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Physics Condensed Matter

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Friday 3 October

Strongly Correlated Electrons

Bimagnon dispersion of La2CuO4 probed by resonant inelastic X-ray scattering

We report on the study of the magnetic excitations of Mott insulator La2CuO4 by using resonant inelastic x-ray scattering (RIXS) and cluster calculations within the framework of exact diagonalization. Our results demonstrate experimentally that the bimagnon excitation in Cu L-edge RIXS is enhanced if the incident x-ray energy is slightly above the absorption edge. Through incident-energy-dependent momentum-resolved RIXS, we investigated the excitation of the bimagnon with predominantly A1 symmetry. The bimagnons of La2CuO4 exhibit a nearly flat dispersion with momentum along the Cu-O bond direction. This observation agrees with the bimagnon dispersion from the calculations on a single-band Hubbard model rather than a Heisenberg model with only the nearest neighbor exchange interaction. This means that the effect of the higher-order spin couplings such as the cyclic or ring exchange interactions caused by the coherent motion of electrons beyond nearest-neighbor sites is important for understanding the bimagnon dynamics of cuprates.
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All authors A. Singh, H. Y. Huang, K. Tsutsui, T. Tohyama, S. Komiya, J. Okamoto, C. T. Chen, A. Fujimori, D. J. Huang

Other Condensed Matter · Cross-listed from quant-ph

Dynamics of Quantum Entanglement Between Photon and Phonon Modes in a Coulomb-coupled Optomechanical Cavity Magnonic Systems

Quantum entanglement is a fundamental phenomenon in quantum information science and a crucial resource for quantum technologies such as precision sensing, secure communication, and computation. In hybrid cavity magno-optomechanical systems, entanglement among cavity photons, magnons, and phonons enables manipulation of quantum states across different modes via radiation pressure-based light-matter interaction. We propose a hybrid optomechanical cavity-magnonic setup with Yttrium iron garnet (YIG) sphere allowing magnons to couple with photons via magnetic-dipole interaction. The system also uses optomechanical and electrostatic interactions to entangle cavity photons and mechanical resonators. We focus on how the magnon nonlinear Kerr effect and varying coupling strengths influence entanglement dynamics. By analysing nonlinear effects alongside other coupling parameters, we identify optimal conditions for initiating and sustaining robust entanglement between the motional modes (phonons) of two Coulomb-coupled mechanical resonators. Our model predicts that adding Coulomb interaction and magnon coupling enhances the degree and tunability of entanglement, making it more resilient to thermal baths at 3 K. This study addresses how to optimize and sustain phonon-phonon entanglement in complex hybrid quantum systems. These findings offer insights relevant to developing quantum memories for continuous variable quantum information processing and other quantum technologies.
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Strongly Correlated Electrons

Spectroscopic evidence of Kondo resonance in 3$d$ van der Waals ferromagnets

Two-dimensional van der Waals (vdW) ferromagnets drive the advancement in spintronic applications and enable the exploration of exotic magnetism in low-dimensional systems. The entanglement of dual $-$ localized and itinerant $-$ nature of electrons lies at the heart of the correlated electron systems giving rise to exotic ground state properties such as complex magnetism, heavy fermionic behavior, Kondo lattice formation, etc. Through temperature-dependent electronic structure of vdW ferromagnets, (Co$_{x}$Fe$_{1-x}$)$_{3}$GeTe$_{2}$, probed using high-resolution photoemission spectroscopy and density functional theory combined with dynamical mean field theory (DFT+DMFT), we provide direct evidence of the emergence of Kondo resonance peak driven by complex interplay between localized and itinerant electrons. In overall agreement with experimental electronic structure and magnetic properties, DFT+DMFT also reveals finite spin band splitting well beyond $T_{C}$. Core levels, valence band photoemission spectra together with DFT+DMFT spectral functions reveal insignificant change across $T_{C}$ indicating non-Stoner magnetism in (Co$_{x}$Fe$_{1-x}$)$_{3}$GeTe$_{2}$. Our results provide a way forward to the understanding of complex interplay between electronic structure, exotic magnetism and heavy fermionic behavior leading to Kondo scenerio in 3$d$ vdW ferromagnets.
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All authors Deepali Sharma, Neeraj Bhatt, Asif Ali, Rajeswari Roy Chowdhury, Chandan Patra, Ravi Prakash Singh, Ravi Shankar Singh

Mesoscale and Nanoscale Physics

Weak localization and antilocalization corrections to nonlinear transport: a semiclassical Boltzmann treatment

The nonlinear transport regime is manifested in the nonlinear current-voltage characteristic of the system. An example of such a nonlinear regime is a setup in which current is injected into the sample and the measured voltage drop is quadratic in the injected current. Such a quadratic nonlinear regime requires inversion symmetry to be broken. This is the same symmetry condition as one needs to observe weak antilocalization, which can be prominent in two-dimensional systems. Here, we study the effects of weak (anti)localization on second-order nonlinear transport in two-dimensional systems using the semiclassical Boltzmann approach. We solve for quasiparticle distribution function up to the second order in the applied external electric field and calculate linear and nonlinear conductivity tensors for a toy model. We find that localization effects could lead to a sign change of the nonlinear conductivity tensor – a phenomenon observed in transition metal dichalcogenide and in single-layer graphene devices.
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Materials Science

Kolmogorov-Arnold Networks in Thermoelectric Materials Design

The discovery of high-performance thermoelectric materials requires models that are both accurate and interpretable. Traditional machine learning approaches, while effective at property prediction, often act as black boxes and provide limited physical insight. In this work, we introduce Kolmogorov–Arnold Networks (KANs) for the prediction of thermoelectric properties, focusing on the Seebeck coefficient and band gap. Compared to multilayer perceptrons (MLPs), KANs achieve comparable predictive accuracy while offering explicit symbolic representations of structure–property relationships. This dual capability enables both reliable predictions and the extraction of physically meaningful functional forms. Benchmarking against literature models further highlights the robustness and generalisability of the approach. Our findings demonstrate that KANs provide a powerful framework for reverse engineering materials with targeted thermoelectric properties, bridging the gap between predictive performance and scientific interpretability.
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All authors Marco Fronzi, Michael J. Ford, Kamal Singh Nayal, Olexandr Isayev, Catherine Stampfl

Mesoscale and Nanoscale Physics

Quantum geometric map of magnetotransport

We propose a quantum geometric map for the magnetononlinear Hall effect (MNHE), the planar Hall effect (PHE), and the ordinary Hall effect (OHE). These magnetotransport phenomena originate from the bilinear charge current of Bloch electrons in electromagnetic fields, incorporating both spin Zeeman coupling and orbital minimal coupling to the applied magnetic field. Benchmarked against Onsager reciprocity, we demonstrate that the spin- and orbital-induced MNHEs are governed by the time-reversal-even Zeeman quantum metric dipole and conventional quantum metric quadrupole, respectively; the spin- and orbital-induced PHEs are dominated by the time-reversal-odd Zeeman Berry curvature dipole and conventional Berry curvature quadrupole, respectively. We further show that the OHE contains an interband contribution that is related to the quantum metric quadrupole, contrary to conventional wisdom. Navigated by this map, we study the previously unexplored spin-induced PHE in the surface Dirac cone of topological insulators, where we uncover a step-like PHE. Our work offers a unified quantum geometric framework for understanding magnetotransport experiments.
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All authors Longjun Xiang, Jinxiong Jia, Fuming Xu, Jian Wang

Mesoscale and Nanoscale Physics

Ginzburg-Landau theory of spin pumping through an antiferromagnetic layer near the Néel temperature

Spin pumping is a microwave-driven means for injecting spins from a ferromagnet into the adjacent target material. The insertion of a thin antiferromagnetic layer between the ferromagnet and the target material is known to enhance the spin pumping signal. Here, in view of describing dynamic fluctuations of the Néel order parameter, we develop Ginzburg-Landau theory of the spin pumping in a ferromagnet/antiferromagnet/heavy metal trilayer in the vicinity of the antiferromagnetic Néel temperature $T_{\rm N}$. When there exists an interfacial exchange interaction between the ferromagnetic spins and the antiferromagnetic Néel order parameter at the ferromagnet/antiferromagnet interface, we find a strongly frequency-dependent enhancement of the pumped spin current that is peaked at $T_{\rm N}$. The present finding offers an explanation for the enhanced spin pumping with strong frequency dependence observed in a Y$_3$Fe$_5$O$_{12}$/CoO/Pt system.
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All authors Yuto Furutani, Hayato Fukushima, Yutaka Yamamoto, Masanori Ichioka, Hiroto Adachi

Thursday 2 October

Materials Science · Cross-listed from physics.app-ph

Impact of Switching Layer Architecture on Power Consumption in RRAM

This work demonstrates that porous helical WOx architectures enable a distinct low-power regime for planar ITO/WOx/ITO resistive random-access devices. While thin film and helical devices behave similarly at a 5 mA compliance, only helical devices sustain reproducible operation at 500 uA, where RESET voltages reduce by ~60%, switching currents decrease by 68-75%, and SET/RESET power drops by ~89% and ~83%. With helical devices operating at 500 uA, the memory window expands 400-600% due to selective suppression of high-resistive-state leakage, yielding both lower-power and improved read margin in a regime inaccessible to thin film devices. These results highlight geometry-driven field enhancement and confinement as practical design principles for low-power, high-margin resistive memories and point toward opportunities in transparent, flexible, and high-surface-area material systems.
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All authors John F. Hardy II, Jack A. Garrard, Guilherme S.Y. Giardini, Carlo R. daCunha

Mesoscale and Nanoscale Physics · Cross-listed from physics.optics

Frequency multiplication in Terahertz band using AlGaN/GaN plasmonic crystals

The plasma oscillations in high-mobility field-effect transistors (HEMTs) have emerged as a key physical mechanism for manipulating electromagnetic radiation in the sub-terahertz (sub-THz) and THz frequency ranges. These collective electron excitations can be excited and tuned electrically offering a compelling route to compact, integrable components for a wide range of next-generation technologies, including sixth-generation (6G) wireless networks, high-resolution biomedical and chemical spectroscopy, industrial process monitoring, and advanced security and defense systems. For these applications, plasmonic crystals – periodic arrays of many strongly coupled FET channels – are particularly promising. In this work, we report on a new class of collective excitations in plasmonic crystals termed rotonic plasmons, which arise at plasmonic mode crossings and exhibit a parabolic dispersion law reminiscent of soft-mode and roton-like spectra. We show that uniform gate modulation across plasmonic crystal unit cells induces periodic variations in the sheet carrier concentration and, consequently, in the plasma frequency. This time-periodic modulation drives nonlinear plasmonic parametric resonances enabling RF-to-THz conversion. By solving the generalized Mathieu equation with damping, we demonstrate that high-amplitude gate pumping enables frequency multiplication and, at cryogenic temperatures (77K) leads to parametric instabilities due to enhanced electron mobility. In plasmonic crystals with lower mobility, RF-to-THz conversion can instead be realized via periodic short-pulse excitation, a regime we introduce as Time-Domain Frequency Multiplication (TDFM). Investigation of AlGaN/GaN low-high plasmonic crystals confirm their potential as tunable, compact THz sources.
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Materials Science

Incorporating Si into Sb2Se3: Tailoring Optical Phase Change Materials via Nanocomposites

Chalcogenide-based optical phase change materials (OPCMs) exhibit a large contrast in refractive index when reversibly switched between their stable amorphous and crystalline states. OPCMs have rapidly gained attention due to their versatility as nonvolatile amplitude or phase modulators in various photonic devices. However, open challenges remain, such as achieving reliable response and transparency spanning into the visible spectrum, a combination of properties in which current broadband OPCMs (e.g., Ge2Sb2Se4Te1, Sb2Se3, or Sb2S3) fall short. Discovering novel materials or engineering existing ones is, therefore, crucial in extending the application scope of OPCMs. Here, we use magnetron co-sputtering to study the effects of Si doping into Sb2Se3. We employ ellipsometry, X-ray diffraction, Raman spectroscopy, and scanning and transmission electron microscopy to investigate the effects of Si doping on the optical properties and crystal structure and compare these results with those from first principles calculations. Moreover, we study the crystallization and melt-quenching of thin films via nano-differential scanning calorimetry (NanoDSC). Our experiments demonstrate that 20% Si doping increases the transparency window in both states, specifically to 800 nm (1.55 eV) in the amorphous phase, while reducing power consumption by lowering the melting temperature. However, this reduction comes at the cost of reducing the refractive index contrast between states and slowing the kinetics of the phase transition.
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All authors Chih-Yu Lee, Yi-Siou Huang, Felix Adams, Chuanyu Lian, Hongyi Sun, Jie Zhao, Zichao Ye, Nathan Youngblood, Juejun Hu, Leslie H Allen, Yifei Mo, Ichiro Takeuchi, Carlos A Rios Ocampo

Materials Science · Cross-listed from cs.LG

High Cycle S-N curve prediction for Al 7075-T6 alloy using Recurrent Neural Networks (RNNs)

Aluminum is a widely used alloy, which is susceptible to fatigue failure. Characterizing fatigue performance for materials is extremely time and cost demanding, especially for high cycle data. To help mitigate this, a transfer learning based framework has been developed using Long short-term memory networks (LSTMs) in which a source LSTM model is trained based on pure axial fatigue data for Aluminum 7075-T6 alloy which is then transferred to predict high cycle torsional S-N curves. The framework was able to accurately predict Al torsional S-N curves for a much higher cycle range. It is the belief that this framework will help to drastically mitigate the cost of gathering fatigue characteristics for different materials and help prioritize tests with better cost and time constraints.
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Mesoscale and Nanoscale Physics

Electron-beam-induced Contactless Manipulation of Interlayer Twist in van der Waals Heterostructures

The ability to dynamically control the relative orientation of layers in two dimensional (2D) van der Waals (vdW) heterostructures represents a critical step toward the realization of reconfigurable nanoscale devices. Existing actuation methods often rely on mechanical contact, complex architectures, or extreme operating conditions, which limit their applicability and scalability. In this work, we present a proof-of-concept demonstration of contactless electrostatic actuation based on electron-beam-induced charge injection. By locally charging an insulating hexagonal boron nitride (hBN) flake on an electrically grounded graphene layer, we create an interfacial electric field that generates in-plane electrostatic torque and induces angular displacement. We validate the induced rotation through in-situ scanning electron microscopy (SEM) and twist-dependent Raman spectroscopy.
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All authors Nicola Curreli, Tero S. Kulmala, Riya Sebait, Nicolò Petrini, Matteo Bruno Lodi, Roman Furrer, Alessandro Fanti, Michel Calame, Ilka Kriegel

Materials Science · Cross-listed from physics.chem-ph

Assessing the impact of contact time on leachate chemistry from recycled concrete aggregates

Recycled concrete aggregate (RCA) is recognized as a readily available, mechanically sufficient construction and demolition waste product that is suitable as a base course substitute for natural, virgin aggregate in pavement construction. Environmentally responsible applications of RCA must consider the high alkalinity, high pH leachate, and heavy metal leaching risks reported in the literature. The existing body of literature does not address discrepancies between field and laboratory measurements of RCA leachate pH, nor are there any existing studies of aged RCA leachate composition as a function of time. To consider the influence of contact time on RCA leachate, the present study evaluates recovered RCA base course samples from the Minnesota Road Research highway construction study site using modified batch test methodology. Leachate pH, alkalinity, and calcium ion (Ca2+) concentration were monitored for 24 hours to understand RCA leachate chemistry during the initial contact period. Leachate pH is high upon initial contact with water (pH > 10) and decreases over time as it reacts with atmospheric carbon dioxide. Calcium ion concentration increases rapidly in the initial contact period, then more gradually as calcium saturation is reached. Alkalinity stabilizes (50-65 mg CaCO3/L) after a dramatic increase during the initial contact period.
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All authors Morgan D. Sanger, Gabrielle Campagnola, Robin Ritchey, Tuncer B. Edil, Matthew Ginder-Vogel

Statistical Mechanics · Cross-listed from physics.soc-ph

From motifs to Lévy flights: Modeling urban mobility in Bogotá's public transport system

In this paper, we study two years of access card validation records from Bogotá's multimodal public transport system, comprising over 2.3 billion trips across bus rapid transit, feeder buses, dual-service buses, and an aerial cable network. From user trajectories constructed exclusively from access records, we derive motifs that reveal recurrent mobility patterns extending beyond simple two-location visits. This approach enables the construction of an integrated origin-destination (OD) matrix covering 2,828 urban zones. Similarity analysis using the Jensen-Shannon divergence confirms the temporal stability of mobility structures across semesters, despite infrastructure changes and fare policy adjustments. From the obtained OD matrices, we derive transition probabilities between zones and uncover a robust power-law relationship with geographical distance, consistent with Lévy flight dynamics. We validate our model using Monte Carlo simulations showing that reproduces both local and long-range displacements, with similar scaling exponents across time. These findings demonstrate that Bogotá's public transport mobility can be effectively modeled through Lévy processes, providing a novel framework for analyzing complex transportation systems based solely on user access records.
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Materials Science

Improper-proper ferroelectric competition as a mechanism for multistate polarisation and ferrielectric-like behaviour

In this paper, we re-explore a simple textbook Landau model describing improper ferroelectricity and show that in the limit where both proper and improper instabilities exist and compete, improper ferroelectrics can display switching between multiple polarisation states. Using first principles calculations we highlight how the hexagonal tungsten bronze materials may be an archetypal case, with the possibility to switch between improper and proper phases. The resulting functional characteristics are akin to "ferrielectrics", with switching behaviour in the form of a triple hysteresis loop. Such functionality could be ideal for creating non-volatile multistate systems for use in memory devices or as a backbone for neuromorphic computing.
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Strongly Correlated Electrons

Spin-dependent orbital selectivity and partial Kondo-screening in magnetically ordered Hund's metal

Hund's metallicity in 3$d$ transition metal oxides constitutes a rare class of compounds, since they have been long understood considering the dominance of Hubbard $U$. $\mathrm{LiV_2O_4}$& $\mathrm{Sr_2CoO_4}$ belong to this rare class of metals; among them, $\mathrm{LiV_2O_4}$ has been the subject of extensive investigations for its unconventional heavy-fermion behavior, while studies on $\mathrm{Sr_2CoO_4}$ remain limited despite its anomalous ferromagnetic ground state. In this study, we report an unusual spin-orbital selective localization in $\mathrm{Sr_2CoO_4}$ leading to a sharp Kondo resonance at $\sim$70 K in the spin-$up$ channel of orbitals of $t_{2g}$ symmetry using a combination of Density functional theory and Dynamical mean field theory (DFT+DMFT) calculations. Correspondingly, an appreciable reduction in the magnetization below $T$=100 K further suggests partial Kondo screening of local moments active at low temperatures, explaining its effective spin magnetization state and upturn in its resistivity observed in experimental reports. We note a significant effect of Hund's induced spin-orbital selective incoherence in dictating the temperature evolution of its macroscopic observables e.g. spin-spin correlation function and effective local moment. Our results reveal a potentially distinct/new form of spin-dependent selectivity induced via Hund's coupling in addition to the conventional orbital-selectivity in the Hund's metals, as a plausible key mechanism in stabilizing their long-range magnetic order.
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Materials Science

The line bundle regime and the scale-dependence of continuum dislocation dynamics

Continuum dislocation dynamics (CDD) has become the state-of-the-art theoretical approach for mesoscale dislocation plasticity of metals. Within this approach, there are multiple CDD theories that can all be derived from the principles of statistical mechanics. In these theories density-based measures are used to represent dislocation lines. Establishing these density measures requires some level of coarse graining with the result of losing track of some parts of the dislocation population due to cancellation in the tangent vectors of unaligned dislocations. The leading CDD theories either treat dislocations as nearly parallel or distributed locally over orientation space. The difference between these theories is a matter of the spatial resolution at which the definition of the relevant dislocation density field holds: for fine resolutions, single dislocations are resolved and there is no cancellation; for coarse resolutions, whole dislocation loops could contribute at a single point and there is complete cancellation. In the current work, a formulation of the resolution-dependent transition between these limits is presented in terms of the statistics of dislocation line orientation fluctuations about a local average line direction. From this formulation, a study of the orientation fluctuation behavior in intermediate resolution regimes is conducted. Two possible closure equations for truncating the moment sequence of the fluctuation distributions relating the two theories mentioned above are evaluated from data, the newly introduced line bundle closure and the previous standard maximum entropy closure relations. The line bundle closure relation is shown to be accurate for coarse-graining lengths up to half the dislocation spacing and the maximum entropy closure is found to poorly agree with the data at all coarse-graining lengths.
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Mesoscale and Nanoscale Physics

A Physical Unclonable Function Based on Variations of Write Times in STT-MRAM due to Manufacturing Defects

A physical unclonable function (PUF) utilizes the unclonable random variations in a device's responses to a set of inputs to produce a unique "biometric" that can be used for authentication. The variations are caused by unpredictable, unclonable and random manufacturing defects. Here, we show that the switching time of a magnetic tunnel junction injected with a spin-polarized current generating spin transfer torque is sensitive to the nature of structural defects introduced during manufacturing and hence can be the basis of a PUF. We use micromagnetic simulations to study the switching times under a constant current excitation for six different (commonly encountered) defect morphologies in spin-transfer-torque magnetic random access memory (STT-MRAM) to establish the viability of a PUF.
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Soft Condensed Matter

Neural-Network-Assisted Boltzmann Approach for Dilute Microswimmer Suspensions

We introduce a neural-network-assisted Boltzmann framework that learns the binary-collision map of microswimmers directly from data and uses it to evaluate collision integrals efficiently. Using a representative model swimmer, the learned map quantitatively predicts translational and rotational diffusivities and enables a linear-stability analysis of isotropy against polar ordering in dilute suspensions. The resulting predictions closely match direct simulations. The present framework is agnostic to active matter models and broadly applicable: once two-body collision data are obtained – either from simulations or experiments – the same surrogate can be used to evaluate kinetic transport across dilute conditions where binary collisions dominate. Because the workflow relies only on pre- and post-collision statistics, the present approach provides a general data-driven route linking particle-scale interactions to macroscopic transport and collective behavior in active suspensions.
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Superconductivity

Finite-size and quenching effects on hyperuniform structures formed during cooling

The outstanding physical properties of hyperuniform condensed matter systems holds significant promise for technological applications and studying effects that may disrupt this hidden order is therefore very important. Vortex matter in superconductors is a model system to study this problem since imaging experiments have revealed that correlated disorder in the host media and finite size effects disrupt the hyperuniformity of the in-plane arrangement of vortices. Here we report simulations of layered interacting elastic lines as a model for the vortex lattice in three-dimensional superconductors, following a cooling protocol that closely mimics the experimental conditions. We show that finite-thickness effects limiting the hyperuniformity range arise both in equilibrium and out-of-equilibrium. Our results provide a theoretical framework to draw a realistic road-map on synthesizing hyperuniform materials when cooling structures on finite host media with disorder.
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All authors A. Cruz-García, J. Puig, R. M. Besana, A. B. Kolton, Y. Fasano

Materials Science · Cross-listed from quant-ph

Quantum simulation of carbon capture in periodic metal-organic frameworks

Carbon capture is vital for decarbonizing heavy industries such as steel and chemicals. Metal-organic frameworks (MOFs), with their high surface area and structural tunability, are promising materials for CO2 capture. This study focuses on Fe-MOF-74, a magnetic Mott insulator with exposed metal sites that enhance CO2 adsorption. Its strongly correlated electronic structure challenges standard DFT methods, which often yield inconsistent predictions. We initially benchmark adsorption energies using various DFT functionals, revealing substantial variability and underscoring the need for more accurate approaches, such as those provided by quantum computing. However, practical quantum algorithms are far less established for simulations of periodic materials, particularly when the plane-wave basis set, often comprising tens of thousands of basis vectors, is used. To address this, we employ an active space reduction strategy based on Wannier functions and natural orbital selection. Localized orbitals around the adsorption site are identified, and MP2 natural orbitals are used to improve convergence of correlation energies. Adsorption energies are then computed using a quantum number-preserving ansatz within the variational quantum eigensolver framework. In addition to classical simulations, we conduct quantum experiments using the sample-based quantum diagonalization method. Although current hardware limits the size of feasible simulations, our approach offers a more efficient and scalable path forward. These results advance the applicability of quantum algorithms to realistic models of carbon capture and periodic materials more broadly.
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All authors Dario Rocca, Jerome F. Gonthier, Joshua Levin, Tobias Schafer, Andreas Gruneis, Byeol Kang, Hong Woo Lee

Disordered Systems and Neural Networks · Cross-listed from physics.bio-ph

Mean-field analysis of a neural network with stochastic STDP

Analysing biological spiking neural network models with synaptic plasticity has proven to be challenging both theoretically and numerically. In a network with N all-to-all connected neurons, the number of synaptic connections is on the order of $N^2$, making these models computationally demanding. Furthermore, the intricate coupling between neuron and synapse dynamics, along with the heterogeneity generated by plasticity, hinder the use of classic theoretical tools such as mean-field or slow-fast analyses. To address these challenges, we introduce a new variable which we term a typical neuron X. Viewed as a post-synaptic neuron, X is composed of the activity state V , the time since its last spike S, and the empirical distribution $\xi$ of the triplet V , S and W (incoming weight) associated to the pre-synaptic neurons. In particular, we study a stochastic spike-timing-dependent plasticity (STDP) model of connection in a probabilistic Wilson-Cowan spiking neural network model, which features binary neural activity. Taking the large N limit, we obtain from the empirical distribution of the typical neuron a simplified yet accurate representation of the original spiking network. This mean-field limit is a piecewise deterministic Markov process (PDMP) of McKean-Vlasov type, where the typical neuron dynamics depends on its own distribution. We term this analysis McKean-Vlasov mean-field (MKV-MF). Our approach not only reduces computational complexity but also provides insights into the dynamics of this spiking neural network with plasticity. The model obtained is mathematically exact and capable of tracking transient changes. This analysis marks the first exploration of MKV-MF dynamics in a network of spiking neurons interacting with STDP.
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Materials Science

Active-Learning Inspired $\textit{Ab Initio}$ Theory-Experiment Loop Approach for Management of Material Defects: Application to Superconducting Qubits

Surface oxides are associated with two-level systems (TLSs) that degrade the performance of niobium-based superconducting quantum computing devices. To address this, we introduce a predictive framework for selecting metal capping layers that inhibit niobium oxide formation. Using DFT-calculated oxygen interstitial and vacancy energies as thermodynamic descriptors, we train a logistic regression model on a limited set of experimental outcomes to successfully predict the likelihood of oxide formation beneath different capping materials. This approach identifies Zr, Hf, and Ta as effective diffusion barriers. Our analysis further reveals that the oxide formation energy per oxygen atom serves as an excellent standalone descriptor for predicting barrier performance. By combining this new descriptor with lattice mismatch as a secondary criterion to promote structurally coherent interfaces, we identify Zr, Ta, and Sc as especially promising candidates. This closed-loop strategy integrates first-principles theory, machine learning, and limited experimental data to enable rational design of next-generation materials.
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All authors Sarvesh Chaudhari, Cristóbal Méndez, Rushil Choudhary, Tathagata Banerjee, Maciej W. Olszewski, Jadrien T. Paustian, Jaehong Choi, Zhaslan Baraissov, Raul Hernandez, David A. Muller, B. L. T. Plourde, Gregory D. Fuchs, Valla Fatemi, Tomás A. Arias

Materials Science

Epitaxially-stabilized growth of wüstite FeO on 4H-SiC

Iron(II) monoxide (FeO) is thermodynamically stable in the halite (wüstite) structure only at elevated temperatures in a typically non-stoichiometric, Fe-deficient, Fe$_{1-z}$O form that tends to phase separate and/or transform into metallic $\alpha$-Fe and magnetite Fe$_3$O$_4$ at ambient conditions. Here we report on the successful growth of up to 180 nm thick $(111)$-oriented FeO heteroepitaxial films on slightly lattice-matched 4H-SiC$(0001)$ using molecular beam epitaxy (MBE). The films have flat, terraced surfaces with tall multi-layer steps. X-ray diffraction (XRD), high-resolution scanning transmission electron microscopy (S/TEM), energy-dispersive X-ray spectroscopy (EDS), and core-level electron energy loss spectroscopy (EELS) collectively confirm the epilayer as phase-pure wüstite FeO, with atomically sharp FeO/SiC interfaces. The films are found to exhibit a slight misfit strain-induced rhombohedral distortion that does not appear to vary over the range of thicknesses examined. These results demonstrate the power of epitaxial stabilization for integrating a thermodynamically unstable, yet functionally interesting material with a commercially available and technologically important semiconductor platform.
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All authors Faisal Kimbugwe, Marzieh Baan, Alexandra Fonseca Montenegro, Roberto C Myers, Tyler J Grassman

Mesoscale and Nanoscale Physics

Symmetry in magnetoelectric electromagnetism and magnetoelectric meta-atoms

While in electromagnetism we have space-time symmetry, magnetoelectric (ME) processes are characterized by space-time symmetry breaking. Our goal is to show that quantum vacuum fields with both time reversal and space inversion symmetry breaking (so-called ME fields) can be observed in subwavelength regions of electromagnetic (EM) radiation. The sources of ME fields are ME meta-atoms, subwavelength elements made of magnetic insulators, where the dynamical ME behavior is due to modulations and topological coupling of magnetization and electric polarization. The interaction between EM and ME systems occurs through virtual structures, ME virtual photons. Experimentally, ME quantum vacuum states can be detected in a microwave cavity. The topic of these studies concerns fundamental aspects of ME quantum electrodynamics (MEQED).
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Superconductivity

Vestigial pairing from fluctuating magnetism and triplet superconductivity

We study the finite-temperature vestigial superconducting phases of a two-dimensional system of fluctuating spin-triplet pairing and spin magnetism. Denoting the respective primary order parameters by $\mathbf{d}$ and $\mathbf{N}$, which are not long-range ordered at finite temperature, the composite fields $\phi_{dd} = \mathbf{d}\cdot\mathbf{d}$ and $\phi_{dN} = \mathbf{d}\cdot\mathbf{N}$ are spin-rotation invariant and can condense at finite temperature. Using a large-$N$ approach that respects the Mermin-Wagner theorem, we here derive the phase diagram which features two vestigial superconductors: $(A)$ a charge-$4e$ superconductor with $\phi_{dd}\neq 0$ and $\phi_{dN} =0$ and $(B)$ a charge-$2e$ state with $\phi_{dN} ,\phi_{dd}\neq 0$. We analyze the temperature and coupling-constant dependent properties of these two superconductors using a perturbative approach and a variational Hartree-Fock study. This reveals non-trivial spectra in the superconductors, which result from the fundamental building blocks being distinct from the usual Cooper pairs–in phase $(A)$, the elementary bosons are bound states of four electrons and, in phase $(B)$, of three electrons and a hole. This work complements the previous study [Nat. Commun. 15, 1713 (2024), arXiv:2301.01344], which focused on the properties of phase $(B)$.
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All authors Yanek Verghis, Denis Sedov, Jakob Weßling, Prathyush P. Poduval, Mathias S. Scheurer

Statistical Mechanics · Cross-listed from quant-ph

Computational access to lattice and long-wavelength physics in quantum mutual information

Quantum mutual information is an important tool for characterizing correlations in quantum many-body systems, but its numerical evaluation is often prohibitively expensive. While some variants of Rényi Mutual Information (RMI) are computationally more tractable, it is not clear whether they correctly capture the long-wavelength physics or are dominated by UV effects, which is of key importance in lattice simulations. We analyze the relevance of lattice effects on the family of $\alpha$-$z$ Rényi mutual informations for ground states of models with conformal field theory descriptions. On the example of massless free fermions we identify distinct regions in the $\alpha$-$z$ plane, where RMI corrections due to the lattice are relevant or irrelevant. We further support these findings with MPS calculations on the transverse field Ising model (TFIM). Our results, accompanied by the open-source Julia package QMICalc$.$jl, provide guidance to using RMI in quantum-many body physics numerical computations.
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All authors Patrick M. Lenggenhager, M. Michael Denner, Doruk Efe Gökmen, Maciej Koch-Janusz, Titus Neupert, Mark H. Fischer

Soft Condensed Matter

Turbulent Dynamics in Active Solids

Turbulence is most commonly associated with high Reynolds number flow, however the framework of turbulent dynamics has been conceptually extended to many other fields, such as magnetohydrodynamic turbulence, elastic wave turbulence in solids, and more recently to low Reynolds number active turbulence in biological fluids. Here we report a form of solid turbulent dynamics in a self-propelled two-dimensional elastic sheet. We show numerically that the polar ordering dynamics in the active elastic solid model (AES) exhibit hallmark features of turbulent dynamics: power-law scaling of the energy spectrum and non-Gaussian statistics of velocity increments. However, there is no energy cascade, in line with previous findings for active turbulence in fluids. These results extend the concept of active turbulence to solid-state active matter, and can be important for understanding collective dynamics in biological active solids such as bacterial colonies and epithelial cell layers.
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Strongly Correlated Electrons

Detecting quantum spin liquid on Kitaev model through a superconducting junction

The Kitaev model belongs to an unconventional class of two-dimensional spin systems characterized by anisotropic, bond-dependent interactions that give rise to Quantum Spin Liquid (QSL) states. These exotic phases, marked by the absence of magnetic ordering even at zero temperature, support fractionalized excitations and emergent gauge fields. A particularly compelling feature of the Kitaev model is its exact solvability, which reveals low-energy excitations in the form of itinerant Majorana fermions-quasiparticles that obey non-Abelian statistics and are of central interest in topological quantum computation due to their inherent robustness against local perturbations and decoherence. Despite extensive theoretical advancements, the experimental identification of QSLs remains challenging, as conventional magnetic probes fail to detect their defining properties. In this work, we present a theoretical investigation of spin current injection from a superconducting metal into a Kitaev quantum spin liquid. By employing a spintronic framework, we derive the dynamics of the injected spin current and demonstrate how its signatures can be traced back to the underlying Majorana excitations in the spin liquid phase. Superconductivity plays a pivotal role in this context, not only as a source of coherent quasiparticles but also as a platform with potential for interfacing with topological quantum devices. Our analysis contrasts the Kitaev-superconductor interface with conventional ferromagnetic junctions, where spin transport is carried by magnons, and highlights distinctive features in the spin current response. These findings open new directions for the detection of QSLs and contribute to the broader effort of integrating topological quantum materials into scalable quantum technologies.
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Statistical Mechanics

One-dimensional long-range Ising model: two (almost) equivalent approximations

We investigate the critical behavior of the one-dimensional Ising model with long-range interactions using the functional renormalization group in the local potential approximation (LPA), and compare our findings with Dyson's hierarchical model (DHM). While the DHM lacks translational invariance, it admits a field-theoretical description closely resembling the LPA, up to minor but nontrivial differences. After reviewing the real-space renormalization group approach to the DHM, we demonstrate a remarkable agreement in the critical exponent $\nu$ between the two methods across the entire range of power-law decays $1/2 < \sigma < 1$. We further benchmark our results against Monte Carlo simulations and analytical expansions near the upper boundary of the nontrivial regime, $\sigma \lesssim 1$.
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All authors Valerio Pagni, Guido Giachetti, Andrea Trombettoni, Nicolò Defenu