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Physics Condensed Matter Mesoscale and Nanoscale Physics

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Monday 31 August

Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.str-el

Bound states, resonances, and their thermodynamic properties in pseudospin-1 systems with short-range impurities

Bound states and resonances induced by short-range impurities modeled by circular potential wells are analyzed in the vicinity of flat and dispersive bands in gapped and gapless pseudospin-1 systems. We find that the bound and resonant states derived from the flat band show unusual characteristics originating from the multicomponent structure of pseudospin-1 fermions, which are distinct from those for pseudospin-$\tfrac{1}{2}$ fermions. Contrary to gapped Dirac systems and unlike bound states in the vicinity of the upper dispersive band, the bound states derived from the flat band occur for any value of the total angular momentum. The energies of these bound states with higher angular momentum $j$ tend to decrease with $|j|$. In addition, it is found that their wave functions are localized at the potential well edge and the localization increases with $|j|$. The signatures of the impurity states in the local density of states are determined. Using the Anderson model for independent electrons in the disorder potential, the thermodynamic potential, entropy density, and heat capacity are obtained. In the regime dominated by bound states derived from the flat band, the entropy density monotonically increases with temperature and saturates, whereas the heat capacity exhibits a single maximum.
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Mesoscale and Nanoscale Physics

Chiral phonons driven by chiral cavities

Lattice vibrations carrying angular momentum give rise to fundamental phenomena such as the phonon Hall effect and the Einstein-de Haas effect, offering new opportunities for manipulating angular momentum in condensed-matter systems. Generating such circularly polarized phonons requires either the use of an external magnetic field, or of polarized light pulses. The latter approach does not require the use of any magnetic response of the material, but it has limitations, in particular regarding the duration of the pulse. Consequently, any effect stemming from phonons generated by light pulses is transient. In this paper, we propose the use of a driven electromagnetic cavity as a route to generate a steady-state population of chiral phonons. We derive a general description of cavity-chiral phonon interaction, with a particular focus on modes of chiral cavities. We show that, under optimized conditions, a significant effective phonon-induced magnetic field can be generated by means of an external drive with realistic power. Our approach is specially tailored for Gamma point phonons with THz frequencies, and opens a new route for investigating chiral phonons with electromagnetic cavities.
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All authors V. A. S. V. Bittencourt, N. Shabala, R. M. Geilhufe, A. Metelmann

Mesoscale and Nanoscale Physics

Entanglement from particle number fluctuations in a second-order topological insulator

Higher-order topological insulators are materials with a bulk energy gap featuring gapless modes at $(d-n)$-dimensional edges, where $n > 1$. Despite this modified bulk-boundary correspondence, their nontrivial topology can nevertheless be observed through the bipartite entanglement spectrum. Inspired by works suggesting fluctuations in conserved quantities could be used to study topology in one-dimensional systems, which likewise feature zero-dimensional edge modes, we extend this treatment to a two-dimensional second-order topological insulator where corner states play an analogous role. We show that the standard bipartite entanglement entropy and particle number fluctuation lack striking signals of topological phase transitions, both in the static case and in the time evolution after a quench, obscured by an area-law term from the subsystem edges. By introducing a quadripartite construction of the subsystem, we show that it is possible to isolate the topological contributions, producing sharp transition peaks in both quantities, observable by studying subsystems much smaller than the full system. As particle number fluctuations are accessible in existing experiments, these results establish a concrete and scalable path to experimental detection of the entanglement in higher-order topological insulators.
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Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.stat-mech

Exact joint eigenvalue densities of non-Hermitian random matrices are Calogero scattering states

Determining exact joint eigenvalue densities is central to random matrix theory. We solve this long-standing problem for non-Hermitian matrices with transposition symmetry (complex symmetric and complex self-dual) at arbitrary matrix size. Up to a Vandermonde factor, they are scattering-state wave functions of the Calogero model, a line of particles interacting through an inverse-square potential, with the coupling strength set by the symmetry. In contrast to many previously known joint densities, the densities cannot be written as a gas of eigenvalues with pairwise interactions. We further compute the complex level spacing distributions and two-point spectral correlation functions, which carry power-law tails, absent in a Coulomb gas. Our results shed light on the interplay among random matrices, integrability, and symmetry.
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Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.stat-mech

Duality between the level statistics of Hermitian and non-Hermitian random matrices

The complex spectral statistics of non-Hermitian random matrices provide a standard diagnostic of dissipative quantum chaos. Yet an analytical understanding of how symmetry enriches these universal correlations remains limited. We establish an exact duality between the spectral statistics of Hermitian and non-Hermitian random matrices in the limit of large matrix size. This duality resolves a longstanding analytical problem by yielding the previously unknown eigenvalue pair-correlation functions for complex symmetric (class AI$^\dagger$) and complex self-dual matrices (class AII$^\dagger$), completing the analytical description of bulk pair correlations in the non-Hermitian threefold way. It further gives closed-form spectral densities near the origin for seven additional symmetry classes. Numerical tests in interacting and dissipative quantum models support the universality of these predictions beyond Gaussian ensembles. The duality suggests a deeper connection between chaos in closed and open quantum systems.
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All authors Ze Chen, Zhenyu Xiao, Yifei Liu, Shinsei Ryu

Mesoscale and Nanoscale Physics

How Landau caterpillars turn into Hofstadter butterflies by tuning the periodic potential strength

It is well-known that the spectrum of two-dimensional electrons in a perpendicular magnetic field is given by discrete flat Landau levels. By contrast, electrons in a two-dimensional tight-binding model give rise to a fractal Hofstadter butterfly spectrum. In this paper, we connect these two opposite limits by showing how a butterfly spectrum emerges from broadened Landau `caterpillars', by continuously increasing the periodic potential strength. We identify a series of topological transitions that isolate a lowest trivial band, a necessary condition for the butterfly to emerge. The resulting butterfly is topologically distinct from the Hofstadter butterfly at fluxes $\phi>1$, due to anomalous behavior of diagonal hopping. Moreover, the hopping parameters of an effective tight-binding model, obtained by a Wannierization procedure at large magnetic field, are highly dependent on the flux, revealing that Wannier orbitals themselves change under the applied magnetic field. Our methods and results are relevant for artificial materials, such as moiré systems, where a full quantum of flux per lattice unit cell is experimentally accessible. On a theoretical level, having Wannierization methods for each specific flux allows more accurate many-body calculations in large magnetic fields.
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Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.str-el

Higher-Winding Fractionalization

Higher-winding skyrmion textures can generate emergent magnetic fields with multiple flux quanta per unit cell. This opens an intriguing route toward fractionalization, allowing fractionalized quantum anomalous Hall states to arise even at integer filling of the microscopic unit cell. We show that, in this setting, increasing lattice-scale inhomogeneity of the emergent magnetic field drives a Berezinskii–Kosterlitz–Thouless (BKT) transition between a fractionalized liquid and a crystalline dielectric state. This transition carries a topological signature: under flux insertion, the many-body polarization defines a quantized winding number that is nonzero in the fractionalized phase and vanishes in the dielectric crystal.
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Mesoscale and Nanoscale Physics · Cross-listed from quant-ph

Engineering multi-photon dissipation with a dc-voltage-biased Josephson junction

Multi-photon dissipation – a key resource for bosonic qubits – is usually realized by parametrically pumping a Josephson coupler at the cost of spurious nonlinear terms. Here we instead engineer it using a dc-voltage-biased SQUID, such that these parasitic terms average out. We activate the conversion of one, two, or four photons of a high-Q mode into a single photon of a lossy mode. We characterize the two-photon dissipation by Wigner tomography, establishing dc-biased junctions as a resource for reservoir engineering and a viable route to cat-qubit stabilization.
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All authors Marco Paradina, Ambroise Peugeot, Roberto Negrin, Oscar Novat, Tristan Villain, Anil Murani, Jean-Loup Ville, Sébastien Jezouin, Raphaël Lescanne, Audrey Bienfait, Benjamin Huard

Mesoscale and Nanoscale Physics

Device characterization of Si$/$SiGe double quantum dots using exchange oscillations in Earth's magnetic field

Exchange-based semiconductor qubits encompass a broad family of encodings constructed from singlet- and triplet-like spin states, several of which are compatible with operation at zero applied magnetic field. Their reliable operation requires characterization of environmental noise, residual idle interactions, and exchange-dependent decay, but this characterization often relies on multi-axis control calibration or deliberately engineered magnetic-field gradients. A simpler zero-applied-field diagnostic is particularly valuable for hybrid semiconductor-superconductor systems, in which magnetic fields can degrade superconducting components. Here, we use the intrinsic magnetic-field gradient produced by residual nuclear spins in isotopically enriched Si/SiGe to implement exchange oscillations between two quantum dots as a characterization tool without a micromagnet, dynamic nuclear polarization, or prior multi-axis calibration. Using Carr-Purcell-Meiboom-Gill exchange sequences, we extend the singlet coherence from $T_2^*=1.17\pm0.02~\mu$s to $T_2^{\mathrm{CPMG}}=74.8\pm1.8~\mu$s with $N=70$ refocusing pulses. The oscillation phase resolves residual exchange in the tens-of-kilohertz regime and enables it to be mapped across the $(1,1)$ charge cell. These results establish intrinsic-gradient exchange oscillations as a simple, more relevant zero-field diagnostic for exchange-only and related semiconductor qubit encodings that is amenable to rapid, high-throughput device characterization.
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All authors Holly G. Stemp, Harry Hanlim Kang, Chih Hwan Yang, Gabriel D. Cutter, Frederike Brockmeyer, Patrick J. Strohbeen, Max Hays, Jeffrey A. Grover, William D. Oliver

Mesoscale and Nanoscale Physics

Interfacial Spin-to-Charge Conversion in Sputtered MoTe2 Heterostructures Probed by Spin Pumping and Spin-Torque Ferromagnetic Resonance

Transition metal dichalcogenides (TMDs) and their Weyl semimetal phases, such as MoTe$_2$, have attracted significant attention for spin-orbit torque applications due to their efficient charge-to-spin conversion. However, whether this conversion originates predominantly from the bulk or the interface remains unclear. Here, we investigate spin-charge interconversion in MoTe$_2$ using spin-pumping and spin-torque ferromagnetic resonance (SP-FMR and ST-FMR). Thickness-dependent measurements reveal large spin-to-charge conversion and spin-torque efficiencies that are essentially independent of MoTe$_2$ thickness, indicating that the conversion is predominantly governed by the Rashba-Edelstein effect at the Py/MoTe$_2$ interface rather than by bulk spin transport. This behavior contrasts with the characteristic thickness dependence observed in Pt heterostructures and is further supported by bidirectional SP-FMR and interface-separation measurements. Our results highlight the dominant role of the Py/MoTe$_2$ interface in enabling efficient spin-charge conversion and spin-orbit torques in TMD-based spintronic devices. These findings highlight the potential of sputtered MoTe$_2$/Py heterostructures for low-power spintronic applications, including magnetic memory and logic devices.
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All authors J. L. Costa, E. Santos, E. L. T. França, J. B. S. Mendes, A. Azevedo

Mesoscale and Nanoscale Physics

Breakdown of Charge-Conjugation Symmetry of Disclinations in 2D Crystals

Disclinations are elementary topological defects in two-dimensional (2D) crystalline membranes, yet their elastic properties remain largely unexplored. Using atomistic simulations, we address the energetics, morphology, and interactions of disclinations in free-standing graphene, a prototypical 2D crystal. We find that while disclinations with positive topological charges follow an expected behavior, negative disclinations exhibit sublinear energy scaling with charge as well as equilibrium shape that deviates sharply from the conventional saddle ansatz. This breakdown of charge-conjugation symmetry leads to qualitatively distinct interactions: positive disclinations repel, whereas negative disclinations display a robust long-range attraction. These trends are shown to be further amplified by self-adhesion in folded membranes. Our results uncover a fundamentally different energetic landscape for negative curvature defects and provide a basis for understanding the stability, self-folding behavior, and defect-driven morphology of graphene and other 2D membranes.
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Mesoscale and Nanoscale Physics

Signatures of inter-sideband coherence in the resonance fluorescence spectrum of an acoustically-modulated quantum dot

We theoretically investigate the inter-sideband phase coherence within the resonance fluorescence spectrum of an acoustically modulated quantum dot using a filtered-field formalism for a Mach-Zehnder configuration. We demonstrate that geometric slant of the interferograms provides an indicator of phase coherence that is resilient to environmental white noise. Specifically, noise-induced spectral diffusion reduces the global fringe intensity, while leaving the characteristic inclination strictly invariant. Our findings establish a framework for verifying single-photon coherence between spectral sidebands, essential for frequency-bin encoding and scalable quantum networking in realistic, noisy solid-state architectures.
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Mesoscale and Nanoscale Physics

Local phase-space Berry curvature and Hall transport in textured twisted bilayer graphene

Slow twist-angle and heterostrain textures in twisted bilayer graphene provide a natural route to phase-space Berry geometry. We show that a purely geometric tetrad/shift sector does not generate mixed Berry curvature once the spin connection is treated consistently. By contrast, a projected textured mini-Dirac cone in twisted bilayer graphene acquires genuine mixed phase-space curvature. We analyze a controlled local Hall-bar limit with a one-dimensional texture and mirror $M_x$. In that limit the pseudogauge gradient renormalizes only the longitudinal conductivity along the textured direction, while a dc nonlinear Hall response appears only when an additional valley-odd tilt generates a Berry-curvature dipole. Both geometric responses peak at the same local filling, $\mu_{\rm loc}=\sqrt{2}\,m$, providing a gate-tunable fingerprint of their common origin. All local-cone parameters and their texture susceptibilities are extracted from a heterostrained Bistritzer-MacDonald model at $\theta=1.3^\circ$. The tilt invoked in the transport estimates corresponds to heterostrain of only $0.03\%-0.2\%$, below values routinely imaged in devices. The resulting theory provides a local analytic framework for textured moiré Dirac materials and cleanly separates geometric, texture-induced, and transport-level ingredients relevant to realistic TBG.
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Mesoscale and Nanoscale Physics

Supermoiré Reconstruction and Topological Mosaics in Twisted Trilayer WSe$_2$ and MoTe$_2$

We investigate lattice relaxation and band structures of helical and alternating twisted trilayer WSe$_2$ and MoTe$_2$ using machine-learning force fields and large-scale ab initio calculations. Interference between the two bilayer moiré lattices generates a supermoiré lattice that, upon relaxation, reconstructs into a few dominant domain types with locally commensurate bilayer moiré lattices. Because the systems lack $C_{2z}$ symmetry, domains otherwise related by this symmetry become energetically and topologically distinct, unlike in twisted trilayer graphene. Band structure calculations show that the topmost valence bands originate from the $K$ ($K'$) valleys and carry domain-dependent valley Chern numbers. The resulting supermoiré lattice hosts a mosaic of topologically inequivalent domains, offering a platform for exploring correlated and topological physics.
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Mesoscale and Nanoscale Physics

Coexistence of polariton bound states in the continuum and 2D radiative excitons

Bound states in the continuum (BICs) enable optical modes with ideally infinite radiative lifetimes despite lying within the radiation continuum. Radiation-matter interaction in periodically patterned planar waveguides embedding two-dimensional (2D) optically active excitations can be described quantum mechanically by diagonalizing a non-Hermitian operator, known as the Hopfield matrix, which can be generalized to incorporate independent photonic and excitonic losses into the polaritonic states. However, since 2D excitons undergo intrinsic wavevector-dependent radiative decay within the light cone, whether the Hopfield formalism can consistently account for this process while preserving polariton BICs has remained an open question. Here we show that a non-Hermitian Hopfield formalism incorporating excitonic radiative losses correctly captures the existence of genuine $k=0$ polariton BICs with diverging radiative lifetimes. The theory provides a unified microscopic framework for radiative excitons and polariton BICs, and an efficient predictive tool for designing photonic-crystal platforms coupled to quantum wells, transition-metal dichalcogenides, and other 2D excitonic materials.
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All authors Simone Zanotti, Marco Liscidini, Dario Gerace, Lucio C. Andreani

Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.mtrl-sci

Emergence and suppression of phonon vortices in two-dimensional crystals: Interplay of lattice symmetry, heavy impurities, and shear

Phonon vortices are vortex-like displacement fields that appear in the vibrational modes of two- dimensional materials. Here, we demonstrate that these vortices arise as symmetry-adapted linear combinations of degenerate planar phonon modes, with the superposition coefficients uniquely de- termined by the lattice point group. This symmetry principle establishes that vortices are intrinsic standing-wave solutions in perfect crystals, requiring neither impurities nor disorder. A heavy mass impurity favors vortex modes over planar modes through stronger resonance-induced frequency soft- ening, whereas shear deformation suppresses vortex modes by breaking rotational symmetry. The competition between these two effects gives rise to a precisely predictable strain threshold. The proposed framework, grounded in symmetry and energy-minimization, provides a useful basis for understanding vibrational topological defects induced by other types of impurities or defects. This study further suggests that defect and shear engineering constitutes an effective tuning strategy for controlling vibrational modes and the associated thermal and mechanical properties of crystals.
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Mesoscale and Nanoscale Physics

Predictive wavelength tailoring of uniform GaSb-based quantum dots for emission at 1.55 um

A detailed study of emission wavelength tailoring of GaSb-based QDs formed by InGaSb-filling of droplet-etched nanoholes in AlGaSb is presented. The study shows that the emission wavelength can be modified from 1.48 um to the center of the telecom C-band at 1.55 mm by independently varying the QD composition and size. More specifically, the optical transition energy shifts linearly as a function of In-content of the QD material at a rate of -4.4 meV/In-percentage, and with the number of monolayers (ML) of material used for filling the nanoholes, at -2.0 meV/ML. These experimentally observed energy shifts are well predicted by simulations yielding rates of -4.3 meV/In-percentage and -2.1 meV/ML, respectively. For the simulation, a uniform In composition, low intermixing, and microscopically measured QD geometry is considered. Additionally, excellent ensemble QD uniformity, with unprecedented inhomogeneous broadening well-below 7 meV across all samples is demonstrated. Finally, photoluminescence of single-QDs reveals narrow excitonic emission lines of 13.8+/-6.7 ueV and low fine-structure splitting values reaching <10 ueV. These results identify GaSb-based LDE QDs as a tunable telecom platform for scaling quantum-photonic applications over long-haul optical fiber networks.
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All authors Markus Peil, Maja Wasiluk, Ziemowit Olinkiewicz, Tymon Przychodni, Robert Matysiak, Teemu Taskinen, Joona Salonen, Abhiroop Chellu, Metin Patli, Joonas Hilska, Anna Musiał, Michał Gawełczyk, Mircea Guina, Teemu Hakkarainen

Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.mtrl-sci

Layer Axial Phonons and Dipolar Thermal Response in Centrosymmetric Thin Films

In nonmagnetic centrosymmetric materials, $\mathcal{PT}$ symmetry enforces vanishing total phonon angular momentum (phonon AM) at every wave vector, making them appear unsuitable as hosts of axial phonons. Here, using first-principles calculations for BaAgAs and representative van der Waal's layered materials, we show that centrosymmetric slabs can still host large hidden layer-resolved phonon AM with both chiral and cycloidal modes. This hidden phonon AM texture produces layer resolved phonon thermal Edelstein-like responses and a real-space phonon AM dipole response, both tunable by strain. Our results establish centrosymmetric layered materials as an exciting platform for hidden axial phonon and multipolar phonon thermal response.
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Mesoscale and Nanoscale Physics

Exact fluctuation relations in voltage- and temperature-biased Laughlin-edge constrictions

We present a comprehensive analysis of non-equilibrium fluctuation-dissipation relations connect- ing experimentally accessible chiral-current auto- and cross-correlations to the tunneling-current noise and conductance in Laughlin edge states coupled through a quantum point contact (QPC). We examine their validity for two chiral Laughlin edges held at different temperatures and voltages and show that the relations remain exact for arbitrary tunneling strength, voltage bias, and edge- state temperatures. We further generalize them to spatially extended QPCs and to tunneling am- plitudes with an explicit voltage dependence, and discuss the conditions and limitations associated with these generalizations. Our results establish that the local tunneling-current noise generated at the QPC can be reliably reconstructed from experimentally accessible auto- and cross-correlations measured downstream, providing a robust route to characterize non-equilibrium transport in chiral edge states.
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All authors Gu Zhang, Gabriele Campagnano, Domenico Giuliano, Igor Gornyi, In`es Safi

Mesoscale and Nanoscale Physics

Moiré-induced lattice reconstruction at buried atomic interfaces

Atomic reconstruction at twisted two-dimensional interfaces governs many of their emergent optical, electronic, and mechanical properties, including sliding ferroelectricity. Despite recent progress in understanding lattice reconstruction in suspended twisted bilayers, structural changes at van der Waals heterointerfaces between multilayer crystals remain largely unexplored. Here we use multi-slice electron ptychography to non-invasively recover the three-dimensional atomic structure at marginally twisted rhombohedral interfaces between thick transition-metal dichalcogenide crystals. With a position precision of ~3 pm and a depth resolution ~1 nm, we resolve the twist-induced lattice reconstruction field per layer, and the resulting dislocation network at the buried interface. Despite the bulk nature, we observe markedly strong in-plane interfacial reconstruction due to suppression of the out-of-plane bending by outer layers, exceeding predictions from our three-dimensional modelling. Furthermore, we extract the strain tensor evolution during the decay of the reconstruction into the bulk, providing a structural foundation for understanding multi-layer moiré systems.
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All authors Nicholas Clark, Frederick Allars, Isaac Soltero, Wendong Wang, David Hopkinson, Hugo de Latour, James G. McHugh, William Talbott, Sam Sullivan-Allsop, Rongsheng Cai, Astrid Weston, Xiao Li, Gareth Tainton, Casey K. Cheung, Francisco Selles, Alex Summerfield, Andrey Kretinin, Christopher S. Allen, Vladimir Falko, Sarah J. Haigh, Roman Gorbachev

Mesoscale and Nanoscale Physics

Dynamics of a nanoscale ferromagnetic vortex

We propose a ferromagnetic vortex stabilized by the interfacial Dzyaloshinskii–Moriya interaction (iDMI) and investigate its properties through theoretical analysis and micromagnetic simulations. Our results demonstrate that this vortex can remain stable even in nanoscale ferromagnetic disks with radii below $5\,\text{nm}$—far smaller than those of conventional nanodot vortices having about $1\,\mu\text{m}$ radius. We analytically solve the nonlinear equation of motion describing the anharmonic vortex oscillation, and identify the critical frequency that determines the stability of the driven oscillation of the vortex. This nanoscale vortex exhibits conventional properties of microscale vortices, including gyrotropic oscillation and resonance frequency shift under an out-of-plane magnetic field. It also exhibits unconventional behaviors, such as a strongly anharmonic potential, nonlinear oscillations, and a Duffing-oscillator-like response under the external AC bias.
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Mesoscale and Nanoscale Physics

Evanescent-mode Casimir-Josephson force and gate-controlled resonances in ballistic graphene Josephson junctions

We develop a microscopic scattering theory of the phase-dependent equilibrium mechanical response of a ballistic superconductor-graphene-superconductor Josephson junction. The calculation is based on an energy-dependent Dirac scattering matrix embedded in a normalized Matsubara determinant, so the reported force correction contains the complete Bogoliubov-de Gennes spectrum of the stated ideal model. At charge neutrality the full determinant approaches a closed-form evanescent-mode result proportional to $\Delta W/L^2$, reaching $2\ln 2\,\Delta W/(\pi L^2)$ at phase difference $\pi$ in the zero-temperature short-junction limit. Gate doping produces propagating channels and Fabry-Pérot structure, causing large oscillations and sign reversals of the phase-dependent force correction $\delta F=F(\phi)-F(0)$. We distinguish the interband-to-intraband Andreev crossover, controlled by $|\mu|/\Delta$, from the evanescent-to-propagating crossover, controlled by $|\mu|L/(\hbar v_F)$. Exact real-energy subgap poles obtained from the same energy-dependent scattering matrix are used to diagnose specular/interband and retro/intraband character; these labels are not treated as separately measurable thermodynamic forces in the mixed regime. We also quantify the difference between the complete determinant result and the frozen-scattering short-junction approximation without identifying that difference with a pure continuum force. The resulting gate- and phase-dependent mechanical signal provides a Dirac-material extension of earlier superconductivity-induced mechanical-force proposals.
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Mesoscale and Nanoscale Physics · Cross-listed from cond-mat.str-el

Holographic Representations of Topological Quantum Criticality: Emergent Symmetry Approach around the Bott Clock

In this article, we apply the idea of emergent symmetries to construct holographic representations of a broad class of topological quantum critical points (tQCPs) that appear in fermionic classes in the Bott clock. We show explicitly that around the Bott clock, an emergent symmetry $U_{EM}$ exists at a tQCP between different symmetry protected gapped phases with protecting symmetry $G_p$ in $d$ spatial dimensions. This emergent symmetry can be used to construct a $(d+1)$ spatial dimensional lattice model with a properly upgraded symmetry such as $U_{EM}\times G_p$ or $U_{EM} \rtimes G_p$, etc. By doubling the degrees of freedom of the adjacent topological class in $d$-dimensions, we successfully show that the $(d+1)$-dimensional lattice models constructed in this way have the desired enlarged symmetry groups that precisely belong to the adjacent topological classes, counterclockwise around the Bott clock. Furthermore, $d$-dimensional boundaries of these $(d+1)$ dimensional lattice models of gapped topological classes are shown to exhibit identical infrared dynamics as the corresponding tQCPs in the $d$-dimensional adjacent topological phases in the Bott clock, with lower symmetries.
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Mesoscale and Nanoscale Physics

Scalar Spin Chirality from Dissipative Pumping and Lamb Shift Precession

Circulating currents in triangular triple quantum dots reverse repeatedly with bias even at zero magnetic flux and for a real Hamiltonian, a phenomenon whose origin has remained unclear. We show that dissipative tunneling prepares an orbital pseudospin, while virtual charge fluctuations generate a noncollinear Lamb field that rotates it toward the chiral direction. Bias changes their relative orientation and thereby reverses the current. This reservoir-induced orbital Hanle effect converts a nonchiral orbital polarization into scalar spin chirality, which an exact ground-multiplet identity links to the circulating current. Hierarchical-equations-of-motion calculations show that the low-bias reversal survives beyond the second-order weak-coupling description, while the quadratic growth of chirality after a sudden voltage switch identifies precession. More broadly, time-reversal-odd responses can emerge in open quantum systems from the interplay between dissipative state preparation and coherent precession.
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Mesoscale and Nanoscale Physics

Singlet-doublet transitions and Josephson currents in a superconducting ring with a quantum dot

We investigate the ground state properties of a superconducting ring embedded with a quantum dot (QD) by using a variational wave-function approach. A theoretical formulation for the treatment of the finite-U Anderson impurity coupled with a superconducting ring are presented. We demonstrate singlet-doublet transitions of the ground state for this system with the QD in the mixed valence regime. It is shown that the supercurrent in the superconductor ring shows oscillations with the external enclosed magnetic flux and exhibits abrupt jumps at the singlet-doublet phase transition points.
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Mesoscale and Nanoscale Physics

Switchable Magnetoelectric Transport in Graphene via a Van der Waals Multiferroic

Electric and magnetic control of transport properties at atomic interfaces is central to the development of next generation electronics and spintronics. Van der Waals multiferroics materials that simultaneously host dielectric and magnetic orders down to the monolayer limit offer a promising platform for such interfacial control, yet the realization of electronic functionalities that exploit the unique attributes of van der Waals multiferroics has largely remained elusive. Here, we realize a van der Waals heterostructure comprising graphene and the multiferroic CuCrP2S6, enabling gate-switchable magnetoelectric transport in graphene, mediated by the multiferroic layer. The charge-neutrality resistance peak of graphene exhibits pronounced hysteresis arising from polarization flip in the multiferroic state. Application of an in-plane magnetic field shifts this peak in a polarization-dependent manner, revealing magnetic-field-induced polarization modulation a direct signature of the magnetoelectric effect. Furthermore, cooling the device under an applied electric field enables domain control of the multiferroic order, allowing reversible switching of the interfacial magnetoelectric transport. These results provide the first demonstration of interfacial magnetoelectric transport in a vdW heterostructure, and establish a pathway for engineering two-dimensional van der Waals interfaces for functional device applications.
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All authors Miuko Tanaka, Shunta Aoki, Ikoi Sato, Hao Ou, Itishree Pradhan, Ngoc Han Tu, Yangsong Chen, Tomohiro Ishii, Kenji Watanabe, Takashi Taniguchi, Michihisa Yamamoto, Masayuki Hashisaka, Jiang Pu, Naoki Ogawa, Toshiya Ideue

Mesoscale and Nanoscale Physics

Universal tuning of Förster resonance energy transfer in gate-programmable conductor-dielectric-conductor heterostructures

We develop a quantum-electrodynamical theory for universal tuning of spontaneous emission and Förster resonance energy transfer (FRET) in a material-agnostic conductor-dielectric-conductor heterostructure. The platform consists of a dielectric spacer of thickness $W$ bounded by two gate-tunable two-dimensional conductors. The only microscopic input from the surrounding materials is the transverse-magnetic and transverse-electric reflection amplitudes $r_{\TM/\TE}(q_\rho,\omega)$ of the two sheets. Starting from the QED photon propagator, we derive the retarded Maxwell dyadic, the vacuum/Hadamard field propagator, and the time-ordered Feynman propagator in the same geometry. The spontaneous-emission rate is controlled by the local vacuum spectral density, while FRET is controlled by the nonlocal retarded/advanced product $\obG_{\text R}(\bx_D,\bx_A;\omega_D)\Im\,\balpha_A(\omega_D)\obG_{\text A}(\bx_A,\bx_D;\omega_D)$. In the transparent limit $r_{\TM}\to 0$, the near-field FRET rate recovers the bulk $x_\rho^{-6}$ law. In the Dirichlet/PEC branch $r_{\TM}\to -1$, the gapless transverse mode is removed and the donor-acceptor coupling acquires a Bessel-$K$ envelope, giving an exponentially screened FRET rate $\Gamma_{D\to A}\propto\exp(-2\pi x_\rho/W)$ at large lateral separation. In the opposite Neumann/PMC-like branch $r_{\TM}\to 1^{-}$, a nearly gapless transverse mode survives and produces a wide quasi-two-dimensional logarithmic propagator, enhancing the nonlocal electromagnetic coupling over a gate-programmable range $x_{\rho,*}\sim W/(1-r_{\TM})$. For graphene-Er implementations, the same retarded Green tensor also separates dissipative on-shell Er-to-graphene decay, governed by its absorptive part, from dispersive virtual-plasmon-mediated Er-Er coupling, governed by its reactive part; a plasmonic band gap can suppress the former while retaining the latter.
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Sunday 30 August

Mesoscale and Nanoscale Physics · Cross-listed from physics.chem-ph

Three-Electrode TiO2 + rGO Cells: Classical Controls and Interpretation within a Quantum-Discord Framework

In three-electrode electrochemical impedance spectroscopy (EIS), the impedance/capacitance response of the working electrode (WE) is measured relative to the reference electrode (RE), whereas the current required by potentiostatic control flows between the WE and the counter electrode (CE). Under classical three-electrode operation, the measured WE-RE response should therefore be independent of the properties of the electrode used as the CE, provided that conventional electrochemical and instrumental artifacts are negligible. Here, we test this expectation in cells containing nanostructured electrodes TiO2 + rGO and examine the results within a framework motivated by quantum discord to describe effective interelectrode correlations. We used dummy-cell measurements, a two-electrode bar-bar control, comparisons between Pt and bar CEs, a dummy circuit introduced into the CE branch, and CE ensemble comparisons to distinguish additive circuit behavior from CE-dependent behavior specific to the three-electrode configuration. In these experiments, the measured three-electrode capacitance response depends on CE, an effect that is not reproduced by the dummy-circuit controls examined. These findings identify a macroscopic CE-dependent capacitance response that departs from the tested classical expectation and is compatible with an effective interelectrode-correlation framework motivated by quantum discord, although the capacitance evidence alone does not constitute a direct measurement of quantum discord.
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Mesoscale and Nanoscale Physics

Chiral superconductors and competing states across a Lifshitz transition in rhombohedral pentalayer graphene

Rhombohedral multilayer graphene hosts a distinctive low-energy electronic structure in which strong Coulomb interactions and nontrivial quantum geometry intertwine to generate exotic quantum states. Recent experiments reported signatures of chiral superconductivity in electron-doped rhombohedral multilayer graphene within the spin- and valley-polarized regime. Here we map the normal-state fermiology surrounding chiral superconductivity in rhombohedral pentalayer graphene. Quantum oscillation measurements reveal an electrically controlled Lifshitz transition between a simply-connected circular quarter-metal Fermi surface and an annular quarter-metal Fermi surface. The Lifshitz boundary itself shifts with perpendicular magnetic field, consistent with the strongly momentum-dependent orbital magnetic moment of the low-energy band. Approaching the transition from either side, the electron effective mass becomes strongly enhanced, implying the formation of a nearly dispersionless band bottom and a strongly reduced kinetic-energy scale. This singular electronic structure produces a regime of exceptionally strong instability in which chiral superconductivity competes with Wigner crystalline phases and reentrant quantum Hall states. In particular, two superconducting regions with signatures of orbital time-reversal-symmetry breaking lie on opposite sides of the Lifshitz boundary and have comparable transition temperatures, yet the annular-side state is suppressed by a substantially smaller perpendicular magnetic field. Our calculation finds comparable chiral pairing tendencies on the two parent Fermi surfaces while producing a much lower orbital-Zeeman pair-breaking scale and an additional finite-momentum pairing tendency for the annular state. These results identify Fermi-surface topology as a key control parameter for chiral superconductivity in rhombohedral graphene.
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All authors Chuanqi Zheng, Cheng Xu, Chushan Li, Chenyu Zhang, Zijing Zhang, Kenji Watanabe, Takashi Taniguchi, Hao Yang, Dandan Guan, Liang Liu, Shiyong Wang, Yaoyi Li, Hao Zheng, Canhua Liu, Jinfeng Jia, Shengwei Jiang, Zhiwen Shi, Guorui Chen, Fengcheng Wu, Yang Zhang, Tingxin Li, Xiaoxue Liu

Mesoscale and Nanoscale Physics

Spin-textured orbitals in altermagnetic artificial atoms

Artificial atoms provide a versatile platform for engineering atomic-like orbitals, yet spin generally remains a passive degree of freedom in their orbital structure. Here, we introduce the concept of altermagnetic artificial atoms formed by confining electrons with momentum-dependent spin splitting. We show that altermagnetism reconstructs conventional confined orbitals into spin-textured orbitals, with spatially distinct distributions of opposite spin components. The resulting confined spectrum retains a twofold degeneracy protected by the combined $C_{4z}\mathcal{T}$ symmetry. These spin textures persist in higher-energy states, where additional radial structures combine with the characteristic angular spin pattern. Furthermore, strain resolves the degenerate orbital pairs into spin-polarized states, and continuously tunes their energy splitting. Our results establish altermagnetic artificial atoms as a route to engineering spin-dependent orbital structures in quantum-confined systems.
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All authors Yue Mao, Yu-Chen Zhuang, Cheng-Ming Miao, Yu-Fei Sun, Qing-Feng Sun