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Physics Condensed Matter

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Tuesday 2 June

Materials Science

Magneto-optical evidence for single-crystal-like magnetic switching of epitaxial antiferromagnetic LaFeO3 films

Strained epitaxial films of the antiferromagnetic orthoferrite LaFeO3 offer a promising platform for antiferromagnetic spintronics, yet their magnetic switching behavior and domain structure have remained largely unexplored due to the small magnitude of the weak ferromagnetic moment. Here, we demonstrate that longitudinal magneto-optical Kerr effect (MOKE) measurements provide a sensitive and direct probe of magnetic switching and domain processes in coherently strained LaFeO3 thin films grown on orthorhombic substrates. By employing DyScO3(110), GdScO3(110), and NdGaO3(110) substrates, we achieve straincontrolled, largely twin-free growth and identify the orientation of the orthorhombic c-axis through the presence or absence of a longitudinal MOKE signal. Compressively strained films exhibit large Kerr signals, rectangular hysteresis loops, and magnetic single-domain remanence over macroscopic areas. Tensile strain on orthorhombic substrates is associated with two competing structural effects on thin film orientation; in-plane magnetization has been identified in some films on GdScO3(110) by MOKE. Angle-dependent MOKE hysteresis follows the Kondorsky model, indicating domain-wall-controlled switching analogous to bulk single crystals. Kerr microscopy reveals abrupt domain nucleation and rapid domain-wall motion, with defects acting as pinning centers and governing the coercive field. Our results establish MOKE as an efficient optical tool for identifying orthorhombic orientation, probing magnetic switching of coupled weak magnetization and Neel vectors, and accessing domain dynamics in LaFeO3 films. This provides a foundation for strain-engineered orthoferrite thin films in antiferromagnetic spintronics and magnonics.
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All authors A. Rieche, W. Hoppe, C. Körner, A. D. Rata, F. Weber, J. B. G. Danziger, E. M. Vocks, F. Wührl, M. Bargheer, W. Widdra, G. Woltersdorf, S. Ebbinghaus, A. Herklotz, K. Dörr

Mesoscale and Nanoscale Physics · Cross-listed from physics.optics

Spatially Uniform and Defect-Tolerant Plasmonic Responses in 3D printed Gold Nanoparticle Assemblies

Three-dimensional (3D) assemblies of gold nanoparticles (AuNPs) offer a rich platform for plasmonic coupling and near-field engineering, yet their optical behavior is often complex due to structural disorder and fabrication-induced variability. Here, we present a systematic optical investigation of large-scale 3D AuNP assemblies fabricated via meniscus-guided assembly, focusing on the reproducibility and spatial uniformity. Spatially-resolved dark-field scattering measurements reveal that high-aspect-ratio AuNP pillars exhibit uniform scattering spectra along their height and across different pillars, despite variations in geometry and structure. Electromagnetic simulations suggest that this robustness arises from an ensemble-averaged plasmonic response governed by many local coupling regions within a finite plasmon delocalization length. Simulated near-field and surface charge distributions suggest that the broad ensemble response remains spatially distributed under representative structural perturbations, consistent with volumetric averaging. Building on this robust platform, we introduce compositional modulation through a core-satellite architecture by incorporating smaller AuNPs. This yields a composition-dependent spectral redistribution, including an additional long-wavelength spectral feature in the core-satellite assemblies. Wavelength-dependent surface-enhanced Raman scattering measurements reveal contrasting responses under 633 and 785 nm excitation, reflecting redistribution of local plasmonic coupling pathways. These results establish design principles for robust 3D plasmonic nanoparticle assemblies with ensemble-averaged and composition-tunable optical responses.
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All authors Vasanthan Devaraj, Sunghyun Kwak, Hyeongjip Kim, Sang-Keun Sung, Jong-Min Lee, Thomas Zentgraf, Won-Geun Kim

Mesoscale and Nanoscale Physics

Tailoring pure valley-Zeeman spin-orbit coupling in WSe$_2$-encapsulated monolayer graphene

Engineering proximity effects in twisted van der Waals heterostructures offers a powerful platform for designing electronic properties. While theoretical predictions of quantum interference in transition metal dichalcogenide-encapsulated graphene can selectively control the spin-orbit coupling component, experimental realizations have remained elusive. Here, we report pure valley-Zeeman spin-orbit coupling in monolayer graphene, achieved by encapsulation between two parallel twisted WSe$_2$ monolayers. We observed a symmetry-enforced reordering of Landau levels, which is driven by the competition between the fixed valley-Zeeman energy and the magnetic-field-dependent cyclotron energy. This reordering is characterized by a transition from symmetry-broken states in the quantum Hall effect to a restored fourfold degeneracy with integer or half-integer quantum Hall sequences. We also demonstrate the ability to completely quench the proximity spin-orbit coupling by tuning the encapsulated geometry.
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All authors Yaqing Han, Siqi Jiang, Jingkuan Xiao, Jiawei Jiang, Yulu Liu, Jiabei Huang, Yu Du, Di Zhang, Fuzhuo Lian, Wanting Xu, Siqin Wang, Kenji Watanabe, Takashi Taniguchi, Xiaoxiang Xi, Alexander S. Mayorov, Renjun Du, Kai Chang, Hongxin Yang, Lei Wang, Geliang Yu

Soft Condensed Matter

Monte-Carlo study of Compositional Heterogeneity in Multicomponent Cluster Crystals

Soft (sub)micron-sized particles with bounded interactions can form cluster crystals, periodic structures in which multiple particles occupy the same lattice site. While the thermodynamics of monodisperse cluster crystals is well understood, less is known about how compositional disorder affects their stability. Using Monte Carlo simulations and density functional theory we show that binary cluster crystals undergo a density driven transition from a homogeneous mixed state to a heterogeneous “alloy" like solid in which lattice sites spontaneously differentiate into populations with distinct compositions and occupancies while preserving the underlying crystal symmetry. The transition is accompanied by a sharp increase in the equilibrium lattice site density and by increased compositional fluctuations, but we see no evidence for macroscopic phase separation. We demonstrate that this transition is governed by competition between clustering and demixing instabilities and derive a simple scaling law for the demixing density as a function of temperature, composition, and particle size mismatch, in quantitative agreement with simulation.
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Disordered Systems and Neural Networks · Cross-listed from stat.ML

An Asymptotic Theory of Chain-of-Thought in In-Context Learning

Chain-of-thought (CoT) reasoning has become a widely used mechanism for eliciting multi-step reasoning in large language models by generating intermediate reasoning steps at inference time. Yet the scaling behavior of generalization with CoT depth remains poorly understood. To address this question, we study a theoretically solvable model of CoT for in-context weight prediction in linear regression, where test-time reasoning is represented as an iterative refinement of the weight-parameter estimate. Using tools from random matrix theory under high-dimensional asymptotics, we derive an exact formula for the generalization error as a function of reasoning depth, pretraining data amount, and context length. Our analysis reveals a sharp phase transition separating exponential and polynomial improvement, saturation, and overthinking, and characterizes how the optimal reasoning depth scales. We further show that deeper reasoning is most effective with sufficiently rich pretraining and in-context information, whereas limited pretraining or context makes longer reasoning prone to error amplification or saturation. We also validate these predictions through experiments on fully learned linear attention and softmax attention models. Our results provide a unified theoretical account of how test-time CoT depth affects generalization.
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Statistical Mechanics

Geometric Bounds on the Finite-Time Performance of Active Machines

Optimizing energy conversion in active matter remains a central challenge in nonequilibrium physics. Here, we develop a unified thermodynamic framework that characterizes the finite-time performance of interacting active machines. We show that cyclic work admits a geometric decomposition into an antisymmetric thermodynamic curvature, governing work extraction, and a symmetric metric, controlling dissipation. Minimal-dissipation protocols follow geodesics in parameter space, while optimal work extraction deviates from them due to a curvature-induced, Lorentz-like effect. This geometric structure directly determines the finite-time scaling of work and dissipation, enabling a mapping onto Onsager-type quasi-linear current–force relations. We show that both the maximal efficiency and the efficiency at maximum power are governed by an asymmetry parameter and a figure of merit, establishing a formal correspondence between active machines and thermoelectric devices with broken time-reversal symmetry. Our results reveal a fundamental geometric origin of energy-conversion performance and provide a general framework for optimizing active machines.
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Mesoscale and Nanoscale Physics

Generation and time evolution of anomalous Floquet Majorana flat edge modes in two-dimensional noncolinear magnet-superconductor heterostructures

We theoretically investigate the realization of gapless Floquet topological superconducting phases in a two-dimensional magnet-superconductor heterostructure (2D Shiba lattice) in the presence of a harmonic drive implemented in the chemical potential. Employing a real-space tight-binding model, we obtain both the regular $0$- and anomalous $\pi$-Floquet Majorana flat edge modes (FMFEMs) in the quasi-energy spectrum. We also study the real-time evolution of the FMFEMs and analyze their local density of states in the presence of such a periodic drive. The topological characterization is performed using the winding number, exploiting the chiral symmetry of the equivalent bulk effective momentum-space Hamiltonian. This is also supported by the corresponding edge state spectra. Furthermore, we employ the Brillouin-Wigner (BW) and Floquet perturbation theory (FPT) to gain analytical insight into the problem. We compare our exact (numerical), BW, and FPT results in terms of the quasi-energy spectra obtained across different frequency regimes. We find good agreement between the exact numerical, BW, and FPT results in the higher-frequency and high-amplitude domain, particularly close to the $0$-quasi-energy modes.
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Statistical Mechanics · Cross-listed from math-ph

Logarithmic Sobolev inequality and hypercontractivity for the Navier-Stokes Fokker-Planck operator

The stochastic incompressible Navier-Stokes equations on $\TT^3$, completed by the fluctuation-dissipation noise, have a Fokker-Planck generator that decomposes into a self-adjoint Ornstein-Uhlenbeck (dissipative) part and an antisymmetric (convective) part. We prove two results about this generator. First, the logarithmic Sobolev inequality holds with the same optimal constant as the pure Ornstein-Uhlenbeck operator, $c_\mathrm{LSI} = \nu\lambda_1$ (where $\nu$ is the viscosity and $\lambda_1$ is the smallest nonzero eigenvalue of the Laplacian on $\TT^3$), independent of the number of retained Fourier modes. Second, the full semigroup is hypercontractive with the same rate as the Ornstein-Uhlenbeck semigroup. Both results follow from a single structural property: the convective generator is antisymmetric in $L^2(P_\mathrm{eq})$ (where $P_\mathrm{eq}$ is the Gibbs measure), and therefore contributes nothing to the Dirichlet form or the $L^q$ norm evolution. The antisymmetry is a consequence of two properties of the incompressible Navier-Stokes nonlinearity: energy conservation and phase-space volume preservation (the Liouville property). These are the same properties that underpin the fluctuation-dissipation theorem for the nonlinear Navier-Stokes equations.
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Statistical Mechanics · Cross-listed from physics.flu-dyn

Turbulence: An Entropic Approach

We show that maximizing the generalized entropic functional $S_{q,\delta}$ subject to standard kinetic energy constraints provides generalized canonical distributions that agree perfectly with measured probability densities of velocity differences at distance $r$ in highly-turbulent Taylor-Couette flow. The end point of the turbulent cascade is described by $\delta =\frac{3}{2}$, a parameter value that also plays an important role in black-hole physics. At this point the Kolmogorov length scale $r=\eta$ is reached and all observable eddy structures of the turbulent flow disappear, in certain analogy to what is observed for black holes at the event horizon. Our approach generalizes statistical mechanics to more general nonadditive entropic functionals $S_{q,\delta}$ such that it is applicable to turbulent flows. This approach asymptotically generates stretched $q$-exponentials as generalized canonical distributions relevant for turbulent flow, with a particular dependence of the stretching exponent $\delta^{-1}$ on $q$ that follows from the well-known escort formalism in nonextensive statistical mechanics. Along this particular line in the parameter space, the physics can be described by $S_q$ on its own with suitable escort constraints, leading to the prediction $\delta^{-1} (r) =2-q(r)$, thus allowing for a consistent thermodynamic description since $S_q$ is both trace-form and composable. We show that the above theoretically derived relation is well satisfied by measured high-precision experimental data for Taylor-Couette flow. At the Kolmogorov length scale $r=\eta$, the endpoint of our scenario, one has $\delta =\frac{3}{2}$ and at this point the third moment of velocity differences ceases to exist and all eddies disappear. We point out various analogies with thermodynamic entropic approaches to black hole physics.
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Strongly Correlated Electrons

Many-Body Non-Hermitian Physics in the Generalized Brillouin Zone

The breakdown of conventional bulk-boundary correspondence (BBC) in non-Hermitian system can be resolved by the generalized Brillouin zone (GBZ) theory. However, extending the GBZ theory to interacting many-body systems remains an open problem. Here, we consider an interacting non-Hermitian model characterized by a circular GBZ. We show that, based on a GBZ transformation, a quasi-reciprocal many-body Hamiltonian can be constructed which, under periodic boundary conditions (PBC), captures the physics of the original non-Hermitian model under open boundary conditions (OBC). Using exact diagonalization (ED), we determine the phase diagram for the quasi-reciprocal many-body Hamiltonian by computing the Zak phase and the structure factor of the charge-density-wave (CDW) phase. We further investigate the entanglement properties and find that the degeneracy of the low-lying entanglement spectrum characterizes each phase in the phase diagram. These findings demonstrate that the topological properties in interacting non-Hermitian system is encoded in the entanglement spectrum of the quasi-reciprocal model. Our work establishes a route to studying many-body non-Hermitian physics within the GBZ formalism.
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All authors Chaoze Lu, Chuanshu Xu, Zhenghao Yang, Xiancong Lu

Strongly Correlated Electrons · Cross-listed from hep-th

Magnetic Symmetries and the Structure of Correlation Functions in Quantum Field Theory

Quantum field theories in the presence of a static and uniform external magnetic field possess two characteristic spatial symmetries: magnetic translations and magnetic rotation. We investigate general consequences of these symmetries on correlation functions from a model-independent perspective, without relying on specific models or perturbative expansions. The projective structure of magnetic translation symmetry constrains correlation functions of charged operators to acquire the Schwinger phase and leads to a factorized form into a gauge-covariant phase factor and a reduced correlator depending only on relative coordinates. We further derive the spectral representation of two-point functions in terms of representations of the magnetic translation algebra, in which the Landau- and symmetric-gauge descriptions arise as different choices of basis. Our results provide a unified symmetry-based framework for quantum field theories in external magnetic fields.
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Materials Science

High-Throughput Discovery of Semimetallic Borophenes with Diverse Dirac States Via Transferable Tight-Binding Approach

Borophene has attracted extensive interest due to its structural flexibility and emergent topological electronic states. However, semimetallic borophenes hosting robust Dirac states remain rare among the large number of predicted allotropes. Here, we develop a transferable tight-binding framework for planar borophenes and combine it with a graph- and group-theory-based random generation strategy to perform high-throughput screening of 522 borophene candidates. Eight previously unreported semimetallic borophenes are identified, hosting diverse topological band crossings, including type-I and type-III Dirac cones, Dirac nodal lines, and quadratic nodal points. Notably, quadratic nodal-point semimetals are predicted in borophene for the first time. Symmetry analysis reveals crystalline-symmetry-protected Dirac states, while first-principles calculations confirm their dynamical and thermal stability. These findings establish borophene as a versatile platform for engineering emergent Dirac physics in two dimensions.
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All authors Yuke Song, Shifang Li, Tao Ouyang, Chao Tang, Jin Li, Chaoyu He

Materials Science

Multiferroicity in the two-dimensional limit in hexagonal LuFeO3 films

Multiferroic oxides, which combine coupled ferroelectric and magnetic orders, are central to understanding correlated quantum phenomena. Yet, as thickness approaches the two-dimensional (2D) limit, both ferroelectricity and magnetism are conventionally expected to vanish due to depolarization fields and finite-size effects, respectively. Here, we demonstrate that hexagonal LuFeO3 (h-LuFeO3) retains coupled ferroelectricity and magnetism at the 2D limit, with a thickness of just one and a half unit cells. Remarkably, the ferroelectric polarization remains comparable to bulk values at room temperature, while long-range magnetism and magnetoelectric coupling persist at low temperatures. We further show that the K3 phonon mode, which mediates the polarization-magnetism coupling, is stable down to the 2D limit. Our results establish h-LuFeO3 as the first oxide system to exhibit genuine 2D-limit multiferroicity, providing a fundamental breakthrough in the long-standing quest to understand and control coupled ferroic orders at the atomic scale.
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All authors Huilin Lai, Junyu Tan, Jinfeng Zhai, Yang Shi, Lili Feng, Huanyu Zhang, Chuanrui Huo, Chuhang Liu, Lijun Wu, Lifeng Yin, Hangwen Guo, Jun Chen, Xiaoshan Xu, Jun Zhao, Yimei Zhu, Shiqing Deng, Wenbin Wang, Jian Shen

Quantum Gases

Observation of interaction-induced fast Thouless pumping of solitons

Thouless pumping provides a paradigmatic platform for studying the effects of interactions on topological transport in periodically driven systems. However, most studies have been constrained by adiabatic conditions, which preclude exploration of interaction-driven novel topological states at high driving frequencies. Here, we experimentally investigate the interplay between interaction and modulation frequency in Thouless pumping realized in a periodically modulated lattice in momentum space of atomic Bose-Einstein condensate. We observe fast Thouless pumping of matterwave solitons at intermediate interactions, with no counterpart in the non- or weakly interacting regimes. Beyond the boundary of topological phase transition induced by interaction, nonadiabatic quantized pumping of solitons emerges at high modulation frequencies over a broad interaction range, in good agreement with theoretical calculations, while the solitons remain trapped in the low-frequency adiabatic pumping regime. Our work opens new avenues for accelerating topological transport in driven quantum systems and engineering fast topological devices.
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All authors Yuqing Li, Jinxiong Jia, Yunfei Wang, Huiying Du, Zhong An, Zhenhua Qiao, Liantuan Xiao, Suotang Jia, Qian Niu, Jie Ma

Mesoscale and Nanoscale Physics

Geometric aspects of spin transport in magnetic multilayers

We discuss spin-dependent transfer-matrix formalism applied to magnetic multilayers in geometric terms. Starting from the stationary Schrödinger equation rewritten as a first-order spatial evolution problem, we interpret the transfer matrix as a path-ordered exponential and relate its matching-matrix construction to a noncompact group constraint. We then connect the induced Möbius action on reflection matrices to an Iwasawa decomposition, identify Weyl-chamber variables as the minimal noncompact transport invariants, and show how torque-related spin structures arise from compact-sector and commutator contributions. A sequence of multilayer examples illustrates the transition from pure spin filtering to controlled spin-orbit mixing and the resulting deformation of Weyl-chamber trajectories. We finally comment on the extension to higher-dimensional internal spaces relevant to orbital transport and realistic calculations.
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Soft Condensed Matter

Attractive Hopfions and Bimerons in Thin Films of Chiral Magnets: Cluster Formation and Lattice Instability in the Conical Phase

We investigate the energetics, interactions, and ordering tendencies of bimerons (cholesteric fingers of the second type, CF–2) and hopfions in thin films of chiral magnets and chiral liquid crystals hosting a conical background state. Although isolated bimerons possess positive eigen-energy with respect to the conical phase, they develop an attractive interaction mediated by the restructuring and partial overlap of their positive-energy shells, i.e., intermediate regions formed relative to the conical state. This attraction promotes the formation of bound pairs and extended bimeron chains, even in parameter regimes where a periodic bimeron lattice is no longer thermodynamically stable. Extending the analysis to three dimensions, we show that circularization of bimerons into hopfions renders their energy finite and gives rise to a well-defined metastability window closely linked to the stability range of cholesteric fingers. Isolated hopfions likewise exhibit an attractive interaction within the conical phase, leading to the formation of hexagonally ordered clusters. The attraction originates from the competition between favorable and unfavorable twist regions and from the energetic cost of the shell structures imposed by the conical background. Despite the presence of attractive pair potentials and cluster formation, we demonstrate that hexagonal hopfion lattices do not exhibit an equilibrium lattice period. Instead, the system evolves toward states in which the conical spiral or the CF–1 phase (cholesteric fingers of the first type) progressively invade the inter-soliton regions, thereby preventing crystallization. Our results reveal a regime of attraction without stable long-range order and clarify the interplay between topology, confinement, and conical-phase frustration in chiral magnet and liquid-crystal thin films.
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Disordered Systems and Neural Networks

Relaxation of the Random Site Coulomb glass Model in Two Dimensions

This study investigates the influence of material density, disorder in onsite energies, and localization length on relaxation dynamics within a two-dimensional random site Coulomb glass model at half-filling. To explore relaxation laws, we calculate the eigenvalue distribution of the linear dynamical matrix using mean-field approximations. Our findings indicate that the system initially undergoes rapid relaxation through energy-lowering transitions. The depletion of the single-particle density of states (DOS) near the Fermi level leads to slow relaxation, with fluctuations diminishing according to a power law. Subsequently, the system adheres to an exponential decay law after a specific period, defined as the relaxation time, which is inversely related to the minimum eigenvalue of the dynamical matrix. As the density of the system decreases, the relaxation rate slows down, resulting in an increase in the relaxation time. For a constant density and localization length, an increase in the disorder of onsite energies results in a longer relaxation time. A significant portion of the eigenvalue spectrum remains unaffected, suggesting that a reduction in localization length concurrent with increased disorder may play an equally vital role in the slow dynamics observed.
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Quantum Gases

Effective scatterings and universal clusters of heteronuclear ultracold mixtures in quasi-low dimensions

We study the effective s-wave scattering of two heteronuclear atoms harmonically confined in quasi-low dimensions, where the atoms have unequal masses and are subject to different confinement frequencies. The resulting effective scattering parameters in low dimensions, including scattering length and effective range, are derived as functions of three-dimensional scattering parameters and confinement strengths. Using realistic Li-K and Li-Cr mixtures as examples, we further compute the binding energies of universal $(1+N)$ clusters in quasi-low dimensions using the effective scattering parameters. Our findings suggest a promising pathway for practically observing universal clusters and their associated many-body phases in low-dimensional ultracold heteronuclear systems.
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Quantum Gases

Scattering and Bound States of Two Heteronuclear Ultracold Atoms in a Quasi-Two-Dimensional Confinement

We solve the two-body problem of ultracold heteronuclear atoms in a quasi-two-dimensional (quasi-2D) geometry. The quasi-2D confinement is realized by a harmonic trap along the longitudinal ($z$-) direction, with different trap frequencies for the two atoms, as in many current experiments on ultracold heteronuclear gases. As a consequence, the longitudinal center-of-mass (CoM) motion is coupled to the relative motion, which significantly complicates the two-body problem. We solve this problem exactly and derive the 2D scattering length $a_{\rm 2D}$, the 2D effective range parameter $R_{\rm 2D}$, and the bound-state energies, as functions of the $s$-wave scattering length and effective range of the two atoms in free three-dimensional (3D) space. We show that multiple 2D scattering resonances can be induced by the coupling between the longitudinal CoM and relative motion. Around these resonances, $a_{\rm 2D}$ varies rapidly with the 3D scattering parameters, while $R_{\rm 2D}$ is strongly enhanced. Since the effective pairwise interaction in quasi-2D ultracold gases is determined by i.e., the two-body scattering amplitudes and bound-state energies, our results can be used for manipulating the effective 2D interatomic interaction in quasi-2D ultracold heteronuclear gases by tuning the confinement frequencies and the 3D scattering parameters.
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Monday 1 June

Disordered Systems and Neural Networks · Cross-listed from physics.comp-ph

Omnisolver: An extensible interface to Ising spin-glass and QUBO solvers: adding a distributed GPU brute-force plugin

This software update extends Omnisolver with omnisolver-bruteforce, a first-class plugin for exact exhaustive search of QUBO and Ising instances on CUDA-enabled GPUs. The update contributes three components: packaging of the single-GPU brute-force kernel of [Computer Physics Communications 260, 107728, 2021] as a first-class Omnisolver plugin with a uniform Python and CLI interface, a Ray-based distributed framework that splits the search into $2^{k}$ fixed-variable subproblems and dispatches them across multiple GPUs and hosts, with a controller that gathers and merges partial results, and numerical stabilization of the fast float32 ground-state path through compensated incremental updates, periodic exact energy re-anchoring, and best-buffer refresh. Stabilization activates automatically for $N \geq 40$ leaving the public sampler API is unchanged. On dense random Ising instances we measure exhaustive solve times up to $N=60$ on $8\times$ NVIDIA H100 (96 GB) GPUs, reaching $\approx\!3.15$ days at $N=60$ in close agreement with the empirical $t_{N+1}=2\,t_N$ doubling rule, with the distributed sampler reaching the full $\approx\!8\times$ speedup over a single H100 from $N\!\gtrsim\!44$ onwards. The plugin thereby serves as a practical ground-truth oracle for state-of-the-art classical heuristics such as the Simulated Bifurcation Machine.
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All authors Konrad Jałowiecki, Jakub Pawłowski, Bartłomiej Gardas, Łukasz Pawela

Strongly Correlated Electrons · Cross-listed from physics.optics

Ultrafast Terahertz and Optical Spectroscopy under Synergetic Extreme Conditions

Elucidating and manipulating emergent phases in complex materials requires direct access to their low-energy collective modes. Terahertz (THz) time-domain and ultrafast optical spectroscopies have emerged as indispensable experimental tools, enabling the probing of intrinsic electrodynamics and the coherent control of non-equilibrium states. At the Synergetic Extreme Condition User Facility (SECUF), we have developed a suite of intense ultrashort light sources covering the near-infrared, mid-infrared, and THz spectral ranges. By integrating these strong-field pulses with extreme sample environments, such as low temperatures, strong magnetic fields, and high pressures, we have established several state-of-the-art spectroscopy platforms. In this article, we outline the technical specifications of each setup and highlight representative user experiments. The presented results underscore the exceptional capability of the THz experimental unit (A4-2) to explore ultrafast dynamics across a multi-parameter thermodynamic phase space.
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All authors Xinbo Wang, Tao Dong, Jianlin Luo, Nanlin Wang

Materials Science · Cross-listed from physics.app-ph

AlN Gate Interlayer for UWBG AlGaN Transistors with Breakdown Field >6.9 MV/cm and PFOM >1.8 GW/cm2

We report the demonstration of regrown epitaxial AlN gate interlayers with ultra-wide bandgap (UWBG) AlGaN polarization-graded field effect transistors (PolFETs). The introduction of the epitaxial AlN gate interlayer enables significant improvement in breakdown strength, with average breakdown field exceeding 6.94 MV/cm, which represents state-of-the-art for lateral field effect transistors, while maintaining excellent on-state current density exceeding 1 A/mm. The integration of epitaxial AlN enables state-of-the-art power-switching figure of merit exceeding 1.87 GW/cm2 at a breakdown voltage exceeding 1.45 kV. This work shows the potential of UWBG AlGaN for next-generation high-power switching and RF applications with enhanced device performance established by a high-quality epitaxially regrown AlN gate interlayer.
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All authors Seungheon Shin, Jonathan Pratt, Joe McGlone, Yinxuan Zhu, Brianna A. Klein, Andrew Armstrong, Andrew A. Allerman, Siddharth Rajan

Mesoscale and Nanoscale Physics

Second-Order Synaptic Memory using Inherent Plasticity of Moiré Superlattices

Achieving synaptic functionality electronically in a single-element quantum material is a fundamental challenge, as conventional methods rely on the introduction of extrinsic charge-traps or polar components. Here, we demonstrate that twisted double bilayer graphene (tDBLG) moiré superlattices, composed purely of carbon, exhibit electronic hysteresis and plasticity in presence of twist-angle disorder. Inversion symmetry breaking at the moiré length scales also gives rise to second-order nonlinear electrical response via disorder-mediated extrinsic mechanisms. Such second-order nonlinearity is highly tunable in both sign and magnitude by varying carrier concentration and vertical displacement field. We harness the coexistence of electronic plasticity and second-order nonlinearity to realize a second-order synaptic memory device. Our findings establish strained moiré carbon systems as a powerful new platform for energy-efficient neuromorphic computing, demonstrating that complex electronic functionality can emerge purely from symmetry breaking physics in a single-element material.
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All authors Tanweer Ahmed, Kenji Watanabe, Takashi Taniguchi, Fèlix Casanova, Luis E. Hueso

Strongly Correlated Electrons

Fast Tensor Network Imaginary Time Evolution by Implicit Stepping on Logarithmic Grids

We present a new method for the efficient imaginary time evolution of quantum many-body wavefunctions represented by matrix product states (MPS). We first show that logarithmic time grids are sufficient to resolve long imaginary time dynamics, yielding an exponential reduction in the number of time steps compared with standard approaches. We then show that A-stable implicit time-stepping methods for ordinary differential equations allow stable propagation for any time step size. The resulting scheme requires only matrix-vector products and linear solves, standard operations in the MPS toolbox. We validate our approach with two examples: a Heisenberg spin chain, which we use to demonstrate a speedup of several orders of magnitude over the standard time-dependent variational principle method with uniform time steps, and a single-site Anderson impurity model with a metallic bath, for which propagation to large imaginary times allows one to observe the exponential dependence of the Kondo temperature on the interaction strength.
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All authors John P. Zima, E. Miles Stoudenmire, Steven R. White, Olivier Parcollet, Jason Kaye

Statistical Mechanics · Cross-listed from math.DS

Ulam Approximation for Nonautonomous Systems: Equivariant Measures and Linear Response

Despite the prevalence of nonautonomous systems in applications, their statistical properties are much less understood than in the autonomous setting. Building on recent results on response theory for nonautonomous systems, we study the approximation of equivariant families and of their linear response by Ulam-type finite-dimensional reductions. First, we show that coarse-graining procedures associated with the classical Ulam method, and more generally with suitable finite-element projections, provide rigorous approximation of equivariant families for sequential systems with memory loss. Second, for systems whose transfer operators are regularizing, we prove that the linear response of the reduced finite-state Markov model converges to the projected linear response of the original system. To the best of our knowledge, a general approximation result of this type has not previously been established in this form, even in the autonomous case. We complement the analysis with numerical experiments on simple but representative time-dependent diffusive models. These results provide a rigorous foundation for the use of Markov approximations in the study of statistical properties of nonautonomous complex systems which almost invariably relies on finite-scale and finite-precision descriptions of their states and dynamics.
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Mesoscale and Nanoscale Physics

Negative temperature coefficient of Gilbert damping in magnetic bilayers

The Gilbert damping of magnetic materials is an important magnetic parameter that determines the switching speed and energy dissipation of spintronic devices. In simple metals, the intrinsic Gilbert damping increases with temperature and diverges near the Curie temperature as a result of spin fluctuations. Here we present atomistic simulations and experimental measurements showing surprising and opposite behavior in Py/Nd bilayers, where the Gilbert damping decreases with increasing temperature. The effect arises because of the enhanced damping at the interface as a result of spin pumping, where elevated temperatures cause a dynamic separation of the interfacial and bulk magnetization during relaxation. Furthermore, the temperature dependence of the damping can be controlled by varying the thickness of the Nd capping layer. Our findings present a new spintronic effect that can be used to modify the dynamic properties of nanoscale materials and devices for enhanced energy efficiency or with improved switching dynamics.
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All authors Lulu Cao, Yuting Gong, Xianyang Lu, Yongbing Xu, Ya Zhai, Jing Wu, Roy W. Chantrell, Richard F. L. Evans

Soft Condensed Matter

Undulatory forcing of an intruder through granular media: effects of frequency and packing fraction

We investigate the motion amid grains of an intruder undergoing an imposed force that oscillates with a given frequency. For that, we made use of discrete numerical simulations where the intruder was a larger disk on which a force oscillating in direction was applied, and the grains consisted of smaller disks. All disks were placed on a surface with basal friction over which they could slide, the system was confined in the sliding directions, and we varied the system packing fraction, oscillation frequency, and magnitude of the forcing. The results show intermittent and very complex motions of the intruder depending on both the packing fraction and frequency of oscillation: it can move sideways while slowly progressing forward, it can be blocked during a long period after and/or before start moving, or it can simply be blocked after a given time. Interestingly, we find that the displacement velocity is much higher when the system packing fraction is above a given threshold, contrary to intuition. The results show that there is an optimal frequency that minimizes the transit time for some ranges of packing fraction, and we propose a model based on the system elasticity that explains this behavior and agrees with the numerical simulations. Our findings shed new light on how to better explore oscillating motion to move objects within granular media.
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Materials Science

Shift current conductivity in monolayer SnS: a tight-binding analysis

We investigate the bulk photovoltaic effect in monolayer SnS using an effective tight-binding model derived from first-principles calculations. By comparing short-range and long-range hopping models, we show that the essential features of the shift current conductivity are captured by a minimal model. The shift current is decomposed into transition intensity and shift vector, enabling identification of dominant interband transitions. The comparison reveals that long-range hopping processes quantitatively modify the peak positions and magnitudes, while the short-range model retains the characteristic low-energy structure of the nonlinear response. Our findings provide a transparent framework for understanding and designing bulk photovoltaic effects in two-dimensional materials.
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Strongly Correlated Electrons

Phase transitions through excited-state level crossings and topological indicators: the case of the XXZ chain with staggered Ising interaction

We combine two ways of determining the phase diagram of the spin-$1/2$ XXZ chain with a staggered Ising interaction and uniform transverse exchange, based on exact diagonalization. The model realizes a competition between Néel order and bond-dimerized phases generated by the alternating Ising interaction. The simplest approach to determine the phase boundaries is to use topological indicators based on generalized position operators (GPOs). We show that in general, the bosonized and numerical results for the topological indicators agree. The second is the method of crossings of excited energy levels (MCEL), which is justified by conformal field theory. Despite the partial loss of translational symmetry induced by the alternating Ising interaction, we show that, with the aid of the GPO to identify the relevant level crossings, the MCEL provides an accurate determination of the phase boundary between the Néel and dimerized phases. While the jumps of a topological indicator based on a GPO provide a qualitatively correct phase diagram, its accuracy is affected when the gap is very small (or the correlation length very large) at one side of the transition, as we show using field-theoretical arguments. The combination of both methods provides a more efficient way of calculating phase diagrams for correlated one-dimensional models than other widely used conventional approaches.
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Strongly Correlated Electrons

The pseudogap in high-$T_c$ superconductors from SU(2) gauge symmetry and dynamic correlation effects

We consider the spectral properties of the two-dimensional Hubbard model, describing the electronic properties of high-$T_c$ compounds, within the SU(2) gauge theory, which assumes the separation of electronic degrees of freedom into those of spinon and chargon subsystems. We use the dynamic mean-field theory (DMFT) approach to describe magnetic long-range order in the chargon subsystem while also treating spinon fluctuations on top of this state. We show that DMFT supplemented by long-wavelength magnetic fluctuations is essential for describing the asymmetry in the damping between the inner and outer regions of the hole pockets and the resulting formation of Fermi arcs in the underdoped regime, especially at low hole doping. The underlying hole pockets in the chargon subsystem can be associated with those observed in quantum oscillation measurements.
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