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Physics Condensed Matter Strongly Correlated Electrons

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Tuesday 13 October · still arriving

Strongly Correlated Electrons · Cross-listed from quant-ph

Explicitly correlated ground states with a feedback-free variational hybrid algorithm

Explicitly correlated methods, which represent dominant short-range correlations by a diagonal Jastrow-type correlator, are designed to accurately describe systems of strongly correlated electrons, such as the fully periodic 2D Fermi–Hubbard model. However, as the reference state is compact in momentum space whereas the correlator acts naturally in real space, there is a fundamental mismatch of bases that classical algorithms resolve only by restricting the reference or the correlator. Here we propose a hybrid algorithm in which a quantum processor prepares a low-entanglement momentum-space matrix product state (MPS), precomputed classically by the transcorrelated method at the cost of a nonvariational energy, rotates it to real space, and measures in bases fixed by the Hamiltonian. Because the measurement bases are independent of the correlator, the correlator can be variationally optimized entirely in classical post-processing with no quantum-classical feedback loop. We demonstrate our algorithm on 32 qubits of Quantinuum's H2-2 with a bond-dimension-4 MPS for the half-filled $4 \times 4$ lattice and achieve a relative ground-state energy error of $16 \pm 4\%$ after postselection, reduced to $3.5 \pm 0.5\%$ by calibration using low-order moments from the MPS. Compared with other feedback-free hybrid algorithms, even under generous assumptions, our method requires fewer samples than quantum-selected configuration interaction and fewer two-qubit gates than quantum Krylov methods.
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Strongly Correlated Electrons

Altermagnetic Ground States on the Ammann–Beenker Tiling

We identify exact altermagnetic ground states of a classical Heisenberg model on a quasicrystal. Considering the Ammann–Beenker tiling as an example, we determine the ground states by exploiting the parity structure of its parent four-dimensional hypercubic lattice. The ground state hosts coplanar altermagnetic order characterized by the preserved spin-group symmetry $[C_{2x}\parallel C_{8z}]$. Without translational symmetry, the momentum-space spin splitting that usually identifies altermagnets is not directly accessible. We instead couple the spins to itinerant electrons and show spin-resolved transport with $g$-wave symmetry, confirming the altermagnetic nature in a nonperiodic system. Our results establish a geometric route to altermagnetic order in quasicrystals, connecting exact magnetic ground states to their spin-resolved transport signatures.
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All authors SeungBeom Hong, YunHo Kim, Moon Jip Park, GiBaik Sim

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

Coherent Phonon Generation from Prethermal Carrier Populations in a Semiconductor

Ultrafast laser excitation of carriers in semiconductors often results in the creation of fully symmetric coherent optical phonons, typically understood in terms of a thermalized transient carrier population. We test this understanding with systematic measurements and first-principles calculations of the photon-energy dependence of ultrafast-laser-driven coherent phonon generation in tellurium, using excitation wavelengths around the electronic band gap. We observe that, contrary to the expectations of models assuming a thermalized carrier population, the coherent amplitude of the fully symmetric $A_1$ mode changes only weakly when tuning wavelength across the band gap. The measured spectral dependence is instead reproduced by a transition-resolved prethermal force weighted by optical matrix elements and band- and momentum-dependent $A_1$ deformation potentials. Fitting this model to the data yields an excited transition state lifetime of a few femtoseconds. These results identify transition selectivity, rather than a thermalized total carrier density, as a key factor controlling coherent-phonon generation in semiconductors excited near a band gap.
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All authors Mingyu Shi, Matteo Savoini, Patrick Friebel, Andrea Annunziata, Thomas Metzger, Yunpei Deng, Laura Cattaneo, Steven L. Johnson

Strongly Correlated Electrons

Unexpected stabilization of a single-$q$ charge density wave in pristine 1T-TiSe$_2$

Over the past decade, studies revisiting the classical charge-density-wave system 1T-TiSe$_2$, long understood to host the $2 \times 2$ triple-$q$ order with equivalent subcomponents, have suggested that these subcomponents may not be identical, challenging a 50-year-old paradigm. Here, we demonstrate not only that these subcomponents are non-identical but also that they develop sequentially rather than simultaneously. By tracking folded-band features, angle-resolved photoemission spectroscopy reveals that a unidirectional $2 \times 1$ single-$q$ order stabilizes first, while the other two components emerge sequentially at lower temperatures, completing the triple-$q$ phase. Our free-energy analysis explains this hierarchy through repulsive coupling among the three subcomponents, as supported by first-principles calculations incorporating phonon anharmonicity. Consequently, the three subcomponents are inequivalent in both phase and amplitude. These results reconcile reported symmetry breaking and differing characteristic temperatures and establish a framework in which ostensibly simple, high-symmetry charge-density order emerges from temperature-dependent competition and cooperation among inequivalent subcomponents.
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All authors Kimoon Higashihira Han, Dongju Hwang, Dongsin Kim, Yeojin Ahn, Jaehun Cha, Seonggeon Gim, Gyubin Lee, Mingi Jho, Chan-young Lim, Sae Hee Ryu, Chris Jozwiak, Aaron Bostwick, Eli Rotenberg, Jonathan D. Denlinger, Makoto Hashimoto, Donghui Lu, Young Woo Choi, Gil Young Cho, Yeongkwan Kim

Strongly Correlated Electrons

Non-Hermitian Statistical Geometry

Particle exchange in two dimensions gives rise to quantum statistics beyond the boson-fermion dichotomy, with central roles in fractional quantum Hall physics, topological quantum computation, and strongly correlated quantum matter. In conventional topological phases, microscopic exchange geometry is compressed into rigid braid and fusion data. We develop a theory of non-Hermitian statistical geometry in which relaxing Hermiticity softens these exchange data into a larger complex space of spectral and relative-geometric degrees of freedom. For two adjacent braid generators, a single projective exchange spectrum is insufficient: their relative eigenline geometry supplies an additional gauge-invariant modulus. On the generic irreducible two-channel branch, braid consistency locks these coordinates through an exact spectrum-geometry relation. Using Riesz projectors and Kato transport, we realize this geometry in a five-arm Kitaev-Majorana network and test spectral and relative-geometric responses in an independent two-dimensional four-vortex Kitaev model. Finite-time dynamics tests the exchange operation, microscopic fusion sewing tests its composition across fusion descriptions, and matched-spectrum controls isolate the role of relative geometry. Nonzero projective Kato curvature shows that braid-consistent, fusion-coherent exchange can depend on the control path. Non-Hermiticity thus exposes exchange geometry, braid consistency re-locks it, fusion coherence further constrains it, and projective flatness determines when geometric exchange becomes intrinsically topological.
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Strongly Correlated Electrons · Cross-listed from quant-ph

Local error correction prolongs time-crystalline memory

Discrete time crystals are non-equilibrium phases of matter with spatiotemporal order and a response that breaks the time-translation symmetry of a periodic external drive. Interactions, spatial disorder and correlated random driving can in theory stabilize this order. In experiments, however, coupling to the environment limits the time crystal lifetime. Here we use stochastic local bit-flip error correction to prolong the time-crystalline response of a driven, spatially disordered two-dimensional Ising model on a superconducting quantum processor, using a repetition code with distances three and five on a honeycomb lattice with up to 68 physical qubits. Even though ancilla qubits, midcircuit syndrome measurements and decoding increase the required quantum and classical resources, the stochastic drive increases the memory decay time by a factor of up to two. At late times we observe that recovery stabilizes spatial order across the lattice. The spin-configuration distributions explain this separation, as recovery suppresses disagreeing bonds while broadening occupies completely reversed states. Syndrome measurements without correction accelerate the memory decay, demonstrating the importance of conditional correction. Our results show that local bit-flip error correction can preserve time-crystalline memory over more drive cycles than the bare dynamics.
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Strongly Correlated Electrons

Direct view of exciton and carrier dynamics in twisted bilayer graphene

Twisted bilayer graphene (tBLG) on H-intercalated SiC (twist angle of $9 \pm 1^{\circ}$) is studied by position\mbox{-}, time\mbox{-}, and angle-resolved photoemission spectroscopy (ARPES). Both graphene layers are hole doped, with a Dirac-point offset of 30~meV. Time-resolved ARPES near the van Hove singularity reveals a spectral feature within the hybridization-induced band gap, together with excited electrons in the conduction band. The in-gap feature exhibits distinct dynamics, and its binding energy and $k$-space location are consistent with the proposed non-hydrogenic “ghost-Fano” exciton arising from destructive interference between two nearly degenerate excitonic channels. Near the Dirac points, the twist separates the largely layer-polarized Dirac cones in momentum space, providing direct layer selectivity. We find markedly different peak electronic temperatures in the two graphene layers, even though their subsequent cooling dynamics are very similar. We attribute this to an ultrafast interlayer redistribution of electronic energy, driven by an interlayer electric field that arises from the different doping in the layers.
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All authors Gianmarco Gatti, Anders S. Mortensen, Zhihao Jiang, Alfred J. H. Jones, Gesa-R. Siemann, Thomas S. Nielsen, Søren Ulstrup, Naina Kushwaha, Bruce Weaver, Yu Zhang, Emma Springate, Charlotte E. Sanders, Vibha Reddy, Ulrich Starke, Philip Hofmann

Strongly Correlated Electrons

Conformal soft modes at elastic instabilities

In case a crystal is close to a continuous elastic phase transition, pronounced critical fluctuations emerge. We show that on the level of linear elasticity theory the displacement vector for these critical modes obeys a condition reminiscent of the conformal Killing equation. For an isostructural instability, four critical modes arise corresponding to one dilation and three special conformal transformations. At crystal symmetry-breaking instabilities, the critical fluctuations include a continuum of modes even for crystals with finite size. For certain cases, these comprise the conformal transformations associated with two-dimensional Minkowski space. These results have implications for critical elastic phenomena as well as for extremal mechanical metamaterials.
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Strongly Correlated Electrons · Cross-listed from cond-mat.supr-con

Observation of stacked vortex structure with number controllable Majorana zero mode in Bi$_{2}$Te$_{3}$/FeTe heterojunction

Creation and control of Majorana zero modes (MZMs) in solid devices is the key challenge in realizing fault tolerant topological quantum computation. Here we report spectroscopic evidence for number controllable MZMs in stoichiometric one quintuple layer Bi$_{2}$Te$_{3}$/FeTe heterostructures, together with the observation of stacked vortices in superconducting islands. Low temperature scanning tunnelling microscopy and spectroscopy reveal a long period moire superlattice arising from lattice mismatch, which induces nanoscale modulation of superconducting gaps. Magnetic vortices exhibit a stacked core structure with two layer derived bound state branches: a dispersive branch evolving into an X-shaped pattern away from the vortex center, and a quantum-limit branch characterized by a spatially unsplit MZMs together with discrete integer quantized Caroli-de Gennes-Matricon states. Notably, MZMs are observed in all measured vortices, and their number can be tuned by magnetic field and the size of Bi$_{2}$Te$_{3}$ islands. These results establish stoichiometric 1QL-Bi$_{2}$Te$_{3}$/FeTe as a patterned superconducting interface that enables isolated and few-vortex Majorana configurations, providing a controlled platform for fuse MZMs.
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All authors Xinru Han, Zhaokun Luo, Quanxin Hu, Xingjian Zhu, Xiaohong Pan, Dan Mu, Xinyu Liang, Zulin Xu, Qiheng Wang, Ryan L. Kong, Mingyuan Li, Zhengliang Zhang, Fazhi Yang, Mojun Pan, Xin Liu, Qiangqiang Gu, Baiqing Lv, Gan Wang, Hong Ding

Monday 12 October

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

Crystal growth, magnetic, and transport properties of the candidate altermagnet Cr$_{1/4}$NbS$_{2}$

Altermagnetism is a rapidly emerging paradigm in condensed matter magnetism, yet the number of experimentally confirmed altermagnetic candidates remains remarkably limited. Cr$_{1/4}$NbS$_2$ has long been theoretically proposed as a promising altermagnet, but there are no reports on experimental investigation of single crystals. Here, we report the successful growth of high-quality single crystals of Cr$_{1/4}$NbS$_2$ and present its structural, thermal, magnetic, and transport properties. Single-crystal X-ray diffraction provides detailed crystallographic information and confirms the hexagonal crystal symmetry ($P6_3/mmc$), one of the criteria for altermagnetic behavior. Resistivity and heat capacity measurements unambiguously identify an antiferromagnetic Néel temperature of $T_N \sim 141$ K. Magnetotransport measurements reveal non-trivial features in the magnetoresistance and Hall response, indicative of quantum diffusive transport phenomena. Cr$_{1/4}$NbS$_2$, synthesized here for the first time in single-crystalline form, therefore serves as an experimental platform for probing the rich spectrum of phenomena predicted for altermagnetic materials.
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All authors Nashra Pistawala, Martin R. Lees, Geetha Balakrishnan, Daniel A. Mayoh

Strongly Correlated Electrons · Cross-listed from quant-ph

Krylov Complexity and Quantum Many-body Scars in Non-Hermitian Kinetically Constrained Models

Thermalization in closed quantum systems and its breakdown are central to understanding the emergence of statistical behavior in isolated many-body systems. Kinetic constraints can hinder thermalization by restricting the allowed dynamics and giving rise to non-ergodic behavior. While various aspects of ergodicity breaking in kinetically constrained models have been extensively studied in Hermitian systems, their behavior in non-Hermitian kinetically constrained models remains less explored. In particular, the inequivalence of left and right eigenstate ensembles in non-Hermitian systems raises the question of whether they exhibit qualitatively different dynamical and eigenstate properties. In this work, we study non-Hermitian generalizations of the paradigmatic PXP and PPXPP models, focusing on their Krylov complexity, eigenstate structure, and dynamics. By exploiting the Arnoldi's algorithm, we find distinct behavior of Krylov complexity in the left and right eigenstate ensembles as non-Hermiticity is increased: in the right ensemble, it exhibits persistent oscillations with an increasing period, while in the left ensemble, it gradually saturates. The characteristic arch-shaped profile of the Arnoldi coefficients is also modified differently in the two ensembles, with a Hermitian-like arch re-emerging in the left ensemble at large non Hermiticity. Additionally, in the non-Hermitian PXP model, the right ensemble retains the characteristic scar structure, while the left ensemble develops additional non-scar eigenstates with anomalously low entanglement and large overlap with the vacuum state. These findings reveal that non-Hermiticity can affect Krylov dynamics and eigenstate structure differently in the left and right ensembles, demonstrating the need to treat them separately when characterizing non-Hermitian kinetically constrained systems.
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All authors Arkaprava Sil, Rudraksh Kaushik, Souvik Kundu, Prasant Mallik, Sudipto Singha Roy

Strongly Correlated Electrons

Quantum skyrmion molecule: two quantum skyrmions bound by coherent magnon exchange

Quantum skyrmions in frustrated spin-$1/2$ magnets are bound states of a few flipped spins in a ferromagnetic background. Using exact diagonalization and density-matrix renormalization group calculations for the $J_1$–$J_2$ triangular-lattice model with easy-axis anisotropy $K$, we ask what happens when two such objects are brought together. The binding energy per flipped spin of a single skyrmion has a minimum at $\Nf^{*}=7$ for $K=0.02$–$0.04$, and skyrmions smaller than $\Nf^{*}$ do not exist as pairs: at any distance they coalesce into a single larger object, and pinning wells cannot prevent it. Two skyrmions of natural size, by contrast, form a bound molecule without pinning or external field, with binding energy $U\simeq-0.007J_1$ at $K=0.03$–$0.04$ and an equilibrium separation of $5.5$ lattice spacings that does not depend on $K$ or on the size of the simulation domain; at $K=0.02$, where the single skyrmion is itself marginally bound, the pair is unbound within our resolution. The two constituents keep their identity ($7+7$ flipped spins) and are coupled by a coherent exchange of magnons, visible as number fluctuations between the two halves of the domain in excess of those of two independent skyrmions and as in-plane spin correlations between the two skyrmion walls that reach $0.16$ across the gap. These correlations follow the vortex pattern of the two textures and lock their relative helicity, the quantum counterpart of the helicity-dependent interaction of classical skyrmions. We discuss the molecule as a self-assembled two-qubit element for skyrmion helicity qubits in a single layer.
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Strongly Correlated Electrons

Phase-Coherent Spin and Lattice Modulations in a Y-type Hexaferrite

Spin-driven multiferroics owe their electric polarization to lattice distortions that follow the magnetic order, yet in incommensurate magnets symmetry normally forbids such a distortion at the fundamental magnetic wavevector, and the distortions themselves are rarely observed. Here we use half-polarized neutron scattering to show that the Y-type hexaferrite Ba$_{0.4}$Sr$_{1.6}$Mg$_2$Fe$_{12}$O$_{22}$ hosts, in its saturated high-field state, a magnetic modulation and a longitudinal lattice modulation at one and the same wavevector, locked in phase. The signature is a large nuclear-magnetic interference asymmetry, $r$ ~ 0.8, of the same sign at the two conjugate satellites and persisting to 275 K. The zone contrast and the field dependence of the satellite indicate an internal, field-induced longitudinal distortion. The modulated state coexists with the transverse-conical magnetoelectric phase and outlives it, revealing a fundamental-wavevector spin-lattice coupling in a magnetic field regime previously regarded as a simple ferrimagnet.
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All authors Oskar Stepančić, Annika Stellhorn, Emma Campillo, Kun Zhai, Niklas Ekström, A. Corani, D. Alba Venero, R. Cubitt, E. Blackburn, L. Shen

Strongly Correlated Electrons

Pairing from repulsive interactions in twisted WSe2 from functional renormalization

Motivated by the observation of superconductivity in twisted bilayer WSe$_2$ over an extended range of displacement fields, reaching from the correlated insulator down to zero field, we analyze the correlated electron phases of this system at hole filling $\nu = -1$ and twist angle $3.65^\circ$ using Hartree–Fock, random phase approximation, and functional renormalization group calculations. We derive a continuum model with gate-screened Coulomb interaction from first principles and compare its instabilities to those of a realistic three-orbital Wannier model with a Hubbard interaction and an artificial single-orbital Hubbard model. In both cases, we find a superconducting instability of mixed $d$-wave singlet and $p$-wave triplet character, arising adjacent to inter-valley-coherent spin-density-wave order in the phase diagram spanned by displacement field and interaction strength. Our additional analysis of the pairing mechanism points to inter-valley coherent spin fluctuations as the pairing glue. The extent of the pairing regime and the associated critical temperatures depend on the model input, and we trace differences to the interaction range entering the projected interaction. Within the continuum model, the gate-screened Coulomb interaction yields pairing down to zero displacement field, bringing theory into agreement with experiment.
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All authors Hannes Braun, Dumitru Călugăru, Pietro M. Bonetti, Haoyu Hu, Yan Zhang, Yi Jiang, Quansheng Wu, Kin Fai Mak, Jie Shan, B. Andrei Bernevig, Michael M. Scherer, Laura Classen

Strongly Correlated Electrons · Cross-listed from quant-ph

Fermionic non-Gaussianity via computable measures and experimentally accessible bounds

Interacting fermions owe both their non-trivial correlations and their computational power to their departure from Gaussianity. Yet, quantifying that departure geometrically faces two challenges: the Gaussian manifold is non-convex, and perturbative treatments are confined to weak interactions. Here, we introduce a geometric measure of fermionic non-Gaussianity, the fidelity distance of a target state to the manifold of fermionic Gaussian states. We construct an iteration formalism to numerically access it, applicable also at strong coupling. Further, we prove a sharpened operator Jensen inequality, of interest in its own right. We use it to derive a witness that involves only two- and four-point fermionic correlators. Numerical benchmarks on the one-dimensional Fermi–Hubbard model show that the quality of the witness improves with system size and, for strong coupling, is tighter than antiflatness. Our results open a scalable route to charting non-Gaussianity of strongly-interacting fermionic quantum simulators.
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Strongly Correlated Electrons

Berry curvature from plane-wave mixing: A three-band model with emergent symmetries

Two-dimensional materials can host topological phases stabilized either by an intrinsic moiré potential or topological crystallization. Crucial to the topology of these phases is the interplay between the (self-consistently generated) potential and the spinor structure, which imbues the band-projected potential with momentum-dependence. Truncating this potential at linear-order in momentum, we obtain a three-band model that captures the low-energy band structure and Berry curvature of such topological bands. We analytically find that the Berry curvature strongly depends on momentum-dependence of the potential. Furthermore, we identify that the model can be tuned to have emergent symmetries, including $U(1)$ and anti-unitary symmetries. Emergent-symmetry breaking perturbations drive the system to regimes hosting topological flat bands, quadratic band touchings, and multiple Dirac cones. We recover many of these features when studying an un-truncated model of a $\lambda$-jellium spinor inside of a periodic potential. Our results reveal a rich interplay of spinor structure and a potential in determining the topology of the ground state.
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Strongly Correlated Electrons · Cross-listed from quant-ph

Entanglement Sudden Death in Gapped Ground States

Spatial sudden death of entanglement refers to the disappearance of quantum correlations between subsystems after a certain distance called the entanglement length. Specifically, given a density matrix $\rho_{ABC}$ on a tripartite system $ABC$ with $B$ spatially separating $A$ and $C$, the entanglement length is the distance $\ell(A,C)$ after which the reduced density matrix $\rho_{AC}$, given by tracing out the $B$ subsystem, is separable. We show in the case of gapped ground states in any dimension that the entanglement length is finite on finite subsystems. Restricting to one-dimensional systems, we prove that normal matrix product states have a finite entanglement length independent of $A$ and $C$, and that a finite pure state with such uniform entanglement length has a matrix product state representation with bond dimension independent of $A$ and $C$. Consequently, in one dimension, entanglement length distinguishes matrix product states from all other pure states.
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Strongly Correlated Electrons

Honeycomb Crystal in a Mass-Asymmetric Electron-Hole Bilayer

A two-dimensional electron gas in a uniform neutralizing background forms a triangular Wigner crystal at low density. In a strongly mass-asymmetric electron-hole bilayer, localized heavy holes instead provide a nonuniform positive background that supports an electron crystal at densities two orders of magnitude higher than for a homogeneous electron gas in the same material. Here we show that correlated mobile electrons can overturn the preference for triangular order, stabilizing a honeycomb electron-hole crystal. Using the powerful real-space neural-network variational Monte Carlo in the Born-Oppenheimer limit with fixed holes, we find that increasing the density drives a transition from a triangular electron-hole crystal to a honeycomb crystal, which eventually melts into itinerant electrons coexisting with the honeycomb or the triangular hole lattice at fixed interlayer separation. Relative to triangular order, honeycomb order emerges when gains in electronic kinetic energy and electron-hole attraction outweigh its higher intralayer Coulomb repulsion, a threshold never reached in the rigid point-dipole model. Moreover, the honeycomb hole lattice supports paramagnetic, antiferromagnetic, and stripe-ordered spin states. Complex polarization indicates a metal-insulator transition, while the states on the honeycomb hole lattice are consistent with a stripe-ordered Dirac semimetal and paramagnetic or antiferromagnetic Mott insulators via mapping to the half-filled Hubbard model. We further propose a BLG/hBN/WS$_2$-WSe$_2$ heterostructure as a platform for the predicted honeycomb crystal, at an experimentally feasible density $n\sim10^{11}~\text{cm}^{-2}$.
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All authors Shengdu Chai, Wangqian Miao, Yuqiang Li, Lei Wang, Xi Dai, X.C. Xie

Strongly Correlated Electrons

Microscopic Theory of the Acoustic Faraday Effect in Spin-Orbit Coupled Magnets

The acoustic Faraday effect probes phonon Hall viscosity through the rotation of transverse acoustic polarization, conventionally interpreted in terms of circular birefringence. We show that magnetic order breaking rotational symmetry generates anisotropic phonon responses and elliptically polarized eigenmodes, so that Faraday rotation cannot be attributed to Hall viscosity alone. To elucidate their microscopic origin and consequences, we derive spin-phonon couplings from a generic $J$-$K$-$\Gamma$-$\Gamma'$ model with interlayer coupling, identifying transverse strain couplings for propagation along the $c$-axis arising from the interplay of Kitaev $(K)$ and $\Gamma$ interactions, along with strain-induced $g$-tensor contributions. Incorporating these couplings into our theory for the Kitaev spin-liquid candidate $\alpha$-RuCl$_3$, we find that symmetry breaking modifies the Faraday response, revealing a Hall viscosity approximately twice the value inferred assuming rotational symmetry. Our results establish a microscopic framework beyond circular birefringence, refining the connection between acoustic Faraday rotation and phonon Hall viscosity in symmetry-broken spin-orbit-coupled magnets.
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Strongly Correlated Electrons

Emergent low-energy thermodynamics and universal $B/T$ scaling in $\alpha$-RuCl$_3$

Quantum spin liquids are exotic states of matter in which strongly interacting spins remain disordered down to zero temperature and host fractionalized excitations. This has motivated an extensive search for their realization in materials. Among candidate systems, $\alpha$-RuCl$_3$ has drawn particular attention as a platform for the quantum spin liquid proposed by Kitaev, in which the low-energy excitations in applied magnetic fields are interpreted as itinerant Majorana fermions and local flux excitations. However, conflicting experimental signatures have cast doubt on whether a Kitaev quantum spin liquid-like state is really the right starting point to interpret the low-energy states in $\alpha$-RuCl$_3$, motivating a closer look at the nature of these excitations. Here we report an extensive high field study of specific heat up to 35 T on $\alpha$-RuCl$_3$. We find that the low-energy thermodynamics exhibit universal $B/T$ scaling with a single effective energy scale proportional to the applied field as long as the magnetic field is not close to the $c$-axis. This behavior persists continuously from the antiferromagnetic phase boundary to the highest fields, suggesting that the perturbative Kitaev limit, with its Majorana and flux excitations, may not be an appropriate starting point for describing the low-energy thermodynamics of $\alpha$-RuCl$_3$ for fields away from the $c$-axis.
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All authors A. Khansili, B. J. Ramshaw, A. Bangura, H.-Y. Kee, R. D. McDonald, F. Assaad, A. Rydh, A. Shekhter, K. A. Modic

Strongly Correlated Electrons · Cross-listed from cond-mat.supr-con

Microscopic Modeling of Interlayer Tunneling in Twisted Bilayer Cuprates

The field of twistronics, recently extended to twisted bilayer cuprate systems, has generated considerable interest due to the prediction of $d+id'$ states close to a $45^\circ$ twist, as suggested by multiple experimental probes. Theoretical studies of these systems using a variety of models and many-body theoretical techniques have revealed multiple competing order parameters. The large variability in experimental results and theoretical predictions demands an accurate microscopic model for these systems, in particular a more realistic description of the interlayer tunneling. In this study, we fit the in-plane hopping and compute the interlayer tunneling amplitudes by calculating the orbital overlap between $d_{x^2-y^2}$ wave functions at each site of the twisted square-lattice model. We observe sign-changing tunneling amplitudes, a strong twist-angle dependence of the direct tunneling term, and long-range tunneling amplitudes that often dominate over direct tunneling. We investigate the band structure, Fermi surfaces, and spectral functions in comparison with those obtained from the phenomenological model and find a substantial redistribution of spectral weight that modifies the competition between different superconducting ground states. We determine the phase diagram as a function of twist angle, filling, and direct tunneling strength, which is controlled by the $c$-axis distance between the monolayers, and observe a reduction in the region of time-reversal-symmetry-breaking (TRSB) $d+id'$ states compared with the phenomenological model. Finally, we investigate the Josephson critical current across the phase diagram and find strongly suppressed critical currents close to a $45^\circ$ twist, consistent with experimental observations.
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All authors Siddhant Panda, Andreas Kreisel, Laura Fanfarillo, P. J. Hirschfeld

Strongly Correlated Electrons

Mutual information across the commensurate–incommensurate crossover and near the Kosterlitz–Thouless point of the spin-$\tfrac12$ $J_1$–$J_2$ Heisenberg chain

What quantum mutual information adds to conventional correlation functions is often unclear. We study the spin-1/2 $J_1$-$J_2$ Heisenberg chain, using DMRG on infinite chains and periodic rings and an SU(2) decomposition of the mutual information into correlation channels. For singlet ground states the two-site mutual information is an exact function of the spin correlator, so any additional content must come from blocks. In the dimerized phase, blocks resolve bond-energy correlations in the SU(2)-scalar channel without an independent asymptotic length: singlet and triplet correlation lengths agree to about 1%. The scalar channel dominates block mutual information at large distances in the commensurate regime up to $J_2/J_1=0.40$, but falls to a few percent beyond the disorder point, which coincides numerically with the Majumdar-Ghosh point $J_2/J_1=1/2$; the structure-factor peak splits only at the Lifshitz point $J_2/J_1=0.520622(2)$. On the gapless side we compare block mutual information on rings extrapolated to infinite size with the two-interval prediction of SU(2)$_1$ conformal field theory across the Kosterlitz-Thouless point $J_2/J_1=0.241167$. There, for block lengths $l\le6$, the correction decays as $l^{-p}$ with $p=1.96$-$2.07$, and any logarithmic term is at least 60 times smaller than in the Heisenberg chain. Expanding in the marginal coupling (from level spectroscopy) the first-order coefficient is consistent with $l^{-2}$ scaling and the second-order coefficient is positive for $x\le1/4$, suggesting that the mutual information relative to the field-theory value becomes stationary at the KT point for large blocks. The scalar-channel share approaches 1/4 at small cross ratio $x$, as expected from SO(4) symmetry; under two stated assumptions its first-order response to the coupling is $(3/8)\ln x-5/8$ at small $x$, matched by the $l=4$ data within 1-3% at $x\le1/9$.
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Strongly Correlated Electrons · Cross-listed from hep-th

Out-of-time-order hydrodynamics and scrambling

Hydrodynamics as an effective field theory (EFT) has been immensely successful for predicting the behaviour of time-ordered correlation functions in the long-time, large-distance regime. In this paper, we analyse the predictions of hydrodynamics for scrambling as probed by out-of-time order correlators (OTOCs). To do so, we consider an all-derivative order generalisation of the Schwinger-Keldysh EFT of hydrodynamics extended to a four-fold time contour required to capture OTOCs. A crucial ingredient of the construction is a local SL(2,R) symmetry, which has previously been suggested as a mechanism for scrambling. We also derive this exact EFT from the microscopic formulation of the maximally chaotic low-temperature limit of the SYK lattice, thereby determining all transport coefficients for this model. As a novel application, we compute the OTOC of energy currents, find that its exponential growth saturates the chaos bound, and match it to expectations based on a shockwave (or scramblon) effective description. Our work shows that the universality of hydrodynamics degrees of freedom extends beyond traditional time-ordered correlators to more complex observables such as OTOCs.
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All authors Marta Bucca, Akash Jain, Márk Mezei, Alexey Milekhin

Strongly Correlated Electrons

Magnetic properties and excitation spectrum of the S = 1/2 three-legged spin ladder, LiMoOP2O7

We report a comprehensive experimental study including density functional theory calculations detailing the magnetic ground state of the $S = 1/2$ Mo$^{5+}$ pyrophosphate, LiMoOP2O7, and its magnetic excitations. Neutron powder diffraction measurements confirm the $P2_1/n$ structural model which is comprised of a three-legged ladder of distorted Mo$^{5+}$ octahedra. Magnetometry and specific heat reveal a long-range magnetic ordering transition at $T_\textrm{N} = 3.5$~K and a field-induced transition at $\mu_{0}$H$_\textrm{c}$ = 1 T. This zero-field long-range magnetic order was determined to be a commensurate $\kappa = 0$ order with an ordered moment that is reduced from the full $S = 1/2$ magnetic moment by 30%. Through inelastic neutron scattering measurements and density functional theory calculations, we define the minimal microscopic model and resolve the spin Hamiltonian up to the seventh leading exchange parameter, resulting in a model with dominant antiferromagnetic leg interactions, weaker ferromagnetic rung interactions, and a significant interlayer ferromagnetic coupling.
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All authors Aly H Abdeldaim, Alexander A. Tsirlin, Jacques Ollivier, Clemens Ritter, Robin S. Perry, Lucy Clark, Gøran J. Nilsen

Strongly Correlated Electrons

Quantum Ising transition on the Cayley tree: boundary criticality, universality, and an effective Bethe line

We investigate quantum criticality in the transverse-field Ising model on finite Cayley trees and demonstrate that their extensive boundary fundamentally changes the nature of the quantum phase transition compared with the infinite, boundary-free Bethe lattice. Using tree tensor-network simulations for systems with up to $N=12286$ sites, we identify a boundary-driven continuous transition at $h_x^c\approx1.76$, distinct from the mean-field Bethe-lattice transition at $h_x^c\approx2.23$. We characterize this transition through finite-size scaling of the magnetization and magnetic susceptibility and extract a consistent set of critical exponents. By introducing next-nearest-neighbor interactions, we demonstrate the robustness of the extracted critical exponents, providing numerical argument for the Ising boundary universality class on the Cayley tree. Furthermore, we show that the physics of the boundary-free Bethe lattice can be efficiently recovered on a finite Cayley tree by fine-tuning a local boundary field. The resulting effective Bethe line, whose existence is tied to the mean-field nature of the bulk transition, effectively screens the extensive boundary and restores both the critical point and the mean-field critical scaling of the infinite Bethe lattice.
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Strongly Correlated Electrons

Destructive Interference of a Charge Density Wave in the Skyrmion Magnet GdRu2Si2

In skyrmion magnets, charge density waves induce higher-order exchange interactions that can select multi-Q ground states. Using resonant X-ray scattering and neutron diffraction, we measure temperature-dependent spin-charge coupling in GdRu2Si2. A minimal Landau model with one critical exponent and two ordering temperatures reproduces all six observed order parameters. Spin-density wave components of the multi-Q ground state drive charge ordering, but the onset of a magnetic helix suppresses it via destructive interference.
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All authors G. D. A. Wood, D. A. Mayoh, F. Orlandi, A. Bombardi, D. D. Khalyavin, P. Manuel, S. H. Moody, P. D. Hatton, R. D. Johnson, T. W. Chamberlain, O. A. Petrenko, M. R. Lees, G. Balakrishnan

Strongly Correlated Electrons

Confinement-deconfinement transitions in the dimer-loop models on two-dimensional non-bipartite lattices

Recent work [Kundu, Damle, Phys. Rev. X 15, 011018 (2025)] has demonstrated that a class of $S=1$ kagome lattice antiferromagnets with competing anisotropies can exhibit unusual low-temperature behavior that is best described in terms of the statistical mechanics of an interesting interpolation between the fully-packed dimer model and the fully-packed loop model on the bipartite honeycomb lattice. On this and other bipartite lattices in two and three dimension, such fully-packed dimer-loop models generically have two distinct power-law correlated Coulomb phases, both of which admit a low-energy description in terms of a fluctuating divergence-free polarization vector field [Phys. Rev. X 15, 011018 (2025); arXiv:2510.11607]. The transition between these phases corresponds to a confinement transition for the $Z_2$ part of the corresponding $U(1)$ flux [Phys. Rev. X 15, 011018 (2025); arXiv:2510.11607]. Here we demonstrate that a variant of such a topological confinement transition can also exist in dimer-loop models on non-bipartite lattices such as the kagome and triangular lattices although the low-energy description does not feature any conserved $U(1)$ flux. In these non-bipartite dimer-loop models, both phases are short-range correlated liquids, and the topological distinction between them is in terms of a $Z_2$-valued winding number instead of the flux of a divergence-free polarization field. In spite of this key difference, this transition appears to be in the same Ising universality class as the analogous transition of the bipartite dimer-loop models. These kagome and triangular lattice dimer-loop models correspond respectively to the low-energy limit of a class of $S=1$ antiferromagnets with competing anisotropies on the ruby lattice comprising a corner-sharing arrangement of fully-frustrated squares and a lattice of corner-sharing fully-frustrated hexagons.
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Strongly Correlated Electrons

Topological Chiral Superconductivity from Doping Correlated Charge Transfer Insulator with Orbital Magnetism

Topological chiral superconductivity has been extensively studied from the perspective of electronic structures in momentum space, while its emergence from real-space processes in strongly interacting systems remains largely unexplored. Here, we study a doped charge-transfer insulator in a strongly repulsive spinless-fermion model with three sublattices and $2\pi$ flux per unit cell. Combining perturbative analysis, exact diagonalization, and density matrix renormalization group simulations, we establish a topological superconducting ground state with $p+ip$ symmetry. In the large charge-transfer gap limit, chiral charge-transfer excitations generate a correlated-hopping process that provides a microscopic mechanism for electron pairing and its chiral structure. The chiral superconductivity persists into the smaller-gap regime, where chiral excitonic two-particle bound state can emerge. Our results establish a concrete real-space route to topological chiral superconductivity upon doping strongly interacting charge-transfer insulators with orbital magnetism.
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All authors Wen Sun, Yuan Yang, Shou-Shu Gong, Wen Huang

Strongly Correlated Electrons · Cross-listed from cond-mat.mes-hall

Nontrivial topological properties from the cooperation of static perturbations and Floquet fields in type-II semi-Dirac semimetals

In this work, we present a comprehensive theoretical study for the topological and anomalous transport properties of type-II SDSMs under three scenarios, i.e., static symmetry-breaking perturbations, periodic Floquet driving by two-frequency orthogonally polarized light (TFOPL), and their cooperative effects in the hybrid scenario. We first show that a static mass $m_z$ opens a bulk gap and drives the system into a Chern insulator with Chern number $C^{\rm per}=\pm 2\,{\rm sgn}(m_z)$. In comparison, TFOPL alone only shifts the positions of Dirac points and cannot open a full gap. Nevertheless, it produces a Berry curvature odd in the $x$-direction, yielding a finite Berry curvature dipole (BCD) along $x$ proportional to the sine of the initial phase, while the $y$-component vanishes. The hybrid scenario, by contrast, exhibits a remarkably rich phenomenology. Specifically, its gap-closure criterion becomes cubic and thus admits up to three real roots when the effective parameter along the $x$-direction is negative, thereby producing multiple light-tunable gap-closing points and a series of topological phase transitions. In particular, the BCD exhibits a double-peak structure with strong enhancement near gap-closing manifolds and synchronized sign reversal of the full vector under external tuning. We further analyze the anomalous Hall conductivity (AHC), anomalous Nernst conductivity (ANC), and anomalous thermal Hall conductivity (ATHC). The AHC and ATHC exhibit quantized plateaus that serve as signatures of Chern-insulator phases, while the ANC, being a Fermi-surface probe, provides complementary local information and can identify light-induced gaps even when global topological invariants remain unchanged. Taken together, these results offer useful insights into the topological properties of 2D type-II SDSMs and related systems.
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Strongly Correlated Electrons

Scalable Quantum Monte Carlo for Shannon-Rényi Entropy: An Experiment-visitable Probe of Quantum Phases and Criticality

The Shannon-Rényi (SR) entropy characterizes the probability distribution of many-body wave functions in a chosen basis and is directly accessible from single-shot measurement snapshots in cold-atom experiments, yet its theoretical evaluation in interacting systems carries exponential cost. Here we construct a field-theoretic spacetime manifold for the SR entropy in which $q$ replicas are glued at the imaginary-time boundaries, recasting it as a ratio of generalized partition functions amenable to large-scale quantum Monte Carlo simulation. On this basis we develop a reweight-annealing framework with two complementary strategies: a virtual-parameter scheme interpolating between unglued and fully glued limits via binomial-weighted partial gluing, and a real-parameter scheme using a physical coupling constant as the annealing variable within stochastic series expansion. Both reduce the computational cost from exponential to polynomial. Most importantly, we establish for the first time a finite-size scaling theory for the SR entropy near a quantum critical point, $S_q=a(g)L^2+S_q^0\left((g-g_c)L^{1/\nu}\right)$; data collapse of its first derivative yields the correlation-length exponent $\nu$ for both the O(3) and Ising universality classes, realized in the spin-$\frac{1}{2}$ columnar dimerized Heisenberg model and the bilayer Heisenberg-Ising model. The same simulations extract the Goldstone-mode count $N_G=2$ and the $Z_2$ ground-state degeneracy $\ln 2$ from subleading terms. These results elevate the SR entropy to a standalone, order-parameter-free diagnostic of quantum criticality with the same scaling status as the entanglement entropy, and close the loop between theory and quantum simulation by enabling quantitative benchmarking of experimental snapshots from state-of-the-art quantum simulators.
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All authors Dong-Xu Liu, Zhe Wang, Zenan Liu Yi-Ming Ding, Zheng Yan