Mathematical Physics
Superintegrable systems of two interacting spin-$\frac12$ particles with first-order vector integrals of motion
O. Ogulcan Tuncer and I. Yurdusen
We study
quantum superintegrability for two interacting non-relativistic
spin-$\frac12$ particles in three-dimensional Euclidean space. The
Hamiltonian contains a central potential together with
spin-orbit,
spin-
spin, tensor, and quadratic
spin-orbit interaction terms, all depending only on the relative distance. We restrict the classification to the $V_4=0$ case, so that the
spin-momentum interaction term is not included. We determine all such systems admitting non-trivial first-order vector integrals of motion. For this purpose, we construct the most general Hermitian first-order vector operator built from the relative position, momentum, orbital angular momentum, and the two
spin vectors. The commutativity condition with the
Hamiltonian leads to an overdetermined system of radial determining equations, whose solution gives the complete list of admissible potentials and the corresponding vector integrals within this class. The results extend the previous classifications of scalar and pseudo-scalar first-order integrals for two particles with
spin. We also discuss selected
symmetry algebras generated by the vector integrals and show, in one representative case, how a scalar reduction leads to exact Coulomb- and oscillator-type solutions.
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Quantum Physics
Nonlinear Response via Sublinear Optics
Mykhaylo Khoma, Valeriia Bilokon, Elvira Bilokon et al. (+1 more)
Sublinear optical response, in which the emitted field scales as a fractional power of the driving field, lies beyond the conventional perturbative hierarchy of nonlinear optics. Here, we show that such a response can be engineered in a hydrogen atom using tracking control. Rather than prescribing the driving waveform, the field is determined self-consistently from the evolving
quantum state to enforce a chosen relation between the optical response and the applied field. We demonstrate accurate tracking for multiple exponents and scaling strengths, establishing that a single atomic system can be driven to realize a family of distinct sublinear responses. The calculations are enabled by a compact wave-packet continuum discretization that treats bound and continuum states on equal footing and is applied here, to the best of our knowledge, for the first time to strong-field optics and
quantum control. These results establish tracking control as a general route to engineering optical responses beyond conventional
polynomial nonlinearities.
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All authors Mykhaylo Khoma, Valeriia Bilokon, Elvira Bilokon, Denys I. Bondar
General Relativity and Quantum Cosmology
Plasma-Induced Modifications of the Shadows of Rotating Bardeen Black Holes with Perfect Fluid Dark Matter
Gowtham Sidharth M and Sanjit Das
We study the optical appearance of a rotating regular Bardeen black hole embedded in perfect fluid dark matter (PFDM) when
photon propagation occurs through a
plasma medium. Three
plasma models are examined: a homogeneous distribution, a radially varying distribution, and a general distribution with both radial and angular dependence. The influence of
plasma on
photon motion and the resulting shadow morphology is analysed using shadow observables. To assess astrophysical viability, the
plasma and PFDM parameters are constrained using the Event Horizon
Telescope bounds on shadow circularity and fractional diameter deviation. The results demonstrate that environmental effects arising from both PFDM and
plasma produce measurable modifications to the shadow, indicating that black-hole imaging can provide useful constraints on the surrounding medium as well as the intrinsic properties of regular rotating black holes.
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Quantum Physics
Rei Sato
We propose an explicit
quantum circuit for
quantum spatial search based on discrete-time
quantum walks on $d$-dimensional
lattices. In this
algorithm, the flip-flop shift operator moves the walker to a neighboring site along the selected spatial direction and reverses the corresponding direction label after the move. By encoding each pair of opposite directions so that they differ only in the least significant
qubit of the coin register, we implement the shift using coin-controlled modular increment and decrement operations on the position registers, together with a single $X$ gate that reverses the direction label. We verify that the proposed
circuits reproduce the theoretical dynamics on two- and three-dimensional periodic
lattices. We further extend the
circuit construction to systems with position-dependent shift rules, such as non-periodic boundaries, and validate this extension on a two-dimensional
lattice. The resource analysis shows logarithmic growth of the
circuit width. For the two-dimensional
lattice, the synthesized depth is consistent with $O(\sqrt{N}(\log N)^{3/2})$, while the three-dimensional depth empirically follows an $O(\sqrt{N})$ dependence over the investigated range. Under a CX-gate depolarizing noise model, CX-optimized
circuits exhibit improved noise robustness. These results provide a practical framework for implementing
quantum spatial search on regular
lattices and extending it to defective and other irregular
lattice structures.
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High Energy Physics (Phenomenology)
Flavor-Dependent QCD Critical Endpoint and Dual-Channel Fluctuations from Multi-Charge Holography
Zhibin Li, Danning Li and Mei Huang
We construct a thermodynamically self-consistent
holographic QCD framework incorporating multiple conserved charges. By introducing three independent bulk $U(1)$ gauge fields, our Einstein-Maxwells-dilaton (EMsD) model naturally accommodates the coupled chemical potential landscape $(\mu_B, \mu_Q, \mu_S)$ inherent to realistic heavy-ion collisions. Crucially, thermodynamic consistency is enforced at the level of
holographic renormalization, ensuring exact Maxwell cross-derivative relations without ad hoc patching. Calibrated exclusively at zero density, the model exhibits genuine predictive power for finite-density thermodynamics. We reveal that finite charge and strangeness densities induce pronounced nonmonotonic shifts in the critical endpoint (CEP) location. Furthermore, by mapping the freeze-out trajectories, we demonstrate that the allowed parameter bands robustly encompass empirical
hadron resonance gas (HRG) fits. Within this physical regime, higher-order cumulant ratios for both net-
baryon and net-charge channels exhibit coherent critical peaks at $\sqrt{s_{NN}} \approx 5\text{--}7\,\text{GeV}$. This hierarchical dual-channel signature provides a decisive, background-free strategy for the ongoing experimental search for the QCD critical point.
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Mathematical Physics
Lagrange points of the restricted three-body problem in spaces of constant curvature
Miguel Ayala, Carlos Barrera-Anzaldo and Luis C. García-Naranjo
We continue the study initiated by Kilin (Reg. Chaot. Dyn. 4, (1999)) and by Martínez and Simó (Celest. Mech. Dynam. Astronom. 128, (2017)) on the classification and stability of the relative
equilibria of the restricted three-body problem in two-dimensional spaces of constant
curvature, which generalize the classical Lagrange points of the planar problem. After formulating the problem as an autonomous Lagrangian system with two degrees of freedom, whose only parameters are the
curvature $\kappa$ and the mass ratio $\mu$ of the primaries, we establish several classification results for the case $\kappa>0$ by combining analytical methods with computer-assisted proofs. These results provide rigorous confirmation of phenomena for which previously only numerical evidence was available. We also provide topological explanations for the qualitative differences between the behavior of relative
equilibria in positive
curvature and that observed in the planar and negative-
curvature cases. Our analysis focuses on the regime of small $\mu$ and indicates that positive
curvature has a stabilizing effect on the triangular
equilibria $\Ll_4$ and $\Ll_5$, whereas negative
curvature appears to have the opposite effect.
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General Relativity and Quantum Cosmology
A wormhole with two black holes
Gérard Clément
We report on a new three-parameter stationary solution of the four-dimensional
vacuum Einstein equations, which describes a Lorentzian wormhole harboring two antipodal co-rotating black holes. These are hung from one of the two spacelike infinities by two semi-infinite
cosmic strings with positive or negative tension. We evaluate the Komar masses and angular momenta of the two black holes, and check that these obey the usual Smarr relation, as well as the generalized first law for a system of collinear black holes and
cosmic strings. While free from Misner strings, this spacetime allows closed timelike curves within a bounded volume. The metric also admits a naked ring singularity for almost all values of the parameters.
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Quantum Physics
Irreversibility, equilibrium and measurement in quantum mechanics
Christopher J. N. Coveney and Peter V. Coveney
Quantum mechanics is widely recognised as being incomplete. It is not consistent with the second law of thermodynamics and does not provide a scientifically credible physical account of the measurement process, the means by which coherence is broken and classically observable states are recorded. This has led to many ad hoc assumptions being used to account for various properties of
quantum systems, among which is the coherence time of
quantum devices that determines their ability to perform computations. Here, we show that all these properties can be accommodated naturally and consistently in the context of mixing
quantum systems which exhibit continuous spectra, as arises in the thermodynamic limit in
quantum statistical mechanics and
quantum gravity. In particular, for isolated systems we show that the time-reversal
symmetry associated with
unitary time
evolution of the
quantum state gives rise to time-
symmetry breaking and a semi-group
evolution which attains thermodynamic
equilibrium at long times. Moreover, the emergence of this non-
unitary time-asymmetry leads to microcanonical
equilibrium states in which all
quantum coherence is lost and is accompanied by the transformation of pure states into mixtures, leading in turn to an increase in
entropy. Inclusion of a macroscopic measurement apparatus shows how the outcome of a measurement corresponds to the von Neumann projection postulate, arising with probabilities in conformance with the Born rule. The mathematical structure of the theory which applies to
quantum systems with continuous spectra is closely analogous to the classical ergodic theory of dynamical systems and the conditions under which they attain
equilibrium states.
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General Relativity and Quantum Cosmology
Gravity-Induced Entanglement of Quantum Clocks as a Signature of Genuinely Quantum Local Position Invariance
Eyuri Wakakuwa
Whether the principles of general relativity extend to a
quantum regime remains one of the open questions in modern physics. In classical general relativity, Einstein's equivalence principle underpins the interpretation of
gravity as spacetime geometry. However, it is not known whether the principle remains valid when the source of
gravity could be
quantum. Here we show that
gravity-induced
entanglement (GIE) of
quantum clocks provides a framework to characterize local position invariance (LPI) in such a regime, which constitutes one of the subprinciples of the equivalence principle. By adapting the existing formulation of
quantum LPI to the context of GIE, we analyze two schemes that address complementary aspects of LPI and differ only in the choice of the initial clock state: one in which
entanglement will be generated if and only if there is a genuinely
quantum violation of LPI, and the other where classical-like LPI violation manifests in the frequency of
entanglement oscillation. Our results suggest that GIE of
quantum clocks offers an approach to investigating fundamental principles of general relativity in the
quantum regime, shedding new light on the interplay between
quantum mechanics and the theory of
gravity.
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Solar and Stellar Astrophysics
Optical Spectroscopy and Temporal Evolution of the Nova V1405 Cas
Gesesew R. Habtie, Ramkrishna Das, Elias Aydi et al. (+1 more)
This paper presents the findings from our study of nova V1405~Cas over the first 1051 days after the outburst. The study includes an analysis of the photometric light curve
evolution, along with a detailed spectroscopic
evolution. Photometric analysis shows that the nova is a very slow nova, with a decline timescale of $t_2 \approx 165$ days. The mass of the white
dwarf is calculated as \( M_{\rm WD} \sim 0.7\~M_{\odot} \). The secondary
star is a low-mass main-sequence
star, with a mass of \( M_{\rm sec} \approx 0.43\~M_{\odot} \). Spectral observations show initial dominance by Balmer emission lines accompanied by prominent P Cygni profiles during the first +339 days. These features disappeared in later epochs, being replaced by high-ionization coronal lines, indicating that the nova had transitioned to the coronal phases by day +371. To investigate the physical conditions of the ejecta and the central source, we conducted photoionization modeling using cloudy. Our model reveals a gradual increase in the temperature and luminosity of the system, and suggests that the ejecta were primarily composed of He, N, Fe, Ne, and Ca, with noticeable temporal variations in their relative abundances. The estimated mean ejected mass is approximately $1.10~\times~10^{-4}\~M_{\odot}$, which is relatively high and suggests a low-mass white
dwarf. Our optical spectroscopic and photometric analyses, combined with detailed photoionization modeling, indicate that the white
dwarf in Nova V1405 Cas is unlikely to be of the ONeMg type.
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All authors Gesesew R. Habtie, Ramkrishna Das, Elias Aydi, Pavol A. Dubovsky
Quantum Physics
Quantum limits to chiroptical molecular discrimination
Mikael P. Backlund
Discriminating enantiomer pairs is of central importance in the molecular sciences. The preferential interaction between
chiral light and matter is commonly employed in this discrimination, despite fundamental challenges. Here we present quantitative error bounds for classifying the handedness of a
chiral, randomly oriented,
quantum optical emitter from the perspective of classical and
quantum hypothesis testing. Most interestingly, we find that a collective measurement on $N$
photons can provide an orders-of-magnitude improvement in error rate relative to a corresponding separable measurement.
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Soft Condensed Matter
Auxetic behaviour in crystals of hard polyhedra
Rinske M. Alkemade, Silvana A. Caipa Cure, Alptuğ Ulugöl et al. (+8 more)
Auxetic materials - systems that, when subjected to a compression in one direction, also compress in one or more perpendicular directions - have intrigued researchers for decades due to their counterintuitive mechanical properties. Their unique behaviour gives auxetic materials potential for a wide range of applications such as shock absorbers, and electrodes in piezoelectric sensors. Most known auxetic materials are realized by connecting rigid, anisotropic units in a hinging manner, which are systems that often are hard to realize experimentally on the microscopic scale. Here, we explore the elastic behaviour of six
crystals composed of discrete space-filling hard polygons or polyhedra. We show that some of these systems show partial auxetic behaviour, emerging from the interplay of
entropy and geometry alone. To demonstrate the feasibility and robustness of this phenomenon, we create two experimental realizations of square-shaped particles, spanning both colloidal particles driven by Brownian motion and granular particles driven by external vibrations, and confirm the emergence of auxeticity in both cases.
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All authors Rinske M. Alkemade, Silvana A. Caipa Cure, Alptuğ Ulugöl, Andrea Plati, Vera Belde, Haadi Naqvi, Felix Verbiest, Giuseppe Foffi, Daniela Kraft, Frank Smallenburg, Laura Filion
Quantum Physics
Single Link Removal Perturbation in Szegedy Quantum Walk: from Graph Completeness Testing to Integrity Monitoring
Sara Giordano and Miguel A. Martin-Delgado
We present a rigorous perturbative analysis of the Szegedy
quantum walk search
algorithm on the complete graph with marked nodes, when a specific anomaly is present in the graph. This is motivated by the problem of monitoring the integrity of dense trusted communication networks with a
quantum-assisted procedure. The
topology of these networks is modeled as a complete graph, and the anomaly of interest is the disappearance of a single communication link which represents the minimal and spectrally hardest structural defect to detect. Building on the graph-completeness testing
algorithm framework, we quantify how the removal of a single unmarked-unmarked edge propagates through the relevant spectral quantities of the Szegedy
quantum walk. Denoting by $n$ the total number of nodes of the graph and by $m$ the number of marked nodes, we prove that the perturbation to the transition
matrix has spectral norm $\Theta(1/n)$, and that the gap
eigenvalue undergoes a strictly negative first-order shift for every $n$ and every number of marked nodes $m$, providing a formal proof of a
conjecture from our completeness testing
algorithm work; in the regime $m = \Theta(n)$ relevant for the search
algorithm, this shift has magnitude $\Theta(1/n^2)$. The corresponding eigenphase shift satisfies $\Delta\theta_\star = \Theta(1/n^2)$ in the same regime. We establish that the rotation angle of the effective subspace under this perturbation is $O(1/n)$ for $m = \Theta(n)$. Finally, we bound the change in success probability to $O(1/\sqrt{n})$ in this same regime of marked nodes, and show that this bound is dominated by the
geometric misalignment of the effective subspace rather than by the spectral shift of the eigenphase. These results provide both the theoretical foundations and the fundamental scaling limits of
quantum walk-based
topology integrity monitoring under minimal structural perturbations.
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High Energy Physics (Phenomenology)
Lorenzo Bartolini, Sven Bjarke Gudnason, Jonas Mager et al. (+1 more)
We construct a
nuclear-matter equation of state (EOS) from
holographic QCD in the Witten-Sakai-Sugimoto (WSS) model, going beyond the homogeneous ansatz by building dense baryonic matter more directly from the solitonic description of
holographic baryons. Employing the two-
baryon interaction potential obtained from the linearized
soliton tails sourced in the curved background by point-like (core) instantons, we assemble an infinite face-centered cubic (FCC)
crystal with nearest neighbors in the most attractive channel as an approximation to the
quantum liquid of
baryons and compute the energy density $\mathcal{E}(n_B)$, the chemical potential $\mu_B$, and the pressure $P$. We calibrate the symmetric-matter EOS by fixing the 't Hooft coupling $\lambda$ and the WSS scale $M_{\rm KK}$ to saturation-density and onset-chemical-potential properties, and by including a
quark-mass term to reproduce the physical pion mass $m_\pi=135\,\mathrm{MeV}$. This fit turns out to remain reasonably close to the parameters required by the
vacuum meson sector, while their modification is consistent with Brown-Rho scaling in a dense medium, and the incompressibility at saturation is of the correct order of magnitude, both in clear contrast to the homogeneous approximation. We then extend to beta-equilibrated matter, using phenomenological input for the
symmetry energy, and obtain hybrid EOS and
neutron-
star observables that are compatible with the NICER constraints.
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All authors Lorenzo Bartolini, Sven Bjarke Gudnason, Jonas Mager, Anton Rebhan
Applied Physics · Cross-listed from eess.IV
Fast reconstruction of tensor tomographic X-ray scattering data for real-time applications
André M. Antunes, Daniël M. Pelt and K. Joost Batenburg
X-ray scattering tensor
tomography reveals nanoscale structural orientation in 3D, but its reliance on slow iterative reconstruction limits real-time use. We introduce an extension of a direct reconstruction approach for parallel-beam geometries that computes algebraic filters approximating multiple iterative updates with a single filtering and back-projection step. By explicitly separating the tomographic projector from a view-dependent mixing operator, the method generalizes across tensor representations and modes of (small-angle) X-ray scattering measurement. Simulated and experimental results show that the approach approximates iterative reconstructions while reducing computation time by over an order of magnitude, realizing a reconstruction of a 53x53x53x28 tensor volume in 1 second on commercially-available hardware. The resulting speed and stability enable high-throughput analysis and open the door to real-time scattering-based imaging.
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Materials Science
Thermal and electrical conductivity of a refractory high-entropy alloy after high-pressure torsion: Electron versus phonon contributions
Jacqueline Hidalgo-Jimenez, Payam Edalati, Md Amirul Islam et al. (+3 more)
The equiatomic refractory high-
entropy alloy TiZrHfNbTa was processed by high-pressure torsion (HPT) to investigate the effect of nanostructuring and defect engineering on thermal and electrical transport properties. Severe plastic deformation (SPD) via the HPT treatment induces substantial accumulation of dislocations, grain refinement to the nanometer level (average: 40 nm), and partial transformation from the BCC phase to the omega phase. While hardness increases to a steady state with processing, the specific heat capacity exhibits a non-monotonic behavior: it decreases at low strains due to the suppression of low-frequency vibrational modes by dislocations, then partially recovers at high strains due to anharmonic vibrations at newly formed high-angle grain boundaries. Thermal conductivity decreases at low strains but shows a slight recovery at high strains, whereas electrical conductivity decreases monotonically to a steady state without recovery. Analysis using the Wiedemann-Franz law reveals that the electronic contribution dominates thermal transport, while the phononic contribution (limited by the scattering of
phonons on defects) is only 11 to 23%, depending on the degree of straining. The contrasting
evolution of thermal and electrical conductivity is ascribed to the transition from dislocation-dominated vibrations at low strains to grain boundary-dominated vibrations at high strains, which affects
phonons and electrons with different efficiencies.
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All authors Jacqueline Hidalgo-Jimenez, Payam Edalati, Md Amirul Islam, Makoto Arita, Bidyut Baran Saha, Kaveh Edalati
Plasma Physics
Combined tools for Particle-In-Cell simulations performed with transversely asymmetric chirped lasers
I. Moulanier, F. Massimo, T. L. Steyn et al. (+1 more)
We introduce the Asymmetric Chirped Electric field reconstruction (ACE) toolbox, a suite of
algorithms enabling the reconstruction of a
laser transverse distribution coupled to a chirped temporal profile. This suite includes the implementation of the reconstructed distribution in Particle In-
Cell simulations in cylindrical and Cartesian geometry. Under the assumption of negligible spatio-temporal couplings, the ACE toolbox extends a previously established method for realistic simulations of the transverse distribution by adding spectral chirping to the modal decomposition of the electric field. The relevance of the ACE toolbox is demonstrated through the modelling of a
Laser Wakefield Acceleration experiment where the produced electron bunch was optimized via spectral chirping of the
laser pulse.
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All authors I. Moulanier, F. Massimo, T. L. Steyn, B. Cros
Exactly Solvable and Integrable Systems
Long-time asymptotic behavior for the defocusing Hirota equation on a finite-genus algebro-geometric background
Taohua Luo, Zhenya Yan and Guoqiang Zhang
In this paper, we investigate the long-time asymptotics for the solution of the Cauchy problem of the defocusing Hirota equation on a finite-genus algebro-
geometric background in the whole $(x,t)$-half-plane, whose method is mainly based on a Riemann-
Hilbert (RH) formulation and Deift-Zhou nonlinear steepest descent method. The critical values of the phase function in the associated RH problem divide the space-time plane into four regions, in which the leading-order term is given by a phase-shifted finite-genus algebro-
geometric solution. The subleading behavior depends on the region: the correction is of order $t^{-1/3}$ and is governed by a Painlevé-XXXIV model RH problem in the transition regions; the leading radiation is of order $t^{-1/2}$ in the Zakharov–Manakov region; and the error is $O(t^{-1})$ in the fast-decay region. These results can also be extended to other higher-order members of the AKNS hierarchy.
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Earth and Planetary Astrophysics
Dynamical formation of long-period exoplanets systems in evolving binary stars
Isabel J. Lima, Rafael R. Sousa, Silvia M. Giuliatti Winter et al. (+4 more)
The dynamical formation and
evolution of long-period
giant exoplanets have not been well constrained due to the few observational parameters. In this study, we explore the dynamical effects in a multi-planetary system around one
star of an evolving wide binary system. We used an interpolated result of a MESA
stellar evolution inside REBOUND N-body integrations to perform simulations with a range of distinct planetary masses in a circumstellar configuration (S-type orbit), centered on a primary
star that evolves from the main sequence
star to a white
dwarf. Control simulations without
stellar evolution were performed to isolate the effects of mass loss. Although few
exoplanets are currently known to possess long-period and moderate eccentricities, we investigated the
evolution mechanisms of long-period gas
giants within this specific regime. Although these
exoplanets often remain undetected due to their wide orbits and long periods, we propose that their formation pathways are robust throughout the
evolution of binary systems. We also simulated an evolved single
star in a multi-planetary system and concluded that the secondary
star made the
exoplanets more unstable and concentrated the survivors within a semi-major axis of 50 au.
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All authors Isabel J. Lima, Rafael R. Sousa, Silvia M. Giuliatti Winter, Diogo Belloni, Ernesto Vieira, Rosana A. N. Araújo, Eder Martioli
Fluid Dynamics
Long rigid fibres in a turbulent channel flow: comparison between experiments and simulations
Defa Sun, Florian Zumbo, Christophe Pitiot et al. (+4 more)
The dynamics of long rigid fibres transported by turbulent channel flow are investigated experimentally and numerically. Experiments use polystyrene fibres of three lengths, $\ell/h=0.25$, $0.5$ and $1$, with moderate inertia, $St^+\approx20$. Their settling velocity is comparable to the friction velocity, causing accumulation near the bottom wall. Measurements are compared systematically with simulations based on a rigid slender-body model. Statistics conditioned on the distance from the wall are used to characterise the effects of fibre length and confinement on translation, orientation and tumbling. Away from the wall, the experimental fibres lag the fluid, with no clear dependence of the velocity deficit on length. Near the wall, the shortest fibres move faster than the local mean flow, whereas longer fibres remain slower, indicating length-dependent sampling of near-wall
turbulence. Confinement also strongly constrains orientation and rotation. Fibres close to the wall predominantly undergo "kayaking" motion, tumbling in planes approximately parallel to it. Orientation statistics collapse when wall distance is normalised by fibre length, identifying $y^+/\ell^+$ as the relevant geometrical variable. Where fibres can acquire a significant wall-normal orientation, "pole-vaulting" events produce a local tumbling-rate maximum at $y^+\approx\ell^+/2$. Its magnitude decreases approximately as $(\ell^+)^{-2}$, consistently with a dimensional estimate based on the near-wall velocity variation sampled along the fibre. Experiments and simulations agree well for orientation and tumbling but differ more for translational velocity. The discrepancies highlight the effect of settling, finite fibre thickness and finite slip Reynolds number that are not fully represented by the model.
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All authors Defa Sun, Florian Zumbo, Christophe Pitiot, Sandra Bosio, Cyrille Claudet, Jeremie Bec, Christophe Brouzet
Chemical Physics · Cross-listed from cs.LG
Predicting Activities in Aqueous Electrolyte Solutions with Hybrid Machine Learning
Zeno Romero, Maximilian Kohns and Fabian Jirasek
Activities in aqueous electrolyte solutions, usually described by ionic activity and osmotic coefficients, are important properties for modeling many processes in industry and nature. Established activity models, such as those of Pitzer or Bromley, require fitting to experimental data for each electrolyte of interest and thus cannot predict properties for unstudied systems. While some predictive approaches exist, they are typically limited in scope and rely on additional ion-specific descriptors. In this work, we introduce a new hybrid model that combines the physics-based Bromley model with a
matrix completion method (MCM) from machine learning. The MCM is employed to predict the electrolyte-specific parameters of the Bromley model, exploiting the fact that these parameters can be arranged in a
matrix with cations and anions as rows and columns, respectively. Due to the lack of experimental data for many electrolytes, the initial parameter
matrix is sparsely populated, making the prediction of the Bromley parameters for unstudied electrolytes a
matrix completion problem. The hybrid model, Bromley-MCM, was trained end-to-end on experimental data for mean ionic activity coefficients and osmotic coefficients of aqueous solutions of 478 electrolytes at 298 K from the Dortmund Data Bank. As output, we obtain a completed
matrix of Bromley parameters for 83 cations and 112 anions, enabling consistent prediction of concentration-dependent activities in aqueous solutions of 9,296 electrolytes at 298~K. This substantially extends the applicability of the Bromley model while maintaining high predictive accuracy, as demonstrated through evaluations on electrolytes excluded from model training.
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High Energy Astrophysical Phenomena
Modes in Transitional Millisecond Pulsars: Evidence of Pulsar Wind-Induced Disk Heating from GRMHD and Radiative Transfer
Raphaël Mignon-Risse, Manuel Linares, Kyle Parfrey et al. (+2 more)
Transitional millisecond
pulsars (tMSPs) alternate between
radio and X-ray
pulsar states, and can represent the missing link between rotation- and
accretion-powered
neutron stars. Their disk state switches stochastically between the low and high X-ray modes, both of unknown physical origin and less luminous than low-mass X-ray binaries. To reveal the source of the X-ray emission, we carry out 2D axisymmetric general-relativistic magnetohydrodynamical simulations of the interaction between an
accretion disk and tMSP magnetosphere. For the first time, we post-process tMSP simulations with a radiative transfer code that incorporates thermal synchrotron, absorption, and Compton scattering processes. By varying the disk density, hence the inflow rate, we explore two disk regimes: one truncated outside and another inside the light cylinder. In the former, most of the X-ray flux comes from the synchrotron emission powered by the wind heating the disk: this "wind" regime could correspond to the high X-ray mode. The latter is the propeller regime and lacks this heating process. However, the propeller episodically expels the disk, activating the wind heating: a 70%-30% mixture of such propeller and wind regimes reproduces the X-ray spectrum of the low X-ray mode. The excess electromagnetic torque in the propeller regime increases the
spin-down rate, averaged over both modes, by a few percent above the disk-free
radio pulsar state, in agreement with observations. Overall, the system is more luminous in X-rays when the flow is truncated outside the light cylinder and supports a contribution from wind-induced disk heating in both low and high X-ray modes.
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All authors Raphaël Mignon-Risse, Manuel Linares, Kyle Parfrey, Alexander Tchekhovskoy, Sean Ressler
Quantum Gases
Programmable Spin Conversion in Gradient Quantum Matter
Mamoru Matsuo, Yuta Sekino and Hiroyuki Tajima
We propose programmable
spin conversion in ultracold gases as gradient
quantum matter, whose
spin-dependent self-energy varies in space.
Quantum kinetic theory shows that a dissipative self-energy
curvature turns a force-driven scalar anisotropy into a
spin source with mixed longitudinal-transverse momentum parity.
Spin-resolved time-of-flight imaging can reveal a transverse
spin texture that changes sign when either the drive or programmed
curvature is reversed. Ultracold gases thereby offer a controllable
spin source for gradient
quantum matter.
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Medical Physics
BART Online Open-Source Sequence Toolbox for Computational MRI
Daniel Mackner, Philip Schaten, Markus Huemer et al. (+4 more)
Purpose In advanced computational MRI techniques, acquisition and reconstruction techniques are jointly designed. For reproducibility, it is therefore important to provide an open implementation of both. At the same time, any use in a clinical environment usually requires a close integration with the MRI scanner. Ensuring long-time reproducibility and maintenance then poses additional challenges. In this work, we aim to provide a fully integrated open-source framework that can meet these demands. Methods A software framework to develop pulse sequences is added to BART, an open-source toolbox for computational MRI. In addition, a vendor-specific driver sequence is developed that can be used to run the sequence on a clinical MRI scanner enabling online adjustment of all relevant sequence parameters. Using the Pulseq format, the exact same sequence can also be reproduced offline using a widely used vendor-neutral open-source standard. Using the Pulseq format, the exact same sequence can also be reproduced offline. As proof-of-concept, quantitative MRI methods for T1 and joint water/fat R2*, B0 mapping using radial FLASH and model-based reconstruction are implemented in the proposed framework. Consistency between online and offline acquisition is validated in phantom and in vivo experiments. Results Quantitative MRI methods highlighting specific challenges of acquisition and reconstruction were successfully implemented in BART. Acquisition parameters and FOV can be adapted online on a clinical MRI system. Quantitative parameter maps from model-based reconstruction agree for online and offline regenerated Pulseq acquisitions. Conclusion This work enables reproducibility of advanced computational MRI methods within a comprehensive end-to-end open-source framework.
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All authors Daniel Mackner, Philip Schaten, Markus Huemer, Viktoria Buchegger, Moritz Blumenthal, Xiaoqing Wang, Martin Uecker
Quantum Physics
Quasi-Non-Hermitian Edge Bursts Induced by Nonuniform Loss
Ze Yang, Wei Li and Fuxiang Li
Non-Hermitian
quantum walks on lossy
lattices with open boundaries can exhibit an anomalous peak of the loss probability at the boundary, known as the non-Hermitian edge burst (NHEB). This phenomenon has been attributed to the combined effect of the non-Hermitian skin effect (NHSE) and a gapless imaginary spectrum. Here we investigate a class of models in which the NHSE is induced by
magnetic flux while the loss is spatially nonuniform. We show that the spatial distribution of loss plays a crucial role in determining the emergence and strength of the NHEB. Notably, even in the absence of the NHSE, a weak boundary accumulation of the loss probability persists. We term this effect a quasi-non-Hermitian edge burst (quasi-NHEB). By analyzing the dependence of the loss probability on the initial position, we further demonstrate that the quasi-NHEB obeys a bulk-edge scaling relation distinct from that of conventional NHEB. Our results show that spatially nonuniform loss alone can generate boundary-localized loss anomalies even without the NHSE, providing new insight into non-Hermitian boundary phenomena and a broader platform for their exploration and potential applications.
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Materials Science
Doping tunable charge density waves in misfit layer compounds
Hugo Le Du, Ludovica Zullo, Justine Cordiez et al. (+14 more)
The ability to tune charge density waves (CDWs) through external control knobs, such as doping, pressure or strain is crucial for exploring the phase diagram of two dimensional (2D) or quasi-2D materials. Yet, controlling CDWs critical temperature and ordering vector remains a challenge for current experimental techniques. In this work, we establish misfit layer compound
heterostructures as a reliable platform to manipulate CDWs in transition metal dichalcogenides. By combining ab initio calculations with low-temperature scanning tunneling microscopy, we show how to achieve doping tunable control over NbSe2 CDW by chemically alloying in the rocksalt subunit. Crucially, we prove that tuning the La Pb ratio in the misfit family (LaxPb1xSe)1.14(NbSe2)2 enables stabilization of different CDW orders, such as 2x2 or 3x3 patterns, and even coexisting phases. This work paves the way for engineering transition metal dichalcogenides with tailored charge density waves within misfit
heterostructures.
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All authors Hugo Le Du, Ludovica Zullo, Justine Cordiez, Robin Salvatore, Daniel Schmieg, Arindam Mukherjee, Giovanni Marini, Dominik Volavka, Francois Debontridder, Marie Herve, Tomas Samuely, Shunsuke Sasaki, Florent Pawula, Etienne Janod, Matteo Calandra, Laurent Cario, Tristan Cren
Pattern Formation and Solitons · Cross-listed from cs.DM
Towards chemistries in dynamical systems
Martin Biehl and Nathaniel Virgo
Chemistry describes aspects of the universe in terms of molecules and their reactions. In this exploratory work we present a way to describe aspects of any dynamical system in similar terms. To describe a dynamical system in this way three decisions have to be made. The first is how many different "places" there are at which molecules or chemical species can occur; the second is how to determine the species present (or not) at each place; and the third is the set of transitions and reactions that can occur between the species in the various places. For these choices to be compatible with the state update of the dynamical system each state must be able to determine transitions that take the currently occurring molecules to those occurring in the updated state. We also propose an additional requirement that there is always a unique way to choose the least amount of transitions occurring during state updates. We discuss gliders in the game of life cellular and argue that when following their definition of according to Randall Beer they satisfy the additional criterion as well. We also point out some issues with the approach.
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Chaotic Dynamics
Quasi-stationary and quasi-ergodic distributions in the Pelikan random map
Samuel Brevitt and Rainer Klages
In this paper we present a concrete example of a substochastic discrete-time Markov chain on a countable state space producing a spectrum of infinitely many quasi-stationary distributions (QSDs) for generic parameter values, with each QSD supporting a distinct escape rate. Our system is motivated by an open variant of the Pelikan dynamical system, a random map introduced in the 1980s. These QSDs, and their stability to perturbative random noise, are tested in numerical simulations. The existence of unique QEDs is also established for some parameter values.
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Quantum Physics
Lower Bounds on Spectral Gaps of Parent Hamiltonians via Tensor Networks
Milán Ádám Rozmán, András Molnár and Norbert Schuch
Proving spectral gaps above the ground space is a central problem in
quantum many-body physics. Yet, finding lower bounds on the gap is notoriously difficult. We revisit the martingale method, originally developed by Fannes, Nachtergaele, and Werner [Fannes '92, Nachtergaele '96] to prove the existence of spectral gaps of parent
Hamiltonians of
Matrix Product States (MPS), and provide improvements to the different steps of the method. Most importantly, we devise a new technique which allows to compute the key quantity in the martingale method – the overlap of local ground spaces – exactly and efficiently. This enables a clear improvement of the method, allowing it to outperform other existing techniques to lower bound gaps, which we demonstrate by benchmarking on several models. Remarkably, our – numerically motivated – approach at the same time also yields a significantly simplified proof of the fact that parent
Hamiltonians of any (well-behaved) MPS are always gapped.
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Quantum Physics
How to improve the discrimination power of classically simulable measurements?
Yiran Wang and Yongming Li
Classically simulable measurements (CSMs) constitute an important class of restricted measurements in the odd-
prime-dimensional magic resource theory, referring to those measurements with positive discrete Wigner functions. Since their discrimination power is weaker than that of global measurements, it is necessary to study how to improve the discrimination power of CSMs. In this paper, we consider three methods to improve the discrimination power of CSMs, including adding magic resources, using
quantum catalysts, and using
quantum memories. Specifically, we relate measurements with positive discrete Wigner functions to completely positive Wigner-preserving measurement channels, thereby transforming the problem of improving the discrimination power of CSMs into the problem of determining how many magic resources are required to simulate
quantum channels using free operations. Based on this, we derive the lower and upper bounds of the simulation cost. Moreover, we provide a concrete example for which these bounds coincide and prove that consumable magic resources can enhance the discrimination power of CSMs. Finally, we establish a no-go
theorem, which shows that for discriminating a pair of states with positive Wigner functions, neither finite-dimensional
quantum catalysts nor finite-dimensional
quantum memories can improve the optimal success probability of discrimination using CSMs.
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