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Physics Condensed Matter

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Monday 13 October

Statistical Mechanics

Spreading fronts: numerical simulations on discrete models and continuous equations

Out-of-equilibrium systems, inherently complex and challenging to understand, are prevalent across various disciplines, including physics where they arise in contexts such as fluid dynamics. In particular, critical out-of-equilibrium systems combine this complexity with the scaling laws and universality classes observed in critical phenomena, with kinetic surface roughening, the study of how a flat surface becomes progressively rougher over time, serving as a prime example. This behavior manifests in a wide variety of contexts, including metal corrosion, cell proliferation, and, notably, the growth of thin films, which can emerge as a result of wetting processes. In this thesis, we conduct extensive numerical simulations to study critical fluctuations and identify universal features of several rough interfaces, generated by simulating discrete models of thin film growth and by performing direct numerical integration of continuum equations. To explore the universal behavior of these interfaces, we identify the critical exponents that characterize the spatio-temporal fluctuations of the front. Additionally, we analyze the dynamics of thin films across different physical scenarios to deepen our understanding of their behavior in out-of-equilibrium conditions, especially in the case where these films are formed by the action of an external force such as Surface Acoustic Waves.
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Materials Science · Cross-listed from quant-ph

Bright Single-Photon Emission from Individual Tin-Vacancy Centers in Multi-Cone Diamond Waveguides

Diamonds containing color centers have recently gathered significant attention for photonic quantum technologies, including quantum sensing, photonic quantum computers, and quantum networks. Among the various color centers, tin-vacancy (SnV) centers are particularly promising due to the high emission efficiency from the zero-phonon line and due to their long spin coherence times. However, the extraction of photons from diamond remains a key challenge. Here we demonstrate high photon extraction from a single SnV center incorporated in a diamond nanopillar with tapered sidewalls and a multi-cone structure. A sharp emission peak with a full width at half maximum (FWHM) of $6\,$nm was observed at a wavelength of $619\,$nm. Furthermore, the second-order correlation function exhibited an antibunching dip well below $g^{(2)}(0) = 0.5$, indicating single-photon emission. Remarkably, the emitter achieved a high saturation count rate of approximately $9\,$Mcps. These results establish our nanopillar platform as a promising candidate for bright and stable quantum sources and sensors based on SnV centers in diamond.
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All authors Pablo Tieben, Jan Rhensius, Takuya F. Segawa, Risei Abe, Konosuke Shimazaki, Shigeki Takeuchi, Andeas W. Schell, Hideaki Takashima

Materials Science · Cross-listed from cs.CV

A Large-Language-Model Assisted Automated Scale Bar Detection and Extraction Framework for Scanning Electron Microscopic Images

Microscopic characterizations, such as Scanning Electron Microscopy (SEM), are widely used in scientific research for visualizing and analyzing microstructures. Determining the scale bars is an important first step of accurate SEM analysis; however, currently, it mainly relies on manual operations, which is both time-consuming and prone to errors. To address this issue, we propose a multi-modal and automated scale bar detection and extraction framework that provides concurrent object detection, text detection and text recognition with a Large Language Model (LLM) agent. The proposed framework operates in four phases; i) Automatic Dataset Generation (Auto-DG) model to synthesize a diverse dataset of SEM images ensuring robust training and high generalizability of the model, ii) scale bar object detection, iii) information extraction using a hybrid Optical Character Recognition (OCR) system with DenseNet and Convolutional Recurrent Neural Network (CRNN) based algorithms, iv) an LLM agent to analyze and verify accuracy of the results. The proposed model demonstrates a strong performance in object detection and accurate localization with a precision of 100%, recall of 95.8%, and a mean Average Precision (mAP) of 99.2% at IoU=0.5 and 69.1% at IoU=0.5:0.95. The hybrid OCR system achieved 89% precision, 65% recall, and a 75% F1 score on the Auto-DG dataset, significantly outperforming several mainstream standalone engines, highlighting its reliability for scientific image analysis. The LLM is introduced as a reasoning engine as well as an intelligent assistant that suggests follow-up steps and verifies the results. This automated method powered by an LLM agent significantly enhances the efficiency and accuracy of scale bar detection and extraction in SEM images, providing a valuable tool for microscopic analysis and advancing the field of scientific imaging.
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All authors Yuxuan Chen, Ruotong Yang, Zhengyang Zhang, Mehreen Ahmed, Yanming Wang

Materials Science

Optimizing Cross-Domain Transfer for Universal Machine Learning Interatomic Potentials

Accurate yet transferable machine-learning interatomic potentials (MLIPs) are essential for accelerating materials and chemical discovery. However, most universal MLIPs overfit to narrow datasets or computational protocols, limiting their reliability across chemical and functional domains. We introduce a transferable multi-domain training strategy that jointly optimizes universal and task-specific parameters through selective regularization, coupled with a domain-bridging set (DBS) that aligns potential-energy surfaces across datasets. Systematic ablation experiments show that small DBS fractions (0.1%) and targeted regularization synergistically enhance out-of-distribution generalization while preserving in-domain fidelity. Trained on fifteen open databases spanning molecules, crystals, and surfaces, our model, SevenNet-Omni, achieves state-of-the-art cross-domain accuracy, including adsorption-energy errors below 0.06 eV on metallic surfaces and 0.1 eV on metal-organic frameworks. Despite containing only 0.5% r$^2$SCAN data, SevenNet-Omni reproduces high-fidelity r$^2$SCAN energetics, demonstrating effective cross-functional transfer from large PBE datasets. This framework offers a scalable route toward universal, transferable MLIPs that bridge quantum-mechanical fidelities and chemical domains.
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All authors Jaesun Kim, Jinmu You, Yutack Park, Yunsung Lim, Yujin Kang, Jisu Kim, Haekwan Jeon, Suyeon Ju, Deokgi Hong, Seung Yul Lee, Saerom Choi, Yongdeok Kim, Jae W. Lee, Seungwu Han

Mesoscale and Nanoscale Physics

Should it really be that hard to model the chirality induced spin selectivity effect?

The chirality induced spin selectivity effect remains a challenge to capture with theoretical modeling. While at least a decade was spent on independent electron models, which completely fail to reproduce the experimental results, the lesson to be drawn out of these efforts is that a correct modeling of the effect has to include interactions among the electrons. In the discussion of the phenomenon ones inevitably encounters the Onsager reciprocity and time-reversal symmetry, and questions whether the observations violate these fundamental concepts, or whether we have not been able to identify what it is that make those concepts redundant in this context. The experimental fact is that electrons spin-polarize by one or another reason, when traversing chiral molecules. The set-ups are simple enough to enable effective modeling, however, overcoming the grand failures of the theoretical efforts, thus far, and formulating a theory which is founded on microscopic modeling appears to be a challenge. A discussion of the importance of electron correlations is outlined, pointing to possible spontaneous breaking of time-reversal symmetry and Onsager reciprocity.
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Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

Tunable multi-photon correlations from a coherently driven quantum dot

Mixing the fields generated by different light sources has emerged as a powerful approach for engineering non-Gaussian quantum states. Understanding and controlling the resulting photon statistics is useful for emerging quantum technologies that are underpinned by interference. In this work, we investigate intensity correlation functions arising from the interference of resonance fluorescence from a quantum emitter with a coherent laser field. We show that the observed bunching behavior results from a subtle interplay between quantum interference and the normalization of the correlation functions. We show that by adjusting the mixing ratio and phase one can achieve full tunability of the second-order correlation, ranging from anti-bunching to bunching. We further extend our analysis to third-order correlation functions, both experimentally and theoretically, to provide new insights into the interpretation of higher-order correlations and offer practical tools for shaping quantum optical fields.
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All authors Thomas K. Bracht, Rachel N. Clark, Petros Androvitsaneas, Matthew Jordan, Samuel G. Bishop, Harry E. Dyte, Moritz Cygorek, Ian A. Farrer, Doris E. Reiter, Anthony J. Bennett

Strongly Correlated Electrons

Spinon band flattening by its emergent gauge field in quantum kagome ice

Fractional excitations provide a key to identifying sought-after topological quantum spin liquid states in realistic materials. Their single-particle dynamics already presents a challenging many-body problem on account of the coupling to their emergent gauge field. Here, we study the spinon excitations of kagome ice, realized at the $2/3$ magnetization plateau of spin ice, by combining up-to-$63$-site exact diagonalization with an analytical state graph mapping. We find a macroscopically degenerate mode in the spinon spectrum. It originates from the destructive interference due to the interaction with surrounding gauge fields, a form of many-body caging. We explicitly construct, and count, the concomitant many-body wave functions. Finally, we discuss the possible role of these flat modes in the magnetization process of kagome antiferromagnets, in particular with regard to the asymmetric termination of the kagome ice magnetisation plateau.
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Soft Condensed Matter

Thin-film flows of granular suspensions on a solid surface

This review article examines the complex dynamics of thin-film flows of granular suspensions spreading over rigid solid substrates with free air interfaces. Such systems feature an involved coupling of the free-surface dynamics with the flow and microstructure of the suspension. In particular, we develop two canonical thin-film situations: drop spreading and dip-coating. In drop spreading, confinement of the particulate phase near the advancing contact line alters both the spreading rate and the interface shape. In dip-coating, understanding the entrainment of fluid and particles becomes challenging as the film thickness approaches the particle size.
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Materials Science

In-plane polar domains enhanced energy storage

Relaxor ferroelectric thin films are recognized for their ultrahigh power density, rendering them highly promising for energy storage applications in electrical and electronic systems. However, achieving high energy storage performance with chemically homogeneous, environmentally friendly and compositionally stable materials remains challenging. In this work, we present a design of dielectrics with high energy storage performance via an in-plane polar domains incorporating polar nanoregions mechanism. Guided by phase-field simulations, we synthesized La/Si co-doping BaTiO3 solid-solution thin films with high chemical homogeneity to realize high energy storage performance. Given that, we achieve a high energy density of 203.7J/cm3 and an energy efficiency of approximately 80% at an electric field of 6.15MV/cm. This mechanism holds significant promise for the design of next-generation high-performance dielectric materials for energy storage and other advanced functional materials.
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All authors Yu Lei, Xiaoming Shi, Sihan Yan, Qinghua Zhang, Jiecheng Liu, Sixu Wang, Yu Chen, Jiaou Wang, He Qi, Qian Li, Ting Lin, Jingfen Li, Qing Zhu, Haoyu Wang, Jing Chen, Lincong Shu, Linkun Wang, Han Wu, Xianran Xing

Mesoscale and Nanoscale Physics

Local-Antisymmetric Flat Band and Coexisting Correlated stripe charge orders in WSe2-Modulated Twisted Bilayer Graphene

Insulating, atomically flat transition metal dichalcogenides (TMDs) like WSe2 are ideal substrates for probing intrinsic graphene properties. Conventionally, their influence on graphene's band structure is assumed negligible, particularly when small moire patterns form. Combining scanning tunneling microscopy/spectroscopy and theoretical analysis, we reveal that the atomic registry in graphene/WSe2 heterostructures profoundly modulates the electronic structure of magic-angle twisted bilayer graphene (MATBG). At special graphene/WSe2 twist angles, an incommensurate moire superlattice hosts three distinct atomic stacking configurations (A, B, X types). These induce position-dependent potentials that asymmetrically shift MATBG's flat bands, transforming them from hole-side to electron-side asymmetric within a single AA-stacked region. This symmetry breaking enables the unprecedented coexistence of orthogonal stripe charge orders in the correlated regime-a phenomenon previously considered mutually exclusive due to Coulomb repulsion. This band modulation arises from the synergistic effects of the graphene/WSe2 interfacial atomic registry and heterostrain within the MATBG, exhibiting multi-field tunability. Our work establishes interfacial atomic registry as a critical, previously overlooked tuning parameter for flat-band physics, opening avenues to engineer correlated quantum states in van der Waals heterostructures.
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All authors Chi Zhang, Shihao Zhang, Mengmeng Zhang, Lin He, Qi Zheng

Materials Science

Entropy Engineering-Regulated Electron-Phonon Coupling for Highly Efficient Photoluminescence in Se-doped WS2

The limited quantum yield of strained monolayer transition metal dichalcogenides grown by vapor-phase methods and during transfer-based stacking poses a fundamental challenge for their optoelectronic applications. Here, we introduce the concept of "entropy engineering" as a transformative strategy to selectively enhance light-matter interactions through controlled electron-phonon coupling. We unveil how tailored entropy introduced via precise selenium doping or interfacial van der Waals proximity can significantly amplify radiative recombination from momentum-dark excitons in WS2 monolayers. Notably, we discover that slight selenium doping drastically enhances the photoluminescence (PL) of WS2 under strain. While both undoped and heavily doped WS2 suffer from strong PL quenching owing to the direct-to-indirect bandgap transition, lightly Se-doped samples exhibit an order-of-magnitude increase in emission intensity. This counterintuitive boost is traced to doping-induced structural disorder, which intensifies electron-phonon interactions and unlocks efficient phonon-assisted emission from otherwise non-radiative indirect excitons. Moreover, we demonstrate that van der Waals coupling to adjacent Se-doped layers can impart interfacial entropy and further augment PL via proximity effects. Our work highlights entropy engineering via controlled doping as a powerful strategy for activating high-efficiency light emission in atomically thin semiconductors.
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All authors Chi Zhang, Quan Shen, Mengmeng Zhang, Zhiming Deng, Taishen Wu, Xuying Zhong, Gang Ouyang, Dongsheng Tang, Qi Zheng, Jiansheng Dong, Weichang Zhou

Materials Science

Frenkel anomaly on co-ordination numbers in liquid CO2 at 100 and 1000 bar studied by Monte Carlo simulation using Kihara potential model

An issue concerning the Frenkel line of liquid CO2 is that its location has not been unequivocally determined. So far, reliable Frenkel lines were identified from velocity autocorrelation functions (VAFs) computed by Molecular Dynamic simulations; however VAFs cannot be directly verified experimentally. By contrast, the co-ordination numbers (CNs) can be measured experimentally by X-ray and neutron scattering or computed by Monte Carlo (MC) simulation, and thus provide an alternative means of determining the location of the Frenkel line. In the present study, the CNs were computed by MC simulation using the Kihara potential, and the Frenkel anomalies were identified at {P = 100 bar, T = 260 K}, in good agreement with previous results based on VAFs, and at {P = 1000 bar, T = 370 K}, which deviates significantly from them.
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Strongly Correlated Electrons

Collinear, incommensurate antiferromagnetism in van der Waals magnet alpha-UTe3

alpha-UTe3, a van der Waals (vdW) actinide compound with a monoclinic ZrSe3-type structure, is a narrow-gap semiconductor with 5f moments. 125Te NMR reveals strongly anisotropic, layer-confined spin fluctuations below about 20 K, with the a-axis component enhanced, and a signal wipeout at the antiferromagnetic (AFM) transition at TN = 5 K. Single-crystal neutron diffraction finds q approx. (0.17, 0.5, 0) and a longitudinal sinusoidal modulation of a-axis moments (amplitude about 0.8 muB) with AFM stacking along b. A CEF singlet-singlet induced-moment framework accounts for the easy-axis anisotropy, the small heat-capacity anomaly at TN, the reduced ordered moment, and the exchange-driven selection of q in this localized 5f vdW magnet, establishing a constrained exchange geometry stabilizing this in-plane incommensurate state.
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All authors H. Sakai, C. Tabata, K. Kaneko, Y. Tokiwa, T. Kitazawa, S. Kambe, Y. Tokunaga, Y. Haga

Superconductivity · Cross-listed from physics.app-ph

Loss investigations of high frequency lithium niobate Lamb wave resonators at ultralow temperatures

Lamb wave resonators (LWRs) operating at ultralow temperatures serve as promising acoustic platforms for implementing microwave-optical transduction and radio frequency (RF) front-ends in aerospace communications because of the exceptional electromechanical coupling (k^2) and frequency scalability. However, the properties of LWRs at cryogenic temperatures have not been well understood yet. Herein, we experimentally investigate the temperature dependence of the quality factor and resonant frequency in higher order antisymmetric LWRs down to millikelvin temperatures. The high-frequency A1 and A3 mode resonators with spurious-free responses are comprehensively designed, fabricated, and characterized. The quality factors of A1 modes gradually increase upon cryogenic cooling and shows 4 times higher than the room temperature value, while A3 mode resonators exhibit a non-monotonic temperature dependence. Our findings provide new insights into loss mechanisms of cryogenic LWRs, paving the way to strong-coupling quantum acoustodynamics and next-generation satellite wireless communications.
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All authors Wenbing Jiang, Xuankai Xu, Jiazhen Pan, Hancong Sun, Yu Guo, Huabing Wang, Libing Zhou, Tao Wu

Superconductivity

Phase-sensitive evidence for pair density waves in a kagome superconductor

Pair density wave (PDW) exhibits periodic amplitude and sign modulations of the superconducting order parameter. Such a pairing state has long been proposed to be highly sensitive to nonmagnetic scattering, but its experimental realization remains elusive. Here we discover a nonmagnetic PDW-breaking effect in a kagome superconductor, using designer atomic nonmagnetic impurities and high-precision scanning tunneling microscopy (STM) at a base temperature of 30mK. We detect 2x2 pair density modulations by Josephson STM with a superconducting tip and 2x2 pairing gap modulations by normal STM. We find that the pairing modulations in both cases are substantially suppressed upon doping the kagome lattice with dilute isovalent nonmagnetic impurities, whereas the charge order and uniform superconductivity remain robust. We further identify the correlation between atomic dopants and the local suppression of PDW. We attribute these findings to a nonmagnetic pair-breaking effect, arising from the phase modulation of PDW in the kagome d-orbital. Taken together with its signatures in other state-of-the-art spectroscopy and transport measurements linked by theory, our findings support the ground state of the kagome superconductor as a correlated topological phase with superconducting loop currents.
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All authors Xiao-Yu Yan, Guowei Liu, Hanbin Deng, Xitong Xu, Haiyang Ma, Hailang Qin, Junyi Zhang, Yuanyuan Zhao, Xiuhao Fan, Wei Song, Muwei Gao, Haitian Zhao, Zhe Qu, Yigui Zhong, Kozo Okazaki, Xiquan Zheng, Yingying Peng, Zurab Guguchia, Xianxin Wu, Da Wang, Qiang-Hua Wang, Hendrik Hohmann, Matteo Dürrnagel, Ronny Thomale, Jia-Xin Yin

Soft Condensed Matter

Impact of elastic inhomogeneity on collective dynamical properties investigated by field theoretical description in real space

Interpreting the vibrational properties of amorphous solids beyond Debye's theory is challenging due to the presence of inhomogeneity on the mesoscopic scale. In this work, we model this inhomogeneity by real-space fluctuating elasticity with a spatially correlated distribution and calculate the dynamical properties using an exact real-space field theoretical approach. Our results clarify that the excess low-frequency density of states (DOS) originates from a selective scattering effect (stronger scattering of short wavelengths) induced by elastic inhomogeneity. The visualization of the local DOS in real space reveals the existence of anomalous modes, highly excited spots, at low frequencies. The findings regarding these highly excited spots and the selectivity of the correlation length were missed in previous perturbative field approaches in wave-vector space, and they align with recent progress from particle-level simulations and experiments. These results provide concrete insights into the low-frequency vibrational anomaly of amorphous solids from the perspective of simple elastic inhomogeneity.
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Materials Science

Generalized quantum limits of electrical contact resistance and thermal boundary resistance

The importance of electrical contact resistance and thermal boundary resistance has increased dramatically as devices are scaled to atomic limits. The use of a rich range of materials with various bandstructures (e.g. parabolic, conical), and in geometries exploiting various dimensionalities (e.g. 1D wires, 2D sheets, and 3D bulk) will increase in the future. Here we derive a single general expression for the quantum limit of electrical contact resistivity for various bandstructures and all dimensions. A corresponding result for the quantum limit of thermal boundary resistance is also derived. These results will be useful to quantitatively co-design, benchmark, and guide the lowering of electrical and thermal boundary resistances for energy efficient devices.
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All authors Alice Ho, Jashan Singhal, Deji Akinwande, Huili Grace Xing, Debdeep Jena

Materials Science

Delayed 1T to 2H Phase Transition Upon Electrochemical Delithiation of LiMoS2

Molybdenum disulfide (MoS2) is a widely studied layered material for electronic, optical, and catalytic applications. It can host lithium ions between the van der Waals layers, which triggers a phase transition between the semiconducting 2H phase and metallic 1T phase. While lithium insertion triggers a phase transition to the 1T phase, the phase behavior upon electrochemical lithium removal is not resolved. In this work, we conduct single-flake electrochemical (de)lithiation of MoS2 using microelectrode arrays. Through both electrochemical voltage analysis and correlative Raman spectroscopy, we show that an electrochemically cycled and delithiated MoS2 flake initially remains in the 1T phase. However, over the course of several days, it transitions back into the thermodynamically stable 2H phase. This result resolves the phase transformation pathway upon delithiation and showcases the ability to electrochemically synthesize the metastable 1T-MoS2 phase.
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All authors Yerin Hong, Juhwan Lim, Jinhong Min, Nishkarsh Agarwal, Robert Hovden, Ageeth A. Bol, Yiyang Li

Mesoscale and Nanoscale Physics

Two-dimensional flat-bands in Moire-diamonds

The discovery of flat-bands in magic-angle twisted bilayer graphene has underscored the potential of moire engineering for correlated states, but such phases are notoriously difficult to realize and highly fragile against perturbations. Here, we propose an alternative route to flat-bands by introducing sp3 hybridization in twisted graphite. Instead of relying on fine-tuned magic angles, our approach identifies flat-band states at relatively large twist angles with short moire periods. In this regime, sp3-induced reconstructions generate electronic states that, once formed, are locked by substantial energy barriers, rendering them robust against external perturbations. Using twisted graphite as a prototype, we uncover a series moire-diamond that host two-dimensional flat conduction of valence bands, where carriers are localized within specific momentum planes but remain dispersive along orthogonal directions. The emergence of dimensional flat-bands opens a new platform for flat-band-driven correlated physics and suggests opportunities for designing quantum materials with highly directional electronic functionalities.
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All authors Yalan Wei, Shifang Li, Yuke Song, Chaoyu He

Superconductivity

Possible Spatial Correlation of Superconducting and Pseudogap Dynamics in a Bi-based Cuprate

Understanding the interplay between superconductivity and the pseudogap phase is essential for elucidating the mechanism of high-temperature superconductivity in cuprates. Here we provide direct spatial evidence that these two states are locally and intrinsically correlated. Using spatially and temporally resolved measurements of photoinduced quasiparticle dynamics in optimally doped Bi$_2$Sr$_{1.7}$La$_{0.3}$CuO$_{6+\delta}$ (La-Bi2201), we reveal micrometer-scale spatial contrasts in the transient reflectivity that arise from local variations in the threshold fluence required to disrupt either the superconducting or pseudogap state. The superconducting response remains spatially uniform, whereas the pseudogap exhibits intrinsic inhomogeneity, yet the spatial variations of their threshold fluences closely track each other, establishing a robust local correlation between the two. These results introduce a bulk-sensitive ultrafast optical methodology for visualizing hidden spatial correlations in correlated materials and provide new benchmarks for understanding the intertwined phases in cuprates.
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All authors T. Shimizu, T. Kurosawa, S. Tsuchiya, R. Tobise, K. Yamane, R. Morita, M. Oda, Y. Toda

Mesoscale and Nanoscale Physics · Cross-listed from math.AP

Hydrodynamics of degenerate Fermi gases on spherical Fermi surfaces

We consider the description of a Fermi gas of free electrons given by the Boltzmann–Fermi–Dirac equation, and aim at providing a precise mathematical understanding of the Fermi ground state and its first-order approximation of excited states on the Fermi sphere. In order to achieve that, using the framework of hydrodynamic limits in collisional kinetic theory, we identify the low-temperature regimes in which charge-density fluctuations concentrate on the Fermi sphere. In three spatial dimensions or higher, we also characterize the thermodynamic equilibra and energy spectra of fluctuations. This allows us to derive the macroscopic hydrodynamic equations describing how charge densities flow and propagate in metals, thereby providing a precise description of plasma oscillations in conductors. The two-dimensional case is fundamentally different and is handled in a companion article. Remarkably, our results establish that excited electrons and their energy can be distributed on the Fermi sphere anisotropically, which deviates from the common intuitive assumption that electrons and their energy should be distributed uniformly in all directions. The hydrodynamic regimes featured in this work are akin to the acoustic limit of the classical Boltzmann equation. However, we emphasize that our derivation holds for arbitrarily fast rates of convergence of the Knudsen number, which significantly extends the applicability of the known proofs of the classical acoustic limit. This suggest that low-temperature limits of Fermi gases provide a promising avenue of research toward a complete understanding of the compressible Euler limit.
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Superconductivity

Magnetic Field-Enhanced Graphene Superconductivity with Record Pauli-Limit Violation

Spin-polarized superconductors offer a rare platform for studying electronic correlations, but few candidate systems have been experimentally confirmed to date. Here, we report the observation of a spin-polarized superconducting state, denoted SC5, in WSe2-proximitized rhombohedral trilayer graphene. At in-plane magnetic field B|| = 0 T, SC5 has a critical temperature of 68 mK and an out-of-plane critical magnetic field of only 12 mT. Surprisingly, these values are significantly enhanced as B|| increases, and the superconductivity persists to B|| = 8.8 T. This value corresponds to a record-high Pauli-limit violation ratio of at least 80 among all superconductors, while the true critical field is beyond the limit of our instrument. We conclude that SC5 experiences a canting crossover from Ising-type to spin-polarized superconductor with increased B||.
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All authors Jixiang Yang, Omid Sharifi Sedeh, Chiho Yoon, Shenyong Ye, Henok Weldeyesus, Armel Cotten, Tonghang Han, Zhengguang Lu, Zach Hadjri, Junseok Seo, Lihan Shi, Emily Aitken, Prayoga P Liong, Zhenghan Wu, Mingchi Xu, Christian Scheller, Mingyang Zheng, Rasul Gazizulin, Kenji Watanabe, Takashi Taniguchi, Dominique Laroche, Mingda Li, Fan Zhang, Dominik M. Zumbühl, Long Ju

Sunday 12 October

Mesoscale and Nanoscale Physics

Quantifying Charge Noise Sources in Quantum Dot Spin Qubits via Impedance Spectroscopy, DLTS, and C-V Analysis

The coherence and fidelity of quantum dot (QD) spin qubits are fundamentally limited by charge noise arising from electrically active trap states at oxide interfaces, heterostructure boundaries, and within the bulk semiconductor. These traps introduce electrostatic fluctuations that couple to the qubit via spin-orbit interactions or charge-sensitive confinement potentials, leading to dephasing and gate errors. In this work, we present a general trap characterization framework for identifying and quantifying the spectral signatures of these trap states using AC impedance spectroscopy, deep-level transient spectroscopy (DLTS), and conventional capacitance-voltage (C-V) analysis. While our case study focuses on strained Ge/SiGe quantum well heterostructures, the approach is broadly applicable to other material systems and qubit types. We demonstrate that each class of traps (oxide interface, quantum well interface, and bulk) exhibits distinct fingerprints across frequency- and time-domain measurements. Oxide traps dominate the low-frequency conductance peaks and appear strongly in Nyquist and transient spectra. QW interface traps, despite being nearly invisible at low densities in conventional C-V and AC impedance analysis, are clearly resolved through multi-exponential decay signatures in time-domain response. Bulk traps contribute to high-frequency admittance and steady-state leakage currents. By correlating each trap type to its characteristic time constant, spatial location, and spectral impact, we provide a diagnostic toolset for disentangling noise sources that degrade qubit performance. This unified methodology bridges traditional defect metrology with emerging qubit noise analysis and enables material- and process-level strategies for coherence optimization in scalable quantum devices.
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Disordered Systems and Neural Networks · Cross-listed from quant-ph

Rigorous estimation of error thresholds of transversal Clifford logical circuits

The threshold theorem promises a path to fault-tolerant quantum computation, provided the physical error rate is below a critical threshold. While transversal gates efficiently implement logical operations, they propagate errors and can lower this threshold relative to a static quantum memory. In this work, we generalize the statistical-mechanical (stat-mech) mapping from quantum memories to logical circuits with transversal gates, thereby enabling rigorous, decoder-independent thresholds for fault-tolerant logical computation. We first demonstrate the framework for two toric code blocks undergoing a transversal CNOT (tCNOT) gate, quantifying two independent error-spreading mechanisms. For persistent bit-flip errors with perfect syndromes, the stat-mech model is a 2D random Ashkin-Teller model. Monte Carlo simulation and finite-size scaling show that the tCNOT reduces the optimal bit-flip threshold to $p=0.080$, a $26\%$ decrease from the toric code memory threshold $p=0.109$. With syndrome errors included, the circuit maps to a 3D random 4-body Ising model with a plane defect, yielding a conservative estimate $p\geq 0.028$, a modest $15\%$ reduction from the memory threshold $p=0.033$. Beyond the tCNOT gate, we derive stat-mech models for all transversal Clifford gates of the toric code, including the fold-transversal Hadamard and $S$ gates, and generalize the framework to arbitrary CSS codes, proving that each transversal gate modifies the stat-mech model only locally in time. By reducing threshold analysis of fault-tolerant logical circuits to the study of classical spin models with local defects, our framework provides a systematic, decoder-independent benchmark for near-term fault-tolerant architectures.
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All authors Yichen Xu, Yiqing Zhou, James P. Sethna, Eun-Ah Kim

Materials Science

Emerging Ferroelectric Domains: Stacking and Rotational Landscape of MoS2 Moire Bilayers

The structures and properties of moire patterns in twisted bilayers of two-dimensional (2D) materials are known to depend sensitively on twist angle, yet their dependence on stacking order remains comparatively underexplored. In this study, we use molecular dynamics simulations to systematically investigate the combined effects of stacking order and rotation in MoS2 bilayers. Beginning from five well-established high-symmetry bilayer stackings, we apply twist angles between 1 and 120 to the top layer, revealing a variety of relaxed moire structures. Our results show that the initial stacking significantly influences the moire domain configurations that emerge at a given twist angle. While all five stacking orders are metastable without twist, they form two moire-equivalent classes- AA/AB and AA',A'B,AB', i.e., for a given twist angle, structures within each class relax to the same moire configuration. Specifically, initial AA and AB stackings give rise to triangular ferroelectric domains near 0+/-3, while AA', A'B, and AB' stackings produce triangular ferroelectric domains near 60+/-3. At precisely 60 and 120 twists, the bilayers relax to into pure high-symmetry stackings, highlighting the rotational relationships between these configurations and explaining the shift of 60 in the ferroelectric rotational range. These findings demonstrate the critical role of stacking order in governing the rich moire landscapes accessible in twistronic systems.
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All authors Anikeya Aditya, Ayu Irie, Nabankur Dasgupta, Rajiv K. Kalia, Aiichiro Nakano, Priya Vashishta

Materials Science · Cross-listed from astro-ph.EP

On the discovery of meteoritic mineral Zolenskyite; The artificial origin should not be overlooked

Recently a new meteoritic mineral, Zolenskyite (Fe0.99Mn0.04Ca0.01Cr1.99S3.98), was discovered from the Indarch meteorite. Zolenskyite was structurally indexed as the monoclinic C2/m CrNb2Se4 - Cr3S4 type structure of synthetic FeCr2S4, with unit cell parameters a = 12.84(1) Å, b = 3.44(1) Å, c = 5.94(1) Å and e̱ta} = 117(1){\deg}. Zolenskyite was reported as high-pressure phase formed from Daubréelite at high pressures and temperatures in highly shocked regions of the EH parent asteroid. Although this discovery provides valuable information about the origin of meteoritic mineral assemblages, the results and conclusions raise controversies with those reported in previous articles where the synthetic FeCr2S4 was described. In this review, an alternative analysis of the supplementary X-ray data from Zolenskyite was made and yields to the monoclinic I2/m Cr3S4 type structure of synthetic FeCr2S4, with unit cell parameters a = 5.940 Å, b = 3.440 Å, c = 11.441 Å and e̱ta} = 90.55{\deg}, in agreement with previous results in the literature and differ from those reported above. Regarding the genesis of Zolenskyite and according to solid-state laboratory synthesis, the transformation of cubic FeCr2S4 phase (ideal composition of Daubréelite) to monoclinic FeCr2S4 (ideal composition of Zolenskyite) requires a process whose replication in Shock metamorphism stages is not well established and remains an open issue to address, together with another open issue related to the real composition of meteoritic minerals, with minor and trace metals, which is often overlooked when compared with synthetic ideal compositions. Whatever the results to be obtained by addressing the above open issues, they will shed more light on the genesis of Zolenskyite. In this context, it is worth to promote an open debate about the hypothesis of artificial origin.
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Materials Science

Electron-hole liquid in biological tissues under ultra high dose rate ionizing radiation

We develop a quantitative model of ionization processes in biological tissues under Ultra High Dose Rate (UHDR) radiation. The underlying conjecture is that of electron-hole liquid (EHL) forming in water based substances of biological tissues. Unlike the earlier known EHL in semiconductor crystals, the charge carriers here are low mobile due to strong interactions with the background (solvated electrons, etc.); hence, EHL resembling ionic melts. Similar to all ionic systems, the Coulomb coupling makes that EHL energetically favorable that leads to recombination barriers suppressing subsequent structural transformations. In particular, generation of secondary reactive species in such EHL becomes limited translating into reduction of biological damages and tissue sparing effect. We show how these processes are sensitive to the tissue quality and frequency dispersion of the dielectric permittivity. Equations for dose and dose rate defining the sparing thresholds are derived.
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Disordered Systems and Neural Networks

Spectral properties of a Non-Hermitian extension of the diluted Wishart ensemble

We develop a theoretical framework based on the cavity and replica methods to analyze the spectral properties of sparse asymmetric correlation matrices of the form $\boldsymbol{F} = (\boldsymbol{X}\boldsymbol{Y}^\top + \omega \boldsymbol{Y}\boldsymbol{X}^\top)/2T$, where $\boldsymbol{X}$ and $\boldsymbol{Y}$ are adjacency matrices of weighted Erdős–Rényi random graphs. We examine how the spectral density evolves as the asymmetry parameter $\omega$ varies from $0 < \omega < 1$ (nearly symmetric matrices) to $-1 < \omega \le 0$ (nearly antisymmetric matrices). Analytical predictions are validated through exact numerical diagonalization, showing excellent agreement with theoretical results in the thermodynamic limit.
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Soft Condensed Matter

Fluidity and morphological stability of an amorphous thin film with radiation-induced defect kinetics

It is common to model ion-irradiated amorphous thin films as if they were highly viscous fluids. In such models, one is frequently concerned with the ion-enhanced fluidity, a measure of the ability of the free interface to relax surface energy. Motivated by usual fluid dynamics problems, the ion-enhanced fluidity is near-universally treated as a constant throughout the amorphous layer. However, for an irradiated thin film, the fluidity is ultimately caused by radiation-induced defect kinetics within the film, leading to regions with greater or lesser fluidity, and sensitive dependence on ion energy, species, flux, irradiation angle, temperature, and other experimental parameters. Here, we develop and analyze a model of radiation-induced defect kinetics coupled to the continuum equations of a viscous thin film. Using realistic parameter values, we show that defect kinetics can meaningfully alter theoretical predictions of surface relaxation and ion-enhanced fluidity. Implications for aligning theoretical and experimental work, especially for surface nano-patterning of silicon induced by low-energy argon irradiation, are discussed.
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Materials Science

Unveiling the growth mode diagram of GaSe on sapphire

The growth of two-dimensional epitaxial materials on industrially relevant substrates is critical for enabling their scalable synthesis and integration into next-generation technologies. Here we present a comprehensive study of the molecular beam epitaxial growth of gallium selenide on 2-inch c-plane sapphire substrates. Using in-situ reflection high-energy electron diffraction (RHEED), in-situ Raman spectroscopy, optical and scanning electron microscopies, we construct a diagram of the gallium selenide growth modes as a function of substrate temperature (530-650 {\deg}C) and Se/Ga flux ratio (5-110). The growth mode diagram reveals distinct regimes, including the growth of layered post-transition metal monochalcogenide GaSe with an unstrained in-plane lattice constant of 0.371$\pm$0.001 nm and a partial epitaxial alignment on sapphire. This work demonstrates a RHEED-based pathway for synthesizing gallium selenide of specific phase and morphology, and the construction of a phase diagram for high vapor pressure III-VI compounds that can be applied to a wide range of other metal chalcogenide materials.
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All authors M. Bissolo, M. Dembecki, J. Belz, J. Schabesberger, M. Bergmann, P. Avdienko, F. Rauscher, A. S. Ulhe, H. Riedl, K. Volz, J. J. Finley, E. Zallo, G. Koblmüller