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Physics Condensed Matter

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Monday 24 August

Materials Science

Composition- and Ordering-Dependent Evolution of Simulated Kikuchi Patterns of Au-Ni Alloys

Understanding how Kikuchi patterns behave with subtle material variations is essential for developing machine learning (ML) based indexing methods for structurally and chemically complex cases, such as phases with potential sub-lattice order or (meta)stable defects with segregation (defect phases). Simulated Kikuchi patterns of the binary Au-Ni system were systematically analysed to investigate the effects of lattice parameter, chemical composition, partial site occupancy and ordering. The full compositional range from pure nickel to pure gold was considered, including a hypothetical ordered L$1_2$ Au$_3$Ni structure. Simulation parameters were optimised by comparison with experimental patterns. Normalized cross correlation showed limited sensibility to subtle differences between patterns. EMsoft simulation results revealed a systematic increase in mean intensity and more reflections contribute significantly as gold content increases. A surprising four-fold increase in mean intensity from 99 % gold to the pure gold sample highlighted limitations of partial site occupancy simulation by EMsoft. Difference maps showed enhanced normalised intensity along the {111} and {200} bands for the sample with 20 % gold compared to higher gold compositions. By isolating lattice parameter and chemical composition effects, chemical composition contributes predominantly to the mean intensity and strong reflections count, although the normalised intensity distribution was affected by both. Introducing L$1_2$ ordering increased the number of strong reflections and mean intensity, and redistributed normalised intensity along {111} and {200} bands and selected zone axis. Normalised intensity distribution and band width, are key descriptions to distinguish the Kikuchi patterns, which can be incorporated in future representation learning based indexing methods.
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All authors Camila A. Teixeira, Lukas Berners, Sandra Korte-Kerzel, Ulrich Kerzel

Strongly Correlated Electrons · Cross-listed from physics.chem-ph

Importance-Reweighted Fock-Space Variational Monte Carlo

Fock-space variational Monte Carlo (FS-VMC) evaluates variational quantities by sampling discrete many-body configurations. In molecular applications, concentrated Born distributions can hinder Markov-chain mixing, while Monte Carlo estimators can also exhibit large variance. We introduce importance-reweighted FS-VMC (IR-FS-VMC), which combines Metropolis–Hastings sampling, an evaluation kernel, and self-normalized importance sampling to estimate the Born-distribution energy, gradient, and stochastic reconfiguration (SR) matrix. Controlled comparisons on equilibrium H2O and Fe2S2 show that the acceptance rate and local-energy variance can respond differently to the sampling and estimation procedure. A single production protocol yields accurate variational energies for H2O dissociation, 36-site hydrogen lattices, and Fe2S2 and Fe4S4 active spaces without system-specific sampling parameters.
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Superconductivity

Revised symmetry rule and intrinsically time-reversal symmetry breaking pairing in multi-orbital superconductors

We investigate the basic symmetry rule for the particle permutation in superconducting (SC) pairing states by examining the numerical solution of the linearized Eliashberg equation for Sr$_2$RuO$_4$. We find that the general multi-band, frequency-dependent SC gap function does not simply transform to itself up to the minus sign with either orbital ($\hat{O}$) or frequency ($\hat{T}$) exchange between two pairing electrons, contradicting the common assumption which has been used without verification. It originates from the fact that paring interactions are not invariant under the $\hat{O}$ or $\hat{T}$ operation, and is demonstrated to be essential to correctly interpret and understand multi-band SC states. One of unique properties implied by our newly found symmetry rule is the possibility of the complex eigenvalue in the linearized gap equation where the corresponding gap functions $\Delta$ always have real and imaginary components both non-zero in real frequencies, inherently breaking the time-reversal symmetry. Our numerical results suggest the possibility of this unique pairing in a real material, Sr$_2$RuO$_4$, for which the Hundness of the material is found to play a key role. The revised symmetry rule not only leads us to more comprehensive understanding of the known SC states, but also opens new possibilities into exotic and unique states.
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Strongly Correlated Electrons · Cross-listed from quant-ph

Deterministic Preparation of Arbitrary Spin Eigenfunctions

Quantum states with conserved total spins, or spin eigenfunctions, are important for studying quantum chemistry and quantum manybody physics problems. A typical class of spin eigenfunctions are Dicke states, which attain maximal spins. While we already have many efficient quantum algorithms to prepare Dicke states, it is not yet clear if we could do so for arbitrary spin eigenfunctions deterministically. Generalizing Bärtschi and Eidenbenz's elegant algorithms for Dicke state preparation, we successfully prepare arbitrary spin eigenfunctions characterized by branching paths and binary spin trees. As a byproduct, we also develop the corresponding classical algorithms to reconstruct all these spin states.
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Soft Condensed Matter

Spontaneous currents determine capillary rise in active matter

The capillary rise of simple passive fluids in a tube is given by Jurin's law of capillary action, which balances surface tension and gravity. For fluids composed of active particles interacting via pairwise forces, a capillary rise was reported despite a negative mechanical surface tension, a phenomenon which remains unexplained. We establish the active form of Jurin's law from the microscopic dynamics. It includes a drag emerging from particle currents that we find responsible for capillary rise. These active currents, alongside negative surface tension, lead to complex and counterintuitive capillary action phenomena that are impossible in equilibrium. In particular the capillary rise of active fluids depends on the shape of the tube, not solely on the tube diameter.
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Mesoscale and Nanoscale Physics

Fidelity susceptibility of Su-Schrieffer-Heeger model with further neighbour hopping term

In this study, topological phase transition in Su-Schrieffer-Heeger (SSH) model with a further neighbour hopping term has been studied in terms of fidelity susceptibility. Topological phase transition point in the standard SSH model has been identified before by noting the divergence of fidelity susceptibility. The same approach has been employed here where fidelity susceptibility is found to diverge at the phase transition points. Additionally, effect of staggered potential on the fidelity susceptibility has been explored. Analytic expression for fidelity susceptibility has been obtained along with its numerical estimation on finite chains by exact diagonalization. Fidelity susceptibility exhibits sharp peaks at the phase transition points in both approaches. Scaling exponent of this divergence has been obtained numerically which is found to agree to that of the standard SSH model without further neighbour terms.
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Statistical Mechanics

Note on Boltzmann's H-Theorem and Detailed Balance Dynamics

The Boltzmann H-theorem states that entropy of an ensemble of thermodynamic states increases until all states become equally probable. The evolution randomly picks one of the states in the ensemble and brings every other state to have the same probability as the selected state. Different realizations of evolution yield a distribution of selected states. We study this distribution numerically and discuss its relevance for equilibrium fluctuations in thermal as well as non thermal systems.
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Materials Science · Cross-listed from physics.optics

Topological space-time waves in complex channels

Structured light in space and time has become a powerful playground in which to explore the fundamental physics of wave systems, while simultaneously introducing new exotic forms of light, from spatio-temporal vortices to toroidal pulses of light. Yet their creation remains restricted by complex optical systems while directly observing their evolution in arbitrary channels remains elusive, complicated by the interplay of dispersion and diffraction and exacerbated by the lack of suitable detection tools. Here we create topological space-time beams in a single step by a resonant response of a symmetry-broken metasurface, mixing spatial, temporal and polarisation degrees of freedom in a single microwave field. Our realisation in the microwave regime allows us to directly observe their dynamics in arbitrary channels, from free-space to complex random media, showing the preservation of topology while the foundational degrees of freedom are scrambled. We use our control to show how to unscramble the space-time properties for the first crosstalk-free transmission of space-time waves. Our work advances the physics of space-time waves, introduces a new toolkit for their creation and control, and offers an exciting roadmap to their exploitation in real-world scenarios, e.g., for robust communications through noisy channels.
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All authors Renwei Zou, Kelsey Everts, Andrew Forbes, Yungui Ma

Materials Science

Observation of current-induced orbital quadrupole accumulation

Spintronics and orbitronics rely on current-induced accumulations of magnetic dipoles: spin and orbital angular momentum. However, electronic orbitals inherently carry multipoles beyond the dipole, with the rank-2 orbital quadrupole as the leading term. Here we use polarization-resolved Kerr microscopy to observe current-induced orbital-quadrupole accumulation at the surfaces of Ti and Pt, metals with markedly different spin–orbit-coupling strengths. By separating the symmetric and antisymmetric components of the off-diagonal optical conductivity, we isolate the time-reversal-even quadrupolar response from the conventional time-reversal-odd magnetic-dipolar one, and find that the quadrupolar optical response exceeds the dipolar one in both metals. First-principles analysis of the measured responses indicates that the quadrupole accumulations are of the same order of magnitude in the two metals despite their widely different spin–orbit-coupling strengths, consistent with a previously unidentified channel of charge-to-orbital conversion that does not require spin–orbit coupling. Our findings establish that current-induced orbital polarization is fundamentally multipolar, expanding current-induced phenomena from the dipolar to the multipolar regime and opening a route to electrical control of orbital-ordered phases.
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All authors Geun-Hee Lee, Yubin Ji, Yongho Park, Changmin An, San Ko, Hye-Won Ko, Jinseob Lim, Jung Hyun Oh, Farzad Mahfouzi, Byong-Guk Park, Kab-Jin Kim, Mark D. Stiles, Kyoung-Whan Kim, Paul M. Haney, Kyung-Jin Lee

Mesoscale and Nanoscale Physics

Antidot superlattices in two-dimensional topological insulators

We investigate the electronic properties of a two-dimensional topological insulator patterned with an array of circular holes. The band structures of the topological insulator superlattices are calculated using the Bernevig-Hughes-Zhang model, discretized with the finite element method. The band topology is studied using the Fukui-Hatsugai-Suzuki method, exploiting the fact that topological charge is conserved when a band gap closes and reopens. We find that when the holes are close to each other and the edge states overlap significantly, the material loses its topological character and becomes a trivial insulator. The results show that patterning topological insulators changes their properties, and this can be achieved with a feature size compatible with current lithographic techniques. This shows the potential to incorporate patterned topological insulators in future electronics.
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All authors Haolin Huang, Jackson S. Smith, Fabio Taddei, Michele Governale, Jared H. Cole

Materials Science

Extreme mixing enables broadband high-temperature electromagnetic absorption in high-entropy perovskites

Developing oxide absorbers with broadband high-temperature electromagnetic absorption performance has long been desirable in the electromagnetic absorption field, yet their absorption performance has remained unsatisfactory. Here, through an extreme mixing strategy, we successfully develop an ultrabroad effective absorption bandwidth (EAB) of 9.3 GHz in high-entropy perovskites up to 600 degree celsius, surpassing the previously reported oxide absorbers. Specifically, we achieve the extreme mixing in high-entropy perovskites by the successful incorporation of up to 13 cation elements, with 8 and 5 cations occupying the A- and B-sites, respectively, using a laser-driven controllable synthesis technique. Such extreme mixing maximally promotes the formation of atomic-scale interfaces to markedly amplify atomic-level interfacial polarization loss for the effective dissipation of electromagnetic wave energy, thereby giving rise to a remarkably broad EAB of 9.3 GHz in high-entropy perovskites up to 600 degree celsius. Owing to the profoundly increased electrical conductivity that causes impedance mismatch at elevated temperatures, however, their EAB deteriorates to 4.6 GHz at 700 degree celsius. This work establishes a new extreme mixing design paradigm for enabling high-entropy oxide absorbers with unprecedented high-temperature EM absorption performance.
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All authors Ziyu Feng, Fangchao Gu, Lei Zhuang, Wu Wang, Hulei Yu, Yanhui Chu

Materials Science

A Topological Magnonic Black-White Hole Crystal

The low-energy dynamics of antiferromagnetic spin waves map onto a massive Klein-Gordon scalar field, providing a solid-state platform for analogue-horizon physics. We show that an inhomogeneous spin current generates an effective magnon flow capable of forming black- and white-hole horizons. Horizon-pair cavities exhibit resonant transport and superradiant-like amplification mediated by magnon-antimagnon mixing. Our central result is that a periodic arrangement of submagnonic and supermagnonic regions forms a non-reciprocal magnonic crystal in which entering the supermagnonic regime makes negative-norm propagating channels available and enables the bulk gap to close and reopen. This drives a topological transition characterized by a change in the Zak phase and the emergence of a hybrid magnon-antimagnon edge state. These results establish a direct connection between analogue-horizon physics and topological magnonics, providing an electrically tunable route for controlling magnonic band topology.
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All authors D. Galvez-Poblete, R. M. Otxoa, A. S. Nunez, S. Allende

Materials Science

Mechanistic Phase-Field Modelling of Woven-Domain Formation in Ferroelectric Material

A recent experimental study reports the spontaneous formation of a three-dimensional woven ferroelectric domain fabric in bulk KTN:Li during sufficiently slow cooling through the ferroelectric transition. The present work develops a nondimensional phase-field framework to examine a physically plausible route by which such a state can emerge. A large-area two-dimensional model first resolves the cooling-rate-dependent formation of a frustrated crossing precursor by combining first-order ferroelectric thermodynamics, electrostatic and elastic interactions, compositional modulation, and effective charge screening. Slow cooling produces a persistent population of charge-associated crossings, whereas the corresponding fast-cooling pathway does not. A three-dimensional extension then incorporates cubic gradient anisotropy, flexoelectric coupling, and strain-gradient regularization to examine whether the planar precursor can develop a genuine woven topology. Within the explored nondimensional parameter regime, slow cooling produces a directly resolved geometrical separation and exchange of depth ordering between the intersecting wall families, whereas the corresponding fast-cooling pathway does not. This distinction is reproduced across independent realisations and remains robust to timestep refinement and changes in computational domain size. The simulations suggest that slow cooling provides a kinetic window for topological selection and that global charge relaxation can coexist with strong local charge concentration at surviving crossings. The model is not calibrated to material-specific KTN:Li coefficients and does not reproduce the experimentally observed low-temperature disappearance of the woven state.
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Superconductivity

Weak coupling theory of nickel-based 327 superconductors

This review provides a comprehensive survey of weak-coupling theoretical approaches applied to understand the emergent superconductivity in the pressurized nickelate bilayer system $La_{3}Ni_{2}O_{7}$. Following the landmark discovery of its high-Tc superconductivity under pressure, this material has rapidly become a new paradigmatic platform in the field of unconventional superconductivity, joining cuprates and iron-based systems. We focus on three pivotal theoretical frameworks: the random phase approximation (RPA), the fluctuation-exchange approximation (FLEX), and the functional renormalization group (FRG). These methods are deployed to analyze the effective pairing interactions and emergent instabilities arising from the low-energy electronic structure, which is commonly modeled by a bilayer two-orbital Hubbard Hamiltonian incorporating the Ni $d_{x^2-y^2}$ and $d_{3z^2-r^2}$ orbitals.
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Materials Science

A Novel Decoupling Method for Investigating Distinct Domain Evolution in Ferroelectric Film

Conventional polarization characterization techniques provide only the averaged response of ferroelectric films, limiting the investigation of domain-dependent reliability mechanisms in HfO2-based ferroelectrics. In this work, a new domain decoupling method is proposed to separately analyze ferroelectric domains with distinct switching behaviors. A three-domain model consisting of upward non-switchable domains, downward non-switchable domains, and switchable domains (Pd) is first introduced to describe heterogeneous domain populations during electrical cycling. By combining complementary switching-current measurements, the responses of different domain populations can be selectively extracted and reconstructed. The proposed method enables quantitative tracking of individual domain populations during cycling. As a demonstration, the method is further applied to analyze the time-dependent evolution of domain populations after electrical cycling. This approach provides a new route for investigating imprint, fatigue, and other reliability-related phenomena in ferroelectric devices.
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All authors Keying Sun, Jiajun Qiu, Hao Li, Zongwei Shang, Lang Zeng, Ming Li, Lining Zhang, Runsheng Wang

Strongly Correlated Electrons

Role of d-electron density of states in the quantum size effect of Pt-Ni and Pt-Pd nanoparticles

We investigated the quantum size effect (QSE) in bimetallic Pt$_{1-x}$Pd$_x$ and Pt$_{1-x}$Ni$_x$ nanoparticles, using $^{195}$Pt nuclear magnetic resonance measurements. The temperature and size dependencies of the anomaly in the nuclear spin-lattice relaxation rate divided by temperature $1/T_1T$ in the Pt$_{1-x}$Pd$_x$ nanoparticles suggest similar electron states between Pt and Pd atoms and are well understood by the QSE. The temperature and composition variations of $1/T_1T$ and Knight shift reveal a systematic increase in the density of states and reduction of the characteristic energy scale $T^*$ with increasing Ni content, consistent with the Kubo gap $\delta_{\mathrm{Kubo}}$. In contrast to Pt$_{1-x}$Cu$_x$ nanoparticles where the QSE is suppressed, the Pt$_{1-x}$Ni$_x$ nanoparticles exhibit clear signatures of quantum energy discretization. This discrepancy highlights the essential role of $d$-electrons in the manifestation of the QSE. Furthermore, analysis of the modified Korringa parameter $K(\alpha)$ suggests enhanced ferromagnetic correlations with increasing Ni concentration, approaching a ferromagnetic quantum critical regime. These results provide experimental evidence that $d$-electron density of states plays a crucial role in the manifestation of the QSE in the nanoparticles formed by the metallic $d$-electron atoms.
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All authors S. Kitagawa, T. Ihara, Y. Kinoshita, K. Ishida, K. Kusada, H. Kitagawa

Mesoscale and Nanoscale Physics

Parity-dependent coupling of molecular spin chains to a superconductor

Topological order can fractionalize the quantum numbers of the underlying particles. A paradigmatic example is the spin-1/2 states at the edges of an antiferromagnetic integer-spin chain, protected by a topological Haldane gap in the bulk and mutually coupled in short chains. Owing to their topological protection, they are natural building blocks for hybrid spin-superconductor quantum systems. Whether fractionalization survives the coupling to a superconducting condensate, however, remains an open question. Here we grow molecular Haldane chains of antiferromagnetically coupled spin-1 triangulene units on a proximitized Au(111)/Nb(110) surface and resolve a parity-dependent coupling of their spin-1/2 edge states to the superconducting condensate by scanning tunnelling spectroscopy. Odd-length chains host Yu-Shiba-Rusinov bound states inside the superconducting gap, originating from the net S=1 ground state, whereas even-length chains form an S=0 ground state decoupled from the superconductor. A two-site superconductor model reveals that this alternation arises from the sign and strength of the inter-edge interaction, a mechanism independently validated by extra-gap spin excitations in tunnelling spectra. Collective many-body spin excitation modes are also detected decoupled from the superconductor by the much larger Haldane gap. The length-tunable coupling of the edge spins to the superconductor opens a route toward molecular spin qubits based on $\pi$-conjugated carbon architectures.
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All authors Katerina Vaxevani, Jon Ortuzar, Stefano Trivini, Georg Monninger, Dongfei Wang, Vilas-Varela, Lucía Gómez-Rodrigo, Diego Peña, Jose Ignacio Pascual

Disordered Systems and Neural Networks · Cross-listed from physics.soc-ph

Evolution of cooperation with Q-learning: how much information do we need?

Cooperation is ubiquitous in both natural and human societies, yet its evolutionary basis remains a major challenge. A long-standing puzzle is whether having more information leads to better decision-making and thus a higher level of cooperation. To address this question, we adopt a recently developed reinforcement learning framework in which individuals learn through trial and error to maximize cumulative rewards - a paradigm that has successfully explained diverse emergent patterns in human behaviors. Specifically, we equip a structured population with the Q-learning algorithm and systematically vary the size of the interactive neighborhood, which serves as a proxy for perceived information. Interestingly, we observe a non-monotonic relationship between cooperation prevalence and neighborhood size in both two-dimensional square lattices and Barabasi-Albert scale-free networks. This inverted U-shaped dependence reveals that an optimal amount of information exists, yielding the highest level of cooperation. Mechanistic analyses show that a moderate neighborhood size enables individuals to strike an optimal balance between information sufficiency and decision-making tractability. This balance allows them to detect reciprocal opportunities while avoiding the deterioration of decision quality due to information overload. Our findings challenge everyday intuition, suggesting that a proper amount of information - not more - is optimal for the emergence of cooperation.
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All authors Yile Ku, Xin Ou, Jiqiang Zhang, Shengfeng Deng, Huiji Yue, Li Chen

Materials Science

Chiral Phonons and Giant Anisotropic Photoresponse in Quasi-1D van der Waals Semiconductor ZrSnS3

Low-dimensional van der Waals semiconductors with reduced symmetry provide a unique platform for exploring anisotropic physical properties. The quasi-one-dimensional family MXQ$_3$ (M = Hf, Zr; X = Sn; Q = S, Se) exhibits notable structural anisotropy, where zigzag atomic chains influence optical phenomena such as birefringence. This study investigates anisotropic lattice dynamics in ZrSnS$_3$ using angle- and polarization-dependent Raman spectroscopy. Temperature-dependent measurements reveal anharmonic phonon behavior, indicating strong phonon-phonon coupling. Density functional theory calculations show good agreement with the experimentally observed Raman spectra, validating the microscopic description of the lattice dynamics. We also observe a helicity-dependent intensity and a reversal in phonon intensity between lower- and higher-frequency modes under circularly polarized light, which is characteristic of chiral phonons governed by the polarization of the Zr/Sn chains. Our first-principles analysis further shows that angular-momentum-like phonon textures can emerge away from the $\Gamma$-point near mode-hybridization and avoided-crossing regions, providing microscopic insight into the observed helicity-dependent Raman signatures. Furthermore, we fabricate an optoelectronic device from a thin ZrSnS$_3$ nanowire, demonstrating a photoresponsivity of 50~mA/W under 520~nm laser excitation (1~mW/cm$^2$). The device exhibits a pronounced, power-scalable anisotropic photoresponse with a clear preferred polarization direction. These results highlight the coupling mechanisms between polarization, lattice vibrations, and charge carriers in ZrSnS$_3$, establishing it as a promising material for polarization-sensitive optoelectronics and directional quantum transport.
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All authors Zahir Muhammad, Shashi B. Mishra, Gayatri, Grzegorz Krasucki, Wajid Ali, Katarzyna Olkowska-Pucko, Obaid Iqbal, Zia Ur Rehman, Aziz Ur Rahman, Maciej R. Molas, Lin Xiaoyang, Weisheng Zhao

Soft Condensed Matter

Collective self-sorting on a chip

We harness two established ingredients for collective demixing: differential speed and curvature to create a self-sorting device. In binary mixtures, motility differences drive spontaneous spatial segregation, while confinement geometry determines how rapidly and strongly this demixing develops. Using particle based simulations, we systematically identify the geometrical conditions that promote efficient segregation and use these results to guide the design of a finite sorting architecture. We then translate these physical mechanisms into a sequence of curved microfluidic units that progressively amplify the separation of the two species and direct them toward distinct collection regions. Experiments with binary Quincke-roller mixtures confirm that an initially mixed suspension progressively demixes as it propagates through the device, leading to strong enrichment downstream. Our results demonstrate how collective active demixing can be converted into a functional continuous sorting strategy, providing a route toward autonomous microfluidic separation based on particle motility and confinement geometry.
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All authors Emanuel F. Teixeira, Thieu van den Bergh, Arjen Klok, Tijn Heesakkers, Alexandre Morin

Materials Science

High-throughput identification of ferromagnetic Kagome candidates in the AT6X4 and AT6X5 families

We present a systematic high-throughput density-functional theory study of the thermodynamic stability, collinear magnetic ground states, and electronic structures of layered kagome compounds in the AT6X4 and AT6X5 families. Using the experimentally reported structure types as templates, we screened 78 substitutional compositions in each family. Our calculations reproduce the stability and antiferromagnetic character of the known Fe-based Ge compounds and identify six additional stable candidates with robust ferromagnetism. Within collinear spin configurations, we find a clear chemistry-dependent trend: stable Fe-based Ge compounds predominantly adopt AFM2 ground states, whereas stable Mn-based Ge compounds consistently favor ferromagnetic order. Exchange analysis further shows that the magnetic phase space is governed by competing interlayer interactions, consistent with the mechanism established for AT6X6 kagome magnets. Representative ferromagnetic members from the two structural families also retain kagome-derived dispersive band features near K, although the AT6X5 phase exhibits stronger band folding and hybridization. Overall, these results establish AT6X4 and AT6X5 as promising layered kagome families for realizing ferromagnetism and kagome-derived electronic states.
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Sunday 23 August

Disordered Systems and Neural Networks

A Heterogeneous General Model for Neuromorphic-Inspired Computation

In recent years, both academia and industry have focused on the development of computational architectures inspired by the distributed, adaptive, and event-driven characteristics of biological neural systems, with the aim of reducing the computational cost associated with conventional training approaches [1]. However, a major challenge is the lack of general models and design guidelines for emerging computational systems and hardware. This work introduces a general model based on an input-dependent stochastic weight network, referred to as a substrate. The substrate weights evolve through input-triggered stochastic updates, with correlations between weight coefficients described by a matrix-valued covariance kernel. The proposed framework is implemented using quadratic polynomial weight functions, where the input amplitude controls the magnitude of the stochastic perturbation and a substrate-dependent distance determines the correlation structure. Numerical simulations show that correlations in the stochastic weight evolution significantly affect the system response, suggesting a potential mechanism for neuromorphic-inspired computation without conventional weight training. The aim of this work is to provide a general formulation of the model and identify its main properties and characteristics. 1 H. Jaeger, Towards a generalized theory comprising digital, neuromorphic and unconventional computing, Neuromorphic Comput. Eng., vol. 1, no. 1, p. 012002, Sep. 2021
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Soft Condensed Matter

A Reduced-Order Dynamical Model for the Ignition of Diver-Induced Cohesive Silt-Out on Sloping Beds

A downward fin thrust near a cohesive seabed lofts sediment. Whether this cloud settles or organizes into a self-sustaining down-slope current determines if a diver loses visibility briefly or catastrophically. We reduce the layer-averaged balances of fluid mass, sediment mass, and momentum to a temporal slab of fixed thickness in the weakly entraining limit. This yields an autonomous planar vector field in dimensionless near-bed speed and suspended load, governed by three dimensionless groups: drag against settling, erosion strength, and near-bed concentration. The field possesses a quiescent equilibrium at the origin and, above a critical bed slope obtained in closed form as the ratio of near-bed concentration times drag-settling number to erosion-strength number, an interior saddle equilibrium. The saddle's stable manifold partitions the state space into basins of decay and unbounded growth, establishing the exact threshold between self-limiting and igniting disturbances. On a flat bed, the origin attracts globally for all admissible erosion laws. For representative silt, the ignition threshold is near a 17-degree bed angle. The closed-form structure is confirmed numerically to machine precision. A closure study demonstrates the critical slope is robust in existence but closure-dependent in value, identifying the linear erosion law as the conservative choice. The model thus isolates bed slope as the controlling parameter for ignition.
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All authors Sandy Hardian Susanto Herho, Iwan Pramesti Anwar, Umar Abdurrahman, Faruq Khadami, Alfita Puspa Handayani, Karina Aprilia Sujatmiko, Dasapta Erwin Irawan

Materials Science · Cross-listed from cs.AI

TRACE: Transition-Aware Residual Control for Multi-Objective Materials Discovery

Multi-objective materials discovery with LLM agents is often limited not only by how many candidates can be proposed, but by how effectively each costly property evaluation informs the next search step. Existing agents mainly store evaluated candidates and their scores, so they know which materials succeeded but not which executable edits caused useful property changes. This makes local refinement difficult when objectives compete and an edit that improves one property may damage another. We propose TRACE, a transition-aware residual control framework that treats evaluated edits as the basic unit of feedback. TRACE records each local refinement as a parent-edit-child transition with observed property deltas, aggregates transition evidence to estimate reusable edit effects, and ranks future edits by their predicted ability to reduce the current candidate's remaining constraint violations while avoiding damage to already satisfied objectives. In a controlled same-backbone comparison, TRACE improves over LLEMA, the state-of-the-art LLM-agent baseline, raising macro-average hit rate from 18.13% to 25.96%.
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All authors Kang Zhou, Yujia Tong, Yong Tao, Jingling Yuan

Superconductivity

Structural disorder and critical voltage scaling in Al/AlOx/Al Josephson junction arrays

The insulating state of one-dimensional Josephson junction (JJ) arrays is governed by collective charge dynamics and disorder-induced pinning, resulting in a finite critical voltage under dc bias. Here, we investigate the influence of fabrication-induced structural defects on the critical-voltage scaling of small-capacitance Aluminium-Aluminium oxide-Aluminium (Al/AlOx/Al) JJ arrays. Controlled variation of the aluminium evaporation rate produces pronounced changes in grain morphology and room-temperature junction resistance. Despite these substantial structural modifications, the normalised critical-voltage scaling is preserved, demonstrating that the collective transport behaviour is remarkably robust against this class of fabrication-induced defects. In contrast, the deliberate introduction of nanoscale gaps into the junctions introduces additional junction-to-junction structural variations that systematically modify the normalised scaling behaviour. Likewise, in situ postfabrication oxidation alters the scaling coefficient while preserving the functional form of the scaling law, indicating that the collective transport is sensitive to specific classes of structural modifications. These results establish which fabrication-induced structural defects influence the collective transport in insulating Al/AlOx/Al Josephson junction arrays, providing new insight into the role of fabrication-induced structural disorder and practical guidance for the design of future Quantum Phase Slip (QPS) devices.
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All authors Amanuel M. Berhane, Susan Coppersmith, Emma Mitchell, Timothy Duty

Soft Condensed Matter

Shapes, forces, and torques of compressed elastic fluid interfaces: beyond axisymmetric configurations

Inspired by the classical Plateau-Douglas problem for soap films bounded by two closed curves, we solve an analogous problem for fluid interfaces with fixed surface area and resistance to out-of-plane bending. The boundaries are planar but need not be symmetric or concentric. The equilibrium surfaces minimize the Willmore bending energy and generalize minimal surfaces such as the catenoid while also exhibiting characteristic features of confined elastic interfaces such as buckling. We systematically classify all possible buckling modes and solution branches by performing a weakly nonlinear analysis and developing a fully nonlinear spectral solver. Our mathematical framework provides insight into the forces and torques required to stabilize cellular membranes and other soft materials and shows that physically relevant asymmetric states can arise even in symmetric systems.
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Mesoscale and Nanoscale Physics

Signatures of localization on the edge of a fractional topological insulator

Recent experiments in van der Waals moiré materials have reported realizations of two-dimensional fractional topological insulators (FTIs). We study transport properties of FTI edges at filling factors $\nu_{\text{FTI}} = 2(1\pm 1/n)$ with integer $n \geq 2$ (even or odd), each of which supports four counter-propagating edge modes. The edge modes can undergo partial localization, leaving two of the four edge modes conducting. We identify three distinct partial-localization channels and, for each channel, determine the reduced theory describing the remaining conducting modes, from which we obtain the minimal quasiparticle charge. We further explore transport properties of each partially localized phase and in particular determine the corresponding edge conductances. We demonstrate that measurements of the conductance together with the minimal quasiparticle charge provide a fingerprint that uniquely distinguishes the three partially localized phases.
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All authors Yuzhuo Tian, Jinhong Park, Alexander D. Mirlin, Jukka I. Väyrynen

Strongly Correlated Electrons

Anomalous dynamical energy flows via nonlinear phononics in spin-Peierls chains

We investigate the nonequilibrium spin-phonon dynamics and energy cascades in a strongly dimerized spin-Peierls chain using a multi-tiered nonlinear phononics architecture. To bypass linear selection rules prohibiting the direct excitation of the Raman-active dimerization mode, a terahertz laser drives an infrared mode that nonlinearly couples to the Raman lattice displacement, subsequently modulating the magnetic exchange. Employing a bond-operator formalism with a second-order cumulant expansion of the Lindblad master equation, we show that maximum energy transfer into the magnetic sector is governed by a dynamical impedance-matching condition rather than the unperturbed triplon density of states. We find that the sustained energy input of continuous-wave driving builds high excitation densities that severely back-act on the lattice, overdamping the primary phonon and smearing magnetic features via power broadening. Conversely, the small time-integrated energy of a pulse keeps the response perturbative, terminating before back-action accumulates and preserving sharp Fano-like quantum interferences. These insights establish limits for controlling dynamic magnetic states without quenching the driving lattice modes.
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All authors Jakob Dolgner, Dirk Manske, James K. Freericks, Mohsen Yarmohammadi

Mesoscale and Nanoscale Physics

Estimating the Fisher information from ARPES in general two-band models

The Quantum Fisher information is frequently studied in the fields of quantum sensing and quantum metrology, as it specifies the sensitivity of a sensor through the Crámer-Rao bound, and in condensed matter physics where it relates to the quantum metric. Measuring the quantum Fisher information is therefore of significant current interest. In this work, we propose a scheme for measuring the quantum Fisher information with respect to any parameter in a general two-band solid state system using angle-resolved photoemission spectroscopy with carefully tuned incidence angles and light polarization. We investigate conditions under which this can be related back to information about the ground state of the material itself changing with system parameters.
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Statistical Mechanics

Time reversal of complex evolution on a quantum computer

The Boltzmann-Loschmidt dispute in 1876-1877 discussed the problem of time reversal of ther- malization from time reversible classical equations of motion. Here, 150 years later, we highlight this problem in the frame of quantum computing. A quantum protocol is proposed that allows to perform a time reversal of complex evolution in the regime of many-body quantum chaos with many qubits. The system represents an evolution of qubits on a square lattice with inter-qubit next-nearest static couplings with a driven pulsed magnetic field. The system entropy grows rapidly to maximal values but returns to initial small values after time reversal. This time reversal is shown to be stable with respect to quantum gate imperfections. However, similar to the Lorenz butterfly effect, there is the butterfly effect of qubit when inversion of only one qubit breaks time reversibility of the whole system. It is argued that this protocol is accessible to nowadays quantum computers and annealers with hundreds of qubits.
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