Peer Revenue Publish or profit

Papers

Fresh from arXiv, typeset properly. Highlighted words trade on the market.

Physics Condensed Matter Strongly Correlated Electrons

cond-mat.str-el Watch Strongly Correlated Electrons (sign in to use)

Tuesday 29 September

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

Accidental accuracy and formal consistency in $GW$+BSE: Exact benchmarks and regime-dependent error cancellation

Standard many-body perturbation theory for optical excitations combines the $GW$ approximation for quasiparticle energies with the Bethe-Salpeter equation (BSE) for the electron-hole response. Formally, the BSE kernel must equal the functional derivative of the self-energy, $K=\delta\Sigma/\delta G$. In routine practice, however, the kernel is built from a statically screened direct interaction and a bare exchange interaction, which breaks this consistency. Using exact diagonalization of the extended Hubbard dimer, we construct a controlled benchmark that isolates the price of this inconsistency. We show that the internally inconsistent practical $GW$+BSE construction frequently yields accurate optical gaps through accidental cancellation between an underestimated $GW$ gap and an oversized bare-exchange kernel, and we map the regions of parameter space where this accidental accuracy occurs. Upon switching on the nearest-neighbor interaction and binding the exciton, the practical construction remains the accurate one throughout the weak-binding regime, with cancellation optima at parts in $10^{3}$, while the frozen-$W$ construction fails at every binding strength. Beyond a binding threshold both static constructions deteriorate, showing that deeply bound excitons require physics beyond any static kernel. Accidental accuracy is therefore a property of the weak-binding regime, and the systematic failure of the frozen-$W$ derivative kernel within the explored parameter space traces to its overscreening of the exchange channel. The accuracy of the practical kernel is an accidental cancellation of two independent errors, an underestimated quasiparticle gap and an oversized exchange term, not a hidden consistency. These results provide a controlled taxonomy of approximation failure in $GW$+BSE and a precise diagnostic for when standard workflows can be trusted.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from cond-mat.supr-con

Imaging phase winding in topological superconductors with a fork-tip Josephson STM

The complex phase winding in a topological superconductor remains challenging to access by conventional real-space probes. We propose a scheme to probe this winding with a fork-tip Josephson STM near an impurity, where two superconducting tips form an interferometer sensitive to phase differences between two positions. The signal remains accessible even if the relative phase between the fork-tip and sample fluctuates, establishing a route towards a local phase-sensitive STM probe of topological superconductivity. We numerically compute the interference pattern to demonstrate that the magnitude and phase of the order parameter can be reconstructed as a function of angle, providing a route towards resolving the longstanding open experimental problem of directly detecting phase winding in topological superconductors.
Read the full abstract

Strongly Correlated Electrons

Neural-quantum-state based downfolding of the three-band Emery model for cuprates and nickelates

Understanding the physics underlying high-temperature superconductivity in cuprates and, more recently, infinite-layer nickelates has remained a central challenge in condensed-matter physics. We establish neural quantum states (NQS), specifically Hidden Fermion Determinant States (HFDS), as a scalable variational approach to the three-band Emery model of the copper- and nickel-oxide layers in these materials. After benchmarking HFDS against matrix product states on width-two geometries, we study ground states of fully two-dimensional (2D) systems of up to $10\times10$ unit cells ($300$ sites). We characterize the momentum-space distribution of dopants and find a pronounced electron-hole dichotomy similar to cuprate experiments. We further downfold the three-band model to effective single-band descriptions by constructing interacting Wannier functions. We consider a wide range of parameters – from the charge-transfer regime relevant to cuprates to the Hubbard-Mott regime of nickelates, as well as systematic scans of the charge-transfer gap that has been demonstrated to impact the critical superconducting temperatures. Across all regimes, the effective model significantly deviates from the usual Fermi-Hubbard model: The typical ratio $U/t$ is enhanced, some parameters experience a significant doping dependence, and sizable terms beyond the conventional Hubbard model are present, most notably a density-assisted hopping $t_n$. Notably, in all effective models, $t_n$ has the largest contribution to particle-hole asymmetry, rather than next-nearest-neighbor hopping contributions. The effective parameters sensitively depend on the charge-transfer energy, doping, and interaction ratios. Our results establish HFDS as an efficient tool for studying the 2D Emery model and demonstrate that single-band descriptions can require interaction terms generated by the underlying multi-band models.
Read the full abstract

Strongly Correlated Electrons

Boundary Criticality in (2+1)-dimensional U(1) Dirac Quantum Spin Liquid

An emergent gauge field can control boundary critical behavior without changing the bulk quantum spin liquid. We investigate the boundary criticality in $(2+1)$-dimensional $U(1)$ Dirac spin liquid, whose low-energy physics is described by massless quantum electrodynamics. Using a perturbative renormalization-group analysis in a half-space, we show that Neumann and Dirichlet boundary conditions for the emergent gauge field lead to distinct boundary universality classes. We determine the boundary scaling dimensions of the fundamental fields and gauge-invariant operators that provide observable signatures. We further propose a fermion-gauge lattice model with tunable boundary interactions as a microscopic setting for realizing and probing these boundary universality classes.
Read the full abstract

All authors Huan Jiang, Zhiming Pan, Xue-Jia Yu, Shao-Kai Jian

Strongly Correlated Electrons · Cross-listed from math-ph

On the Spectrum of Some Temperley-Lieb Spin Chains

We review mathematical results about the spectrum of spin-$s$ chains with a nearest neighbor interaction given by the projection onto the singlet state of two spin-$s$ degrees of freedom. Up to normalization, these interaction terms generate a Temperley-Lieb algebra at loop parameter $d=2s+1$. We also present several new results. First, we prove a ferromagnetic ordering of energy levels across symmetry sectors of the model, thus generalizing a previous result of Nachtergaele, Spitzer and Starr (2004) for the spin-$\tfrac12$ $XXZ$ chain. This enables us to determine a uniform lower bound on the finite volume spectral gap for these spin chains. By combining a variational estimate with Knabe's finite size criterion, we show that the exact spectral gap of the GNS Hamiltonian of the fully polarized state is $1-2/d$. Furthermore, this value serves as a lower bound for the gap of the maximally mixed ground state. Finally, we show that the ground state projectors on open chains satisfy the Jones-Wenzl recursion, thereby recovering a known result that the degeneracies are the quantum integers $[L+1]_q$ for $q+q^{-1}=d$. We discuss how the high degeneracy of the ground states allows the model to break a continuous symmetry while remaining gapped, and renders that gap unstable.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

3/8 charge-density wave instability in the kagome metal CsV$_3$Sb$_5$

The kagome metal CsV$_3$Sb$_5$ exhibits charge density wave (CDW) and superconducting transitions, both of which are substantially affected by pressure. Recent x-ray diffraction experiments identify a new charge-ordered phase at a pressure coinciding with the dip of the superconducting dome. This CDW phase displays a distinctive wavevector $\mathbf{Q} = (3/8, 0, 1/2)$ and monoclinic symmetry, in contrast to the $2\times2\times 2$ and $2\times2\times 4$ orders reported at ambient pressure. In this letter, we show that density functional perturbation theory (DFPT) calculations on a fine reciprocal-space grid predict the leading lattice instability of CsV$_3$Sb$_5$ to be at this wavevector. Finite-displacement calculations reveal that while anharmonic effects stabilize the conventional $L_2^-$ CDW at ambient pressure, the competing $3/8$ instability becomes energetically favorable above $\sim$1 GPa, consistent with experimental observations. Interestingly, the nesting function displays a peak at the same wavevector. A Landau free energy analysis explains the emergence of the monoclinic distortion observed in x-ray diffraction, in addition to several bond-ordering patterns that may be relevant to the observed trends in the superconducting $T_c$.
Read the full abstract

All authors Luca Buiarelli, Hyeonseo H. Park, Ethan T. Ritz, Rafael M. Fernandes, Turan Birol

Strongly Correlated Electrons · Cross-listed from cond-mat.mes-hall

Interlayer Fermi Polarons in Bilayer MoTe$_2$

Atomic bilayers of transition metal dichalcogenides (TMDs) host quantum phases governed by the layer degree of freedom, including bilayer Wigner crystals, fractional Chern insulators, and exciton condensates. These phases are probed primarily through exciton spectroscopy, yet it remains poorly understood how excitons and carriers interact to form Fermi polarons in bilayers, where both the impurity and the Fermi sea carry a layer pseudospin. Progress has been limited because most TMD bilayers have momentum-indirect optical bandgaps, in which non-radiative decay and inhomogeneous broadening obscure the intrinsic spectra. Here, we show that bilayer MoTe$_2$, unlike most TMD bilayers, retains a direct optical bandgap, providing a clean platform for studying bilayer Fermi-polaron physics. In a dual-gated device, an out-of-plane electric field continuously tunes the hybridization between intralayer and interlayer excitons, forming layer-coherent excitons. Upon electrostatic doping, the excitonic spectrum evolves into multiple polaron branches, controlled by both carrier doping and the out-of-plane electric field. Among these, we identify a polaron with no analog in monolayers, in which a layer-coherent exciton is dressed by carriers in the opposite layer, and is quantitatively captured by our field-theoretic model. Our results establish that pseudospin structure in both the impurity and the bath reshapes polaron formation, opening new avenues to many-body states such as Bose-Einstein condensates with interlayer coherence.
Read the full abstract

All authors Ruihao Ni, Eugen Dizer, Maximilian Wolf, Son T. Le, Sharadh Jois, Jeffrey J. Schwartz, Liuxin Gu, Rundong Ma, Suji Park, Beini Gao, Lifu Zhang, Houk Jang, Takashi Taniguchi, Kenji Watanabe, Aubrey T. Hanbicki, Adam L. Friedman, Richard Schmidt, You Zhou

Strongly Correlated Electrons

Variational Monte Carlo for the Hubbard model

In these lecture notes, we introduce the variational Monte Carlo method for the Hubbard model. First, we briefly introduce the single-orbital Hubbard model and its multi-orbital extension, focusing only on electronic models. Then, we introduce the general scheme under which variational Monte Carlo works and we present the variational wave functions that can properly describe superconductive and magnetic states in single-orbital and multi-orbital Hubbard models. We also detail how to perform Monte Carlo calculations for the given wave functions. We also describe how to optimize a variational wave function with the stochastic reconfiguration method. Finally, we present a few results for correlation functions that can be computed in variational Monte Carlo, to determine, for instance, the presence of charge or spin order and superconductivity.
Read the full abstract

Strongly Correlated Electrons

Strong-to-Weak Spontaneous Symmetry Breaking of Dephased Fermions

Strong-to-weak spontaneous symmetry breaking (SWSSB) is a novel phase transition in mixed states associated with the loss of global charge information. In this work we study fermions with $U(1)$ symmetry under infinite density dephasing and derive the SWSSB properties of the resulting mixed states. Our central observation is that at infinite dephasing every Renyi correlator is exactly the spin-spin correlator of a compact XY model, whose Boltzmann weight is the squared full-counting-statistics generating function of a classical ensemble built from the parent state. For the Renyi-2 correlator it is the full counting statistics of the parent state itself. We complement the infinite dephasing mapping with a novel diagrammatic expansion for the Renyi-1 correlator, applicable to any diagonal mixed state, which computes the couplings of the Renyi-1 XY model. We also study a replica field theory for even Renyi index quantities, applicable at finite dephasing. Our analysis indicates that fully dephased metals display long-range SWSSB in $d\geq 2$, as confirmed numerically and experimentally in $d=2$, and quasi-long-range SWSSB in $d=1$. For insulating parent states both an SWSSB and a trivial phase are possible at infinite dephasing depending on UV details. Long-range SWSSB in $d\geq 3$, or quasi-long-range SWSSB in $d=2$, survives above a nonuniversal, Renyi-index-dependent threshold and is lost when the parent state is deep in the insulating phase, with the exception of quantum Hall insulators which generically have quasi-long-range SWSSB. For even Renyi indices we also determine the stability of the SWSSB phase away from infinite dephasing and derive the universality class of the SWSSB transition.
Read the full abstract

Strongly Correlated Electrons

Correlation-assisted topological and metamagnetic transitions in Rashba-coupled superconductors: $t$-$J$-$U$ model study

Unconventional superconductivity commonly emerges in systems characterized by strong electronic correlations, with layered copper-oxides serving as a canonical example. Observation of spin-momentum locking within Bi-family of the cuprates, compatible with the presence of non-negligible Rashba-type spin-orbit coupling (RSOC), calls for an investigation of the joint effects of electronic correlations and RSOC on pairing in copper-oxide and related superconductors. Employing statistically-consistent variational approximation (SGA), we carry out such an analysis by constructing the phase diagram for the case of square-lattice t-J-U model incorporating RSOC. We also investigate the effects of time-reversal-symmetry breaking by Zeeman field, as well as characterize emergent topological superconducting (TSC) states. Chern number $C = \pm 4$ TSC is found in a broad regime of on-site Coulomb repulsion close to half-filling. The latter is not governed by correlations and emerges also within the weak-coupling Bogoliubov-de Gennes (BdG) scheme. Yet, we identify a distinct $C = \pm 2$ TSC state that is driven specifically by electronic correlations via a topological transition occurring with no bulk quasiparticle gap closure, and is accompanied by discontinuous metamagnetic and Lifshitz transitions. Moreover, a qualitatively distinct doping evolution of the $d$- and $p$-wave components of the underlying mixed-parity SC order parameter above the metal-to-insulator transition is demonstrated. Our work points toward the relevance of joint correlation and RSOC effects beyond BdG scheme to phase diagrams of RSOC-coupled superconductors.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

From Chemical Complexity to Tunable Magnetic Ordering in Highly Disordered High-Entropy Spinel Oxides

High-entropy stabilization chemistry is redefining materials design by transforming configurational disorder, arising from the deliberate incorporation of multiple principal cations, into a thermodynamic advantage that promotes phase stability and enables emergent functionalities. In this work, we investigate the evolution of magnetic ordering in spinel-type high entropy oxides by systematically varying the cation composition of the B site within a fixed high-entropy A-site matrix, (Ni$_{0.2}$Mg$_{0.2}$Co$_{0.2}$Cu$_{0.2}$Zn$_{0.2}$)B$_2$O$_4$. Upon introducing multicomponent B-site configurations, we uncover a strikingly linear dependence of the magnetic transition temperature (T$_C$) on the T$_C$s of the corresponding single B-site high-entropy systems. Remarkably, this trend persists even in highly complex (Ni$_{0.2}$Mg$_{0.2}$Co$_{0.2}$Cu$_{0.2}$Zn$_{0.2}$)(Cr$_{0.2}$Mn$_{0.2}$Fe$_{0.2}$Ga$_{0.2}$X$_{0.2}$)$_2$O$_4$, X = Al and Ti. Despite the material's extremely high degree of disorder, absence of a dominant magnetic ion or a straightforward superexchange pathway, detailed magnetization measurements, low-temperature X-ray magnetic circular dichroism, and neutron powder diffraction studies reveal robust long-range ferrimagnetic ordering. These results reveal an emergent predictability in ferrimagnetic high-entropy spinel oxides, where, despite extreme configurational disorder and competing interactions, robust ferrimagnetic order can arise from, rather than be hindered by, extreme configurational disorder. This establishes a pathway for predictively tuning magnetic transition temperatures in high-entropy oxides beyond conventional ordered systems.
Read the full abstract

All authors Neha Sharma, Sushanta Mandal, Nikita Sharma, Amritpal, Sangeeta Thakur, Viktor Ukleev, Chen Luo, Florin Radu, S. D. Kaushik, Tirthankar Chakraborty, Sanjoy Kr. Mahatha, Denis Pelloquin, Sourav Marik

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

Chemical-Disorder-Induced Non-metallic Transport in Thermodynamically Metallic Mo4TGa16Ge (T = Co, Rh or Ir)

Flat-band electronic states can be highly sensitive to chemical perturbations, offering opportunities to access a broader range of electronic behaviors beyond that of parent materials. Here, we report the discovery of a new series of compounds, Mo4TGa16Ge (T = Co, Rh, or Ir), derived from the strongly correlated flat-band superconductor, Mo4PtGa17, via nominally preserving the total valence electron counts. All three materials crystallize in a noncentrosymmetric cubic space group, F-43m, with Ge selectively occupying one of the Ga sites in the parent compound. Although the total electron count remains the same, Mo4TGa16Ge exhibits significantly distinct properties from Mo4PtGa17. Theoretical calculations predict metallic electronic structures with narrow, dominant Mo-d states at the Fermi energy, while low-temperature heat capacity results demonstrate finite Sommerfeld coefficients. However, electrical transport measurements show predominantly non-metallic behaviors with small observed activation energies, excluding the possibilities of conventional semiconducting behaviors. Combining chemical bonding analysis, electronic structure and compositional determination from X-ray crystallography and spectroscopy, we propose that the coexistence of the non-metallic transport features and the thermodynamically metallic behaviors can be attributed to the high sensitivity of the narrow-band materials to chemical disorders. Thus, the discovery and investigation of Mo4TGa16Ge provide a chemically tunable platform for studying disorder-controlled transport in flat-band intermetallics.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from hep-lat

Boundary Condition dependent Universality Classes on a Hyperbolic Lattice

We study the ferromagnetic Ising model on finite hyperbolic tessellations of Euclidean AdS$_2$ with open and wired boundary conditions. Because a finite fraction of spins remains at the boundary as the lattice grows, these conditions select distinct thermodynamic behaviours. In the $\{5,4\}$ tessellation, Monte-Carlo simulations using efficient worm algorithms on open boundaries (OBC) yield a transition near $\beta_c J=0.632(3)$, with susceptibility data collapsing under scaling by the total number of spins $N$. The fitted finite-size exponents, $1/\bar{\nu} \simeq 0.162$ and $\gamma/\bar{\nu} \simeq 0.743$, differ substantially from the mean-field volume scaling. Wired boundaries (WBC), which correlate boundary spins, instead show a transition around $\beta_c J=0.348(4)$ to an ordered phase consistent with the mean-field exponents. While the mean-field criticality with WBC is consistent with previous studies and with the suppression of independent boundary fluctuations, the OBC exponents hint at the presence of a new universality class. Results from other tessellations support the robustness of the observed scaling with OBC. We discuss a possible route to interpolate between the different boundary conditions. Our findings show that boundary dynamics must be specified when characterizing critical behaviour on hyperbolic lattices.
Read the full abstract

All authors Pallabi Dey, Debasish Banerjee, Arnab Kundu, Ritam Sinha

Strongly Correlated Electrons

Uniform-Charge-Density $d$-Wave Superconductivity in the Pure $t$-$J$ Model at $1/8$ Doping on an Infinite Cylinder

The ground state of the square-lattice $t$-$J$ model at $1/8$ hole doping has been the subject of a long-standing controversy, with conflicting numerical reports of stripe order versus superconductivity. Here, we address this debate using the variational uniform matrix product state (VUMPS) method, which optimizes the wave function directly in the thermodynamic limit along the cylinder axis and eliminates the boundary pinning effects that can arise in finite-cylinder calculations. On an infinite cylinder of circumference $L_y = 8$, we find a uniform-charge-density $d$-wave superconducting ground state with quasi-long-range pairing correlations. The dominant pairing occurs at zero center-of-mass momentum, while no sizable finite-momentum pairing component is detected. Twisted-boundary-condition calculations reveal a finite superconducting phase stiffness, with the order-parameter phase winding smoothly to follow the applied flux, providing an independent probe of the robustness of the superconductivity. Moreover, both charge and spin correlations decay rapidly, with no signatures of long-range stripe or magnetic order, in contrast to an $L_y=6$ cylinder at $1/6$ doping where the same method readily identifies stripe order. Our results provide methodologically distinct evidence in the long-standing stripe–superconductivity debate in the pure $t$-$J$ model and reveal uniform $d$-wave superconductivity in a minimal model of doped Mott insulators.
Read the full abstract

Strongly Correlated Electrons

Evolution of Magnetism in Ce$_4$Ge$_7$ under Magnetic Field and Pressure

We report the magnetic and transport properties of single-crystalline Ce$_4$Ge$_7$, which crystallizes in a non-centrosymmetric orthorhombic structure (space group C222$_1$). It undergoes an antiferromagnetic transition at $T_N$ = 7.3 K. When a magnetic field is applied along the $b$-axis, a metamagnetic transition occurs at 1.3 T (at 2 K). Correspondingly, this transition gives rise to an anomalous Hall effect, which is dominated by the intrinsic Karplus-Luttinger mechanism. Under hydrostatic pressure, $T_N$ of Ce$_4$Ge$_7$ initially increases slightly and is then gradually suppressed. For pressures above $P_c$ = 10.2 GPa, no magnetic order is observed. The divergence of the $A$ coefficient, the maximum of the residual resistivity, and the non-Fermi liquid behavior around $P_c$ indicate the possible existence of an antiferromagnetic quantum critical point in Ce$_4$Ge$_7$.
Read the full abstract

All authors Kaixin Ye, Qihe Yu, Yongjian Li, Yanan Zhang, Ye Chen, Rui Li, Lin Jiao, M. Smidman, Yongjun Zhang, Yu Liu, Huiqiu Yuan

Strongly Correlated Electrons · Cross-listed from cond-mat.quant-gas

Finite-momentum trimers and Cooper quartets in a one-dimensional Fermi gas with coexistent $s$- and $p$-wave interactions

We study finite-momentum trimers and Cooper quartets in a one-dimensional two-component Fermi gas with coexistent $s$- and $p$-wave interactions, regularized in the relative momentum of each pair so that they remain Galilean invariant. Pauli blocking alone then makes the trimer dispersion deviate from free center-of-mass motion, so the trimer energy can be lowest at finite total momentum. Allowing this motion expands the $abb$ region among pairs and trimers and removes the region where an odd-wave pair is lowest. The $aabb$ quartet lies below all these branches at every sampled coupling, and in a strip starting on the crossing of the two dimer-pair channels its lowest breakup channel is a moving $abb$ trimer and an atom. At weak interspecies attraction, a variational bound shows that two odd-wave Cooper pairs bind into a quartet, whose binding exceeds that of the coexisting trimer by orders of magnitude as the attraction weakens. At stronger interspecies attraction, the quartet binding relative to two unlike-species dimers disappears when the odd-wave interaction is switched off, although the even-wave interaction dominates the interaction energy. Relative to the in-vacuum case, the Fermi sea enhances the weak-coupling quartet binding, and at fixed scattering lengths the quartet binding grows with density while the coexisting trimer becomes much shallower. These results show that neither the most strongly bound pair nor the dominant interaction energy alone determines whether the quartet binds.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from physics.comp-ph

From Bellissard's gap labeling to atomistic quasiperiodic bilayers

Bellissard's framework uses covariant observables to describe aperiodic solids. We examine how butterfly-like spectra in twisted bilayers can be related to bulk gap labels and topological response. A bulk gap permits a spectral projector and an integrated density of states. A topological response requires an additional pairing of that projector. In an illustrative finite honeycomb bilayer, an exact second-moment identity isolates the interlayer contribution to spectral variance. Angle-resolved spectra, finite state counts, an uncoupled reference, and size and broadening checks show how coupling redistributes spectral weight without assigning a bulk gap label. We then examine the requirements for atomistic electronic-structure calculations, including nonorthogonal orbitals, projected densities of states, and basis functions that move during relative sliding. The resulting framework specifies the steps needed to connect atomistic spectra with bulk state counting and topological response.
Read the full abstract

Strongly Correlated Electrons

Ergodicity in a hole-doped Anderson spin insulator

An interacting many-body system being localized in the presence of disorder can fail to serve as its own bath. In an electronic system, the charge and spin degrees of freedom can act as thermal baths for each other. In this paper, we study the stability of an Anderson insulator in the spin sector with respect to charge doping. We consider one-dimensional two-component fermions in a lattice with large onsite repulsion ($t-J_{XX}$ model) and with a single hole in a random magnetic field. In the absence of the hole the spin sector is localized in arbitrarily weak random magnetic fields. We argue that a single hole thermalizes the spin chain in the weak disorder limit. In this regime our numerical results indicate ergodicity of the system as a whole and delocalization of the hole. At larger magnetic fields the hole eventually localizes with a finite localization length, and the Anderson spin insulator is restored.
Read the full abstract

Strongly Correlated Electrons

Quantized Hyperfine Field at an Implanted $\mu^+$ Site in PrPb$_3$: Interplay between Localized $f$ Electrons and an Interstitial Charged Particle

The local effect of an interstitial hydrogen-like particle on localized $f$ electrons was studied in PrPb$_3$ by means of $\mu^+$ spin rotation and relaxation. Spontaneous $\mu^+$ spin precession with harmonic frequencies was observed for the first time in $f$ electron compounds. We demonstrate that the signal is derived from a coupling between the $\mu^+$ spin and the hyperfine-enhanced nuclear spin of nearest neighbor (nn) $^{141}$Pr with Ising-like anisotropy. The signal also suggests a marked suppression of spin dynamics of the nn $^{141}$Pr in comparison with that of the bulk $^{141}$Pr. These facts strongly indicate modification of the $f$ electronic state due to the interstitial charged particle.
Read the full abstract

All authors T. U. Ito, W. Higemoto, K. Ohishi, N. Nishida, R. H. Heffner, Y. Aoki, A. Amato, T. Onimaru, H. S. Suzuki

Strongly Correlated Electrons

Probing the electronic structure of $\mathrm{UTe}_2$ with ARPES and high-energy spectroscopy

$\mathrm{UTe}_2$ has emerged as one of the most intensively studied strongly correlated materials in recent years owing to its unconventional superconductivity and the possible realization of a spin-triplet, topologically nontrivial pairing state. A central open issue concerns the nature of the $\mathrm{U}\,5f$ electrons and their participation in low-energy quasiparticle states. In this review, we summarize recent spectroscopic studies of $\mathrm{UTe}_2$ using momentum-resolved angle-resolved photoemission spectroscopy (ARPES) and element- and configuration-sensitive X-ray probes, including X-ray absorption spectroscopy (XAS), X-ray absorption near-edge structure (XANES), X-ray magnetic circular dichroism (XMCD), resonant X-ray emission spectroscopy (RXES), and resonant inelastic X-ray scattering (RIXS). A key finding is the pronounced technique dependence of the inferred electronic structure. We synthesize the present spectroscopic picture by integrating these results with modern electronic-structure calculations such as density functional theory plus dynamical mean-field theory (DFT+DMFT). These findings support an intermediate-valence ground state with significant admixture of $5f^2$ and $5f^3$ configurations in $\mathrm{UTe}_2$, and they delineate key experimental and theoretical benchmarks needed to connect the normal-state electronic structure to the superconducting mechanism.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from hep-th

Emergent Symmetries in Ensemble Averages

It is widely believed that there are no exact global symmetries in quantum gravity. We review recent works showing that global symmetries can nevertheless emerge after ensemble averages of theories, as encountered in holography. As a precision case study, we discuss the ensemble average of two-dimensional Narain-type conformal field theories associated with an even quadratic form of general signature, which is computed by the Siegel-Weil formula and interpreted as a sum over geometries in a three-dimensional Abelian Chern-Simons theory. Global symmetries of the bulk anyons can emerge after the average, as T-dualities relating different theories in the ensemble are "folded" into symmetries of a single theory (duality origami). We discuss the relation to the Swampland program, including the emergence of global symmetries at infinite distance. Finally, we recast strong-to-weak spontaneous symmetry breaking (SWSSB) of mixed states as an emergence of symmetries in ensemble averages; in holography, wormholes connecting the two sides of a thermofield-double construction provide its bulk realization. This motivates a new Swampland conjecture.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from cond-mat.mtrl-sci

Frustrated Gd3+ Double Perovskites as High-Performance Magnetocaloric Materials for Sub-100 mK Adiabatic Demagnetization Refrigeration

Achieving temperatures below 100 mK is essential for advancing quantum technologies and exploring fundamental quantum phenomena. While paramagnetic salts have traditionally enabled adiabatic demagnetization refrigeration (ADR), their limitations have driven the search for more effective alternatives. In this work, we present Gd3+-based double perovskites, Ba2GdSbO6 and Sr2GdSbO6, as high-performance magnetocaloric materials. Starting ADR from 2 K and 5 T, these compounds reach 67 mK and 68 mK in small finite magnetic fields, and 83 mK and 78 mK in zero field, respectively, which are the lowest reported ADR temperatures for Gd3+ magnets (S = 7/2) under these conditions. The frustrated geometry and the complex interplay of exchange and dipolar interactions suppress their antiferromagnetic ordering temperatures to 100 and 166 mK for Ba2GdSbO6 and 190 mK for Sr2GdSbO6, while maintaining an outstanding entropy density of 189 mJ K-1 cm-3 and 201 mJ K-1 cm-3, respectively. Notably, Ba2GdSbO6 sustains sub-100 mK cooling even at finite fields of 0.5 T, making it particularly promising for practical ADR applications.
Read the full abstract

All authors Tim Treu, Marvin Klinger, Christian Heil, Hans-Albrecht Krug von Nidda, Vinicius E. S. Frehse, Mamoun Hemmida, Anton Jesche, Alexander A. Tsirlin, Philipp Gegenwart

Monday 28 September

Strongly Correlated Electrons

Artificial versus Natural Atoms: The uncanny capability of the many-body Schrödinger equation to produce emergent behavior

The paper reviews the theoretical and experimental progress achieved in the last 25 years in understanding the novel physics of artificial atoms and molecules as arising from the formation of Wigner molecules (WMs) of localized (to a stronger or lesser extent) fermionic or bosonic particles, which are finite quantum analogs of the more familiar bulk Wigner crystal. The term artificial atoms, as used here, encompasses a broad range of recently fabricated quantum nanodevices and experimental apparatuses consisting of a finite number of mutually repelling confined particles, including two-dimensional semiconductor and moiré transition metal dichalcogenide quantum dots, as well as trapped ultracold neutral atoms or ions. These nano-sized or micro-sized artificial devices and apparatuses (in single well or multi-well of variable-shape arrangements) hold a great promise for technological applications in the field of quantum information and quantum computers, as well as for advances in fundamental many-body physics. Prominent quantum effects of Wigner molecularization are the strong quenching of the spectral energy gaps, the appearance of rovibational spectra (in analogy with natural molecules), entanglement, and pinning due to an external perturbation. In high magnetic fields or at rapid rotation, WMs provide an alternative theory to the fractional quantum Hall effect. The physics of Wigner molecules is shown to derive from the solutions of the many-body Schrödinger equation (MBSE) in the regime of strong interparticle correlations arising from the dominance of the potential over the kinetic energy, or from a high magnetic field, as well as from a rapid rotation... (continues in the paper).
Read the full abstract

Strongly Correlated Electrons

Quantum metric induced nonlinear transport in the hidden loop-current phase of kagome metal RbV$_3$Sb$_5$

A hidden low-temperature phase with possible loop-current order has been proposed in the kagome metals AV$_3$Sb$_5$ (A=K, Rb or Cs), but its experimental signatures remain subtle and indirect. Here, we use third-order nonlinear transport to probe this hidden phase in RbV$_3$Sb$_5$. At ~35 K, the longitudinal cubic response develops a strong kink and pronounced directional anisotropy with a strong departure from common relaxation time scaling, while the transverse cubic response acquires a magnetic field-odd component at the same temperature. Their coincident onset identifies the third-harmonic response as a sensitive marker of the low-temperature electronic reconstruction with time-reversal broken symmetry. Crucially, we find that the quantum metric quadrupole contributes directly to the longitudinal third-order response. In a loop-current charge-density-wave model, its direction selective enhancement captures the observed angular reconstruction. Our work shows how higher-order nonlinear transport translates subtle changes in electronic symmetry and quantum metric into measurable electrical signatures in quantum materials that is important for studying complex electronic phases of matter.
Read the full abstract

All authors Jia-Chen Shi, Shupeng Xu, Utkarsh Khandelwal, Nashra Pistawala, Luminita Harnagea, Steven J. May, Ritesh Agarwal

Strongly Correlated Electrons

Magnetic properties and Fermi-surface topology of kagome magnet HoV$_6$Sn$_6$

We report a study of the magnetic properties and Fermi-surface topology of the kagome magnet HoV$_6$Sn$_6$ using magnetization and tunnel-diode-oscillator (TDO) measurements. The temperature-dependent magnetization exhibits Curie-Weiss behavior at high temperatures and reveals long-range magnetic order below $T_c$ $\approx$ 2.4 K. Below Tc, the field-dependent magnetization reveals pronounced magnetic anisotropy, with saturation moments of $\approx$ 9.5 and 7 $\mu_B$ /Ho for fields applied along the out-of-plane and in-plane directions, respectively. To probe the Fermi surface, we perform TDO measurements in magnetic fields up to 41.5 T and at temperatures down to 0.35 K. The TDO signal exhibits well-defined quantum oscillations with multiple frequencies extending up to $\sim$ 9 kT. Angular- and temperature-dependent measurements are used to determine the Fermi-surface geometry and cyclotron effective masses, respectively. To elucidate the electronic structure, we perform first-principles calculations of the electronic bands, density of states (DOS), and Fermi surface. The calculated band structure exhibits flat-band features, van Hove singularities, and Dirac-like crossings near the Fermi level. The DOS near the Fermi level is dominated by the V-d orbitals, indicating that the V kagome layers play a major role in determining the low-energy electronic properties of HoV6Sn6. Our calculations further support a ferromagnetic ground state with the Ho moments oriented along the c axis, consistent with neutron-scattering measurements. The calculated quantum-oscillation frequencies from the Fermi-surface pockets of HoV6Sn6 are in overall good agreement with the experimentally observed frequencies. Our combined experimental and theoretical results provide insight into the magnetic anisotropy and electronic structure of HoV$_6$Sn$_6$ and reveal its multiband Fermi-surface topology.
Read the full abstract

All authors Tucker Beekmann, Ganesh Pokharel, Wyatt Edward Ackerman, Stephen D. Wilson, David E. Graf, Keshav Shrestha

Strongly Correlated Electrons

Magnetic excitations of the strongly-anisotropic triangular XXZ model: a projected spin-product state approach

Recent experiments have sparked interest on the ground-state properties and on the excitation spectrum of the spin-$1/2$ triangular XXZ model with strong Ising-like anisotropy. In this work, we introduce and analyze a “projected” coherent-state approximation to the model, constructed by projecting spin-product states onto the low-energy configurations of the triangular Ising antiferromagnet. Within this approximation, we discuss the structure of the ground-state ordering and the magnetization curve under a longitudinal field. We then discuss the excitation spectrum by linearizing equations of motion deriving from a time-dependent variational principle. This leads to a natural description of spin-wave-like excitations within the strongly constrained Hilbert space. At zero field, the variational approximation leads to a very flat landscape of quasi-degenerate states, which results in a low-energy pseudo-Goldstone mode in the excitation spectrum. We compare our results to experimental measurements on the cobaltite K$_{2}$Co(SeO$_{3}$)$_{2}$ (KCSO). Our approximation leads to a dramatic improvement as compared to linear spin-wave theory. However, there remain deviations in the value of the pseudo-Goldstone gap and in the dispersion near $M$ points at low field.
Read the full abstract

Strongly Correlated Electrons

Excitonic Stripe Order in the Two-Orbital Hubbard-Kanamori Model

Excitonic condensation and stripe formation are two distinct manifestations of electronic correlations. While excitonic order naturally arises in multi-orbital systems, stripe order is a prominent feature of doped correlated-electron models. Here, we investigate an excitonic analogue of stripe order in the two–orbital Hubbard-Kanamori model on the square lattice, characterized by a spatial modulation of inter-orbital particle-hole coherence and, in the orbital-parity-symmetric limit, spontaneous breaking of a relative orbital $\mathbb{Z}_2$ symmetry. Using unrestricted real-space Hartree-Fock calculations complemented by random-phase-approximation instability analysis, we determine how the Kanamori interactions select different excitonic channels. The sign of Hund's exchange controls the spin character of the condensate: ferromagnetic Hund coupling favors triplet excitonic order, whereas antiferromagnetic Hund coupling stabilizes singlet excitonic order. Upon doping, commensurate excitonic density waves develop incommensurate textures, including excitonic stripes and, in the triplet sector, spiral excitonic density waves. We further show that crystal-field splitting strongly reorganizes the excitonic instability by modifying inter-orbital nesting and can stabilize triplet excitonic order even in the absence of pair hopping. Our results establish excitonic stripes as a distinct symmetry-broken state of multi-orbital correlated systems and identify microscopic routes for their stabilization.
Read the full abstract

All authors Rafael D. Soares, Luke Staszewski, Chunhan Feng, Alexander Wietek

Strongly Correlated Electrons

Spectroscopy of phonon-coupled integer and fractional Chern insulators: emergence of polarons and chirality deficit of graviton mode

Strong electron-phonon coupling can destabilize both Chern insulators (CIs) and fractional Chern insulators (FCIs) in favor of charge order, but whether the instabilities in CI and FCI share a common microscopic mechanism remains unclear. In this paper, we address this question by studying a flat-band Haldane model coupled to dynamical Holstein phonons at integer and fractional fillings using density-matrix renormalization group with local basis optimization. We find that the low-energy effects of phonons are dominated by their dressing of charge-neutral collective modes. In the CI and FCI, phonons dress excitons and magnetorotons into composite modes that we identify as exciton polarons and magnetoroton polarons, respectively. These modes soften strongly upon approaching the transition, while the momenta of their energy minima anticipate the ordering wave vectors of the charge-ordered phases. The phonon spectrum, in turn, acquires dispersive features inherited from the exciton and magnetoroton modes, providing direct lattice signatures of these neutral excitations. Within the FCI phase, electron-phonon coupling also enhances the opposite-chirality spectral weight of the graviton response, thereby resulting in a chirality deficit. Our results provide a unified excitation-based picture of phonon-driven instabilities in CIs and FCIs and establish lattice dynamics as a probe of their neutral collective modes.
Read the full abstract

Strongly Correlated Electrons · Cross-listed from quant-ph

Digital Quantum Algorithms for Generating and Utilizing Spin Squeezed States

Spin squeezed states (SSSs) are conventionally viewed as analog resources for quantum metrology. Here we develop algorithms to efficiently generate and exploit SSSs on a digital quantum computer. We introduce an adaptive local-circuit protocol that prepares SSSs with squeezing parameter $\xi$ in depth $\mathrm{O}\left(\log{1/\xi}\right)$, yielding an exponential improvement over non-adaptive approaches. We prove that this depth is optimal for permutation symmetric SSSs by deriving a matching lower bound on entanglement entropy. We further leverage the squeezing paradigm to deterministically prepare the Dicke states using asymptotically fewer resources than prior methods. Remarkably, classical simulations of our preparation protocols under realistic noise models predicts a metrological gain of 4.2 dB beyond the standard quantum limit with 55 superconducting qubits in total including ancillae. Our work paves the way for performing quantum metrology on near-term digital quantum devices.
Read the full abstract

Strongly Correlated Electrons

Advancing Fuzzy-Sphere CFTs: $\mathrm{SO}(3)$-Rotation-Resolving Exact Diagonalization, 3D Ising Heavy Primaries, and Quasi-Hole-Space Projection

Fuzzy-sphere regularization has recently emerged as a powerful framework for studying three-dimensional conformal field theories (CFTs). In this work, we exploit symmetry and Hilbert-space structures to substantially advance this framework. We develop an exact-diagonalization algorithm that resolves the full $\mathrm{SO}(3)$ rotational symmetry, reducing computational costs by factors of several hundred. For the three-dimensional Ising CFT, we identify around 100 primary operators, including a large number of previously unknown heavy scalar primaries up to scaling dimension $\Delta\approx16.5$. We also resolve the tension between previous fuzzy-sphere and bootstrap results regarding the parity-odd scalar primary. Furthermore, we identify a branch of scalar primaries associated with $\phi^n$ operators in the $\phi^4$ Lagrangian description, beginning with the identity, $\sigma$, $\epsilon$, $\epsilon'$, and $\sigma'$. Their wave functions exhibit a semi-classical structure closely related to states invariant under area-preserving diffeomorphisms of the sphere. Finally, we show that critical points involving fractional quantum Hall states can be studied within a substantially reduced Hilbert space spanned by quasi-hole states of the corresponding model quantum Hall wave functions like the Laughlin state. This suggests a general strategy for exploring CFTs intertwined with topologically ordered phases.
Read the full abstract