise Coulomb-Buckingham potential versus extensive ab initio data using a genetic algorithm to study O2-P2 phase transitions in Na\textsubscript{x}CoO\textsubscript{2}. Our density functional theory~(DFT) and classical potential calculations show that phase transition barriers decrease upon desodiation and are further lowered if dynamic conditions are considered through molecular dynamics simulations. Our developed classical potential is able to capture phase transitions and its related increase in the Na-ion diffusivity under standard lab conditions at the $\upmu$s timescale of molecular dynamics simulation. Furthermore, it is found that the phase transition occurs gradually via various OPn phases.
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Materials Science · Cross-listed from physics.app-ph

Optimization for growth condition of ultrathin hexagonal boron nitride on dielectric substrates via LPCVD

Hexagonal Boron Nitride (h-BN) is a highly intriguing candidate for heterostructure optoelectronic applications, such as Deep Ultraviolet photodetectors, UV sensing and communication systems and solar cells. This is primarily due to its unique properties, including a layer dependent wide energy bandgap, superior mechanical strength, high thermal conductivity, high band-edge absorption coefficient, and exceptional transparency in the UV region. The widely adopted synthesis method for h-BN thin films is Chemical Vapor Deposition (CVD) Method, which often utilizes catalytic substrates like copper (Cu) and Nickel (Ni). However, integrating the synthesized h-BN into device applications requires a subsequent transfer process to the target substrate. This transfer step introduces significant material damage, such as folding, cracking and polymer residues, which ultimately degrade the optoelectronic properties of the material and compromise device performance. To overcome this major challenge, there is a strong need to synthesize high-quality h-BN films directly onto dielectric substrates such as silicon (Si), SiO2, quartz, sapphire or AlN without the need for transfer. The primary difficulty in direct synthesis lies in achieving homogenous, high crystallinity films with controllable thickness due to the absence of a catalytic effect. In this work, we investigated the optimization of growth parameters for the direct synthesis of ultrathin h-BN films on non-catalytic quartz substrates, which are highly transparent in the UV region, using the Low-pressure Chemical Vapor Deposition (LPCVD) method. The optimal synthesis conditions were determined to be 1050oC for 60 min, achieved by the decomposition of 150 mg Ammonia Borane (AB) precursor at 80oC. This optimization is crucial for advancing large-scale, high-performance h-BN based DUV photodetector fabrication.
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All authors Meryem Bozkaya, Muhammet Nasuh Ar{\i}k, Ali Altuntepe, Hakan Ateş, Recep Zan

Superconductivity

Layer-Resolved Impurity States Reveal Competing Pairing Mechanisms in Trilayer Nickelate Superconductor La$_4$Ni$_3$O$_{10}$

Trilayer Ruddlesden-Popper nickelate superconductor $\mathrm{La}_4 \mathrm{Ni}_3 \mathrm{O}_{10}$ has generated considerable interest due to its unconventional superconductivity and complex electronic structure. Notably, $\mathrm{La}_4 \mathrm{Ni}_3 \mathrm{O}_{10}$ features a mixed Ni valence state and an asymmetric trilayer configuration, leading to distinct quasiparticle distributions and local density of states (LDOS) between the inner and outer NiO$_2$ planes. In this work, we investigate impurity-induced states in $\mathrm{La}_4 \mathrm{Ni}_3 \mathrm{O}_{10}$ using a two-orbital model combined with $T$-matrix formalism, focusing on the contrasting roles of intra- and interlayer pairing channels. Our self-consistent mean-field analysis reveals that interlayer pairing results in partially gapless Fermi surfaces, with unpaired quasiparticles concentrated in the outer layers and a pronounced low-energy LDOS. We demonstrate that impurity effects vary significantly depending on both the pairing symmetry and impurity location: interlayer-dominant pairing produces sharp resonance states when impurities are in the inner layer, whereas impurities in the outer layer lead to in-gap enhancements without sharp resonances; in contrast, intralayer-dominant pairing generally yields increased in-gap LDOS without sharp impurity resonances, regardless of impurity position. These findings suggest that single-impurity spectroscopy can serve as a powerful probe to distinguish between competing superconducting pairing mechanisms in trilayer nickelates and highlight the rich physics arising from their multilayer structure.
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Mesoscale and Nanoscale Physics

Mesoscopic superfluid to superconductor transition

Spectrum tomography for the energy ($E$) of a ring-shaped Bose-Hubbard circuit is illustrated. There is an inter-particle interaction $U$ that controls superfluidity (SF) and the transition to the Mott Insulator (MI) regime. The circuit is coupled to an electromagnetic cavity mode of frequency $\omega_0$, and the coupling is characterized by a generalized fine-structure-constant $\alpha$ that controls the emergence of superconductivity (SC). The ${(U,\alpha,\omega_0,E)}$ diagram features SF and SC regions, a vast region of fragmented possibly chaotic states, and an MI regime for large $U$. The mesoscopic version of the Meissner effect and the Anderson-Higgs mechanism are discussed.
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Statistical Mechanics

Boundary Criticality of Complex Conformal Field Theory: A Case Study in the Non-Hermitian 5-State Potts Model

Conformal fields with boundaries give rise to rich critical phenomena that can reveal information about the underlying conformality. While most existing studies focus on Hermitian systems, here we explore boundary critical phenomena in a non-Hermitian quantum 5-state Potts model which exhibits complex conformality in the bulk. We identify free, fixed and mixed conformal boundary conditions and observe the conformal tower structure of energy spectra, supporting the emergence of conformal boundary criticality. We also studied the duality relation between different conformal boundary conditions under the Kramers-Wannier transformation. These findings should facilitate a comprehensive understanding for complex CFTs and stimulate further exploration on the boundary critical phenomena within non-Hermitian strongly-correlated systems.
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All authors Yin Tang, Qianyu Liu, Qicheng Tang, W. Zhu

Materials Science

Mid-infrared intraband transitions in InAs colloidal quantum dots

III-V colloidal quantum dots are widely studied for their applications as detectors and emitters from visible to short-wave infrared. They might also be used in the mid-infrared if they can be stably n-doped to access their intraband transitions. Mid-infrared intraband transitions are therefore studied for InAs, InAs/InP, and InAs/ZnSe colloidal quantum dots with an energy gap at 1.4 micron. Using electrochemistry, the quantum dot films show state-resolved mobility, state-resolved electron filling, and intraband absorption in the 3-8 micron range. The InAs/ZnSe films need a more reducing potential than InAs, but the InAs/InP films need a lower reduction potential. As a result, we found that dry films of InAs/InP dots show stable n-doping of the 1Se state, with a steady-state intraband absorption in the 3-5 micron range, and intraband luminescence at 5 micron. low-toxicity, high thermal stability, and stable n-doping, InAs quantum dots become an interesting material for mid-infrared applications.
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Strongly Correlated Electrons

Critical Density-Wave Vestigial Phases of Commensurate Pair Density Wave

The pair-density-wave (PDW) is an exotic pairing state hosting a spatially modulated pairing order parameter, which has attracted great interest. Due to its simultaneously breaking U(1)-gauge and translational symmetries, intriguing vestigial phases which restore only one broken symmetry can emerge at an intermediate temperature regime. Previously, investigations on the vestigial phases of PDW were mainly focused on incommensurate PDW. However, the experimentally observed PDW is usually commensurate, whose vestigial phases have not been systematically investigated. Here we study the vestigial phases of 2D commensurate PDW with $n$-times expanded unit vectors, hosting different numbers of wave vectors. Based on the Ginzburg-Landau theory, we get the low energy effective model Hamiltonian. Subsequent renormalization group (RG) and Monte-Carlo (MC) studies are conducted to obtain the phase diagram and spatial dependent correlation functions. Our RG and MC calculations consistently yield the following result. For $n\le 4$, besides the charge-4e/2e superconductivity, there exists the translational symmetry broken charge-density-wave (CDW) vetigial phase. Intriguingly, for $n\ge 5$, the restore of the translational symmetry with increasing temperature is realized through two successive Berezinskii-Kosterlitz-Thouless transitions. Such a two-step process leads into two critical vestigial phases, i.e. the critical-PDW and the critical-CDW phases, in which the discrete translational symmetry is quasily broken, leading into a power-law decaying density-density correlation even at 2D. Our work appeals for experimental verifications.
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All authors Chu-Tian Gao, Jing Zhou, Yu-Bo Liu, Fan Yang

Materials Science

Dynamic Screening Effects on Auger Recombination in Metal-Halide Perovskites

The performance of modern light-emitting technologies, from lasers to LEDs, is limited by nonradiative losses, with Auger recombination being the dominant channel at device-relevant carrier densities. Reliable modeling of this process is essential, yet conventional treatments neglect dynamic dielectric effects, limiting the predictive reliability at operating conditions. We develop a general framework that incorporates the frequency-dependent screened Coulomb interaction $W_{00}(\mathbf{q},\omega)$, computed from low-scaling GW, into both direct and phonon-assisted Auger amplitudes. Demonstrated on orthorhombic $\gamma$-CsPbI$_3$ (band gap $E_g\approx1.73$ eV) and $\gamma$-CsSnI$_3$ ($E_g\approx1.30$ eV), the approach shows that dynamic screening enhances the dielectric response, lowering the room-temperature Auger coefficient by $\sim$50-60 %. This renormalization shifts the crossover between radiative and nonradiative recombination by nearly a factor of two in carrier density. Dynamic dielectric screening thus emerges as a quantitative determinant of Auger recombination, offering a transferable framework for predictive modeling across polar semiconductors where frequency-independent screening models are inadequate.
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Mesoscale and Nanoscale Physics

Spin-Texture Spin-valve with a van der Waals Magnet

All-electrical methods for nucleating, detecting, and manipulating spin textures in two-dimensional (2D) van der Waals (vdW) magnets can serve as fundamental building blocks for multi-state spintronic memory, logic, and neuromorphic computing applications. Unlike conventional ferromagnets, vdW ferromagnets such as Fe5GeTe2 with strong Dzyaloshinskii-Moriya interactions stabilize nanoscale chiral spin textures, including skyrmions and stripe domains. However, the sub-100 nm size of these spin textures has limited their study to sophisticated microscopy techniques. Here, we demonstrate all-electrical detection of spin textures in vdW itinerant ferromagnet Fe5GeTe2 using pure spin transport in a lateral graphene spin-valve device at room temperature. By engineering nanoscale constrictions or notches in Fe5GeTe2, we create spin textures that inject distinct spin polarizations into the graphene channel, where they are nonlocally sensed by a reference conventional ferromagnetic detector at room temperature. This enables the observation of anomalous multi-level spin-valve switching and Hanle spin precession signals, which are due to unique spin textures in Fe5GeTe2 and in sharp contrast to single-domains and conventional magnet-based devices. This all-electrical approach can provide direct access to the spin textures on an integrated 2D spintronic circuit without the need for ex-situ microscopic characterizations.
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All authors Bing Zhao, Roselle Ngaloy, Lars Sjöström, Saroj P. Dash

Soft Condensed Matter

Static Dielectric Permittivity Profiles and Coarse-graining Approaches for Water in Graphene Slit Pores

The dielectric response of nano-confined fluids is crucial across technologies and biological systems, yet its calculation and interpretation from molecular simulations are often muddled by unclear boundary conditions. We re-derive the Green–Kubo relation for the spatially resolved linear dielectric response of fluids in planar confinement, explicitly accounting for boundary conditions and showing that equilibrium-derived profiles agree with those obtained from external fields. We identify common misconceptions in the literature and outline how microscopic dielectric behavior can be coarse-grained to connect with experimental observables. Simulations show that water retains a bulk-like dielectric response down to $\sim 1\,\mathrm{nm}$ confinement. The reduced effective dielectric response that governs capacitance arises from the placement of the dielectric interface. Using effective-medium theory, we demonstrate that long-range reductions reported in experiments and theory are consistent with bulk-like behavior beyond about $1\,\mathrm{nm}$ from the surface. The effective response naturally maps onto an interfacial capacitance, and the dielectric properties of simulated water are robust across simulation setups and water models, reflecting universal polarization correlations.
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All authors Philipp Stärk, Henrik Stooß, Philip Loche, Douwe Jan Bonthuis, Roland R. Netz, Alexander Schlaich

Materials Science

Separation of Hoke and Schottky effects for improvement of mixed halide perovskite solar cell stability

Ion migration in halide perovskites is a key factor limiting the operational stability of solar cells due to formation of halogen ion enriched domains and accumulation layers. The present work demonstrates the manifestation of ion migration in two ways via Hoke and Schottky effects. Both effects are induced by external exposure but have its peculiar way of solar cell performance degradation. We demonstrate the effects of ion migration on the device performance by measuring time dependent short-circuit current and different impedance characteristics that allow to see how charge-carrier separation property degrades. The Schottky effect leads to the rapid decrease of charge-carrier separation characteristic of solar cell while Hoke effect leads to the slow defect accumulation in the perovskite layer leading to the enhanced Shockley-Read-Hall recombination. Separation of these two effects can be realized by simple increase of transport layer thickness. A thick transport layer blocks losses of charge-carrier selectivity in a solar cell and leads to an enormous increase of T80 time, from 15 seconds up to 60 minutes.
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All authors Vladimir Ivanov, Eduard Ageev, Denis Danilov, Eduard Danilovskiy, Dmitry Gets

Materials Science

Alteraxial Phonons in Collinear Magnets

Axial phonons, carrying angular momentum through rotational lattice vibrations, offer a promising platform for exploring phonon-magnetic coupling effects. However, how the interplay of lattice and magnetism determine the phonon angular momentum (PAM) of axial phonons remains elusive. Here, based on magnetic point group theory, we establish a symmetry framework to classify phonons in collinear magnets (e.g. ferromagnets, antiferromangets, altermagnets) into three distinct categories: ferroaxial, antiferro-nonaxial, and alteraxial phonons, which are distinguished by their different PAM patterns. Beyond the ferroaxial phonons featuring $s$-wave PAM, we reveal a complete series of alteraxial phonons, characterized by higher-order-wave PAM patterns ranging from $p$- to $j$-wave. Notably, alteraxial phonons are not limited to altermagnets, but also emerge in ferromagnets and antiferromagets. Our high-throughput search predicts hundreds of candidate magnetic materials hosting alteraxial phonons. Ab initio calculations on representative magnets further confirm the existence and distinct symmetry-enforced nodal structures of PAM in alteraxial phonons. Our work provides a complete classification for axial phonons in collinear magnetic systems and paves the way for engineering magneto-phononic phenomena.
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All authors Fuyi Wang, Junqi Xu, Xinqi Liu, Huaiqiang Wang, Lifa Zhang, Haijun Zhang

Strongly Correlated Electrons

Interlayer coupling driven phase evolution in hyperbolic $1T$-TaS$_2$

Understanding how microscopic interactions control macroscopic phase transitions is central to quantum materials, where charge density waves (CDWs), Mott states, and superconductivity often compete. In $1T$-TaS$_2$, this competition is tied to a sequence of CDW phases and a hysteretic metal-insulator transition, but details of the transition, especially the role of interlayer coupling, remain unresolved. In this work, spectroscopic ellipsometry is used to determine the uniaxial dielectric response of bulk $1T$-TaS$_2$ from room temperature down to the commensurate insulating state. The room-temperature data reveal natural type-II hyperbolic behavior in the visible range, with negative in-plane and positive out-of-plane permittivity. Temperature-dependent ellipsometry combined with anisotropic Bruggeman effective medium analysis shows that the metallic domains responsible for percolation evolve from disc-like to needle-like shapes, and that, upon heating, an additional intermediate phase emerges. These results identify the transition in $1T$-TaS$_2$ as a three-dimensional, interlayer-driven percolation process and establish this material as a natural, tunable hyperbolic medium.
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Strongly Correlated Electrons

Valence band-satellite, temperature dependent magnetic and spectral study of {\alpha}-Fe

We investigate the influence of correlations and plasmonic excitation on valence band-satellite of $\alpha$-Fe, along with magnetic and spectral properties as function of temperature. Coulomb interaction parameters are obtained by systematically employing various schemes in constrained random phase approximation (cRPA). This study identifies the presence of valence band satellite in Fe at $\sim$6 eV binding energy supported by (i) substantial incoherent spectral weight in the valence band spectra obtained from Density Functional Theory plus Dynamical Mean Field Theory (DFT+DMFT) and (ii) plasmonic excitations in the frequency range $\sim$6-8 eV suggested by $G_0W_0$ calculations. We note presence of significant contribution of temperature-dependent Pauli-spin susceptibility indicating competing degree of itinerancy. $e_g$ state shows a strong temperature driven non-Fermi-liquid behavior emerging near $T_c$. Our results reveal a high-temperature orbital-selective loss of coherence eventually leads to a orbital selective collapse of magnetization at $T_c$, suggesting a ferromagnetic phase characterized by strong correlation- and temperature- dependent spectral features.
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Quantum Gases

Quasiparticle spectra of mixtures of dipolar and non-dipolar condensates at zero and finite temperatures

We examine the low-lying collective quasiparticle modes of a quasi-one-dimensional mixture of Bose-Einstein condensates having dipolar and non-dipolar atomic species. The dipolar atomic species have permanent magnetic dipolar moments. We employ Hartree-Fock-Bogoliubov theory to investigate the distinct collective spectra at zero and finite temperatures corresponding to phase separation phenomena stemming from the dipole-dipole interaction of dipolar atomic species. When the dipolar interaction is tuned to be repulsive, the number of zero-energy modes decreases, reflecting the system's tendency towards mixing. For a large number of atoms, we show that the attractive (repulsive) dipolar interaction strengths lead to ground states with non-dipolar (dipolar) atomic species at the periphery, and this leads to a discontinuity in quasiparticle mode evolution. We finally reveal that miscibility driven by thermal fluctuations at finite temperatures exhibits dipole mode hardening, confirmed by the loss of long-range phase coherence through the correlation function. The mode mixing in the dispersion relations ascertains a dipolar strength-dependent miscibility transition and the low-lying quasiparticle mode evolution.
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Strongly Correlated Electrons

Interplay of Kekulé bond order and lattice instability in $\mathrm{C}_6\mathrm{Li}$

Understanding the interplay between charge order and lattice instability in quantum materials remains a central challenge, as their coexistence often obscures causal relationships. This work introduces $\mathrm{C}_6\mathrm{Li}$ as a novel platform to investigate charge order mediated by two distinct mechanisms. We show that the hybridization between carbon $\pi$ and lithium $s$ orbitals generates an effective long-range hopping within Li-centered hexagons. This hopping drives a Kekulé bond order, whose structure varies with charge density and the sign of the hopping. This bond order induces a Kekulé lattice distortion via electron-phonon coupling. In the limit where lithium atoms are distant from the graphene layer, a Fermi surface nesting-driven Kekulé bond order emerges, stabilized by the electron-phonon interaction. Our results establish $\mathrm{C}_6\mathrm{Li}$ as a tunable platform for elucidating the causal hierarchy between electronic and structural orders in quantum materials.
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All authors Yuanhao Zhang, Zi Yuan, Xiangru Kong, Weijiang Gong, Shaozhi Li

Mesoscale and Nanoscale Physics

Atomic-scale probe of molecular magneto-electric coupling

Van der Waals heterostructures are a core tool in quantum material design. The recent addition of monolayer ferroelectrics expands the possibilities of designer materials. Ferroelectric domains can be manipulated using electric fields, thus opening a route for external control over material properties. In this paper we explore the possibility of engineering magneto-electric coupling in ferroelectric heterostructures by studying the interface of bilayer SnTe with iron phthalocyanine molecules as a model system. The molecules act as sensor spins, allowing us to sample the magneto-electric coupling with nanometer precision through scanning tunneling microscopy. Our measurements uncover a structural, and therefore material-independent and intrinsic, mechanism to couple electric and magnetic degrees of freedom at the nanoscale.
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All authors Mohammad Amini, Linghao Yan, Orlando J. Silveira, Adolfo O. Fumega, Viliam Vaňo, Jose L. Lado, Shawulienu Kezilebieke, Peter Liljeroth, and Robert Drost

Materials Science · Cross-listed from cs.LG

Materium: An Autoregressive Approach for Material Generation

We present Materium: an autoregressive transformer for generating crystal structures that converts 3D material representations into token sequences. These sequences include elements with oxidation states, fractional coordinates and lattice parameters. Unlike diffusion approaches, which refine atomic positions iteratively through many denoising steps, Materium places atoms at precise fractional coordinates, enabling fast, scalable generation. With this design, the model can be trained in a few hours on a single GPU and generate samples much faster on GPUs and CPUs than diffusion-based approaches. The model was trained and evaluated using multiple properties as conditions, including fundamental properties, such as density and space group, as well as more practical targets, such as band gap and magnetic density. In both single and combined conditions, the model performs consistently well, producing candidates that align with the requested inputs.
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Disordered Systems and Neural Networks · Cross-listed from physics.optics

Anomalous Wave-Packet Dynamics in One-Dimensional Non-Hermitian Lattices

Non-Hermitian (NH) systems have attracted great attention due to their exotic phenomena beyond Hermitian domains. Here we study the wave-packet dynamics in general one-dimensional NH lattices and uncover several unexpected phenomena. The group velocity of a wave packet during the time evolution in such NH lattices is not only governed by the real part of the band structure but also by its imaginary part. The momentum also evolves due to the imaginary part of the band structure, which can lead to a self-induced Bloch oscillation in the absence of external fields. Furthermore, we discover the wave-packet dynamics can exhibit disorder-free NH jumps even when the energy spectra are entirely real. Finally, we show that the NH jumps can lead to both positive and negative temporal Goos–Hänchen shifts at the edge.
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Quantum Gases · Cross-listed from nucl-th

Absence of charged pion condensation in a magnetic field with parallel rotation

We investigate the critical temperature of a relativistic Bose-Einstein condensate of charged bosons driven by rotation in a parallel magnetic field [Y. Liu and I. Zahed, Phys. Rev. Lett. 120, 032001 (2018)]. For non-interacting bosons, the critical temperature can only be determined for a system with fixed angular momentum. We find that the critical temperature of the non-interacting system vanishes due to the fact that the system is quasi-one-dimensional, indicating that non-interacting bosons cannot undergo Bose-Einstein condensation. For interacting bosons, we investigate a system with quartic self-interaction. We show that the order parameter vanishes and the off-diagonal long-range order is absent at any nonzero temperature because of the quasi-one-dimensional feature, in accordance with the Coleman-Mermin-Wagner-Hohenberg theorem.
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Materials Science

First principle study of electronic, magnetic and thermoelectric properties of Co$_2$YPb (Y = Tc, Ti, Zr and Hf) full Heusler: Application to embedded automotive systems

In this study, theoretical investigation on structural, electronic, magnetic, elastic and thermoelectric properties of the full Heusler Co$_2$YPb (Y = Tc, Ti, Zr and Hf) alloys have been performed within density functional theory (DFT). The exchange and correlation potential is addressed using two approximations: the generalized gradient approximation (GGA) and the GGA augmented by the Tran–Blaha-modified Becke-Johnson (mBj-GGA) approximation, which provides a more accurate description of the energy band gap. The electronic and magnetic properties reveal that the full-Heusler alloys Co$_2$YPb (with Y = Tc, Ti, Zr, and Hf) display half-metallic ferromagnetic behavior. Furthermore, the elastic properties suggest that Co$_2$YPb are mechanically stable, with ductile characteristics. Full Heusler alloys P-type exhibit positive Seebeck coefficients and high ZT values, indicating good thermoelectric performance in terms of electrical and thermal conductivity. This leads us to the conclusions that these compounds are very interesting in improving the performance of embedded automotive systems and can also be used in spintronic devices.
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All authors N. Saidi, A. Abbad, W. Benstaali, K. Bahnes

Strongly Correlated Electrons

On the Role of the Canonical Transformation in the Single-Channel Kondo Model

This pedagogical work presents the significant role that canonical transformation plays in the interpretation of the Abelian bosonized single-channel SU(2) Kondo model, emphasizing its effect on the scaling dimension $\Delta$. The transformation shifts the longitudinal exchange coupling and modifies the scaling dimension of the spin-flip vertex $\tau_{\pm} e^{\pm i\beta \phi}$. Rather than fixing $\Delta$ to the fermionic value $\tfrac{1}{2}$, we keep $\alpha$ explicit, which allows us to identify how different choices lead to marginal or relevant regimes through $(1-\Delta(\alpha))J_\perp$. This approach offers a direct way to trace the scaling behavior from the bosonized Hamiltonian and shows how the RG flow connects to the definition of the Kondo temperature, where the resistance diverges, without switching to other methods.
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